Self-Absorption Corrections for Plutonium Measurements With the Tomographic Gamma Scanner - 17325
The Tomographic Gamma Scanner (TGS) is a Non-Destructive Assay (NDA) instrument that combines high-resolution gamma spectroscopy with low spatial resolution three-dimensional image reconstruction in order to reduce bias and improve precision for measurements of drummed waste. The TGS technique is especially suited to measure containers with non-uniform source distributions and low-to me-dium-density heterogeneous matrices, compared with traditional NDA methods. Canberra recently built, installed, and commissioned a TGS system, intended primarily for the measurement of plutonium (Pu) bearing waste, at a European nu-clear fuel reprocessing facility. Pu assays using the TGS technique present technical challenges distinct from those typically encountered in traditional LLW applications. Among these is the need to apply corrections for self-absorption effects that occur on scales smaller than the TGS spatial resolution, and can compromise the assay result if not included in the TGS imaging methodology. We present a brief review of the Self Absorption Correction (SAC) technique, and discuss the complications involved with its application to the TGS methodology with examples from our recent experience. This work continues a Canberra history of further developing and refining a technique to solve emerging problems, having commercialized the original methodology by partnering with the research institution that pioneered it. The TGS and the SAC methodologies were originally developed by Los Alamos National Laboratory (LANL) and John Fleissner respectively, and this work illustrates how Canberra has implemented an advancement of these techniques in a new TGS system. (authors)