Sealing fractures to increase underground storage security: Lessons learned from a multiscale multim
Explore the source record for details and available documents.
Hajirezaie, Sassan↗
SEARCH · Search NASA
Results for “UNDERGROUND STORAGE”
Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.
Quote a phrase for an exact phrase match. Source license links do not imply unrestricted reuse.
From Fossil Fuels to Green Mines: Understanding Hydrogen-Shale Interactions for Secure Underground Storage
Hydrogen-powered mining trucks are rapidly gaining traction as a key driver of decarbonization in the mining industry. This surge necessitates a decisive shift towards renewable energy sources, primarily for hydrogen production. However, the inherent intermittency of renewables poses a challenge for continuous operations, demanding efficient storage solutions for hydrogen fuel. Hydrogen, derived from renewables, requires large-scale storage, with underground hydrogen storage (UHS) in depleted oil and gas reservoirs projected to provide this capacity. An impermeable seal (caprock) overlying depleted reservoirs is crucial for preventing leakage and ensuring secure storage. Shale, a potential caprock, has been recognized for its effectiveness in containing natural gas for geological time-periods. This study investigates the impact of hydrogen exposure on the matrix permeability of Marcellus shale, a key factor influencing its sealing capacity. A novel time-resolved approach was employed, measuring matrix permeability after each exposure to understand the dynamic interactions between hydrogen and the shale matrix. Samples were exposed to hydrogen in pressure reactions at realistic reservoir conditions at varying time durations. Preliminary results reveal an initial increase in permeability, while subsequent exposures show a decrease, indicating potential microstructural changes.
08 HYDROGEN↗
Hydrogen underground storage for grid electricity storage: An optimization study on techno-economic analysis
Here, this study performs a techno-economic analysis of hydrogen underground storage systems for grid electricity storage, evaluating their economic viability at the plant scale using dynamic optimization. It explores the feasibility of various system configurations and revenue models in the context of volatile electricity prices and the necessity for multiple revenue streams. The hypothesis tested is that large-scale hydrogen storage, despite its low round-trip efficiency, can be economically viable with the right mix of revenue streams. This study uses scenario-based analysis to assess the impacts of different system configurations, including engaging in time-shifting arbitrage, ancillary service markets and blending hydrogen with natural gas. Results indicate potential annual net cash flows of up to $\$$1.5 million from ancillary services integration and $\$$5.2 million from natural gas blending, contingent on specific system sizes. The study concludes that hydrogen underground storage for grid electricity storage can be profitable, and emphasizes that proper system design and precise electricity price forecasting are crucial for optimizing system performance and economic returns. This research sets the stage for further investigations into the scalability of hydrogen storage systems and their broader implications for grid electricity storage and energy market dynamics.
25 ENERGY STORAGE↗
Analysis of synergies in converting underground storage sites: Natural gas to hydrogen with co-located CO2 storage
This study examines the untapped potential of synergistically converting underground natural gas storage (UGS) into underground hydrogen storage (UHS) with co-located CO2 storage. Current approaches to subsurface storage technology (SST) development often prioritise single-use scenarios, overlooking the benefits of integrating multiple technologies. We investigate converting UGS assets into UHS through gradual cushion-gas injection over multiple years, rather than injecting all cushion gas in the first year, and include on-site CO2 storage to offset site emissions. Mechanistic modelling shows this gradual transition reduces the Levelised Cost of Storage (LCOS) of H2 by 1.2-13.1% while retaining energy output within 3% of the current status quo. We also show that combined UHS and CO2 storage hubs can reduce the LCOS of CO2 by 45-77% for only a 3-10% increase in hydrogen LCOS relative to the status quo. This analysis framework may help future-proof SST sites and support a resilient, economically beneficial energy transition.
Mouli-Castillo, Julien↗
Integrated geological, economic, and risk assessment of underground hydrogen storage
Underground hydrogen storage (UHS) is a promising option to buffer variable renewable power and support the hydrogen economy. Yet this technology is early-stage, and key uncertainties remain about how coupled processes such as geochemical and geomechanical impacts affect long-term storage security. In this paper, we seek to integrate the results from a large, multi-scale research program to quantify core feasibility metrics and situate these studies within ongoing efforts. Through this work, we evaluate hydrogen recoverability during storage by assessing diffusive losses, losses to geochemical interactions and their subsequent impact on geomechanical properties, and losses to residual saturation during injection and withdrawal. Molecular and laboratory studies show that lithologic heterogeneity, pore geometry, and mineral surface chemistry govern hydrogen–rock interactions, controlling loss pathways. High-pressure coreflooding is used to estimate relative permeabilities and measure parameters needed for reservoir-scale sensitivity analyses. These core-scale experiments found early hydrogen breakthrough at low saturations driven by capillary and viscous fingering, which limits pore-space utilization at early times, while repeated injection and withdrawal cycles improve deliverability over time. Technoeconomic factors and purity requirements for end uses are also considered as part of our comprehensive feasibility analysis. Finally, we underscore the importance of geophysical monitoring and tailored injection strategies to maintain integrity and efficiency. Together, these results provide a quantitative foundation for safe, scalable deployment of UHS and highlight priorities for future integrated studies.
08 HYDROGEN↗
Economic assessment of seismic monitoring for underground hydrogen storage
Underground hydrogen storage (UHS) plays a key role in the energy landscape. However, like other subsurface engineering technologies, UHS may cause leakage into the groundwater or atmosphere and possibly induce local seismicity. To reduce these risks, seismic monitoring could be a viable technique to track the UHS plume, detect leakages, and locate induced seismicity events. Seismic monitoring has been proposed to safely monitor UHS, but research in this area is still new and requires field studies. Lab and theoretical studies have demonstrated the validity of seismic monitoring for UHS. Therefore, it is imperative to analyze the economic feasibility of seismic monitoring for UHS. Hence, we develop a cost model and open-source Python code for seismic monitoring that considers types of seismometers, comprehensive operational scenarios, detection thresholds, and long-term leakage monitoring. A case study is further provided to validate the cost model on reservoir simulations of UHS. We find that the levelized cost for a 10-year operating UHS site will range on the order of ∼0.003 $\$$/kg. The methods developed in this study could also be applied to the monitoring of groundwater, gas, and/or wastewater injection.
08 HYDROGEN↗
Concrete Testing Case for Closure of Handford’s 241-C Underground Storage Tanks
Sixty percent of the nation's highly toxic and radioactive mixed wastes are stored at Hanford in 177 deteriorating underground storage tanks. To close or remove these storage tanks from service and place them in a condition that is protective of human health and the environment, the tanks must be physically stabilized to prevent subsidence once wastes have been retrieved. Remaining residual liquid waste in the tanks that cannot be removed must be solidified and the solid wastes encapsulated to meet the Nuclear Regulatory Commission, Department of Energy, Environmental Protection Agency, and the State of Washington requirements. The Department of Energy has developed cementitious flowable concretes to restrict access and provide chemical stabilization for radionuclides. Formulation, laboratory, and field testing for application at Hanford began with flowable, self-leveling structural and non-structural fills. A slump flow equal to or greater than 610 mm, 0% bleed water, and 0.1% (by volume) shrinkage measurements were key parameters guiding reformulation efforts that resulted in highly flowable, self-consolidating concretes that met Hanford 241-C Tank closure short- and long-term regulatory and engineering performance requirements.
formula development↗
Permanent Closure of the TAN-680 Diesel Underground Storage Tank 98TAN00650 (DEQ Facility ID# 6-120618)
This closure package documents the site assessment and petitions for permanent closure of the Idaho National Laboratory (INL) Test Area North (TAN) diesel underground storage tank 98TAN00650 (DEQ Facility ID# 6-120618), in accordance with the regulatory requirements established in 40 CFR 280.71, “Permanent Closure and Changes-In-Service”.
02 PETROLEUM↗
Cyclic loading–unloading impacts on geomechanical stability of multiple salt caverns for underground hydrogen storage
Underground caverns in a salt dome are promising geologic features to store hydrogen because of salt’s extremely low permeability and self-healing behavior. The salt cavern storage community, however, has not fully understood the geomechanical behaviors of salt rock driven by quick operation cycles of injection–production, which may significantly impact the cost-effective storage-recovery performance of multiple caverns. Our field-scale generic model captures the impact of cyclic loading–unloading on the salt creep behavior and deformation under different cycle frequencies, operating pressure, and spatial order of operating cavern(s). This systematic simulation study indicates that the initial operation cycle and arrangement of multiple caverns play a significant role in the creep-driven loss of cavern volumes and cavern deformation. Finally, our future study will develop a new salt constitutive model based on geomechanical tests of site-specific salt rock to probe the cyclic behaviors of salt precisely both beneath and above the dilatancy boundary, including reverse (inverse transient) creep, the Bauschinger effect, and damage-healing mechanism.
08 HYDROGEN↗
Cyclic loading-unloading impacts on salt cavern stability: Implication for underground hydrogen storage
Underground caverns in salt formations are promising geologic features to store hydrogen (H2) because of salt’s extremely low permeability and self-healing behavior. Successful salt-cavern H2 storage schemes must maximize the efficiency of cyclic injection-production while minimizing H2 loss through adjacent damaged salt. The salt cavern storage community, however, has not fully understood the geomechanical behaviors of salt rocks driven by quick operation cycles of H2 injection-production, whic
Chang, Kyung Won↗
Evolution of Geomechanics for Underground Storage within Salt
Explore the source record for details and available documents.
Lord, Anna Snider↗
Sampling and Analysis Plan for LSL2 Underground Storage Tank Evaluation of PFAS in Soil: Protection of Groundwater
This SAP gathers all pertinent information relevant to the sampling and analysis of soil at the removal site for a former 10,000-gallon UST and reference sites in the vicinity of the excavation site. Data Quality Objectives establishes the process and steps for the acquisition of data. Data Flow Diagram establishes the decisions and next steps. Quality Assurance Project Plan establishes the quality requirements for data collection, including planning, implementation, and assessment of sampling, field measurements, and laboratory analysis. The work is being completed for DOE-SC Pacific Northwest Site Office.
12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗
Measurement of hydrogen relative permeabilities for underground storage in the Simpson Group formation - Anadarko Basin
Abstract for AGU26
03 NATURAL GAS↗
Characterizing Hydrogen Storage Potential in U.S. Underground Gas Storage Facilities
Abstract Underground hydrogen storage is a long‐duration energy storage option for a low‐carbon economy. Although research into the technical feasibility of underground hydrogen storage is ongoing, existing underground gas storage (UGS) facilities are appealing candidates for the technology because of their ability to store and deliver natural gas. We estimate that UGS facilities in the United States (U.S.) can store 327 TWh (9.8 MMT) of pure hydrogen. A complete transition to hydrogen storage would reduce the collective working‐gas energy of UGS facilities by ∼75%; however, most (73.2%) UGS facilities could maintain current energy demand using a 20% hydrogen‐natural gas blend. U.S. UGS facilities can buffer 23.9%–44.6% of the high and low hydrogen demand projected for 2050, respectively, which exceeds the current percentage of natural gas demand buffered by storage. Thus, transitioning UGS infrastructure to hydrogen could substantially reduce the number of new hydrogen storage facilities needed to support a hydrogen economy.
08 HYDROGEN↗
MR13A-3183: Microbial and Geochemical Characterization of Groundwater: Implications for Underground Hydrogen Storage Leakage
Underground hydrogen storage (UHS) in geological formations is a key element of the clean energy transition as it enables the decarbonization of the transportation and industrial sectors by decoupling hydrogen production and storage. UHS has many benefits, including low cost, much wider availability, large storage capacity, well-established infrastructure, and increased safety because of geological sealing capabilities. However, the impact of hydrogen (H2) biogeochemical interactions in the presence of subsurface microorganisms is largely neglected from UHS perspectives. These interactions might affect the effectiveness of storage and can even cause H2 to leak into the shallow aquifers. Leakage of H2 into groundwater can change the geochemistry and induce several microbial-driven processes. Microorganisms, such as sulfate-reducers, are naturally abundant in groundwater and consume H2 to produce hydrogen sulfide (H2S), which can contaminate the freshwater drinking groundwater and cause damage to infrastructure. Hydrogen leakage can also trigger microbial reactions responsible for metal mobility, which can impact the water quality. However, the kinetics of these reactions and the temporal impact of hydrogen leakage in groundwater are still unknown. Therefore, a time series hydrogen-groundwater interaction experiment was conducted, and the changes in fluid chemistry and headspace gas composition will be analyzed along with DNA sequencing results to understand the extent and kinetics of biogeochemical reactions that occur if hydrogen leaks into groundwater. In the experiments, Ultra High Purity (UHP) hydrogen gas will be injected into glass vials with groundwater samples, for a designated time period. For each glass-sealed vial, 16S rRNA gene sequencing, IC, ICP-MS, and GC-TCD will be performed. The experiments provide insights into plausible impacts of hydrogen leakage into shallow drinking water aquifers.
Clark, Allison [West Virginia University (WVU)]↗
Hydrogen Storage for Flexible Fossil Fuel Power Generation: Integration of Underground Hydrogen Storage with Gas Turbine (Final Report)
As the nation continues to encourage, through market structures and financial incentives, the proliferation of intermittent renewable electricity, how to optimize the ever-changing electric grid and identify means to retain and improve resilience, while ensuring continued reductions in GHG emissions, will be critical. According to Bloomberg, wind & solar generated 10.5% of US electricity in 2020 and that percentage continues to grow. In support of expanding renewable energy use, and to address its intermittent nature, this project will develop the Hydrogen Storage for Flexible Fossil Fuel Power Generation platform that is dispatchable, reliable, repeatable and have the ability to produce zero or negative carbon power while interfacing with geology capable of CO2 and hydrogen storage. GTI Energy (GTIE) and team members Illinois State Geological Survey (ISGS), Mitsubishi Heavy Industries America (MHIA), Ameren Illinois, Hexagon Purus, and the Low Carbon Resources Initiative (LCRI) completed a Phase I Conceptual Study under contract DE-FE0032012 for Hydrogen Storage for Flexible Fossil Fuel Power Generation: Integration of Underground Hydrogen Storage with Gas Turbine. The Hydrogen Storage for Flexible Fossil Fuel Power Generation platform addresses the intermittent nature of the expanding use of Variable Renewable Energy (VRE) generation. The low cost of the electricity (COE) generated results in greater dispatch and more operation at higher power levels (higher efficiency), fewer short intervals, and fewer start/stop cycles. The reliable, resilient system can produce zero carbon power and store hydrogen. It will demonstrate hydrogen storage in geologic formations like those used in natural gas underground storage thus enabling large scale storage of hydrogen in sedimentary strata across the United States rather than in geographically restricted salt caverns. The Phase I study confirmed the system is feasible and generates power at lower cost than other low carbon approaches. The demonstration defines the pathway for broad commercial application and will accelerate the development of larger systems suitable for centralized utility scale electricity production. The study advanced the maturity of the H 2 storage-based system with flexible power generation by completing a Pre-FEED study (Phase II). The Pre-FEED focused on the selected Energy Farm on the University of Illinois Urbana-Champaign (UIUC) site that includes above ground and underground hydrogen storage, low-carbon hydrogen production (GTI’s Compact Hydrogen Generator, CHG) with underground CO2 sequestration, and a 40-MW class gas turbine. The Pre-FEED addressed the entire system and its interconnection to the natural gas and electric grid and mitigation of key risks, such as storage behavior, load-following, and system operation. During Phase 1 of the project, the team completed key tasks, which moved the entire demonstration project, specific components and approaches closer to commercialization. These Phase I Accomplishments include: Completing System Requirements Review; Completing System Layout and Modeling - Heat & Mass Balance and Process Flow Diagram; Completing modelling of 9 turbine performance cases; Evaluating rock strata for underground storage of hydrogen and sequestration of carbon dioxide; Completing initial modelling of underground storage of hydrogen and withdrawal with evaluation of loss and water production; Identifying roadable storage for above ground hydrogen storage; Identifying existing electrical infrastructure for receiving/delivering electricity; Identifying existing gas supply infrastructure for receiving natural gas; Document concept design/development plans in required reports. Conclusions: The 12-month Feasibility study in Phase I study was completed and confirmed the system is feasible and generates power at lower cost than other low carbon approaches and even lower cost than the reference NGCC plant without carbon capture when taking advantage of 45Q carbon credits. The study enabled the fidelity of the concept to be improved and allowed identification of the requirements for the system. Defining the individual system and component requirements was performed via the system requirements review with the whole team. These requirements were then incorporated into and iterated with our Heat & Mass Balance process model and process flow diagrams were generated to reflect the overall system. This information was then used to complete the TEA and show economic feasibility. Large scale non-salt geologic storage of hydrogen is an enabling technology for a hydrogen-fired turbine that can be retrofitted into large-scale electric generating units (EGU). Our demonstration will include 428 MWh or ~4 hours full load of hydrogen storage (above and underground). Carbon capture inherent to the CHG process can capture 90% CO 2 (with upgrades to >98%). This system provides a COE of 23% savings relative to an NGCC with a post combustion amine system. Our proposed storage system decouples carbon capture and hydrogen production from power production; therefore, we expect our proposed system’s efficiency and variable COE to be superior resulting in overall higher dispatch and reduced deep cycling. Our demonstration will be full to multi-day hydrogen storage and has the potential for longer (seasonal) duration commercially. The demonstration defines the pathway for broad commercial application and will accelerate the development of larger systems suitable for centralized utility scale electricity production.
03 NATURAL GAS↗
Risk Assessment Considerations for Underground Hydrogen Storage in Depleted Gas Reservoirs
Underground hydrogen storage (UHS) in depleted reservoirs presents a promising solution for large-scale energy storage as hydrogen demand grows. As the UHS industry emerges, robust risk assessments are critical to ensuring safe operation of the storage facilities and minimizing the risk of accidents. This work explores risk assessment protocols for underground natural gas storage (UGS) in depleted reservoirs and identifies key considerations for repurposing these facilities for UHS. By examining the differences in physical and chemical properties between hydrogen and natural gas, this work highlights new and modified hazards that merits a reevaluation of traditional natural gas risk assessment practices. This investigation synthesizes insights from previous literature reviews and interviews with UGS industry experts and operators to identify key areas for adapting risk assessment methodologies for hydrogen. The insights gleaned from expert interviews indicate that existing risk assessment standards are non-prescriptive, leading to diverse company-specific risk assessment methodologies requiring substantial additions to become practical. Due to a lack of concrete risk assessment requirements, experience, and relevant data, this uncertainty is expected to be magnified considerably when considering hydrogen. This study identifies several areas for potential modification of existing risk assessment practices that could be considered by those developing standards or performing risk assessments for UHS. Specifically, risk assessments may be improved by including risks unique to hydrogen in existing standards, changing the magnitude of different risk factors in existing risk assessment protocols, and improving methods of data collection and communication across the industry to address large areas of uncertainty.
08 HYDROGEN↗