DOE OSTI2023
The Sum-of-Fractions method is a technique used to assure that homogeneous mixtures of fissile and fissionable isotopes are below a minimum margin of k eff or reactivity. Current work by Pacific Northwest National Laboratory examines different mixtures of 233 U, 235 U, and 239 Pu to determine critical mass limits for mixtures of transuranic actinides lacking a validation basis. To provide a validation basis for these limits, the work presented here describes the results of a sensitivity and uncertainty analysis of various mixtures of these isotopes in various concentrations moderated and reflected by light water and polyethylene. The TSUNAMI-1D sequence in the SCALE code system was used to generate sensitivity coefficients for three different concentrations of mixtures of 233 U, 235 U, and 239 Pu. The TSUNAMI-IP sequence was then used for similarity assessment (c k ) with critical benchmark experiment sensitivity data files (SDFs) from the Oak Ridge National Laboratory Verified, Archived Library of Inputs and Data and the Nuclear Energy Agency SDF database. The VADER sequence in SCALE was used for statistical testing and to generate upper subcritical limits from the data to develop a basis for validating critical mass limits.
07 ISOTOPE AND RADIATION SOURCES↗