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Results for “XUV-assisted HHG”

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Extended quantitative rescattering model for simulating high-order harmonic streaking spectra by synchronization of an intense IR laser and a time-delayed attosecond XUV pulse

In this work, we theoretically investigate the modulated high-harmonic generation (HHG) driven by an intense few-cycle infrared (IR) laser field and a weak extreme-ultraviolet (XUV) pulse at a delayed time. We establish an extended quantitative rescattering (EQRS) model to simulate the HHG streaking spectra, with the ideas of correcting the IR ionization and the transition from the ground to continuum states in the strong-field approximation. The EQRS model has an accuracy comparable to that from “exactly” solving the time-dependent Schrödinger equation (TDSE). We reveal that the fringes in the streaking spectra are caused by the interference between the attosecond XUV pulse and harmonics resulting from different recombination pathways under the intense IR laser. We then demonstrate that the XUV pulse can be accurately retrieved by treating the single-atom TDSE results or macroscopic propagation results as the “input” data. This work provides with a tool for efficiently simulating and thoroughly analyzing the XUV-assisted HHG, which could also enhance its capability for tracing the electron dynamics involved in the strong-field phenomena.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

High harmonic generation in mixed XUV and NIR fields at a free-electron laser

Abstract We present the results of an experiment investigating the generation of high-order harmonics by a femtosecond near-infrared (NIR) laser pulse in the presence of an extreme ultraviolet (XUV) field provided by a free-electron laser (FEL), a process referred to as XUV-assisted high-order harmonic generation (HHG). Our experimental findings show that the XUV field can lead to a small enhancement in the harmonic yield when the XUV and NIR pulses overlap in time, while a strong decrease of the HHG yield and a red shift of the HHG spectrum is observed when the XUV precedes the NIR pulse. The latter observations are in qualitative agreement with model calculations that consider the effect of a decreased number of neutral emitters but are at odds with the predicted effect of the correspondingly increased ionization fraction on the phase matching. Our study demonstrates the technical feasibility of XUV-assisted HHG experiments at FELs, which may provide new avenues to investigate correlation-driven electron dynamics as well as novel ways to study and control propagation effects and phase matching in HHG.

47 OTHER INSTRUMENTATION↗