Impact of Dynamic Oxidant Chemistry on GOCART Aerosols in GEOS-FP
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Patricia Castellanos↗
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Global- to Micro-Scale Evolution of the Pinatubo Aerosol: Using Composite Data Sets to Build the Picture and Assess Consistency of Different Measurements
This paper brings together experimental. evidence required to build realistic models of the global evolution of physical, chemical, and optical properties of the aerosol resulting from the 1991 Pinatubo volcanic eruption. Such models are needed to compute the effects of the aerosol on atmospheric chemistry, dynamics, radiation, and temperature. Whereas there is now a large and growing body of post-Pinatubo measurements by a variety of techniques, some results are in conflict, and a self-consistent, unified picture is needed, along with an assessment of remaining uncertainties. This paper examines data from photometers, radiometers, impactors, optical counters/sizers, and lidars operated on the ground, aircraft, balloons, and spacecraft.
Russell, P. B.↗
Pinatubo Aerosol Evolution: Using Composite Data Sets to Build the Global- To Micro-Scale Picture and Assess Consistency of Different Measurements
This paper brings together experimental evidence required to build realistic models of the global evolution of physical, chemical, and optical properties of the aerosol resulting from the 1991 Pinatubo volcanic eruption. Such models are needed to compute the effects of the aerosol on atmospheric chemistry, dynamics, radiation, and temperature. Whereas there is now a large and crowing body of post-Pinatubo measurements by a variety of techniques, some results are in conflict, and a self-consistent, unified picture is needed, along with an assessment of remaining uncertainties. This paper examines, data from photometers, radiometers, impactors, optical counter/sizers, and lidars operated on the ground, aircraft, balloons, and spacecraft. Example data sources include: (1) Tracking sunphotometers and lidars at Mauna Loa Observatory (MLO) and on the DC-8. (2) Particle spectrometers and wire impactors on the ER-2 and DC-8. (3) Dustsondes (particle counter/sizers on balloons). and (3) SAGE II, SAM II, AVHRR, CLAES, and ISAMS sensors on a variety of satellites. We assess the mutual consistency of these disparate data sets and recommend 'consensus' properties and uncertainties in the process of developing a composite data set. Recommended properties include the spatial and temporal evolution of particle chemical composition, shape, wavelength-and temperature-dependent refractive index, size distribution, and optical depth spectra. Supporting references are cited and representative data shown.
Russell, Philip B.↗
Pinatubo Aerosol Evolution: Using Composite Data Sets to Build the Global- to Micro-Scale Picture and Assess Consistency of Different Measurements
This paper brings together experimental evidence required to build realistic models of the global evolution of physical, chemical, and optical properties of the aerosol resulting from the 1991 Pinatubo volcanic eruption. Such models are needed to compute the effects of the aerosol on atmospheric chemistry, dynamics, radiation, and temperature. Whereas there is now a large and growing body of post-Pinatubo measurements by a variety of techniques, some results are in conflict, and a self-consistent, unified picture is needed, along with an assessment of remaining uncertainties. This paper examines data from photometers, radiometers, impactors, optical counters/sizers, and lidars operated on the ground, aircraft, balloons, and spacecraft. Example data sources include: - Tracking sunphotometers and lidars at Mauna Loa Observatory (MLO) and on the DC-8 - Particle spectrometers and wire impactors on the ER-2 and DC-8 - Dustsondes (particle counters/sizers on balloons) - SAGE II, SAM II, AVHRR, CLAES, and ISAMS sensors on a variety of satellites. We assess the mutual consistency of these disparate data sets and recommend 'consensus" properties and uncertainties in the process of developing a composite data set. Recommended properties include the spatial and temporal evolution of particle chemical composition, shape, wavelength and temperature-dependent refractive index, size distribution, and optical depth spectra. Supporting references are cited and representative data shown.
Russell, P. B.↗
The Joint Aerosol-Monsoon Experiment: A New Challenge to Monsoon Climate Research
Aerosol and monsoon related droughts and floods are two of the most serious environmental hazards confronting more than 60% of the population of the world living in the Asian monsoon countries. In recent years, thanks to improved satellite and in-situ observations, and better models, great strides have been made in aerosol, and monsoon research respectively. There is now a growing body of evidence suggesting that interaction of aerosol forcing with water cycle dynamics in monsoon regions may substantially alter the redistribution of energy at the earth surface and in the atmosphere, and therefore significantly impact monsoon rainfall variability and long term trends. In this talk, I will describe issues related to societal needs, scientific background, and challenges in studies of aerosol-water cycle interaction in Asian monsoon regions. As a first step towards addressing these issues, the authors call for an integrated observation and modeling research approach aimed at the interactions between aerosol chemistry and radiative effects and monsoon dynamics of the coupled ocean-atmosphere-land system. A Joint Aerosol-Monsoon Experiment (JAMEX) is proposed for 2007-2011, with an enhanced observation period during 2008-09, encompassing diverse arrays of observations from surface, aircraft, unmanned aerial vehicles, and satellites of physical and chemical properties of aerosols, long range aerosol transport as well as meteorological and oceanographic parameters in the Indo-Pacific Asian monsoon region. JAMEX will leverage on coordination among many ongoing and planned national programs on aerosols and monsoon research in China, India, Japan, Nepal, Italy, US, as well as international research programs of the World Climate Research Program (WCRP) and the World Meteorological Organization (WMO).
Lau, William K. M.↗
SAGE 1 data user's guide
A guide for using the data products from the Stratospheric Aerosol and Gas Experiment 1 (SAGE 1) for scientific investigations of stratospheric chemistry related to aerosol, ozone, nitrogen dioxide, dynamics, and climate change is presented. A detailed description of the aerosol profile tape, the ozone profile tape, and the nitrogen dioxide profile tape is included. These tapes are the SAGE 1 data products containing aerosol extinction data and ozone and nitrogen dioxide concentration data for use in the different scientific investigations. Brief descriptions of the instrument operation, data collection, processing, and validation, and some of the scientific analyses that were conducted are also included.
Mcmaster, Leonard R.↗
Coupled Aerosol-Chemistry-Climate Twentieth-Century Transient Model Investigation: Trends in Short-Lived Species and Climate Responses
The authors simulate transient twentieth-century climate in the Goddard Institute for Space Studies (GISS) GCM, with aerosol and ozone chemistry fully coupled to one another and to climate including a full dynamic ocean. Aerosols include sulfate, black carbon (BC), organic carbon, nitrate, sea salt, and dust. Direct and BC snow-albedo radiative effects are included. Model BC and sulfur trends agree fairly well with records from Greenland and European ice cores and with sulfur deposition in North America; however, the model underestimates the sulfur decline at the end of the century in Greenland. Global BC effects peak early in the century (1940s); afterward the BC effects decrease at high latitudes of the Northern Hemisphere but continue to increase at lower latitudes. The largest increase in aerosol optical depth occurs in the middle of the century (1940s-80s) when sulfate forcing peaks and causes global dimming. After this, aerosols decrease in eastern North America and northern Eurasia leading to regional positive forcing changes and brightening. These surface forcing changes have the correct trend but are too weak. Over the century, the net aerosol direct effect is -0.41 Watts per square meter, the BC-albedo effect is -0.02 Watts per square meter, and the net ozone forcing is +0.24 Watts per square meter. The model polar stratospheric ozone depletion develops, beginning in the 1970s. Concurrently, the sea salt load and negative radiative flux increase over the oceans around Antarctica. Net warming over the century is modeled fairly well; however, the model fails to capture the dynamics of the observedmidcentury cooling followed by the late century warming.Over the century, 20% of Arctic warming and snow ice cover loss is attributed to the BC albedo effect. However, the decrease in this effect at the end of the century contributes to Arctic cooling. To test the climate responses to sulfate and BC pollution, two experiments were branched from 1970 that removed all pollution sulfate or BC. Averaged over 1970-2000, the respective radiative forcings relative to the full experiment were +0.3 and -0.3 Watts per square meter; the average surface air temperature changes were +0.2 degrees and -0.03 C. The small impact of BC reduction on surface temperature resulted from reduced stability and loss of low-level clouds.
Koch, Dorothy↗
SAGE 2 satellite data set validation
The results of a validation study of data obtained by the Stratospheric Aerosol and Gas Experiment 2 satellite experiment (SAGE 2) are given. Preliminary SAGE 2 data have been available for the period October, 1984 to May, 1985. In addition, the results of two correlative experimental measurement series have been studied in detail, as well as climatological data obtained by other techniques, including ground-based and airborne lidar. The study shows the SAGE 2 data to be of great potential value to studies of the microphyiscs of stratospheric aerosols, the chemistry of trace gases and stratospheric dynamics. A small number of unidentified errors in the current preliminary data set are described. These will be removed from the next version of the data set which is anticipated to be of archival quality.
Kent, G. S.↗
Atmospheric Research 2014 Technical Highlights
Atmospheric research in the Earth Sciences Division (610) consists of research and technology development programs dedicated to advancing knowledge and understanding of the atmosphere and its interaction with the climate of Earth. The Division's goals are to improve understanding of the dynamics and physical properties of precipitation, clouds, and aerosols; atmospheric chemistry, including the role of natural and anthropogenic trace species on the ozone balance in the stratosphere and the troposphere; and radiative properties of Earth's atmosphere and the influence of solar variability on the Earth's climate. Major research activities are carried out in the Mesoscale Atmospheric Processes Laboratory, the Climate and Radiation Laboratory, the Atmospheric Chemistry and Dynamics Laboratory, and the Wallops Field Support Office. The overall scope of the research covers an end-to-end process, starting with the identification of scientific problems, leading to observation requirements for remote-sensing platforms, technology and retrieval algorithm development; followed by flight projects and satellite missions; and eventually, resulting in data processing, analyses of measurements, and dissemination from flight projects and missions. Instrument scientists conceive, design, develop, and implement ultraviolet, infrared, optical, radar, laser, and lidar technology to remotely sense the atmosphere. Members of the various Laboratories conduct field measurements for satellite sensor calibration and data validation, and carry out numerous modeling activities. These modeling activities include climate model simulations, modeling the chemistry and transport of trace species on regional-to-global scales, cloud resolving models, and developing the next-generation Earth system models. Satellite missions, field campaigns, peer-reviewed publications, and successful proposals are essential at every stage of the research process to meeting our goals and maintaining leadership of the Earth Sciences Division in atmospheric science research. Figure 1.1 shows the 20-year record of peer-reviewed publications and proposals among the various Laboratories. This data shows that the scientific work being conducted in the Laboratories is competitive with the work being done elsewhere in universities and other government agencies. The office of Deputy Director for Atmospheric Research will strive to maintain this record by rigorously monitoring and promoting quality while emphasizing coordination and integration among atmospheric disciplines. Also, an appropriate balance will be maintained between the scientists' responsibility for large collaborative projects and missions and their need to carry out active science research as a principal investigator. This balance allows members of the Laboratories to improve their scientific credentials, and develop leadership potentials. Interdisciplinary research is carried out in collaboration with other laboratories and research groups within the Earth Sciences Division, across the Sciences and Exploration Directorate, and with partners in universities and other government agencies. Members of the Laboratories interact with the general public to support a wide range of interests in the atmospheric sciences. Among other activities, the Laboratories raise the public's awareness of atmospheric science by presenting public lectures and demonstrations, by making scientific data available to wide audiences, by teaching, and by mentoring students and teachers. The Atmosphere Laboratories make substantial efforts to attract and recruit new scientists to the various areas of atmospheric research. We strongly encourage the establishment of partnerships with Federal and state agencies that have operational responsibilities to promote the societal application of our science products. This report describes our role in NASA's mission, provides highlights of our research scope and activities, and summarizes our scientists' major accomplishments during calendar year 2014. The composition of the organization is shown in Figure 1.2 for each code. This report is published in a printed version with an electronic version on our atmospheres Web site, http://atmospheres.gsfc.nasa.gov/.
Technical↗
Atmospheric Research 2016 Technical Highlights
Atmospheric research in the Earth Sciences Division (610) consists of research and technology development programs dedicated to advancing knowledge and understanding of the atmosphere and its interaction with the climate of Earth. The Divisions goals are to improve understanding of the dynamics and physical properties of precipitation, clouds, and aerosols; atmospheric chemistry, including the role of natural and anthropogenic trace species on the ozone balance in the stratosphere and the troposphere; and radiative properties of Earth's atmosphere and the influence of solar variability on the Earth's climate. Major research activities are carried out in the Mesoscale Atmospheric Processes Laboratory, the Climate and Radiation Laboratory, the Atmospheric Chemistry and Dynamics Laboratory, and the Wallops Field Support Office. The overall scope of the research covers an end-to-end process, starting with the identification of scientific problems, leading to observation requirements for remote-sensing platforms, technology and retrieval algorithm development; followed by flight projects and satellite missions; and eventually, resulting in data processing, analyses of measurements, and dissemination from flight projects and missions. Instrument scientists conceive, design, develop, and implement ultraviolet, infrared, optical, radar, laser, and lidar technology to remotely sense the atmosphere. Members of the various laboratories conduct field measurements for satellite sensor calibration and data validation, and carry out numerous modeling activities. These modeling activities include climate model simulations, modeling the chemistry and transport of trace species on regional-to-global scales, cloud resolving models, and developing the next-generation Earth system models. Satellite missions, field campaigns, peer-reviewed publications, and successful proposals are essential at every stage of the research process to meeting our goals and maintaining leadership of the Earth Sciences Division in atmospheric science research. Figure 1.1 shows the 22-year record of peer-reviewed publications and proposals among the various laboratories.
Atmospheric↗
Atmospheric Research 2018 Technical Highlights
Atmospheric research in the Earth Sciences Division (610) consists of research and technology development programs dedicated to advancing knowledge and understanding of the atmosphere and its interaction with the climate of Earth. The Division’s goals are to improve understanding of the dynamics and physical properties of precipitation, clouds, and aerosols; atmospheric chemistry, including the role of natural and anthropogenic trace species on the ozone balance in the stratosphere and the troposphere; and radiative properties of Earth’s atmosphere and the influence of solar variability on the Earth’s climate. Major research activities are carried out in the Mesoscale Atmospheric Processes Laboratory, the Climate and Radiation Laboratory, the Atmospheric Chemistry and Dynamics Laboratory, and the Wallops Field Support Office. The overall scope of the research covers an end-to-end process, starting with the identification of scientific problems, leading to observation requirements for remote sensing platforms, technology and retrieval algorithm development; followed by flight projects and satellite missions; and eventually, resulting in data processing, analyses of measurements, and dissemination from flight projects and missions.
Highlights↗
Retrieval of Aerosol Properties from Multi-Spectral Extinction Measurements
The direct-beam spectral extinction of solar radiation contains information on atmospheric composition in a form that is essentially free from the data analysis complexities that often arise from multiple scattering. Ground based Multi-Filter Shadowband Radiometer (MFRSR) measurements provide such information for the vertical atmospheric column path, while solar occultation measurements from a satellite platform provide horizontal slices through the atmosphere. We describe application of a Multi-Spectral Atmospheric Column Extinction (MACE) analysis technique used to analyze MFRSR data also to occultation measurements made by SAGE II. For analysis, we select the 1985 Nevado del Ruiz volcanic eruption period to retrieve atmospheric profiles of ozone and NO2, and changes in the stratospheric aerosol size and optical depth. The time evolution of volcanic aerosol serves as a passive tracer to study stratospheric dynamics, and changes in particle size put constraints on the sulfur chemistry modeling of volcanic aerosols. Paper presented at The '99 Kyoto Aerosol-Cloud Workshop, held Dec 1-3, 1999, Kyoto, Japan
Lacis, Andrew A.↗
Retrieval of Aerosol Properties from Multi-Spectral Extinction Measurements
The direct-beam spectral extinction of solar radiation contains information on atmospheric composition in a form that is essentially free from the data analysis complexities that often arise from multiple scattering. Ground based Multi-Filter Shadowband Radiometer (MFRSR) measurements provide such information for the vertical atmospheric column path, while solar occultation measurements from a satellite platform provide horizontal slices through the atmosphere. We describe application of a Multi-Spectral Atmospheric Column Extinction (MACE) analysis technique used to analyze MFRSR data also to occultation measurements made by SAGE 11. For analysis, we select the 1985 Nevado del Ruiz volcanic eruption period to retrieve atmospheric profiles of ozone and NO2, and changes in the stratospheric aerosol size and optical depth. The time evolution of volcanic aerosol serves as a passive tracer to study stratospheric dynamics, and changes in particle size put constraints on the sulfur chemistry modeling of volcanic aerosols.
Lacis, Andrew A.↗
Developing a Model-based Capability to Analyze Requirements for the Climate Observing System
Models are foundational for estimating states of the earth's climate system, both as tools to extrapolate information in time and space, and as observation 'operators' used to relate what is analyzed and predicted to what is observed. Expanding the simulation approach further, observing system simulation experiments (OSSEs) are designed to mimic the complete process of analyzing the climate state by replacing real observations with entirely simulated ones determined from a model-based depiction of nature. OSSEs provide a framework to 'fly' simulated satellite instruments through a synthetic atmosphere and investigate the trade-spaces of measurements for various satellite configurations and sampling strategies, and assess their measurement impact on modeling and forecasting capabilities. Such a tool is a crucial but as yet unfulfilled need for future mission selection and design. The components of a state-of-the-art OSSE system are being assembled at the Global Modeling and Assimilation Office (GMAO, Code 610.1) at NASA/GSFC, leveraging on the GMAO's existing modeling and data assimilation infrastructure for numerical weather prediction (NWP). The OSSE framework is based on the GMAO's Goddard Earth Observing System atmospheric general circulation model, version 5 (GEOS-5) and the Gridpoint Statistical Interpolation (GSI) observational analysis scheme, combined with the Goddard Chemistry, Aerosol, Radiation, and Transport (GOCART) model developed by the Atmospheric Chemistry and Dynamics Branch (Code 613.3). This system is an evolving, key component of Goddard's planned development of an Integrated Earth System Analysis (IESA) capability, which will bring together into a single, fully interactive system Goddard's modeling and assimilation efforts in atmosphere, ocean and chemistry and aerosols to provide a comprehensive analysis and prediction system for weather and climate In addition to providing a state-of-the-art capability for assimilating current observation types, GEOS-5, and the future IESA, provide the capability to identify the need for, and assess the potential impact of, future observing systems under consideration for improving weather and climate prediction.
Gelaro, Ronald↗
Connecting Regional Aerosol Emissions Reductions to Local and Remote Precipitation Responses
The unintended climatic implications of aerosol and precursor emission reductions implemented to protect public health are poorly understood. We investigate the precipitation response to regional changes in aerosol emissions using three coupled chemistry-climate models: NOAA Geophysical Fluid Dynamics Laboratory Coupled Model 3 (GFDL-CM3), NCAR Community Earth System Model (CESM1), and NASA Goddard Institute for Space Studies ModelE2 (GISS-E2). Our approach contrasts a long present-day control simulation from each model (up to 400 years with perpetual year 2000 or 2005 emissions) with 14 individual aerosol emissions perturbation simulations (160-240 years each). We perturb emissions of sulfur dioxide and/or carbonaceous aerosol within six world regions and assess the significance of precipitation responses relative to internal variability determined by the control simulation and across the models. Global and regional precipitation mostly increases when we reduce regional aerosol emissions in the models, with the strongest responses occurring for sulfur dioxide emissions reductions from Europe and the United States. Precipitation responses to aerosol emissions reductions are largest in the tropics and project onto the El Nino Southern Oscillation (ENSO). Regressing precipitation onto an Indo-Pacific zonal sea level pressure gradient index (a proxy for ENSO) indicates that the ENSO component of the precipitation response to regional aerosol removal can be as large as 20% of the total simulated response. Precipitation increases in the Sahel in response to aerosol reductions in remote regions because an anomalous interhemispheric temperature gradient alters the position of the Intertropical Convergence Zone (ITCZ). This mechanism holds across multiple aerosol reduction simulations and models.
Westervelt, Daniel M.↗
Laboratory for Atmospheres 2008 Technical Highlights
The 2008 Technical Highlights describes the efforts of all members of the Laboratory for Atmospheres. Their dedication to advancing Earth Science through conducting research, developing and running models, designing instruments, managing projects, running field campaigns, and numerous other activities, is highlighted in this report. The Laboratory for Atmospheres (Code 613) is part of the Earth Sciences Division (Code 610), formerly the Earth Sun Exploration Division, under the Sciences and Exploration Directorate (Code 600) based at NASA s Goddard Space Flight Center in Greenbelt, Maryland. In line with NASA s Exploration Initiative, the Laboratory executes a comprehensive research and technology development program dedicated to advancing knowledge and understanding of the atmospheres of Earth and other planets. The research program is aimed at understanding the influence of solar variability on the Earth s climate; predicting the weather and climate of Earth; understanding the structure, dynamics, and radiative properties of precipitation, clouds, and aerosols; understanding atmospheric chemistry, especially the role of natural and anthropogenic trace species on the ozone balance in the stratosphere and the troposphere; and advancing our understanding of physical properties of Earth s atmosphere. The research program identifies problems and requirements for atmospheric observations via satellite missions. Laboratory scientists conceive, design, develop, and implement ultraviolet, infrared, optical, radar, laser, and lidar technology for remote sensing of the atmosphere. Laboratory members conduct field measurements for satellite data calibration and validation, and carry out numerous modeling activities. These modeling activities include climate model simulations, modeling the chemistry and transport of trace species on regional-to-global scales, cloud-resolving models, and development of next-generation Earth system models. Interdisciplinary research is carried out in collaboration with other laboratories and research groups within the Earth Sciences Division, across the Sciences and Exploration Directorate, and with partners in universities and other Government agencies. The Laboratory for Atmospheres is a vital participant in NASA s research agenda. Our Laboratory often has relatively large programs, sizable satellite missions, and observational campaigns that require the cooperative and collaborative efforts of many scientists. We ensure an appropriate balance between our scientists responsibility for these large collaborative projects and their need for an active individual research agenda. This balance allows members of the Laboratory to continuously improve their scientific credentials. Members of the Laboratory interact with the general public to support a wide range of interests in the atmospheric sciences. Among other activities, the Laboratory raises the public s awareness of atmospheric science by presenting public lectures and demonstrations, by making scientific data available to wide audiences, by teaching, and by mentoring students and teachers. The Laboratory makes substantial efforts to attract new scientists to the various areas of atmospheric research. We strongly encourage the establishment of partnerships with Federal and state agencies that have operational responsibilities to promote the societal application of our science products. This report describes our role in NASA s mission, gives a broad description of our research, and summarizes our scientists major accomplishments during calendar year 2008. The report also contains useful information on human resources, scientific interactions, and outreach activities.
Cote, Charles E.↗
An Aerosol Physical Chemistry Model for the Upper Troposphere
This report is the final report for the Cooperative Agreement NCC2-1000. The tasks outlined in the various proposals are: (1) Development of an aerosol chemistry model; (2) Utilization of satellite measurements of trace gases along with analysis of temperatures and dynamic conditions to understand ice cloud formation, dehydration and sedimentation in the winter polar regions; (3) Comparison of the HALOE and SAGE II time dependencies of the Pinatubo aerosol decay. The publications are attached.
Lin, Jin-Sheng↗
Differential Absorption Lidar (DIAL) Measurements from Air and Space
Differential absorption lidar (DIAL) systems have been used for the measurement of ozone, water vapor, and aerosols from aircraft platforms for over 18 years, yielding new insights into atmospheric chemistry, composition, and dynamics in large-scale field experiments conducted all over the world. The successful deployment of the lidar in-space technology experiment (LITE) in September 1994 demonstrated that space-based lidars can also collect valuable information on the global atmosphere. This paper reviews some of the contributions of the NASA Langley Research Center's airborne ozone and water vapor DIAL systems and space-based LITE system to the understanding of the atmosphere and discusses the feasibility and advantages of putting DIAL systems in space for routine atmospheric measurements of ozone and/or water vapor and aerosols and clouds. The technology and applications of the differential absorption lidar (DIAL) technique have progressed significantly since the first DIAL measurements of Schotland, and airborne DIAL measurements of ozone and water vapor are frequently being made in a wide range of field experiments. In addition, plans are underway to develop DIAL systems for use on satellites for continuous global measurements. This paper will highlight the history of airborne lidar and DIAL systems, summarize the major accomplishments of the NASA Langley DIAL program, and discuss specifications and goals for DIAL systems in space.
Browell, E. V.↗