Determination of aerosol size distributions from lidar measurements
Aerosol size distribution from lidar light scattering polarization properties, constructing inversion model
Browning, S. R.↗
SEARCH · Search NASA
Results for “aerosol size distribution”
Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.
Quote a phrase for an exact phrase match. Source license links do not imply unrestricted reuse.
Aerosol size distribution, composition, and CO2 backscatter
The aerosol size distribution, composition, and CO2 backscatter at 10.6 microns (beta-CO2) were measured continuosly at the Mauna Loa Observatory (Hawaii) during January-March and November-December, 1988 periods to compare the characteristics of periods associated with appreciable Asian dust transport to that site (January-March) with those of periods characterized by low-dust condition. The aerosol size distribution in the range 0.15 micron to 7.6 microns was measured at temperatures of 40, 150, and 340 C to differentiate between volatile and nonvolatile aerosols. Large ranges of variability was found in measurements of aerosol size distribution during both periods, but the average distributions were similar for both the high-dust and the low-dust periods. However, values for beta-CO2 were more elevated (by about six times) during periods associated with active Asian dust transport to the observatory site than during the low-dust periods.
Clarke, Antony D.↗
A diagnostic stratospheric aerosol size distribution inferred from SAGE II measurements
An aerosol size distribution model for the stratosphere is inferred based on 5 years of Stratospheric Aerosol and Gas Experiment (SAGE) II measurements of multispectral aerosol and water vapor extinction. The SAGE II aerosol and water vapor extinction data strongly suggest that there is a critical particle radius below which there is a relatively weak dependence of particle number density with size and above which there are few, if any, particles. A segmented power law model, as a simple representation of this dependence, is used in theoretical calculations and intercomparisons with a variety of aerosol measurements including dustsondes, longwave lidar, and wire impactors and shows a consistently good agreement.
Thomason, Larry W.↗
Three optical methods for remotely measuring aerosol size distributions.
Three optical probing methods for remotely measuring atmospheric aerosol size distributions are discussed and contrasted. The particular detection methods which are considered make use of monostatic lidar (laser radar), bistatic lidar, and solar radiometer sensing techniques. The theory of each of these measurement techniques is discussed briefly, and the necessary constraints which must be applied to obtain aerosol size distribution information from such measurements are pointed out. Theoretical and/or experimental results are also presented which demonstrate the utility of the three proposed probing methods.
Reagan, J. A.↗
Retrieval of stratospheric aerosol size distribution from atmospheric extinction of solar radiation at two wavelengths
A parametric study is presented of the effects of the size distribution and composition of stratospheric aerosols on the value R, the ratio of the extinction of solar radiation at wavelength 0.45 micron to the extinction at wavelength 1.0 micron. The aerosol size distributions under study comprise nine analytical expressions, including most of the stratospheric aerosol models used by investigators. The aerosol compositions considered are the supercooled sulfuric-acid droplets, with different weight percentages of H2SO4 in the aerosol. It is found that whereas R is not very sensitive to either the composition or the radii limits of the stratospheric aerosols under consideration, it is quite sensitive to the value of the variable parameter governing the mode radius of the size distribution of aerosol particles. The results of the parametric study underlie the method proposed here of retrieving the size distribution of aerosol particles in the stratosphere from the experimental results of the extinction of solar radiation at two wavelengths.
Yue, G. K.↗
Analytic modeling of aerosol size distributions
Mathematical functions commonly used for representing aerosol size distributions are studied parametrically. Methods for obtaining best fit estimates of the parameters are described. A catalog of graphical plots depicting the parametric behavior of the functions is presented along with procedures for obtaining analytical representations of size distribution data by visual matching of the data with one of the plots. Examples of fitting the same data with equal accuracy by more than one analytic model are also given.
Deepack, A.↗
Retrieval of aerosol size distribution moments from multiwavelength particulate extinction measurements
Two methods for inferring aerosol size distribution moments from multiwavelength particulate extinction measurements are studied. The methods are an eigenvalue technique that approximates an appropriate moment-weighting function by a linear combination of kernel functions and a conversion ratio approach that uses the ratio of the particulate extinction measurements at two wavelengths to choose a model moment-to-extinction conversion ratio. The techniques are applied to infer the third moment, or volume, of the aerosol size distribution from actual particulate extinction measurements taken as part of the Stratospheric Aerosol and Gas Experiment II during a correlative measurement experiment in Brazil in April 1985.
Livingston, John M.↗
Aerosol size distributions obtained by inversion of spectral optical depth measurements
Columnar aerosol size distributions have been inferred by numerically inverting particulate optical depth measurements as a function of wavelength. An inversion formula which explicitly includes the magnitude of the measurement variances is derived and applied to optical depth measurements obtained in Tucson with a solar radiometer. It is found that the individual size distributions of the aerosol particles (assumed spherical), at least for radii greater than or approximately equal to 0.1 micron, fall into one of three distinctly different categories. Approximately 50% of all distributions examined thus far can best be represented as a composite of a Junge distribution plus a distribution of relatively monodispersed larger particles centered at a radius of about 0.5 micron. Scarcely 20% of the distributions yielded Junge size distributions, while 30% yielded relatively monodispersed distributions of the log-normal or gamma distribution types. A representative selection of each of these types will be presented and discussed. The sensitivity of spectral attenuation measurements to the radii limits and refractive index assumed in the numerical inversion will also be addressed.
King, M. D.↗
In Situ Aerosol Size Distributions and Clear Column Radiative Closure During ACE-2
As part of the second Aerosol Characterization Experiment (ACE-2) during June and July of 1997, aerosol size distributions were measured on board the CIRPAS Pelican aircraft through the use of a DMA and two OPCS. During the campaign, the boundary layer aerosol typically possessed characteristics representative of a background marine aerosol or a continentally influenced aerosol, while the free tropospheric aerosol was characterized by the presence or absence of a Saharan dust layer. A range of radiative closure comparisons were made using the data obtained during vertical profiles flown on four missions. Of particular interest here are the comparisons made between the optical properties as determined through the use of measured aerosol size distributions and those measured directly by an airborne 14-wavelength sunphotometer and three nephelometers. Variations in the relative humidity associated with each of the direct measurements required consideration of the hygroscopic properties of the aerosol for size distribution based calculations. Simultaneous comparison with such a wide range of directly measured optical parameters not only offers evidence of the validity of the physicochemical description of the aerosol when closure is achieved, but also provides insight into potential sources of error when some or all of the comparisons result in disagreement. Agreement between the derived and directly measured optical properties varied for different measurements and for different cases. Averaged over the four case studies, the derived extinction coefficient at 525 nm exceeded that measured by the sunphotomoter by 2.5% in the clean boundary later, but underestimated measurements by 13% during pollution events. For measurements within the free troposphere, the mean derived extinction coefficient was 3.3% and 17% less than that measured by the sunphotometer during dusty and nondusty conditions, respectively. Likewise, averaged discrepancies between the derived and measured scattering coefficient were -9.6%, +4.7%, +17%, and -41% for measurements within the clean boundary layer, polluted boundary layer, free troposphere with a dust layer, and free troposphere without a dust layer, respectively. Each of these quantities, as well as the majority of the > 100 individual comparisons from which they were averaged, were within estimated uncertainties.
Collins, D. R.↗
Aerosol size distributions - Remote determination from air-borne measurements of the solar aureole
Aerosol-size distributions were determined remotely using an airborne scanning photometer. This instrument consists of a sunshade, optics, and a large-dynamic-range photodetector-amplifier system that scans about the vertical, recording both the direct attenuated solar beam and the diffuse sky radiance in the almucantar of the sun at an effective wavelength of 0.54 micron. Inversion of the measured radiances determined aerosol radii from approximately 0.2 to 8.0 microns. Data were taken during flights over western Lake Superior and southwestern Wisconsin. Inverted aerosol-size distributions are compared with results obtained by other methods.
Twitty, J. T.↗
In Situ Aerosol-Size Distributions and Clear-Column Radiative Closure During ACE-2
As part of the second Aerosol Characterization Experiment (ACE-2) during June and July of 1997, aerosol-size distributions were measured on board the CIRPAS Pelican aircraft through the use of a Differential Mobility Analyzer (DMA) and 2 Optical Particle Counters (OPCs). During the campaign, the boundary-layer aerosol typically possessed characteristics representative of a background marine aerosol or a continentally influenced aerosol, while the free-tropospheric aerosol was characterized by the presence or absence of a Saharan dust layer. A range of radiative closure comparisons were made using the data obtained during vertical profiles flown on 4 missions. Of particular interest here are the comparisons made between the optical properties as determined through the use of measured aerosol-size distributions and those measured directly by an airborne 14-wavelength sunphotometer and 3 nephelometers. Variations in the relative humidity associated with each of the direct measurements required consideration of the hygroscopic properties of the aerosol for size-distribution-based calculations. Simultaneous comparison with such a wide range of directly-measured optical parameters not only offers evidence of the validity of the physicochemical description of the aerosol when closure is achieved, but also provides insight into potential sources of error when some or all of the comparisons result in disagreement. Agreement between the derived and directly-measured optical properties varied for different measurements and for different cases. Averaged over the 4 case studies, the derived extinction coefficient at 525 nm exceeded that measured by the sunphotometer by 2.5% in the clean boundary layer, but underestimated measurements by 13% during pollution events. For measurements within the free troposphere, the mean derived extinction coefficient was 3.3% and 17% less than that measured by the sunphotometer during dusty and non-dusty conditions, respectively. Likewise, averaged discrepancies between the derived and measured scattering coefficient were -9.6%, +4.7%, +17%, and -41% for measurements within the clean boundary layer, polluted boundary layer, free troposphere with a dust layer, and free troposphere without a dust layer, respectively. Each of these quantities, as well as the majority of the more than 100 individual comparisons from which they were averaged, were within estimated uncertainties.
Collins, R.↗
The Angstrom Exponent and Bimodal Aerosol Size Distributions
Powerlaws have long been used to describe the spectral dependence of aerosol extinction, and the wavelength exponent of the aerosol extinction powerlaw is commonly referred to as the Angstrom exponent. The Angstrom exponent is often used as a qualitative indicator of aerosol particle size, with values greater than two indicating small particles associated with combustion byproducts, and values less than one indicating large particles like sea salt and dust. In this study, we investigate the relationship between the Angstrom exponent and the mode parameters of bimodal aerosol size distributions using Mie theory calculations and Aerosol Robotic Network (AERONET) retrievals. We find that Angstrom exponents based upon seven wavelengths (0.34, 0.38, 0.44, 0.5, 0.67, 0.87, and 1.02 micrometers) are sensitive to the volume fraction of aerosols with radii less then 0.6 micrometers, but not to the fine mode effective radius. The Angstrom exponent is also known to vary with wavelength, which is commonly referred to as curvature; we show how the spectral curvature can provide additional information about aerosol size distributions for intermediate values of the Angstrom exponent. Curvature also has a significant effect on the conclusions that can be drawn about two-wavelength Angstrom exponents; long wavelengths (0.67, 0.87 micrometers) are sensitive to fine mode volume fraction of aerosols but not fine mode effective radius, while short wavelengths (0.38, 0.44 micrometers) are sensitive to the fine mode effective radius but not the fine mode volume fraction.
Schuster, Gregory L.↗
Simulation of the Aerosol Size Distribution Using a Neural Network Surrogate for the Modal Aerosol Module (MAM7)
One objective of atmospheric simulations is to quantify the distribution of aerosols and their properties. Accurate parameterizations of the processes governing aerosol mass, particle number, and particle size distribution are important for predicting the Earth’s net radiative balance and aerosol-cloud interactions. The Modal Aerosol Module (MAM7) is a two-moment aerosol model that simulates mass, number, and size distribution of seven modes comprised of internally mixed aerosol species. The two-moment scheme adds significant computational expense but allows for the prediction of varying particle size distribution relative to the bulk method which predicts only total mass. In this work, we developed a neural network surrogate model for MAM7 (MAMnet) to predict the aerosol number concentration in NASA’s Global Earth Observing System (GEOS) without adding prohibitive computational expense. MAMnet, can be driven by output from a single moment, mass-based, aerosol scheme (Goddard Chemistry Aerosol and Radiation model (GOCART)) or from reanalysis products (Modern-Era Retrospective analysis for Research and Applications, Version 2 (MERRA-2)). MAMnet was trained using number concentrations from a 5-year GEOS/MAM7 simulation at 1-degree horizontal resolution and using the total mass calculated across modes as inputs, as well as temperature and air density. The model architecture for MAMnet was based on AlexNet, the 2012 winner of the ImageNet Large Scale Visual Recognition Challenge. While some modifications were necessary to accommodate our problem, important aspects of the network were preserved. MAMnet was able to reproduce zonal dynamics and spatial distributions of the aerosol number concentration however predictability in the upper troposphere was poor.
Katherine H Breen↗
Retrieval of aerosol size distributions from scattering and extinction measurements in the presence of multiple scattering
A fast technique, based on approximation to atmospheric radiative transfer in the solar aureole, is presented for the retrieval of aerosol size distribution from multispectral measurements of both scattered sky radiance and extinction by aerosol media. In this approximation, it is assumed that for a relatively clear day, the sky radiance is due to single scattering by molecules and aerosols, and to multiple scattering by molecules alone. The accuracy of this approximation is discussed in connection with the inversion of scattered radiation data. Results for aerosol size distributions retrieved from multispectral solar extinction measurements by the nonlinear least squares method are discussed, and the retrievals are found to be accurate when checked against ground truth measurements.
Deepak, A.↗
The inversion of aureole measurements to derive aerosol size distributions
An iterative method to invert size distributions from simulated scattered radiance measurements at small angles from the sun has been investigated. The inferred size distributions were represented by piecewise linear and cubic spline functions. Various relevant characteristics were investigated and it was found that: (1) the inverted size distribution was insensitive to the number of knots in the piecewise linear spline; (2) within the range of sensitivity, the choice of initial guess had little effect on the inverted size distribution; (3) five per cent random noise in the simulated radiances appreciably deteriorated the result but variations are still tolerable when compared with other methods for determining size distributions; (4) the inverted distribution was insensitive to the index of refraction used in the kernel for particle radii greater than 1 micron; (5) the choice of wavelength between 0.40 and 0.70 microns has a negligible effect on the inverted distribution; (6) a range of tropospheric aerosol size distributions gives acceptable inverted results; and (7) the cubic spline representation can give reasonable inverted distributions, but may become unstable.
Twitty, J. T.↗
Application of modified Twomey techniques to invert lidar angular scatter and solar extinction data for determining aerosol size distributions
Polarization properties of the angularly scattered laser light from a volume of air are used to determine the size distribution of the aerosol particles within the volume by the use of appropriate inversion techniques. Similar techniques are employed to determine a mean size distribution of the particulates within a vertical column through the atmosphere from determinations of the aerosol optical depth as a function of wavelength. In both of these examples, a modification of an inversion technique originally described by Twomey has been employed. Details of this method are presented as well as results from actual measurements employing bistatic lidar and solar radiometer.
Herman, B. M.↗
Aerosol Size Distribution Properties Associated With Cold-Air Outbreaks in the Norwegian Arctic
The aerosol particles serving as cloud condensation and ice nuclei contribute to key cloud processes associated with cold-air outbreak (CAO) events but are poorly constrained in climate models due to sparse observations. Here we retrieve aerosol number size distribution modes from measurements at Andenes, Norway, during the Cold-Air Outbreaks in the Marine Boundary Layer Experiment (COMBLE) and at Zeppelin Observatory, approximately 1000 km upwind from Andenes at Svalbard. During CAO events at Andenes, the sea-spray-mode number concentration is correlated with strong over-ocean winds with a mean of 8±4 cm−3 that is 71 % higher than during non-CAO conditions. Additionally, during CAO events at Andenes, the mean Hoppel minimum diameter is 6 nm smaller than during non-CAO conditions, though the estimated supersaturation is lower, and the mean number concentration of particles that likely activated in-cloud is 109±61 cm−3 with no statistically significant difference from the non-CAO mean of 99±66 cm−3. For CAO trajectories between Zeppelin Observatory and Andenes, the upwind-to-downwind change in number concentration is the largest for the accumulation mode with a mean decrease of 93±95 cm−3, likely attributable primarily to precipitation scavenging. These characteristic properties of aerosol number size distributions during CAO events provide guidance for evaluating CAO aerosol–cloud interaction processes in models.
accumulation mode particle scavenging↗
Use of In Situ Cloud Condensation Nuclei, Extinction, and Aerosol Size Distribution Measurements to Test a Method for Retrieving Cloud Condensation Nuclei Profiles From Surface Measurements
If the aerosol composition and size distribution below cloud are uniform, the vertical profile of cloud condensation nuclei (CCN) concentration can be retrieved entirely from surface measurements of CCN concentration and particle humidification function and surface-based retrievals of relative humidity and aerosol extinction or backscatter. This provides the potential for long-term measurements of CCN concentrations near cloud base. We have used a combination of aircraft, surface in situ, and surface remote sensing measurements to test various aspects of the retrieval scheme. Our analysis leads us to the following conclusions. The retrieval works better for supersaturations of 0.1% than for 1% because CCN concentrations at 0.1% are controlled by the same particles that control extinction and backscatter. If in situ measurements of extinction are used, the retrieval explains a majority of the CCN variance at high supersaturation for at least two and perhaps five of the eight flights examined. The retrieval of the vertical profile of the humidification factor is not the major limitation of the CCN retrieval scheme. Vertical structure in the aerosol size distribution and composition is the dominant source of error in the CCN retrieval, but this vertical structure is difficult to measure from remote sensing at visible wavelengths.
Ghan, Stephen J.↗