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At least 19 records

Beta decay of rb86

Measuring of rubidium 86 beta decay using lithium drifted surface barrier silicon detectors

BETA RADIATION

Cold equation of state in a strong magnetic field - Effects of inverse beta-decay

The influence of a high magnetic field (B is greater than 10 exp 12 G) on the degenerate matter equation of state appropriate to a neutron star is studied. The regime dominated by relativistic electrons up to the neutron drip density is highlighted. The equilibrium matter composition and equation of state, allowing for inverse beta-decay. Two different equilibrium models are determined: an ideal neutron-proton-electron (npe) gas and the more realistic model of Baym, Pethick, and Sutherland (1971) consisting of a Coulomb lattice of heavy nuclei embedded in an electron gas. For a sufficiently high field strength, the magnetic field has an appreciable effect, changing the adiabatic index of the matter and the nuclear transition densities. The influence of a strong field on some simple nonequilibrium processes, including beta-decay and inverse beta-decay (electron capture) is also considered. The effects produced by the magnetic field are mainly due to the changes in the transverse electron quantum orbits and the allowed electron phase space induced by the field.

Lai, Dong

Beta-decay, Bremsstrahlen, and the origin of molecular chirality

A brief review is presented of the Vester-Ulbricht beta-decay Bremsstrahlen hypothesis for the origin of optical activity, and of subsequent experiments designed to test it. Certain experiments along these lines, begun in 1974 and involving the irradiation of racemic and optically active amino acids in a 61.7 KCi Sr-90-Y-90 Bremsstrahlen source, have now been completed and are described. After 10.89 years of irradiation with a total Bremsstrahlen dose of 2.5 x 10 to the 9th rads, crystalline DL-leucine, norleucine, and norvaline suffered 47.2, 33.6, and 27.4 percent radiolysis, respectively, but showed no evidence whatsoever of asymmetric degradation. Dand L-Leucine underwent about 48 percent radiolysis and showed 2.4-2.9 percent radioracemization. Other samples in solution were too severely degraded to analyze. Probable intrinsic reasons for the failure of the Vester-Ulbricht mechanism to afford asymmetric radiolysis in the present and related experiments involving beta-decay Bremsstrahlen are enumerated.

Bonner, W. A.

Experimental evidence for beta-decay as a source of chirality by enantiomer analysis

Earlier experiments testing the Vester-Ulbricht beta-decay hypothesis for the origin of molecular chirality are reviewed, followed by descriptions of experiments involving attempted asymmetric radiolysis of DL-amino acids using quantitative gas chromotography as a probe for optical activity. The radiation sources included Sr-90-Y-90, C-14, and P-32 Bremsstrahlen, longitudinally polarized electrons from a linear accelerator and longitudinally polarized protons from a cyclotron. With the possible exception of the linear accelerator irradiations, these experiments failed to produce g.c.-detectable enantiomeric excesses, even at 50-70 percent gross radiolysis. Thus no unambiguous support for the Vester-Ulbricht hypothesis is found in any of the attempted asymmetric radiolyses performed to date. Radioracemization, a possible reason for these failures, is discussed.

Bonner, W. A.

Experiments on the origin of molecular chirality by parity non-conservation during beta-decay

Experiments are described to test a theory for the origin of optical activity wherein the longitudinally polarized electrons resulting from parity violation during radioactive beta decay, and their resulting circularly polarized Bremsstrahlung, might interact asymmetrically with organic matter to yield optically active products. Experiments involve subjecting a number of racemic and optically active amino acid samples to irradiation in a 61700 Ci90SR-90Y beta radiation source for a period of 1.34 years, then examining them for any asymmetric effects by means of optical rotatory dispersion and analytical gas chromatography. In the cases of D,L-leucine, norleucine, norvaline and proline as solids, of D,L-leucine in solution and of D,L-tyrosine in alkaline solution no optical rotation was observed during CRD measurements in the 250-630 nm spectral region. While slight differences were noted in the percent radiolysis of solid D- (12.7%) and L-leucine (16.2%) as determined by GC, no enrichment of either enantiomer was found.

Bonner, W. A.

Experiments on the origin of molecular chirality by parity non-conservation during beta-decay

Experiments are described to test a theory for the origin of optical activity wherein the longitudinally polarized electrons resulting from parity violation during radioactive beta-decay, and their resulting circularly polarized bremsstrahlung, might interact asymmetrically with organic matter to yield optically active products. The historical background to this subject is briefly reviewed. Our experiments involve subjecting a number of racemic and optically active amino acid samples to a beta-radiation source for a period of 1.34 years (total dose: 411 Mrads), then examining them for any asymmetric effects by means of optical rotatory dispersion and analytical gas chromatography.

Bonner, W. A.

On the origin of biological chirality via natural beta-decay

An hypothesis to account for the chirality (handedness) of some biological molecules is given. Experimental evidence suggests that longitudinally polarized electrons having the chirality of terrestrial beta-decay electrons remove dextro-leucine from a racemic mixture. If, by a similar mechanism, the terrestrial environment provided more levo- than dextro-amino acids, that would account for the chirality now observed in organic molecules. An isotope of potassium has been proposed as the natural beta-emitter responsible for biomolecular chirality; however, Carbon 14 may be an even more plausible candidate. Ready availability of the carbon isotope in the terrestrial environment of 4.5 aeons ago, and the role of leucine in protein synthesis indicate that these two agents may have been chief factors in the evolution of biomolecular chirality. Suggestions for further research in this area are made.

Noyes, H. P.

Beta decay and the origins of biological chirality - Experimental results

Preliminary experimental results are presented of an investigation of the possible role of preferential radiolysis by electrons emitted in the beta decay of radionuclides, a parity-nonconserving process, in the universal causation of the optical activity of biological compounds. Experiments were designed to measure the asymmetry in the production of triplet positronium upon the bombardment of an amino acid powder target by a collimated beam of positrons as positron helicity or target chirality is reversed. No asymmetry down to a level of 0.0007 is found in experiments on the D and L forms of cystine and tryptophan, indicating an asymmetry in positronium formation cross section of less than 0.01, while an asymmetry of 0.0031 is found for leucine, corresponding to a formation cross section asymmetry of about 0.04

Gidley, D. W.

Beta decay and the origin of biologial chirality - New experimental results

The hypothetical connection developed by Vester and Ulbricht (1959), between the handedness of beta particles in radioactive decay and the (L) sign of biologial chirality is investigated in a radiolysis experiment. The experiment measured the predicted asymmetry in the formation triplet or 'ortho-' positronium (oPs) in amino acid enantiomers by low energy positrons under conditions of helicity reversal. The positrons were focused on amino acid powder samples. By measuring the time between positron arrival and emission of gamma rays, long-lived oPs were separated from other species. It is found that the asymmetry in leucine (0.8 x 10 to the -4th) is consistent with the theoretical prediction of 10 to the -6th. Neither the experimental limits nor the theoretical estimates are found to rule out a mechanism like that described by Vester and Ulbricht as the cause of the sign of the observed chiral polarization.

Van House, J.

Segmented Ge detector rejection of internal beta activity produced by neutron irradiation

Future Ge spectrometers flown in space to observe cosmic gamma-ray sources will incorporate segmented detectors to reduce the background from radioactivity produced by energetic particle reactions. To demonstrate the effectiveness of a segmented Ge detector in rejecting background events due to the beta decay of internal radioactivity, a laboratory experiment has been carried out in which radioactivity was produced in the detector by neutron irradiation. A Cf-252 source of neutrons was used to produce, by neutron capture on Ge-74 (36.5 percent of natural Ge) in the detector itself, Ge-75 (t sub 1/2 = 82.78 min), which decays by beta emission with a maximum electron kinetic energy of 1188 keV. By requiring that an ionizing event deposit energy in two or more of the five segments of the detector, each about 1-cm thick, the beta particles, which have a range of about 1-mm, are rejected, while most external gamma rays incident on the detector are counted. Analysis of this experiment indicates that over 85 percent of the beta events from the decay of Ge-75 are rejected, which is in good agreement with Monte Carlo calculations.

Varnell, L. S.

Electronic considerations for externally segmented germanium detectors

The dominant background source for germanium gamma ray detector spectrometers used for some astrophysics observations is internal beta decay. Externally segmented germanium gamma ray coaxial detectors can identify beta decay by localizing the event. Energetic gamma rays interact in the germanium detector by multiple Compton interactions while beta decay is a local process. In order to recognize the difference between gamma rays and beta decay events, the external electrode (outside of detector) is electrically partitioned. The instrumentation of these external segments and the consequence with respect to the spectrometer energy signal is examined.

Madden, N. W.

Lu-Hf total-rock isochron for the eucrite meteorites

The isotope Lu-176 (2.6% of natural lutetium) decays by beta(-) to Hf-176, with a long half life. The first Lu-Hf isochron is presented. The eucrite meteorites, a suite of planetary igneous rocks of known age, 4,550 Myr, define a 10-point total-rock isochron with a slope of 0.0934 + or - 40, leading to a value of 3.53 + or - 0.14 x 10 to the 10th yr for the beta(-) decay half life of Lu-176. The isochron intercept of 0.27973 + or - 12 gives the initial Hf-176/Hf-177 for the inner solar system at the time of accretion.

Patchett, P. J.