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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 19 records
All sourcesNASA NTRSDOE OSTI
NASA NTRS1990

Model test of CCN-cloud albedo climate forcing

Cloud condensation nuclei (CCN) influence cloud albedo through their effect on the cloud droplet size distribution. A number of studies have evaluated the climatic impact of the CCN-cloud albedo feedback, but all have assumed that cloud distributions, cloud thicknesses, and cloud liquid water contents would remain constant as the climate adjusted. This assumption has been tested using the Livermore version of the National Center for Atmospheric Research Community Climate Model. The results indicate that there are no significant compensating changes in cloud properties that would counteract the 1.7 percent global albedo increase resulting from a fourfold increase in marine CCN concentration. Furthermore, when ocean surface temperatures are decreased 4 C in a manner broadly consistent with the enhanced cloud albedos, an increase in cloud fraction of 3.5 percent and a reduction in cloud altitude are predicted, leading to a positive feedback from clouds that would imply a climate impact roughly double that calculated from cloud droplet size distribution change alone.

Ghan, S. J.↗
DOE OSTI2023

Influences of cloud vertical overlapping on the calculated cloud albedo and their validation with satellite observations

Cloud albedo is expected to influence cloud radiative forcing in addition to cloud fraction, and inadequate description of the cloud overlapping effects on the cloud fraction may influence the simulated cloud fraction, and thus the relative cloud radiative forcing (RCRF) and cloud albedo. In this study, we first present a new formula by extending that presented previously in Liu et al. (2011) to consider multilayer clouds directly in the relationship between cloud albedo, cloud fraction and RCRF, and then quantitatively evaluate the effects of different cloud vertical overlapping structures, represented by the decorrelation length scales (L cf ), on the simulated cloud albedos. We use the BCC_AGCM2.0_CUACE/Aero model with simultaneous validation by observations from the Clouds and the Earth's Radiation Energy System (CERES) satellite. When L cf < 4 km (i.e., the cloud overlap is closer to the random overlap), the simulated cloud albedos are generally in good agreement with the satellite-based albedos for December– February and June–August; when L cf ≥ 4 km (i.e., the cloud vertical overlap is closer to the maximum overlap), the difference between simulated and observed cloud albedos became larger, due mainly to significant differences in cloud fractions and RCRF. Further quantitative analysis shows that the relative Euclidean distance, which represents the degree of overall model–observation disagreement, increases with the L cf for all three variables (cloud albedo, cloud fraction and RCRF), indicating the importance of cloud vertical overlapping in determining the accuracy of the calculated cloud albedo for multilayer clouds.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS2004

Entrainment, Drizzle, and Stratocumulus Cloud Albedo

Globally averaged cloud changes from GCMs on average show a doubling of the Twomey effect, which is the change in cloud albedo with respect to changes in droplet concentrations for fixed cloud water and droplet dispersion. In contrast, ship-track measurements show a much more modest amplification of the Twomey effect, suggesting that the GCMs are exaggerating the indirect aerosol effect. We have run large-eddy simulations with bin microphysics of marine stratocumulus from multiple field campaigns, and find that the large-eddy simulations are in much better agreement with the ship-track measurements. The inversion strength over N. Pacific stratocumulus (as measured during DYCOMS-II) is generally much stronger than over N. Atlantic stratocumulus (as measured during ASTEX), and we have found that the response of cloud water to increasing droplet concentration changes sign as the inversion strengthens. For the different environmental conditions, we will show the overall response of cloud albedo to droplet concentrations, and decompose the response into its contributing factors of changes in cloud water, droplet dispersion, and horizontal inhomogeneity.

Ackerman, A. S.↗
NASA NTRS1991

Cloud albedo control by cloud-top entrainment

Marine stratus and stratocumulus clouds exert a considerable influence on the earth's heat budget, mainly due to their high albedos relative to the ocean surface. It is therefore important to understand the processes that control the radiative properties of these extensive cloud systems, particularly during daylight hours. Aircraft measurements of a stratocumulus cloud deck taken around local noon during the 1987 field phase of the First International Satellite Cloud Climatology Project Regional Experiment are the topic of this paper. A mixing line analysis of data from a series of flight tracks across a strong gradient in cloud albedo provides evidence that variations in the water vapor content of the air above the marine inversion can be responsible for the albedo change. The implications of this unexpected result for climate modeling are discussed.

Hanson, Howard P.↗
NASA NTRS1992

Natural versus anthropogenic factors affecting low-level cloud albedo over the North Atlantic

Cloud albedo plays a key role in regulating earth's climate. Cloud albedo depends on column-integrated liquid water content and the density of cloud condensation nuclei, which consists primarily of submicrometer-sized aerosol sulfate particles. A comparison of two independent satellite data sets suggests that, although anthropogenic sulfate emissions may enhance cloud albedo immediately adjacent to the east coast of the United States, over the central North Atlantic Ocean the variability in albedo can be largely accounted for by natural marine and atmospheric processes that probably have remained relatively constant since the beginning of the industrial revolution.

Falkowski, Paul G.↗
NASA NTRS1993

Effect of anthropogenic sulfate aerosols on low-level cloud albedo over oceans

By reducing cloud droplet size, anthropogenic sulfate aerosols are capable of increasing cloud albedo and thus possibly changing the climate. To test the detectability of this effect, we examined satellite-measured low-level cloud albedo off the east coasts of North America and Asia at midlatitudes where anthropogenic sulfate sources are large and aerosols are transported eastward over the oceans by prevailing westerlies. The satellite data demonstrate enhanced cloud albedo near the coastal boundaries where sulfate concentrations are large. Similar trends are absent over ocean regions of the Southern Hemisphere that are removed from anthropogenic sulfate sources.

Kim, Youngseung↗
DOE OSTI2024

Present-day correlations are insufficient to predict cloud albedo change by anthropogenic aerosols in E3SM v2

Cloud albedo susceptibility to droplet number perturbation remains a source of uncertainty in understanding aerosol–cloud interactions and thus both past and present climate states. Through the Energy Exascale Earth System Model (E3SM) v2 experiments, we probe the effects of competing processes on cloud albedo susceptibility of low-lying marine stratocumulus in the northeast Pacific. In present-day conditions, we find that increasing precipitation suppression by aerosols increases cloud albedo susceptibility, whereas increasing cloud sedimentation decreases it. By constructing a hypothetical model configuration exhibiting negative susceptibility under all conditions, we conclude that cloud albedo change due to aerosol perturbation cannot be predicted by present-day co-variabilities in E3SM v2. As such, our null result herein challenges the assumption that present-day climate observations are sufficient to constrain past states, at least in the context of cloud albedo changes to aerosol perturbation.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2023

Evaluation of liquid cloud albedo susceptibility in E3SM using coupled eastern North Atlantic surface and satellite retrievals

The impact of aerosol number concentration on cloud albedo is a persistent source of spread in global climate predictions due to multi-scale, interactive atmospheric processes that remain difficult to quantify. We use 5 years of geostationary satellite and surface retrievals at the US Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) eastern North Atlantic (ENA) site in the Azores to evaluate the representation of liquid cloud albedo susceptibility for overcast cloud scenes in the DOE Energy Exascale Earth System Model version 1 (E3SMv1) and provide possible reasons for model–observation discrepancies. The overall distribution of surface 0.2 % CCN concentration values is reasonably simulated, but simulated liquid water path (LWP) is lower than observed and layer mean droplet concentration (N d ) comparisons are highly variable depending on the N d retrieval technique. E3SMv1's cloud albedo is greater than observed for given LWP and N d values due to a lower cloud effective radius than observed. However, the simulated albedo response to N d is suppressed due to a correlation between the solar zenith angle (SZA) and N d created by the seasonal cycle that is not observed. Controlling for this effect by examining the cloud optical depth (COD) shows that E3SMv1's COD response to CCN concentration is greater than observed. For surface-based retrievals, this is only true after controlling for cloud adiabaticity because E3SMv1's adiabaticities are much lower than observed. Assuming a constant adiabaticity in surface retrievals as done in top-of-atmosphere (TOA) retrievals narrows the retrieved ln N d distribution, which increases the cloud albedo sensitivity to ln N d to match the TOA sensitivity. The greater sensitivity of COD to CCN is caused by a greater Twomey effect in which the sensitivity of N d to CCN is greater than observed for TOA-retrieved N d , and once model–observation cloud adiabaticity differences are removed, this is also true for surface-retrieved N d . The LWP response to N d in E3SMv1 is overall negative as observed. Despite reproducing the observed LWP–N d relationship, observed clouds become much more adiabatic as N d increases, while E3SMv1 clouds do not, associated with more heavily precipitating clouds that are partially but not completely caused by deeper clouds and weaker inversions in E3SMv1. These cloud property differences indicate that the negative LWP–N d relationship is likely not caused by the same mechanisms in E3SMv1 and observations. The negative simulated LWP response also fails to mute the excessively strong Twomey effect, highlighting potentially important confounding factor effects that likely render the LWP–N d relationship non-causal. N d retrieval scales and assumptions, particularly related to cloud adiabaticity, contribute to substantial spreads in the model–observation comparisons, though enough consistency exists to suggest that aerosol activation, drizzle, and entrainment processes are critical areas to focus E3SMv1 development for improving the fidelity of aerosol–cloud interactions in E3SM.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2022

Projecting Stratocumulus Transitions on the Albedo—Cloud Fraction Relationship Reveals Linearity of Albedo to Droplet Concentrations

Satellite images show solid marine stratocumulus cloud decks (Sc) that break up over the remote oceans. The Sc breakup is initiated by precipitation and is accompanied by a strong reduction in the cloud radiative effect. Aerosol has been shown to delay the Sc breakup by postponing the onset of precipitation, however its climatic effect is uncertain. Here we introduce a new approach that allows us to re-cast currently observed cloud cover and albedo to their counterfactual cleaner world, enabling the first estimate of the radiative effect due to delayed cloud breakup. Using simple radiative approximation, the radiative forcing with respect to pre-industrial times due to delayed Sc breakup is –0.39 W m –2 . The radiative effect changes nearly linearly with aerosol due to the droplet concentration control on the cloud cover, suggesting a potentially accelerated warming if the current trend of reduction in aerosol emissions continues.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2023

Distinct regional meteorological influences on low-cloud albedo susceptibility over global marine stratocumulus regions

Abstract. Marine stratocumuli cool the Earth effectively due to their high reflectance of incoming solar radiation and persistent occurrence. The susceptibility of cloud albedo to droplet number concentration perturbations depends strongly on large-scale meteorological conditions. Studies focused on the meteorological dependence of cloud adjustments often overlook the covariability among meteorological factors and their geographical and temporal variability. We use 8 years of satellite observations sorted by day and geographical location to show the global distribution of marine low-cloud albedo susceptibility. We find an overall cloud brightening potential for most marine warm clouds, which is more pronounced over subtropical coastal regions. A weak cloud darkening potential in the annual mean is evident over the remote SE Pacific and SE Atlantic. We show that large-scale meteorological fields from the ERA5 reanalysis data, including lower-tropospheric stability, free-tropospheric relative humidity, sea surface temperature, and boundary layer depth, have distinct covariabilities over each of the eastern subtropical ocean basins where marine stratocumuli prevail. This leads to a markedly different annual cycle in albedo susceptibility over each basin. Moreover, we find that basin-specific regional relationships between key meteorological factors and albedo susceptibilities are absent in a global analysis. Our results stress the importance of considering the geographical distinctiveness of temporal meteorological covariability when scaling up the local-to-global response of cloud albedo to aerosol perturbations.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS1994

Cloud condensation nucleus-sulfate mass relationship and cloud albedo

Analysis of previously published, simultaneous measurements of cloud condensation nucleus number concentration and sulfate mass concentration suggest a nonlinear relationship between the two variables. This nonlinearity reduces the sensitivity of cloud albedo to changes in the sulfur cycle.

Hegg, Dean A.↗
NASA NTRSDate not supplied

Reducing OCO-2 regional biases through novel 3D cloud, albedo, and meteorology estimation

This ROSES project tests the addition of novel 3D cloud, albedo fine structure, temperature and water vapor profile to the OCO-2 retrieved system. All new parameters have been added to the ReFRACtor / TROPESS system for testing. Currently, we are comparing 3d-cloud retrievals from OCO-2 radiances to the MODIS-derived EAR3T cloud properties. The water and temperature profile retrievals have been implemented and result in improved XCO2 comparisons to TCCON, and now are implementing principal-component analysis (PCA) to reduce the number of parameters added. We are also studying ECOSTRESS spectral library, AVIRIS-ng, OCO-2 spectral residuals, and albedo retrievals with additional parameters to determine the appropriate characterization of albedo. We find that the current albedo parametrization (2nd order polynomial) is adequate for ocean and vegetation, but not adequate for soil and rock observations.

Reducing OCO-2↗
NASA NTRS1990

Measurements of the light-absorbing material inside cloud droplets and its effect on cloud albedo

Most of the measurements of light-absorbing aerosol particles made previously have been in non-cloudy air and therefore provide no insight into aerosol effects on cloud properties. Here, researchers describe an experiment designed to measure light absorption exclusively due to substances inside cloud droplets, compare the results to related light absorption measurements, and evaluate possible effects on the albedo of clouds. The results of this study validate those of Twomey and Cocks and show that the measured levels of light-absorbing material are negligible for the radiative properties of realistic clouds. For the measured clouds, which appear to have been moderately polluted, the amount of elemental carbon (EC) present was insufficient to affect albedo. Much higher contaminant levels or much larger droplets than those measured would be necessary to significantly alter the radiative properties. The effect of the concentrations of EC actually measured on the albedo of snow, however, would be much more pronounced since, in contrast to clouds, snowpacks are usually optically semi-infinite and have large particle sizes.

Twohy, C. H.↗
NASA NTRS2004

Entrainment, Drizzle, and Cloud Albedo

Increased aerosol and hence droplet concentrations in polluted clouds are expected to inhibit precipitation and thereby increase cloud water, leading to more reflective clouds that partially offset global warming. Yet polluted clouds are not generally observed to hold more water. Much of the uncertainty regarding the indirect aerosol effect stems from inadequate understanding of such changes in cloud water. Detailed simulations show that the relative humidity of air overlying stratocumulus is a leading factor determining whether cloud water increases or decreases when precipitation is suppressed. When the overlying air is dry, cloud water can decrease as droplet concentrations increase.

Ackerman, A. S.↗
NASA NTRS2010

The Characterization of Deep Convective Cloud Albedo as a Calibration Target Using MODIS Reflectances

There are over 25 years of historical satellite data available to climate analysis. The historical satellite data needs to be well calibrated, especially in the visible, where there is no onboard calibration on operational satellites. The key to the vicarious calibration of historical satellites relies on invariant targets, such as the moon, Dome C, and deserts. Deep convective clouds (DCC) also show promise of being a stable invariant or predictable target viewable by all satellites, since they behave as solar diffusers. However DCC have not been well characterized for calibration. Ten years of well-calibrated MODIS is now available. DCC can easily be identified using IR thresholds, where the IR calibration can be traced to the onboard black-bodies. The natural variability of DCC albedo will be analyzed geographically and seasonally, especially difference of convection initiated over land or ocean. Functionality between particle size and ozone absorption with DCC albedo will be examined. Although DCC clouds are nearly Lambertion, the angular distribution of reflectances will be sampled and compared with theoretical models. Both Aqua and Terra MODIS DCC angular models will be compared for consistency. Normalizing angular geostationary DCC reflectances, which were calibrated against MODIS, with SCIAMACHY spectral reflectances and comparing them to MODIS DCC reflectances will inspect the usage of DCC albedos as an absolute calibration target.

Doelling, David R.↗