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NASA NTRS1981

Comparison between two Aitken counters and with cloud condensation nuclei counters at the 1980 International CCN Workshop

The Pollak and the TSI 3020 counters agreed to within about 10% at concentrations below 1000 cu cm, whereas above that concentration, substantial systematic differences were observed. When the test aerosol was monodisperse and the CCN counters were operated at supersaturations that should nucleate all the aerosol, the Pollak counter read about 6% to 20% lower than the CCN counter in the concentration range from 250/cu cm to 1800/cu cm. The TSI 3020 read about 20% lower than the CCN counter at concentrations less than 1000/cu cm, and a factor of about two higher at concentrations above 1000/cu cm.

Rogers, C. F.↗

NASA NTRS1997

A Balloon-Borne Cloud Condensation Nuclei Counter

A balloon-borne instrument was constructed for observations of vertical profiles of cloud condensation nucleus (CCN) concentrations, active at 1% supersaturation. Droplet concentration in the static thermal-gradient diffusion chamber is deduced from the amount of scattered laser light detected by a photodetector. The photodetector is calibrated using a video camera and computer system to count the number of droplets produced from NaCl aerosol. Preliminary data are available from nine early morning profiles obtained at Laramie, Wyoming, between June 1995 and January 1997. To complement the CCN measurements, instruments that measure condensation nuclei (CN) and aerosols with diameter greater than 0.30 micrometers (D(sub 0.3) were also included on the balloon package. CCN concentrations exhibited a general decrease from the surface to the top of the boundary layers, were generally uniform through well-mixed layers, and show variability above well-mixed layers. In general, the structure of the CCN profile appears to be closely related to the structure in the CN and D(sub 0.3) profiles. Summer profiles generally have CCN concentration greater than 200/cu cm up to 500 mbar, whereas winter profiles are less than 200/cu cm at all levels.

Delene, David J.↗

NASA NTRS1981

The Third International Cloud Condensation Nuclei Workshop

Twenty-five instruments were tested, including size characterization devices and two Aitken counters. The test aerosols were supplied to the instruments by an on-line generation system, thereby eliminating the need for storage bags. Cloud condensation chambers and haze chambers are highlighted.

Kocmond, W. C.↗

NASA NTRS1985

Cloud Microphysics by Thermal Wave Methods

This experiments series is the first application of a low-gravity experimental technique to the study of cloud microphysics. The low-gravity environment is provided by the parabolic maneuver of NASA's KC-135 aircraft. The primary objective is to compare experimental observations of cloud droplet growth and evaporation in a convection free environment with a numerical model of the process. Beyond that, the work also involves the development and testing of low-gravity research techniques. In particular, passive methods of thermal control have been devised and used effectively. The study to date has shown that the method is particularly suitable for looking at interactions between adjoining portions of the cloud drop field and interactions of the drop field with a solid interface. After final analysis of the data, it is expected the results will shed light on the development of cloud droplet size spectra in natural clouds as well as the performance of certain types of cloud physics instrumentation, particularly continuous flow diffusion chambers and loud condensation nuclei counters.

Anderson, B. J.↗

NASA NTRS1989

Observations of condensation nuclei in the Airborne Antarctic Ozone Experiment - Implications for new particle formation and polar stratospheric cloud formation

This paper discusses the results of the ER-2 Condensation Nucleus Counter operated in the Airborne Ozone Experiment in August, September, and October 1987, providing data on the mixing ratio of aerosol condensation nuclei (CN) with diameters between about 0.02 and 1 micron. It is shown that the vertical profile of the CN mixing ratio is closely related to that of N2O, and that, between the -71 and -53 deg latitude, the location of the minima in the CN mixing ratio profile was near the 160 ppbv N2O isopleth, indicating that the processes of mixing and subsidence, which determine the inclination of that isopleth, also strongly affect the spatial distribution of the sulfate aerosol. Evidence for new sulfate particle formation is presented and related to the amount of subsidence experienced by air parcels in the formation of the polar vortex. Concentrations of CN are compared with those of larger particles (with diameters between 0.81 micron and 9.75 microns) to study polar stratospheric cloud formation mechanisms.

Wilson, J. C.↗

NASA NTRS1989

Balloon-borne measurements of aerosol, condensation nuclei, and cloud particles in the stratosphere at McMurdo Station, Antarctica, during the spring of 1987

Measurements of the vertical profile of particles with condensation nuclei counters and eight channel aerosol detectors at McMurdo Station, Antarctica, in 1987 verified observations made in 1986 concerning the absence of upwelling in the polar vortex and the presence of a condensation nuclei layer in conjunction with the ozone hole region. New observations of a bimodal aerosol size distribution, consisting of a large-particle mode mixed in with the small-particle sulfate mode, at temperatures below -79 C are consistent with the presence of nitric acid-water particles at low concentrations. Higher concentrations of large particles were observed in association with nacreous clouds. An unusual particle layer which contained enhanced concentrations of both the small-particle (sulfate) mode and the large-particle (nitric acid) mode was detected at temperatures below -85 C, suggesting simultaneous nucleation and growth phenomena. The vortex condensation nuclei layer was observed to form at the same time as the ozone hole, indicating that formation of the layer is triggered by photochemical processes and may be important in controlling ozone depletion above 22 km.

Hofmann, D. J.↗

NASA NTRS1990

Aerosol measurements in the stratocumulus project

Cloud Condensation Nuclei (CCN) and Condensation Nuclei (CN) were measured from the National Center for Atmospheric Research (NCAR) Electra throughout the marine stratocumulus project. The total particle concentration was measured with a condensation nucleus counter. The CCN were measured with the Desert Research Institute (DRI) instantaneous CCN spectrometer. This instrument simultaneously measures the concentration of aerosol active at up to 100 different critical supersaturations (Sc). This is accomplished by exposing the sample to a fixed supersaturation field and using the size of the droplets produced in this cloud chamber to deduce the Sc of the nuclei upon which they have grown. Droplet size is associated with Sc through a calibration which is accomplished by passing soluble aerosols of known size and composition through the cloud chamber. This procedure results in a calibration curve of Sc vs. droplet size. This then allows the channel number to be directly associated with Sc. Thus, number concentration vs. Sc is obtained and this is a CCN spectrum. Since the instrument operates continuously, the measurements at all Sc's are available simultaneously. Samples are drawn directly from the ambient air and data is displayed in nearly real time. Samples were integrated over times of about 10 seconds so that substantial spatial resolution is available. Calibrations were performed once or twice a day and were found to be consistent. Preliminary results are shown.

Hudson, James G.↗

NASA NTRS1981

Simultaneous operation of three CCN counters and an isothermal haze chamber at the 1980 International CCN Workshop

Four devices were operated for the detection and characterization of cloud condensation nuclei (CCN) and fog condensation nuclei (FCN). In chronological order of development, the CCN devices are the conventional continuous-flow diffusion chamber (CFD), the rapid-cycle CCN spectrometer, and the instantaneous CCN spectrometer. The FCN detection device is an isothermal haze chamber (IHC). These four instruments are discussed and general comments on their performance at the workshop are given.

Hudson, J. G.↗

NASA NTRS1994

Cloud-Aerosol Interactions in Tropical Storms

During the Coupled Ocean-Atmosphere Response Experiment (COARE) of the Tropical Ocean and the Global Atmosphere (TOGA) program we measured cloud and aerosol particles aboard the NASA DC-8 over the warm pool of the western Pacific. Instruments on the aircraft included a condensation nuclei counter, optical particle counters, two-dimensional shadow probes and an ice crystal replicator. The size range covered by these instruments was from =0.01 micron to 6.4 mm diameter; particle shapes were determined for particles of sizes D greater than 1 micron.

Puesschel, R. F.↗

NASA NTRS1988

Aerosol measurements in the winter/spring Antarctic stratosphere. I - Correlative measurements with ozone. II - Impact on polar stratospheric cloud theories

Aerosol measurements collected from August 25-November 3, 1986 at McMurdo Station using balloon-borne optical particle counters are examined in order to study the relationship between aerosol and ozone distribution and the formation of polar stratospheric clouds (PSCs). Ozone, aerosol, and condensation nuclei profiles, and pressure, temperature, and humidity measurements are analyzed. It is observed that the height of the stratospheric sulfate layer decreases over the period of measurement suggesting that upwelling in the votex is not important in the zone depletion process. Three theories on PSC formation are described, and the effects of the aerosol measurements on the theories are considered. The three theories are: (1) the original theory of water vapor pressure over a solution of H2SO4 of Steele et al. (1983) and Hamill and Mc Master (1984); (2) the nitric acid theory of PSCs of Toon et al. (1986) and Hamill et al. (1986); and (3) the quasi-cirrus cloud theory of Heymsfield (1986).

Hofmann, D. J.↗

NASA NTRS2003

Toward Aerosol/Cloud Condensation Nuclei (CCN) Closure during CRYSTAL-FACE

During July 2002, measurements of cloud condensation nuclei were made in the vicinity of southwest Florida as part of the Cirrus Regional Study of Tropical Anvils and Cirrus Layers-Florida Area Cirrus Experiment (CRYSTAL-FACE) field campaign. These observations, at supersaturations of 0.2 and 0.85%, are presented here. The performance of each of the two CCN counters was validated through laboratory calibration and an in situ intercomparison. The measurements indicate that the aerosol sampled during the campaign was predominantly marine in character: the median concentrations were 233 cm-3 (at S = 0.2%) and 371 cm(sup -3) (at S = 0.85%). Three flights during the experiment differed from this general trend; the aerosol sampled during the two flights on 18 July was more continental in character, and the observations on 28 July indicate high spatial variability and periods of very high aerosol concentrations. This study also includes a simplified aerosol/CCN closure analysis. Aerosol size distributions were measured simultaneously with the CCN observations, and these data are used to predict a CCN concentration using Kohler theory. For the purpose of this analysis, an idealized composition of pure ammonium sulfate was assumed. The analysis indicates that in this case, there was good general agreement between the predicted and observed CCN concentrations: at S = 0.2%, N(sub predicted)/N(sub observed)= 1.047 (R(sup 2)= 0.911)); at S = 0.85%, N(sub predicted)/N(sub observed)=1.201 (R(sup 2)= 0.835)). The impacts of the compositional assumption and of including in-cloud data in the analysis are addressed. The effect of removing the data from the 28 July flight is also examined; doing so improves the result of the closure analysis at S = 0.85%. When omitting that atypical flight, N(sub predicted)/N(sub observed) = 1.085 (R(sup 2) = 0.770) at S = 0.85%.

VanReken, Timothy M.↗

NASA NTRS1998

Vertical Profiles of Cloud Condensation Nuclei, Condensation Nuclei, Optical Aerosol, Aerosol Optical Properties, and Aerosol Volatility Measured from Balloons

Under the support of this grant a balloon-borne gondola containing a variety of aerosol instruments was developed and flown from Laramie, Wyoming, (41 deg N, 105 deg W) and from Lauder, New Zealand (45 deg S, 170 deg E). The gondola includes instruments to measure the concentrations of condensation nuclei (CN), cloud condensation nuclei (CCN), optically detectable aerosol (OA.) (r greater than or equal to 0.15 - 2.0 microns), and optical scattering properties using a nephelometer (lambda = 530 microns). All instruments sampled from a common inlet which was heated to 40 C on ascent and to 160 C on descent. Flights with the CN counter, OA counter, and nephelometer began in July 1994. The CCN counter was added in November 1994, and the engineering problems were solved by June 1995. Since then the flights have included all four instruments, and were completed in January 1998. Altogether there were 20 flights from Laramie, approximately 5 per year, and 2 from Lauder. Of these there were one or more engineering problems on 6 of the flights from Laramie, hence the data are somewhat limited on those 6 flights, while a complete data set was obtained from the other 14 flights. Good CCN data are available from 12 of the Laramie flights. The two flights from Lauder in January 1998 were successful for all measurements. The results from these flights, and the development of the balloon-bome CCN counter have formed the basis for five conference presentations. The heated and unheated CN and OA measurements have been used to estimate the mass fraction of the aerosol volatile, while comparisons of the nephelometer measurements were used to estimate the light scattering, associated with the volatile aerosol. These estimates were calculated for 0.5 km averages of the ascent and descent data between 2.5 km and the tropopause, near 11.5 km.

Deshler, T.↗

NASA NTRS2015

Investigation of the CCN Activity, BC and UVBC Mass Concentrations of Biomass Burning Aerosols during the 2013 BASELInE Campaign

Biomass-burning (BB) aerosols, acting as cloud condensation nuclei (CCN), can influence cloud microphysical and radiative properties. In this study, we present CCN measured near the BB source regions over northern Southeast Asia (Doi Ang Khang, Thailand) and at downwind receptor areas (Lulin Atmospheric Background Station, Taiwan), focusing exclusively on 13-20 March 2013 as part of 2013 spring campaign of the Seven SouthEast Asian Studies (7-SEAS) intensive observation. One of the campaigns objectives is to characterize BB aerosols serving as CCN in SouthEast Asia (SEA). CCN concentrations were measured by a CCN counter at 5 supersaturation (SS) levels: 0.15%, 0.30%, 0.45%, 0.60%, and 0.75%. In addition, PM2.5 and black carbon mass concentrations were analyzed by using a tapered element oscillating microbalance and an aethalometer. It was found the number-size distributions and the characteristics of hygroscopicity (e.g., activation ratio and k) of BB aerosols in SEA have a strong diurnal pattern, and different behaviors of patterns were characterized under two distinct weather systems. The overall average value was low (0.05-0.1) but comparable with previous CCN studies in other BB source regions. Furthermore, a large fraction of UV-absorbing organic material (UVBC) and high Delta-C among BB aerosols were also observed, which suggest the existence of substantial particulate organic matter in fresh BB aerosols. These data provide the most extensive characterization of BB aerosols in SEA until now.

biomass burning aerosol↗

NASA NTRS1980

Laboratory investigations of cloud nuclei from combustion of Space Shuttle propellant

Small quantities of solid rocket motor propellant, of the type to launch the Space Shuttle, were burned at ambient pressure in the laboratory to provide aerosol samples for characterization. A portion of each sample was injected into an isothermal cloud chamber and the remainder into a 770-liter holding tank. Portable ice nucleus (IN) counters, filter devices for IN determinations and a cloud condensation nucleus (CCN) counter sampled from the tank. The measurements show that particles resulting from the combustion of the propellant are active IN (3.3 times 10 to the 8th to 1.5 times 10 to the 11th/g active at 20 C). The portable counters and filters detected significantly fewer IN than the isothermal cloud chamber. The propellant aerosol is a prolific source of CCN that swamped the instrument.

Hindman Ii, E. E.↗

NASA NTRS1978

Vertical profiles of condensation nuclei

Condensation nuclei measurements using a low supersaturation (about 10%) thermal gradient diffusion cloud chamber (TGDCC) and a high supersaturation (about 200%) expansion type instrument were compared on a series of three balloon flights over Laramie, Wyoming. In general, the two instruments produced similar vertical profiles but some discrepancies remain unexplained. Agreement between the two would indicate that the low supersaturations used in the TGDCC were still large enough to cause the instrument to count essentially all of the particles present. The TGDCC condensation nuclei (CN) counter was flown at several sites in both the Northern and Southern Hemispheres. The results indicate the existence of a relative maximum in the CN mixing ratio associated with the upper equatorial troposphere and what appears to be a worldwide constant mixing ratio of CN above 20-25 km.

Rosen, J. M.↗

NASA NTRS1974

In situ measurements of particulate number density and size distribution from an aircraft

Two different commercial particulate measuring instruments were flown aboard the NASA Convair 990. A condensation nuclei monitor was utilized to measure particles larger than approximately 0.003 micron in diameter. A specially designed pressurization system was used with this monitor at cabin altitude pressure. A near-forward light scattering counter was used to measure the number and size distribution particles in the size range from 0.5 to 5 microns and greater in diameter. Considerable variation in number density was encountered for both classes of particles at the test altitudes ranging from 5 to 12 km. Presence of clouds could be detected by the light scattering instrument because large numbers of particles would then be registered by the instrument, especially in the size range above 5.0 microns in diameter.

Briehl, D.↗

NASA NTRS1994

Condensation nuclei measurement in the stratosphere for the NASA ACE program

A condensation nucleus counter which operated at stratospheric pressures was developed, designed, and constructed. It was calibrated in the laboratory. Its response as a function of particle size and concentration was reported. This was the first time that the response of such an instrument was verified in the laboratory. An inlet was constructed which provided near isokinetic sampling. The resulting instrument, the U-2 CNC, was deployed on NASA U-2 aircraft in the study of the climatic effects of aerosol. These studies occurred in March, April, May, July, November, and December of 1992 and in April, May, June, and December of 1983. The U-2 CNC was used in the study of the aerosol cloud resulting from the eruption of El Chichon. It permitted the observation of new particle formation in the stratosphere.

Wilson, James Charles↗

NASA NTRS1990

Measurements of condensation nuclei in the Airborne Arctic Stratospheric Expedition - Observations of particle production in the polar vortex

The ER-2 Condensation Nucleus Counter (ER-2 CNC) was operated in the Airborne Arctic Stratospheric Expedition (AASE) in January and February 1989. The ER-2 CNC measures the mixing ratio of particles, CN, with diameters from approximately 0.02 to approximately 1 micron. The spatial distribution of CN in the Arctic polar vortex was found to resemble that measured in the Antarctic in the Spring of 1987. The vertical profile of CN in the vortex was lowered by subsidence. At altitudes above the minimum in the CN mixing ratio profile, CN mixing ratios correlated negatively with that of N2O, demonstrating new particle production. CN serve as nuclei in the formation of Polar Stratospheric Clouds (PSCs) and the concentration of CN can affect PSC properties.

Wilson, J. C.↗