Influence of particle size distribution on reflected and transmitted light from clouds
Particle size distribution effects on incident radiation from clouds calculated by Monte Carlo method
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Particle size distribution effects on incident radiation from clouds calculated by Monte Carlo method
Particle size distribution influence on reflected and transmitted light from clouds calculated by Monte Carlo technique
Increased aerosols can modify the shape of the cloud Particle Size Distribution (PSD), thereby influencing the radiative properties of clouds, known as the Dispersion Effect (DE). However, a global, observation-based quantification of its impact on Aerosol-Cloud Interactions (ACI) is lacking, leading to DE being typically ignored in satellite-based estimates of ACI forcing. Here we propose a physics-based method that combines polarimetric satellite data on cloud PSD to achieve global observational quantification of DE’s impact on ACI in liquid-phase stratiform clouds. Globally, DE offsets ACI changes induced by droplet number concentration variation and liquid water path adjustment by 7% and −1.4%, respectively. Furthermore, a parameterization based on the global dataset of PSD shape parameters is developed to improve DE estimation in large-scale models. Both the quantification and parameterization enhance our understanding of DE and facilitate the inclusion of this non-negligible impact of DE on ACI in estimating aerosol climate forcing.
Noctilucent cloud particle size composition and origin from sounding rocket flight and control collecting surfaces
Use of an improved single-particle light-scattering instrument for measurement of cloud microstructure in field studies. Cloud particle size and number information is measured over 12 sizing intervals, in the range from 4 to 85 microns in diameter. The microstructure can be observed in real time and with a spatial resolution not previously reported. The general features of water cloud droplet size and number distributions are consistent with previous direct capture and replication studies. The transition from water to ice phase regions in cumuliform clouds can be inferred from dramatic changes observed in the distribution features. Results are also presented for stratus and cirrus cloud penetrations.
AEROPOL infrared polarimeter was built for measurements microns between 1.1 and 3.5 microns, with a 1.5 degree field of view, using a wire grid polarization analyzer. A PbS detector is cooled by condensed Freon-13. The instrument operates under minicomputer control, giving a polarization least squares solution each 2.5 seconds. AEROPOL was flown on the NASA CV-990 aircraft, in a remote-sensing study of terrestrial cloud particle sizes and shapes.
An airborne remote sensing study of cloud particle sizes and shapes, performed with an IR polarimeter is described. Linear polarization for a given wavelength was measured as a function of the phase angle. Liquid water clouds are found to exhibit considerable detail in their polarization curves, including a positive cloudbow near 40-degrees phase angle, and negative polarization at phase angles of less than 20 degrees and greater than (roughly) 100 degrees. A polarization vs phase angle curve obtained for thick tropical cirrus clouds showed negative polarization at large and small phase angles, and positive polarization at angles between 20 and 145 degrees. There is no indication of a cloudbow or other detailed structure.
An infrared polarimeter was built to measure the degree of linear polarization and the direction of vibration of radiation scattered upwards by clouds, between 1.1 and 3.5 microns, with a 1.5-deg field of view, using a rotating wire-grid polarization analyzer. A PbS detector is cooled to 192 K by condensing freon-13. This AEROPOL instrument operates under minicomputer control, giving a polarization least-squares solution every 2.5 s. The polarimeter was flown on the NASA CV-990 aircraft, in a remote-sensing study of terrestrial cloud particle sizes and shapes.
Multiple scattering calculations are performed in order to investigate the nature of the circular polarization of sunlight reflected by planetary atmospheres. Contour diagrams as a function of size parameter and phase angle are made for the integrated light from a spherical but locally plane-parallel atmosphere of spherical particles. To investigate the origin of the circular polarization, results are also computed for second-order scattering and for a simpler semiquantitative model of scattering by two particles. Observations of the circular polarization of the planets are presently too meager for accurate deduction of cloud particle properties. However, certain very broad constraints can be placed on the properties of the dominant cloud particles on Jupiter and Saturn. The cloud particle size and refractive index deduced for the Jupiter clouds by Loskutov, Morozhenko, and Yanovitskii from analyses of the linear polarization are not consistent with the circular polarization. The few available circular polarization observations of Venus are also examined.
Preliminary results of the nephelometer experiments conducted aboard the large sounder, day, north, and night probes of the Pioneer Venus mission are presented. The vertical structures of the Venus clouds observed simultaneously at each of the four locations from altitudes of from 63 kilometers to the surface are compared, and similarities and differences are noted. Tentative results from attempting to use the data from the nephelometer and cloud particle size spectrometer on the sounder probe to identify the indices of refraction of cloud particles in various regions of the Venus clouds are reported. Finally the nephelometer readings for the day probe during impact on the surface of Venus are presented.
Airborne in situ exhaust cloud measurements were conducted to obtain definitions of cloud particle size range, Cl2 content, and HCl partitioning. Particle size distribution data and Cl2 measurements were made during the May, August, and September 1977 Titan launches. The measurements of three basic effluents - HCl, NO sub X, and particles - against minutes after launch are plotted. The maximum observed HCl concentration to the maximum Cl2 concentration are compared and the ratios of the Cl2 to the HCl is calculated.
The evidence for solid mode 3 particles in the clouds of Venus is reexamined. The sampling characteristics of the cloud particle size spectrometer (LCPS) are reviewed, and reasons are pointed out for believing that relatively small differences in interpreting the measurements of this instrument could produce systematic errors. It is shown that all of the Pioneer Venus and Venera measurements can be understood if it is assumed that the large particles observed by the LCPS form the tail of the mode 2, H2SO4 size distribution.
Coincident measurements of cirrus cloud microphysical properties such as particle size distribution and particle shape and morphology, and measurements of infrared intensity and flux were made. Data was acquired nearly simultaneously in space and time by a KingAir in cloud and by an ER-2 at an altitude of 19 km. Upwelling infrared intensities and fluxes measured from the ER-2 and observations of cloud particle size distributions and particle phase and morphology made from the KingAir are discussed. Broad-band flux measurements were available both in and below the cirrus layer from the KingAir.
Theoretical calculations predict that cloud reflectance in near infrared windows such as those at 1.6 and 2.2 microns should give lower reflectances than at visible wavelengths. The reason for this difference is that ice and liquid water show significant absorption at those wavelengths, in contrast to the nearly conservative scattering at wavelengths shorter than 1 micron. In addition, because the amount of absorption scales with the path length of radiation through the particle, increasing cloud particle size should lead to decreasing reflectances at 1.6 and 2.2 microns. Measurements at these wavelengths to date, however, have often given unpredicted results. Twomey and Cocks found unexpectedly high absorption (factors of 3 to 5) in optically thick liquid water clouds. Curran and Wu found expectedly low absorption in optically thick high clouds, and postulated the existence of supercooled small water droplets in place of the expected large ice particles. The implications of the FIRE data for optically thin cirrus are examined.
Advances in lidar and radar technology have potential for providing new and better information on climate significant parameters of cirrus. Consequently, the NOAA Wave Propagation Lab. is commencing CLARET (Cloud Lidar And Radar Exploratory Test) to evaluate the promise of these new capabilities. Parameters under study include cloud particle size distribution, height of cloud bases, tops, and multiple layers, and cloud dynamics revealed through measurement of vertical motions. The first phase of CLARET is planned for Sept. 1989. The CO2 coherent Doppler lidar and the sensitive K sub a band radar hold promise for providing valuable information on cirrus that is beyond the grasp of current visible lidars.
Data collected during flight 9 of the Stratosphere-Troposphere Exchange Project (STEP), in Australia (1987), are used in an attempt to define the nature of one particular cirrus outflow region and its radiative impact. To explore the mechanisms by which air is exchanged between the stratosphere and troposphere, a series of instruments was flown on the NASA ER-2 high-altitude research aircraft to make measurements relevant to the radiative budget of tropical clouds. The data acquired included upwelling infrared radiance at 10.5 and 6.5 microns (spectral bandwidth of 1 micron); net infrared flux (spectral bandwidth of 3 to 40 microns); cloud particle size distribution; water-vapor and total water (vapor plus condensed phase); aerosol particle size distribution; and ambient temperature.
A new instrument, the Probe Infrared Laser Spectrometer (PIRLS), is described for in situ sensing of the gas composition and particle size distribution of Titan's atmosphere on the NASA/ESA Cassini mission. For gas composition measurements, several narrow-band (0.0001/cm) tunable lead-salt diode lasers operating near 80 K at selected mid-IR wavelengths are directed over a path length defined by a small reflector extending over the edge of the probe spacecraft platform; volume mixing ratios of 10 to the -9th should be measurable for several species of interest. A cloud-particle-size spectrometer using a diode laser source at 780 nm shares the optical path and deployed reflector; a combination of imaging and light scattering techniques is used to determine sizes of haze and cloud particles and their number density as a function of altitude.
The extinction characteristics of thin ice-crystal clouds over the oceanic convective rain belts in the tropics and midlatitudes, obtained from the infrared interferometer spectrometer flown on Nimbus 4 satellite in 1970 are examined. It is observed that the optical depth of these clouds in the RF window region is less than 3 and their spectral features are consistent with the cloud particle size of about 10 micron. These optically-thin ice-crystal clouds are extensions of the anvil clouds generated by deep convective systems. The existence of such clouds extending from the upper troposphere into the lower stratosphere in the polar regions during winter and early spring is indicated, and the result of a theoretical simulation are analyzed.