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NASA NTRS2021

Less Atmospheric Radiative Heating By Dust Due to the Synergy of Coarser Size and Aspherical Shape

Mineral dust aerosols cool and warm the atmosphere by scattering and absorbing solar (shortwave: SW) and thermal (longwave: LW) radiation. However, significant uncertainties remain in dust radiative effects, largely due to differences in the dust size distribution and spectral optical properties simulated in Earth system models. Dust models typically underestimate the coarse dust load (more than 2.5 µm in diameter) and assume a spherical shape, which leads to an overestimate of the fine dust load (less than 2.5 µm) after the dust emissions in the models are scaled to match observed dust aerosol optical depth at 550 nm (DAOD550). Here, we improve the simulated dust properties with data sets that leverage measurements of size-resolved dust concentration, asphericity factor, and refractive index in a coupled global chemical transport model with a radiative transfer module. After the adjustment of size-resolved dust concentration and spectral optical properties, the global and annual average of DAOD550 from the simulation increases from 0.023 to 0.029 and falls within the range of a semi-observationally based estimate (0.030 ± 0.005). The reduction of fine dust load after the adjustment leads to a reduction of the SW cooling at the top of the atmosphere (TOA). To improve agreement against a semi-observationally based estimate of the radiative effect efficiency at TOA, we find that a less absorptive SW dust refractive index is required for coarser aspherical dust. Thus, only a minor difference is estimated for the net global dust radiative effect at TOA (−0.08 vs. −0.00 W m−2 on a global scale). Conversely, our sensitivity simulations reveal that the surface warming is substantially enhanced near the strong dust source regions (less cooling to −0.23 from −0.60 W m−2 on a global scale). Thus, less atmospheric radiative heating is estimated near the major source regions (less heating to 0.15 from 0.59 W m−2 on a global scale), because of enhanced LW warming at the surface by the synergy of coarser size and aspherical shape.

simulated dust properties↗

NASA NTRS2022

Importance of Different Parameterization Changes for the Updated Dust Cycle Modeling in the Community Atmosphere Model (Version 6.1)

The Community Atmosphere Model (CAM6.1), the atmospheric component of the Community Earth System Model (CESM; version 2.1), simulates the life cycle (emission, transport, and deposition) of mineral dust and its interactions with physio-chemical components to quantify the impacts of dust on climate and the Earth system. The accuracy of such quantifications relies on how well dust-related processes are represented in the model. Here we update the parameterizations for the dust module, including those on the dust emission scheme, the aerosol dry deposition scheme, the size distribution of transported dust, and the treatment of dust particle shape. Multiple simulations were undertaken to evaluate the model performance against diverse observations, and to understand how each update alters the modeled dust cycle and the simulated dust direct radiative effect. The model–observation comparisons suggest that substantially improved model representations of the dust cycle are achieved primarily through the new more physically-based dust emission scheme. In comparison, the other modifications induced small changes to the modeled dust cycle and model–observation comparisons, except the size distribution of dust in the coarse mode, which can be even more influential than that of replacing the dust emission scheme. We highlight which changes introduced here are important for which regions, shedding light on further dust model developments required for more accurately estimating interactions between dust and climate.

mineral dust parameterizations↗

NASA NTRS2013

Shape-induced Gravitational Sorting of Saharan Dust During Transatlantic Voyage: Evidence from CALIOP Lidar Depolarization Measurements

Motivated by the physical picture of shape-dependent air resistance and, consequently, shape-induced differential sedimentation of dust particles, we searched for and found evidence of dust particle asphericity affecting the evolution and distribution of dust-scattered light depolarization ratio (delta). Specifically, we examined a large data set of Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) observations of Saharan dust from June to August 2007. Observing along a typical transatlantic dust track, we find that (1) median delta is uniformly distributed between 2 and 5 km altitudes as the elevated dust leaves the west coast of Africa, thereby indicating uniformly random mixing of particle shapes with height; (2) vertical homogeneity of median delta breaks down during the westward transport: between 2 and 5 km delta increases with altitude and this increase becomes more pronounced with westward progress; (3) delta tends to increase at higher altitude (greater than 4 km) and decrease at lower altitude (less than 4 km) during the westward transport. All these features are captured qualitatively by a minimal model (two shapes only), suggesting that shape-induced differential settling and consequent sorting indeed contribute significantly to the observed temporal evolution and vertical stratification of dust properties. By implicating particle shape as a likely cause of gravitational sorting, these results will affect the estimates of radiative transfer through Saharan dust layers.

CALIPSO↗

NASA NTRS2014

CALIPSO Observations of Transatlantic Dust: Vertical Stratification and Effect of Clouds

We use CALIOP nighttime measurements of lidar backscatter, color and depolarization ratios, as well as particulate retrievals during the summer of 2007 to study transatlantic dust properties downwind of Saharan sources, and to examine the influence of nearby clouds on dust. Our analysis suggests that (1) under clear skies, while lidar backscatter and color ratio do not change much with altitude and longitude in the Saharan Air Layer (SAL), depolarization ratio increases with altitude and decreases westward in the SAL (2) the vertical lapse rate of dust depolarization ratio, introduced here, increases within SAL as plumes move westward (3) nearby clouds barely affect the backscatter and color ratio of dust volumes within SAL but not so below SAL. Moreover, the presence of nearby clouds tends to decrease the depolarization of dust volumes within SAL. Finally, (4) the odds of CALIOP finding dust below SAL next to clouds are about of those far away from clouds. This feature, together with an apparent increase in depolarization ratio near clouds, indicates that particles in some dust volumes loose asphericity in the humid air near clouds, and cannot be identified by CALIPSO as dust.

CALIPSO↗

DOE OSTI2020

Apparent dust size discrepancy in aerosol reanalysis in north African dust after long-range transport

North African dust reaches the southeastern United States every summer. Size-resolved dust mass measurements taken in Miami, Florida, indicate that more than one-half of the surface dust mass concentrations reside in particles with geometric diameters less than 2.1 µm, while vertical profiles of micropulse lidar depolarization ratios show dust reaching above 4 km during pronounced events. These observations are compared to the representation of dust in the Modern-Era Retrospective analysis for Research and Applications, version 2 (MERRA-2) aerosol reanalysis and closely related Goddard Earth Observing System model version 5 (GEOS-5) Forward Processing (FP) aerosol product, both of which assimilate satellite-derived aerosol optical depths using a similar protocol and inputs. These capture the day-to-day variability in aerosol optical depth well, in a comparison to an independent sun-photometer-derived aerosol optical depth dataset. Most of the modeled dust mass resides in diameters between 2 and 6 µm, in contrast to the measurements. Model-specified mass extinction efficiencies equate light extinction with approximately 3 times as much aerosol mass, in this size range, compared to the measured dust sizes. GEOS-5 FP surface-layer sea salt mass concentrations greatly exceed observed values, despite realistic winds and relative humidities. In combination, these observations help explain why, despite realistic total aerosol optical depths, (1) free-tropospheric model volume extinction coefficients are lower than those retrieved from the micro-pulse lidar, suggesting too-low model dust loadings in the free troposphere, and (2) model dust mass concentrations near the surface can be higher than those measured. The modeled vertical distribution of dust, when captured, is reasonable. Large, aspherical particles exceeding the modeled dust sizes are also occasionally present, but dust particles with diameters exceeding 10 µm contribute little to the measured total dust mass concentrations after such long-range transport. Remaining uncertainties warrant a further integrated assessment to confirm this study's interpretations.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS2020

Apparent dust size discrepancy in aerosol reanalysis in north African dust after long-range transport

MEERA-2 aerosols reanalysis↗

NASA NTRS2011

A Sensitivity Study on the Effects of Particle Chemistry, Asphericity and Size on the Mass Extinction Efficiency of Mineral Dust in the Earth's Atmosphere: From the Near to Thermal IR

To determine a plausible range of mass extinction efficiencies (MEE) of terrestrial atmospheric dust from the near to thermal IR, sensitivity analyses are performed over an extended range of dust microphysical and chemistry perturbations. The IR values are subsequently compared to those in the near-IR, to evaluate spectral relationships in their optical properties. Synthesized size distributions consistent with measurements, model particle size, while composition is defined by the refractive indices of minerals routinely observed in dust, including the widely used OPAC/Hess parameterization. Single-scattering properties of representative dust particle shapes are calculated using the T-matrix, Discrete Dipole Approximation and Lorenz-Mie light-scattering codes. For the parameterizations examined, MEE ranges from nearly zero to 1.2 square meters per gram, with the higher values associated with non-spheres composed of quartz and gypsum. At near-IR wavelengths, MEE for non-spheres generally exceeds those for spheres, while in the thermal IR, shape-induced changes in MEE strongly depend on volume median diameter (VMD) and wavelength, particularly for MEE evaluated at the mineral resonant frequencies. MEE spectral distributions appear to follow particle geometry and are evidence for shape dependency in the optical properties. It is also shown that non-spheres best reproduce the positions of prominent absorption peaks found in silicates. Generally, angular particles exhibit wider and more symmetric MEE spectral distribution patterns from 8-10 micrometers than those with smooth surfaces, likely due to their edge-effects. Lastly, MEE ratios allow for inferring dust optical properties across the visible-IR spectrum. We conclude the MEE of dust aerosol are significant for the parameter space investigated, and are a key component for remote sensing applications and the study of direct aerosol radiative effects.

Hansell, R. A., Jr.↗

NASA NTRS2000

Desert Dust Layers Over Polluted Marine Boundary Layers: ACE-2 Measurements and ACE-Asia Plans

Aerosols in ACE-Asia are expected to have some commonalties with those in ACE-2, along with important differences. Among the commonalities are occurrences of desert dust layers over polluted marine boundary layers. Differences include the nature of the dust (yellowish in the East Asia desert outflow, vs. reddish-brown in the Sahara Outflow measured in ACE-2) and the composition of boundary-layer aerosols (e.g., more absorbing, soot and organic aerosol in-the Asian plume, caused by coal and biomass burning, with limited controls). In this paper we present ACE-2 measurements and analyses as a guide to our plans for ACE-2 Asia. The measurements include: (1) Vertical profiles of aerosol optical depth and extinction (380-1558 nm), and of water vapor column and concentration, from the surface through the elevated desert dust, measured by the 14-channel Ames Airborne Tracking Sunphotometer (AATS-14); (2) Comparisons of airborne and shipborne sunphotometer optical depths to satellite-retrieved values, with and without desert dust; (3) Comparisons between airborne Sunphotometer optical depth and extinction spectra and those derived from coincident airborne in situ measurements of aerosol size distribution, scattering and absorption; (4) Comparisons between size distributions measured in situ and retrieved from sunphotometer optical depth spectra; (5) Comparisons between aerosol single scattering albedo values obtained by several techniques, using various combinations of measurements of backscatter, extinction, size distribution, scattering, absorption, and radiative flux. We show how analyses of these data can be used to address questions important to ACE-Asia, such as: (1) How do dust and other absorbing aerosols affect the accuracy of satellite optical depth retrievals? How important are asphericity effects? (2) How important are supermicron dust and seasalt aerosols to overall aerosol optical depth and radiative forcing? How well are these aerosols sampled by aircraft inlets and instruments? (3) How consistent are suborbital in situ and remote measurements of aerosols, among themselves and with satellite retrievals? What are the main reasons for observed inconsistencies?

Russell, Philip B.↗

DOE OSTI2024

On the force exerted on a non-spherical asymmetric dust grain from homogeneous, stationary, isotropic, non-magnetized plasma

Whereas the conventional wisdom suggests that the force between non-magnetized homogeneous, stationary, isotropic plasma, and the dust grain is only possible for the case of relative plasma–grain velocity, it is shown that stationary non-spherical asymmetric dust grain immersed in stationary, non-magnetized, isotropic plasma can experience a force caused by the grain–plasma interactions. The component of the force due to scattering of plasma particles in the limit of infinite Debye length is considered analytically. Both the particle scattering and absorption force components are modeled numerically in the limits of infinite and finite Debye length using a newly developed 2D3V Aspherical Particle-in-Cell code. The code simulates interactions of dust grain of selected non-spherical asymmetric shape with plasmas using dust shape conforming coordinates. Here, the simulations confirm the existence of the force on non-spherical asymmetric grain in stationary non-magnetized plasma and show that the plasma screening effects can lead to reversal of the force direction.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

NASA NTRS2012

CALIPSO Observations of Transatlantic Dust: Vertical Stratification and Effect of Clouds

CALIOP nighttime measurements of lidar backscatter, color and depolarization ratios during the summer of 2007 are used to study transatlantic dust properties downwind of Saharan sources, and to examine the interaction of clouds and dust. We discuss the following findings: (1) while lidar backscatter doesn't change much with altitude in the Saharan Air Layer (SAL), depolarization and color ratios both increase with altitude in the SAL; (2) lidar backscatter and color ratio increase as dust is transported westward in the SAL; (3) the vertical lapse rate of dust depolarization ratio increases within SAL as plumes move westward; (4) nearby clouds barely affect the backscatter and color ratio of dust volumes within SAL but not so below SAL. Finally, (5) the odds of CALIOP finding dust below SAL next to clouds are about 2/3 of those far away from clouds. This feature, together with an apparent increase in depolarization ratio near clouds, indicates that particles in some dusty volumes lose asphericity in the humid air near clouds, and cannot be identified by CALIPSO as dust.

Yang, Weidong↗

NASA NTRS2011

Light Scattering by Wavelength-Sized Particles "Dusted" with Subwavelength-Sized Grains

The numerically exact superposition T-matrix method is used to compute the scattering cross sections and the Stokes scattering matrix for polydisperse spherical particles covered with a large number of much smaller grains. We show that the optical effect of the presence of microscopic dust on the surfaces of wavelength-sized, weakly absorbing particles is much less significant than that of a major overall asphericity of the particle shape.

Mishchenko, Michael I.↗

NASA NTRS2014

A Multi-Wavelength Investigation of the Radio-Loud Supernova PTF11qcj and its Circumstellar Environment

We present the discovery, classification, and extensive panchromatic (from radio to X-ray) follow-up observations of PTF11qcj, a supernova (SN) discovered by the Palomar Transient Factory (PTF). Our observations with the Karl G. Jansky Very Large Array show that this event is radio-loud: PTF11qcj reached a radio peak luminosity comparable to that of the famous gamma-ray-burst-associated SN 1998bw (L (sub 5 gigahertz) approximates 10 (sup 29) ergs per second per hertz). PTF11qcj is also detected in X-rays with the Chandra Observatory, and in the infrared band with Spitzer. Our multi-wavelength analysis probes the SN interaction with circumstellar material. The radio observations suggest a progenitor mass-loss rate of approximately 10 (sup -4) the mass of the sun per year times (v (sub omega) divided by 1000 kilometers per second), and a velocity of approximately 0.3-0.5 c (the speed of light in a vacuum) for the fastest moving ejecta (at around 10 days after explosion). However, these estimates are derived assuming the simplest model of SN ejecta interacting with a smooth circumstellar wind, and do not account for possible inhomogeneities in the medium and asphericity of the explosion. The radio data show deviations from such a simple model, as well as a late-time re-brightening. The X-ray flux from PTF11qcj is compatible with the high-frequency extrapolation of the radio synchrotron emission (within the large uncertainties). A light echo from pre-existing dust is in agreement with our infrared data. Our pre-explosion data from the PTF suggest that a precursor eruption of absolute magnitude M (sub r) approximately equal to -13 mag may have occurred approximately 2.5 years prior to the SN explosion. Overall, PTF11qcj fits the expectations from the explosion of a Wolf-Rayet star. Precursor eruptions may be a feature characterizing the final pre-explosion evolution of such stars.

Radio↗

NASA NTRS2009

NASA Tech Briefs, March 2009

Topics covered include: Improved Instrument for Detecting Water and Ice in Soil; Real-Time Detection of Dust Devils from Pressure Readings; Determining Surface Roughness in Urban Areas Using Lidar Data; DSN Data Visualization Suite; Hamming and Accumulator Codes Concatenated with MPSK or QAM; Wide-Angle-Scanning Reflectarray Antennas Actuated by MEMS; Biasable Subharmonic Membrane Mixer for 520 to 600 GHz; Hardware Implementation of Serially Concatenated PPM Decoder; Symbolic Processing Combined with Model-Based Reasoning; Presentation Extensions of the SOAP; Spreadsheets for Analyzing and Optimizing Space Missions; Processing Ocean Images to Detect Large Drift Nets; Alternative Packaging for Back-Illuminated Imagers; Diamond Machining of an Off-Axis Biconic Aspherical Mirror; Laser Ablation Increases PEM/Catalyst Interfacial Area; Damage Detection and Self-Repair in Inflatable/Deployable Structures; Polyimide/Glass Composite High-Temperature Insulation; Nanocomposite Strain Gauges Having Small TCRs; Quick-Connect Windowed Non-Stick Penetrator Tips for Rapid Sampling; Modeling Unsteady Cavitation and Dynamic Loads in Turbopumps; Continuous-Flow System Produces Medical-Grade Water; Discrimination of Spore-Forming Bacilli Using spoIVA; nBn Infrared Detector Containing Graded Absorption Layer; Atomic References for Measuring Small Accelerations; Ultra-Broad-Band Optical Parametric Amplifier or Oscillator; Particle-Image Velocimeter Having Large Depth of Field; Enhancing SERS by Means of Supramolecular Charge Transfer; Improving 3D Wavelet-Based Compression of Hyperspectral Images; Improved Signal Chains for Readout of CMOS Imagers; SOI CMOS Imager with Suppression of Cross-Talk; Error-Rate Bounds for Coded PPM on a Poisson Channel; Biomorphic Multi-Agent Architecture for Persistent Computing; and Using Covariance Analysis to Assess Pointing Performance.

Source record↗