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A review of coarse mineral dust in the Earth system

Mineral dust particles suspended in the atmosphere span more than three orders of magnitude in diameter, from <0.1 µm to more than 100 µm. This wide size range makes dust a unique aerosol species with the ability to interact with many aspects of the Earth system, including radiation, clouds, hydrology, atmospheric chemistry, and biogeochemistry. This review focuses on coarse and super-coarse dust aerosols, which we respectively define as dust particles with a diameter of 2.5–10 µm and 10–62.5 µm. We review several lines of observational evidence indicating that coarse and super-coarse dust particles are transported farther than previously expected and that the abundance of these particles is substantially underestimated in current global models. We synthesize previous studies that used observations, theories, and model simulations to highlight the impacts of coarse and super-coarse dust aerosols on the Earth system, including their effects on dust-radiation interactions, dust-cloud interactions, atmospheric chemistry, and biogeochemistry. Specifically, coarse and super-coarse dust aerosols produce a net positive direct radiative effect (warming) at the top of the atmosphere and can modify temperature and water vapor profiles, influencing the distribution of clouds and precipitation. In addition, coarse and super-coarse dust aerosols contribute a substantial fraction of ice-nucleating particles, especially at temperatures above –23 °C. They also contribute a substantial fraction to the available reactive surfaces for atmospheric processing and the dust deposition flux that impacts land and ocean biogeochemistry by supplying important nutrients such as iron and phosphorus. Furthermore, we examine several limitations in the representation of coarse and super-coarse dust aerosols in current model simulations and remote-sensing retrievals. Because these limitations substantially contribute to the uncertainties in simulating the abundance and impacts of coarse and super-coarse dust aerosols, we offer some recommendations to facilitate future studies. Overall, we conclude that an accurate representation of coarse and super-coarse properties is critical in understanding the impacts of dust aerosols on the Earth system.

54 ENVIRONMENTAL SCIENCES↗

Impact of Dust-Cloud-Radiation-Precipitation Dynamical Feedback on Subseasonal-to-Seasonal Variability of the Asian Summer Monsoon in Global Variable-Resolution Simulations With MPAS-CAM5

In this study, we investigate the effects of increased dust emission from the Middle East deserts on subseasonal-to-seasonal (S₂S) variability of the Asian summer monsoon (ASM). Numerical experiments are performed using the Model for Prediction Across Scales (MPAS) coupled with the Community Atmosphere Model (CAM5) physics, with regional refinement at 30 km grid resolution over South Asia and the surrounding regions. Result shows that increased dust emission and transport from the Middle East/West Asia region induces a strong dust-cloud-radiation-precipitation-circulation feedback, resulting in a colder surface over the desert regions and the western Tibetan Plateau, but warmer and moister troposphere with enhanced cloudiness and precipitation over the Pakistan/Northwest India (PNWI) region. The latter changes are amplified by the dust aerosol induced Elevated Heat Pump (EHP) mechanism along the West Himalayas/Iranian Plateau foothill regions, most pronounced during May-June. During July-August, cloud radiation feedback further enhances the warming of the upper troposphere, and cooling of the land surface over the PNWI and adjacent regions over West Asia. The upper tropospheric heating and increased precipitation over PNWI spur a large-scale anomalous Rossby wavetrain and a northward displacement of the subtropical jetstream, manifesting in a contraction of the South Asian High and westward shift of the Western Pacific Subtropical High. As a result, the entire ASM precipitation-cloud system is displaced westward. Precipitation and cloudiness are intensified over northwest and western India and west Asia, but suppressed over southern and central East Asia. Analyses of the S₂S variability of the upper level vorticity balance suggests that heating by Middle East dust plays an important role in exciting, and anchoring a teleconnection pattern through interactions among dust-cloud radiation, precipitation heating over the PNWI, the development of an upper level Rossby wavetrain, and the northward shift of the boreal summer jetstream over Eurasia.

54 ENVIRONMENTAL SCIENCES↗

Importance of Different Parameterization Changes for the Updated Dust Cycle Modeling in the Community Atmosphere Model (Version 6.1)

The Community Atmosphere Model (CAM6.1), the atmospheric component of the Community Earth System Model (CESM; version 2.1), simulates the life cycle (emission, transport, and deposition) of mineral dust and its interactions with physio-chemical components to quantify the impacts of dust on climate and the Earth system. The accuracy of such quantifications relies on how well dust-related processes are represented in the model. Here we update the parameterizations for the dust module, including those on the dust emission scheme, the aerosol dry deposition scheme, the size distribution of transported dust, and the treatment of dust particle shape. Multiple simulations were undertaken to evaluate the model performance against diverse observations, and to understand how each update alters the modeled dust cycle and the simulated dust direct radiative effect. The model–observation comparisons suggest that substantially improved model representations of the dust cycle are achieved primarily through the new more physically-based dust emission scheme. In comparison, the other modifications induced small changes to the modeled dust cycle and model–observation comparisons, except the size distribution of dust in the coarse mode, which can be even more influential than that of replacing the dust emission scheme. We highlight which changes introduced here are important for which regions, shedding light on further dust model developments required for more accurately estimating interactions between dust and climate.

mineral dust parameterizations↗

Synergy of Satellite-Surface Observations for Studying the Properties of Absorbing Aerosols in Asia

Through interaction with clouds and alteration of the Earth's radiation budget, atmospheric aerosols significantly influence our weather and climate. Monsoon rainfalls, for example, sustain the livelihood of more than half of the world's population. Thus, understanding the mechanism that drives the water cycle and freshwater distribution is high-lighted as one of the major near-term goals in NASA's Earth Science Enterprise Strategy. Every cloud droplet/ice-crystal that serves as an essential element in portraying water cycle and distributing freshwater contains atmospheric aerosols at its core. In addition, the spatial and temporal variability of atmospheric aerosol properties is complex due to their dynamic nature. In fact, the predictability of the tropical climate system is much reduced during the boreal spring, which is associated with the peak season of biomass burning activities and regional/long-range transport of dust aerosols. Therefore, to accurately assess the impact of absorbing aerosols on regional-to-global climate requires not only modeling efforts but also continuous observations from satellites, aircraft, networks of ground-based instruments and dedicated field experiments. Since 1997 NASA has been successfully launching a series of satellites the Earth Observing System - to intensively study, and gain a better understanding of, the Earth as an integrated system. Through participation in many satellite remote-sensing/retrieval and validation projects over the years, we have gradually developed and refined the SMART (Surface-sensing Measurements for Atmospheric Radiative Transfer) and COMMIT (Chemical, Optical & Microphysical Measurements of In-situ Troposphere) mobile observatories, a suite of surface remote sensing and in-situ instruments that proved to be vital in providing high temporal measurements, which complement the satellite observations. In this talk, we will present SMART-COMMIT which has played key roles, serving as network or supersite, in major international research projects such as the Joint Aerosol Monsoon Experiment (JAM EX), a core element of the Asian Monsoon Years (AMY, 2008-2012). SMART-COMMIT deployments during 2008 AMY/JAMEX were conducted in northwestern China to characterize the properties of dust-laden aerosols and in the vicinity of Beijing for mega-city aerosols. In 2009, SMART-COMMIT also participated in the JAMEX/RAJO-MEGHA (Radiation, Aerosol Joint Observations-Monsoon Experiment in the Gangetic-Himalayan Area; Sanskrit for Dust-Cloud) to study the aerosol properties, solar absorption and the associated atmospheric warming, and the climatic impact of elevated aerosols during the pre-monsoon season in South Asia. We will show results from these field experiments, as well as discuss a new initiative of 7-SEAS (7 South East Asian Studies) to study the interaction of anthropogenic aerosols with regional meteorology, particularly with clouds.

Tsay, Si-Chee↗