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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 19 records
All sourcesNASA NTRSDOE OSTI
DOE OSTI2019

Homonuclear dipolar recoupling of arbitrary pairs in multi-spin systems under magic angle spinning: A double-frequency-selective ZQ-SEASHORE experiment

We introduce a useful method for measuring the internuclear distances within arbitrarily selected pairs of like nuclei in dipolar-coupled multi-spin systems. The approach uses a combination of the zero-quantum shift-evolution-assisted selective homonuclear recoupling (ZQ-SEASHORE) technique developed by Hu and Tycko [ J. Chem. Phys. 2009, 131, 045101] and double-frequency-selective radio-frequency pulse. The double-frequency-selective pulse inverts polarizations of two spins simultaneously, and thus applications of the method presented here are only limited by the spectral resolution, and not by the number of interacting spins. Our experiments demonstrate the validity of the method and present analytical expressions for the dephasing curve.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2026

Calibration and Data Analysis of a Frequency Selectable Laser Source for CMB Detector Characterization

Cosmic Microwave Background (CMB) experiments study faint radiation left over from the early universe. The CMB was created when the universe became cool enough for light to travel freely through space, and today it gives scientists one of the earliest images of the universe. One important goal of modern CMB experiments is to measure this radiation with higher precision in order to search for evidence that supports the theory of cosmic inflation. To do this, scientists use extremely sensitive detectors that must be calibrated accurately. The Frequency Selectable Laser Source, or FLS, is a new calibration tool that can send selected frequencies to detectors and help measure their response. During my internship, I worked on the FLS after it returned to Fermilab from Chile, where it had been used to characterize detectors at the Simons Observatory. The system came back in parts, so the first part of my project was helping rebuild the optical and mechanical setup. After the system was rebuilt, we performed alignments to maximize the receiver photocurrent. We then collected calibration measurements over different frequency ranges, including 543 GHz to 568 GHz, 740 GHz to 766 GHz, and 60 GHz to 500 GHz. These measurements were used to check waterline calibration and reflectivity features and compare new data with previous data. Another major part of my project was learning Python so I could understand previous analysis code, modify it for new files, and write my own code to compare the mean response between datasets. The results showed that the new data was close to previous measurements and that waterline features near 556 GHz and 752 GHz were found within less than 1.5 GHz of the expected values. I also completed the reflectivity analysis for five prisms in two polarization orientations. In the original orientation, the results were consistent between the five prisms and close to values measured on a different system at the University of Chicago. I then collected a second set of measurements on my own with the polarization of the laser rotated by 90 degrees and compared them with the original data using the same Python workflow. The measured reflectivity increased for all five prisms in the new orientation, showing that the prism reflectivity depends on polarization. Future work will focus on using the FLS to characterize real CMB detectors.

Pumarino, Rafael [Unlisted]↗
DOE OSTI2026

Calibration and Data Analysis of a Frequency Selectable Laser Source for CMB Detector Characterization

Cosmic Microwave Background (CMB) experiments study faint radiation left over from the early universe. The CMB was created when the universe became cool enough for light to travel freely through space, and today it gives scientists one of the earliest images of the universe. One important goal of modern CMB experiments is to measure this radiation with higher precision in order to search for evidence that supports the theory of cosmic inflation. To do this, scientists use extremely sensitive detectors that must be calibrated accurately. The Frequency Selectable Laser Source, or FLS, is a new calibration tool that can send selected frequencies to detectors and help measure their response. During my internship, I worked on the FLS after it returned to Fermilab from Chile, where it had been used to characterize detectors at the Simons Observatory. The system came back in parts, so the first part of my project was helping rebuild the optical and mechanical setup. After the system was rebuilt, we performed alignments to maximize the receiver photocurrent. We then collected calibration measurements over different frequency ranges, including 543 GHz to 568 GHz, 740 GHz to 766 GHz, and 60 GHz to 500 GHz. These measurements were used to check waterline calibration and reflectivity features and compare new data with previous data. Another major part of my project was learning Python so I could understand previous analysis code, modify it for new files, and write my own code to compare the mean response between datasets. The results showed that the new data was close to previous measurements and that waterline features near 556 GHz and 752 GHz were found within less than 1.5 GHz of the expected values. I also completed the reflectivity analysis for five prisms in two polarization orientations. In the original orientation, the results were consistent between the five prisms and close to values measured on a different system at the University of Chicago. I then collected a second set of measurements on my own with the polarization of the laser rotated by 90 degrees and compared them with the original data using the same Python workflow. The measured reflectivity increased for all five prisms in the new orientation, showing that the prism reflectivity depends on polarization. Future work will focus on using the FLS to characterize real CMB detectors.

Pumarino Meza, Rafael [Unlisted, US; Fermilab]↗
DOE OSTI2026

Calibration and Data Analysis of a Frequency Selectable Laser Source for CMB Detector Characterization

Cosmic Microwave Background (CMB) experiments study faint radiation left over from the early universe. The CMB was created when the universe became cool enough for light to travel freely through space, and today it gives scientists one of the earliest images of the universe. One important goal of modern CMB experiments is to measure this radiation with higher precision in order to search for evidence that supports the theory of cosmic inflation. To do this, scientists use extremely sensitive detectors that must be calibrated accurately. The Frequency Selectable Laser Source, or FLS, is a new calibration tool that can send selected frequencies to detectors and help measure their response. During my internship, I worked on the FLS after it returned to Fermilab from Chile, where it had been used to characterize detectors at the Simons Observatory. The system came back in parts, so the first part of my project was helping rebuild the optical and mechanical setup. After the system was rebuilt, we performed alignments to maximize the receiver photocurrent. We then collected calibration measurements over different frequency ranges, including 543 GHz to 568 GHz, 740 GHz to 766 GHz, and 60 GHz to 500 GHz. These measurements were used to check waterline calibration and reflectivity features and compare new data with previous data. Another major part of my project was learning Python so I could understand previous analysis code, modify it for new files, and write my own code to compare the mean response between datasets. The results showed that the new data was close to previous measurements and that waterline features near 556 GHz and 752 GHz were found within less than 1.5 GHz of the expected values. I also completed the reflectivity analysis for five prisms in two polarization orientations. In the original orientation, the results were consistent between the five prisms and close to values measured on a different system at the University of Chicago. I then collected a second set of measurements on my own with the polarization of the laser rotated by 90 degrees and compared them with the original data using the same Python workflow. The measured reflectivity increased for all five prisms in the new orientation, showing that the prism reflectivity depends on polarization. Future work will focus on using the FLS to characterize real CMB detectors.

Pumarino Meza, Rafael [Unlisted, US; Fermilab]↗
DOE OSTI2017

Full Waveform Inversion with Multisource Frequency Selection of Marine Streamer Data

The theory and practice of multisource full waveform inversion of marine supergathers are described with a frequency-selection strategy. The key enabling property of frequency selection is that it eliminates the crosstalk among sources, thus overcoming the aperture mismatch of marine multisource inversion. Tests on multisource full waveform inversion of synthetic marine data and Gulf of Mexico data show speedups of 4× and 8×, respectively, compared to conventional full waveform inversion.

58 GEOSCIENCES↗
DOE OSTI2026

Background cancellation for frequency-selective quantum sensing

A key challenge in quantum sensing is the detection of weak time dependent signals, particularly those that arise as specific frequency perturbations over a background field. Conventional methods usually demand complex dynamical control of the quantum sensor and heavy classical post-processing. We propose a quantum sensor that leverages time independent interactions and entanglement to function as a passive, tunable, thresholded frequency filter. By encoding the frequency selectivity and thresholding behavior directly into the dynamics, the sensor is responsive only to a target frequency of choice whose amplitude is above a threshold. This approach circumvents the need for complex control schemes and reduces the post-processing overhead.

Puig, Ricard [Los Alamos; Ecole Polytechnique, Lau↗
DOE OSTI2019

Dynamics of frequency-selective operation of a CO laser tunable in a wide spectral range

This paper presents a computational/theoretical analysis of the generation of a single pulse by a frequency-selective electron-beam sustained discharge CO laser. The calculations have been performed using a theoretical model in which the entire set of VV exchange processes involving CO molecules at high vibrational levels is taken into full account. We present calculated pulse shapes for a wide range of transitions, including transitions between high vibrational levels, and examine the possibility of raising the laser output intensity by optimising the density and composition of the gain medium. (paper)

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2026

An upgraded frequency-selectable laser source (FLS) calibrator for CMB bandpass characterization

One of the biggest challenges for Cosmic Microwave Background (CMB) experiments comes from the uncertainty in instrument bandpass calibration. Uncertainties in bandpass can limit foreground removal and spectral fitting, which are critical for inflationary and galaxy cluster measurements. CMB experiments currently use Fourier Transform Spectrometers (FTSes) to measure instrument bandpasses. However, FTS systems are currently systematics-limited, so significant improvements in bandpass measurements require novel calibrators. To this end, we developed a Frequency-selectable Laser Source (FLS) calibrator, which uses a laser with adjustable frequency coupled to a system that allows for laser power attenuation. Following initial testing with the first FLS prototype, we developed an upgraded version of the calibrator with improved performance. We present the upgrades to the FLS calibrator, the characterization of the upgraded calibrator and new laser source, and plans for testing with microwave instruments in the field.

Saunders, Lauren J. [Fermilab] (ORCID:000000016367↗
DOE OSTI2025

Frequency-Selectable Laser Source (FLS) Calibrator for CMB Bandpass Characterization

One of the biggest challenges for Cosmic Microwave Background (CMB) experiments comes from our detector bandpass calibration. Uncertainties in bandpass can severely limit our measurements by limiting foreground removal and spectral fitting, which is particularly important for high-$\ell$ observations like cluster science using the Sunyaev-Zeldovich (SZ) effect. Currently, CMB experiments typically use a Fourier Transform Spectrometer (FTS) to measure the detector bandpasses. However, the resolution of the FTS is dependent on the length of the interferometer arms, leading to a need for increasingly large FTS instruments as CMB experiments require tighter constraints on detector bandpasses. Additionally, systematic effects like shifts in bandpass shape from uneven illumination from the FTS further limit the calibration uncertainties. As a complement to the FTS, we have developed a Frequency-selectable Laser Source (FLS) calibrator, which uses a laser with adjustable frequency housed in a calibrator that allows for varying degrees of laser power attenuation. We present several tests used to characterize the first prototype design of the FLS calibrator, as well as the improvements to the calibrator design currently underway.

Saunders, Lauren [Fermilab]↗
DOE OSTI2025

Highly Sensitive Measurements of Methylene Dynamics With a Frequency-Selective Double-Quantum Sideband Method

Probing the fast dynamics of surface sites using NMR spectroscopy is highly challenging owing to the sites’ high dilution and the difficulties often associated with isotopic enrichment. Intra-CH 2 1 H- 1 H dipolar couplings are ideal probes of motions given that they only involve 1 H’s and the tensor has a well-defined size and orientation. Here, we introduce a frequency-selective variant of the double-quantum sideband method to measure like-spin 1 H- 1 H dipolar coupling constants. The experiment dramatically reduces the instrument time required to measure dynamically-averaged intra-CH 2 dipolar couplings. We demonstrate the performance of the sequence using silica-supported silanes as model highly-mobile surface species.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2025

Frequency-Selectable Laser Source for Cosmic Microwave Background Experiments

Cosmic Microwave Background (CMB) experiments measure remnant radiation from the early universe and use that data to determine fundamental properties of the universe. We can constrain key parameters, such as \textit{r}, the cosmic tensor-to-scalar ratio, and $N_\text{eff}$, the effective number of relativistic species, by analyzing the CMB power spectra. Improving our measurements of the CMB requires improving our instrument systematics, one of the most important of which is detector bandpass. Current experiments use a Fourier Transform Spectrometer (FTS) to measure bandpass. However, the FTS is systematics limited, and cannot achieve the accuracy needed to make improved CMB measurements. For this reason, we are developing a new instrument, the Frequency-Selectable Laser Source (FLS) to decrease the uncertainty in bandpass by an order of magnitude. In this paper, we describe work completed to support the version 2 upgrade to the FLS. Using ray-tracing software, we modeled the FLS optics to set physical tolerances for the new design. We also discuss the laser calibration, and future work to be completed in further development of the FLS upgrade.

Rosen-Turits, Gabriel M. [Fermilab]↗
DOE OSTI2025

Frequency-Selectable Laser Source (FLS) for Cosmic Microwave Background Experiments

Cosmic Microwave Background (CMB) experiments measure remnant radiation from the early universe and use that data to determine fundamental properties of the universe. We can constrain key parameters, such as \textit{r}, the cosmic tensor-to-scalar ratio, and $N_\text{eff}$, the effective number of relativistic species, by analyzing the CMB power spectra. Improving our measurements of the CMB requires improving our instrument systematics, one of the most important of which is detector bandpass. Current experiments use a Fourier Transform Spectrometer (FTS) to measure bandpass. However, the FTS is systematics limited, and cannot achieve the accuracy needed to make improved CMB measurements. For this reason, we are developing a new instrument, the Frequency-Selectable Laser Source (FLS) to decrease the uncertainty in bandpass by an order of magnitude. In this paper, we describe work completed to support the version 2 upgrade to the FLS. Using ray-tracing software, we modeled the FLS optics to set physical tolerances for the new design. We also discuss the laser calibration, and future work to be completed in further development of the FLS upgrade.

Rosen-Turits, Gabriel M.↗
DOE OSTI2018

Frequency-selective excitation of high-wavevector phonons

We demonstrate here the selective excitation of a narrow frequency band of TA phonons throughout the Brillouin zone of germanium using a sinusoidally modulated picosecond laser pulse. The pulse is produced through the combination of two chirped and delayed pulses using a stabilized interferometer. The phonon excitations are probed by time- and momentum- resolved x-ray diffuse scattering.

36 MATERIALS SCIENCE↗
DOE OSTI2018

Extraordinary electromagnetic transmission by antenna arrays and frequency selective surfaces having compound unit cells with dissimilar elements

The various embodiments presented herein relate to extraordinary electromagnetic transmission (EEMT) to enable multiple inefficient (un-matched) but coupled radiators and/or apertures to radiate and/or pass electromagnetic waves efficiently. EEMT can be utilized such that signal transmission from a plurality of antennas and/or apertures occurs at a transmission frequency different to transmission frequencies of the individual antennas and/or aperture elements. The plurality of antennas/apertures can comprise first antenna/aperture having a first radiating area and material(s) and second antenna/aperture having a second radiating area and material(s), whereby the first radiating/aperture area and second radiating/aperture area can be co-located in a periodic compound unit cell. Owing to mutual coupling between the respective antennas/apertures in their arrayed configuration, the transmission frequency of the array can be shifted from the transmission frequencies of the individual elements. EEMT can be utilized for an array of evanescent of inefficient radiators connected to a transmission line(s).

47 OTHER INSTRUMENTATION↗
DOE OSTI2018

MEMS terahertz-to-infrared band converter using frequency selective planar metamaterial

A MEMS terahertz-to-infrared converter has been developed based on the unique properties of metamaterials that allow for selective control of the absorptivity and emissivity of the sensors. The converter consists of a sensing element structurally made of planar metamaterial membranes, connected to a substrate frame by four symmetrically-located thermal insulators. Upon THz absorption, the temperature of the sensing element increases and the outward infrared flux from the backside of the element is read by a commercial long-wave infrared camera. Two configurations were designed and fabricated with metamaterial absorptivity optimized for 3.8THz and 4.75THz quantum cascade lasers. The first sensor, fabricated with an oxidized aluminum backside, exhibits higher responsivity, but lower conversion efficiency than the second sensor, fabricated with a metamaterial backside. The spectral characteristics of the metamaterial on the two sides can be optimized to improve both responsivity and sensitivity, while keeping the sensors’ thermal time constant sufficiently small for real time imaging. No dedicated electronics or optics are required for readout making metamaterial-based MEMS THz-to-IR converters very attractive for THz imaging as means of a simple attachment to commercial IR cameras.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2023

Tuning the output of a laser

In a general aspect, a laser system includes a laser and a frequency comb generator system. The laser is configured to generate a laser signal, and the frequency comb generator system is configured to generate a frequency comb based on the laser signal. The frequency comb includes frequency comb signals at respective comb frequencies. The laser system also includes a frequency comb dispersion system configured to spatially separate the frequency comb signals onto respective optical channels of the frequency comb dispersion system. The laser system additionally includes a frequency selector system configured to generate a selected frequency signal from the frequency comb signals after separation. The selected frequency signal includes a target separated frequency comb signal. The laser system also includes a frequency shifter configured to alter the selected frequency signal toward a target output frequency of the laser system.

Liu, Chang↗
DOE OSTI2019

Wide-Angle Spectrally Selective Absorbers and Thermal Emitters Based on Inverse Opals

Engineered optical absorbers are of significant interest for applications ranging from stray light reduction to energy conversion. Here, we demonstrate a large-area (centimeter-scale) metamaterial that features near-unity frequency-selective absorption in the mid-infrared wavelength range. The metamaterial comprises a self-assembled porous structure known as an inverse opal, here made of silica. The structure’s large volume fraction of voids, together with the vibrational resonances of silica in the mid-infrared spectral range, reduce the metamaterial’s refractive index to close to that of air and introduce considerable optical absorption. As a result, the frequency-selective structure efficiently absorbs incident light of both polarizations even at very oblique incidence angles. The absorber remains stable at high temperatures (measured up to ~900 °C), enabling its operation as a frequency-selective thermal emitter. The excellent performance of this absorber/emitter and ease of fabrication make it a potential surface coating for passive radiative cooling, laser safety, and other large-area applications.

42 ENGINEERING↗