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At least 19 records

Effect of inversion asymmetry on the superconducting and exciton condensates of bilayer graphene

Inversion asymmetry in bilayer graphene can be tuned by the displacement field. As a result, the band dispersion in biased bilayer graphene acquires flatband regions near the Dirac points along with a nontrivial band geometry. We analyze the effect of inversion asymmetry on the critical temperature and superfluid stiffness of the superconducting state of AB-stacked graphene bilayer and the exciton condensate in double layers formed by two AB-stacked graphene bilayers. We find that the geometric superfluid stiffness in bilayer graphene superconductors is negligible due to the small superconducting gap. Furthermore, since the geometric superfluid stiffness is maximized for a constant order parameter, it can be neglected in biased bilayer graphene superconductors with any pairing symmetry. In contrast, the displacement field enhances the geometric superfluid stiffness in exciton condensates. It is most prominent at low densities and high displacement fields. Here, a consequence of the geometric superfluid stiffness is a modest enhancement of the Berezinskii-Kosterlitz-Thouless transition temperature in bilayer graphene’s exciton condensate.

BKT transition↗

Enhancing Spin Filters by Use of Bulk Inversion Asymmetry

Theoretical calculations have shown that the degrees of spin polarization in proposed nonmagnetic semiconductor resonant tunneling spin filters could be increased through exploitation of bulk inversion asymmetry (BIA). These enhancements would be effected through suitable orientation of spin collectors (or spin-polarization- inducing lateral electric fields), as described below. Spin filters -- more precisely, sources of spin-polarized electron currents -- have been sought for research on, and development of, the emerging technological discipline of spintronics (spin-transport electronics). The proposed spin filters were to be based on the Rashba effect, which is an energy splitting of what would otherwise be degenerate quantum states, caused by a spinorbit interaction in conjunction with a structural-inversion asymmetry (SIA) in the presence of interfacial electric fields in a semiconductor heterostructure. The magnitude of the energy split is proportional to the electron wave number. In a spin filter, the spin-polarized currents produced by the Rashba effect would be extracted by quantum-mechanical resonant tunneling.

Ting, David↗

Structural inversion asymmetry in epitaxial ultrathin films of Bi(111)/InSb(111)B

Bismuth (Bi) films hold potential for spintronic devices due to strong spin-orbit coupling. Understanding the growth, surface states, and interactions with the substrate is key to their functionalization. Large-area high-quality (111) Bi ultrathin films were grown on InSb (111)B substrates by molecular beam epitaxy (MBE). Strong film-substrate interactions epitaxially stabilize the (111) orientation and lead to nonequivalent interface potentials. Analysis of angle-resolved photoemission spectroscopy (ARPES) measurements, employed to characterize the evolution of the surface states with film thickness, indicate a crossing at the $\overline{M}$ point, suggesting a topologically trivial phase in the thin film. In conclusion, the results show the presence of interfacial bonds to the substrate breaks inversion symmetry, preventing the semimetal-to-semiconductor transition predicted for freestanding bismuth layers, highlighting the importance of controlled functionalization and surface passivation of two-dimensional materials.

Inbar, Hadass S. [Univ. of California, Santa Barba↗

Device Concepts Based on Spin-dependent Transmission in Semiconductor Heterostructures

We examine zero-magnetic-field spin-dependent transmission in nonmagnetic semiconductor heterostructures with structural inversion asymmetry (SIA) and bulk inversion asymmetry (BIA), and report spin devices concepts that exploit their properties. Our modeling results show that several design strategies could be used to achieve high spin filtering efficiencies. The current spin polarization of these devices is electrically controllable, and potentially amenable to highspeed spin modulation, and could be integrated in optoelectronic devices for added functionality.

resonant tunneling↗

A Segmentation Algorithm for Characterizing Rise and Fall Segments in Seasonal Cycles: An Application to XCO2 to Estimate Benchmarks and Assess Model Bias

There is more useful information in the time series of satellite-derived column-averaged carbon dioxide (XCO2) than is typically characterized. Often, the entire time series is treated at once without considering detailed features at shorter timescales, such as nonstationary changes in signal characteristics – amplitude, period and phase. In many instances, signals are visually and analytically differentiable from other portions in a time series. Each rise (increasing) and fall (decreasing) segment in the seasonal cycle is visually discernable in a graph of the time series. The rise and fall segments largely result from seasonal differences in terrestrial ecosystem production, which means that the segment's signal characteristics can be used to establish observational benchmarks because the signal characteristics are driven by similar underlying processes. We developed an analytical segmentation algorithm to characterize the rise and fall segments in XCO2 seasonal cycles. We present the algorithm for general application of the segmentation analysis and emphasize here that the segmentation analysis is more generally applicable to cyclic time series. We demonstrate the utility of the algorithm with specific results related to the comparison between satellite- and model-derived XCO2 seasonal cycles (2009–2012) for large bioregions across the globe. We found a seasonal amplitude gradient of 0.74–0.77 ppm for every 10∘ of latitude in the satellite data, with similar gradients for rise and fall segments. This translates to a south–north seasonal amplitude gradient of 8 ppm for XCO2, about half the gradient in seasonal amplitude based on surface site in situ CO2 data (∼19 ppm). The latitudinal gradients in the period of the satellite-derived seasonal cycles were of opposing sign and magnitude (−9 d per 10∘ latitude for fall segments and 10 d per 10∘ latitude for rise segments) and suggest that a specific latitude (∼2∘ N) exists that defines an inversion point for the period asymmetry. Before (after) the point of asymmetry inversion, the periods of rise segments are lesser (greater) than the periods of fall segments; only a single model could reproduce this emergent pattern. The asymmetry in amplitude and the period between rise and fall segments introduces a novel pattern in seasonal cycle analyses, but, while we show these emergent patterns exist in the data, we are still breaking ground in applying the information for science applications. Maybe the most useful application is that the segmentation analysis allowed us to decompose the model biases into their correlated parts of biases in amplitude, period and phase independently for rise and fall segments. We offer an extended discussion on how such information about model biases and the emergent patterns in satellite-derived seasonal cycles can be used to guide future inquiry and model development.

Calle, Leonardo↗

A Segmentation Algorithm for Characterizing Rise and Fall Segments in Seasonal Cycles: an Application to Xco2 to Estimate Benchmarks and Assess Model Bias

There is more useful information in the time series of satellite-derived column-averaged carbon dioxide (XCO2) than is typically characterized. Often, the entire time series is treated at once without considering detailed features at shorter timescales, such as nonstationary changes in signal characteristics – amplitude, period and phase. In many instances, signals are visually and analytically differentiable from other portions in a time series. Each rise (increasing) and fall (decreasing) segment in the seasonal cycle is visually discernable in a graph of the time series. The rise and fall segments largely result from seasonal differences in terrestrial ecosystem production, which means that the segment's signal characteristics can be used to establish observational benchmarks because the signal characteristics are driven by similar underlying processes. We developed an analytical segmentation algorithm to characterize the rise and fall segments in XCO2 seasonal cycles. We present the algorithm for general application of the segmentation analysis and emphasize here that the segmentation analysis is more generally applicable to cyclic time series. We demonstrate the utility of the algorithm with specific results related to the comparison between satellite- and model-derived XCO2 seasonal cycles (2009–2012) for large bioregions across the globe. We found a seasonal amplitude gradient of 0.74–0.77 ppm for every 10∘ of latitude in the satellite data, with similar gradients for rise and fall segments. This translates to a south–north seasonal amplitude gradient of 8 ppm for XCO2, about half the gradient in seasonal amplitude based on surface site in situ CO2 data (∼19 ppm). The latitudinal gradients in the period of the satellite-derived seasonal cycles were of opposing sign and magnitude (−9 d per 10∘ latitude for fall segments and 10 d per 10∘ latitude for rise segments) and suggest that a specific latitude (∼2∘ N) exists that defines an inversion point for the period asymmetry. Before (after) the point of asymmetry inversion, the periods of rise segments are lesser (greater) than the periods of fall segments; only a single model could reproduce this emergent pattern. The asymmetry in amplitude and the period between rise and fall segments introduces a novel pattern in seasonal cycle analyses, but, while we show these emergent patterns exist in the data, we are still breaking ground in applying the information for science applications. Maybe the most useful application is that the segmentation analysis allowed us to decompose the model biases into their correlated parts of biases in amplitude, period and phase independently for rise and fall segments. We offer an extended discussion on how such information about model biases and the emergent patterns in satellite-derived seasonal cycles can be used to guide future inquiry and model development.

segmentation algorithm↗

Hydrogen Bonding Analysis of Structural Transition-Induced Symmetry Breaking and Spin Splitting in a Hybrid Perovskite Employing a Synergistic Diffraction-DFT Approach

Two-dimensional (2D) hybrid organic–inorganic perovskites (HOIPs) offer an outstanding opportunity for spin-related technologies owing in part to their tunable structural symmetry breaking and distortions driven by organic–inorganic hydrogen (H) bonds. However, understanding how H-bonds tailor inorganic symmetry and distortions and therefore enhance spin splitting for more effective spin manipulation remains imprecise due to challenges in measuring H atom positions using X-ray diffraction. Here, we report a thermally induced structural transition (at ~209 K) for a 2D HOIP, (2-BrPEA) 2 PbI 4 [2-BrPEA = 2-(2-bromophenyl)ethylammonium], which induces inversion asymmetry and a strong spin splitting (ΔE > 30 meV). While X-ray diffraction generally establishes heavy atom coordinates, we utilize neutron diffraction for accurate H atom position determination, demonstrating that the structural transition-induced rearrangement of H-bonds with distinct bond strengths asymmetrically shifts associated iodine atom positions. Further, consequences of this shift include an increased structural asymmetry, an enhanced difference between adjacent interoctahedra distortions (i.e., Pb–I–Pb bond angles), and therefore significant spin splitting. We further show that H-only density-functional theory (DFT) relaxation of the X-ray structure shifts H atoms to positions that are consistent with the neutron experimental data, validating a convenient pathway to more generally improve upon HOIP H-bonding analyses derived from quicker/less-expensive X-ray data.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Promises and technological prospects of two-dimensional Rashba materials

The Rashba spin–orbit coupling effect, primarily arising from structural-inversion asymmetry in periodic crystals, has garnered considerable attention due to its tunability and potential applications in spintronics. Its capability to manipulate electron spin without an external magnetic field opens new avenues for spintronic device design, particularly in semiconductor technology. Within this framework, 2D Rashba materials hold special interest due to their inherent characteristics, which facilitate miniaturization and engineering capabilities. In this Perspective article, we provide an overview of recent advancements in the research of 2D Rashba materials, aiming to offer a comprehensive understanding of the diverse manifestations and multifaceted implications of the Rashba effect in material science. Rather than merely presenting a list of materials, our approach involves synthesizing various viewpoints, assessing current trends, and addressing challenges within the field. Our objective is to bridge the gap between fundamental research and practical applications by correlating each material with the necessary advancements required to translate theoretical concepts into tangible technologies. Furthermore, we highlight promising avenues for future research and development, drawing from insights gleaned from the current state of the field.

Physics↗

Spin lifetime tuning in zincblende heterostructures and applications to spin devices

We present analytical expressions for the D'yakonov-Perel' spin relaxation rates under the combined action of bulk and structural inversion asymmetry for zincblende heterostructures when terms up to linear and third order in k are included in the Hamiltonian. We see for heterostructures that, under the right conditions, the lowest-order-in-k component of the spin relaxation tensor can be made to vanish for all spin components at the same time. We study how the inclusion of terms of higher order in k affects these results.

spin filters↗

NASA Tech Briefs, October 2007

Topics covered include; Wirelessly Interrogated Position or Displacement Sensors; Ka-Band Radar Terminal Descent Sensor; Metal/Metal Oxide Differential Electrode pH Sensors; Improved Sensing Coils for SQUIDs; Inductive Linear-Position Sensor/Limit-Sensor Units; Hilbert-Curve Fractal Antenna With Radiation- Pattern Diversity; Single-Camera Panoramic-Imaging Systems; Interface Electronic Circuitry for an Electronic Tongue; Inexpensive Clock for Displaying Planetary or Sidereal Time; Efficient Switching Arrangement for (N + 1)/N Redundancy; Lightweight Reflectarray Antenna for 7.115 and 32 GHz; Opto-Electronic Oscillator Using Suppressed Phase Modulation; Alternative Controller for a Fiber-Optic Switch; Strong, Lightweight, Porous Materials; Nanowicks; Lightweight Thermal Protection System for Atmospheric Entry; Rapid and Quiet Drill; Hydrogen Peroxide Concentrator; MMIC Amplifiers for 90 to 130 GHz; Robot Would Climb Steep Terrain; Measuring Dynamic Transfer Functions of Cavitating Pumps; Advanced Resistive Exercise Device; Rapid Engineering of Three-Dimensional, Multicellular Tissues With Polymeric Scaffolds; Resonant Tunneling Spin Pump; Enhancing Spin Filters by Use of Bulk Inversion Asymmetry; Optical Magnetometer Incorporating Photonic Crystals; WGM-Resonator/Tapered-Waveguide White-Light Sensor Optics; Raman-Suppressing Coupling for Optical Parametric Oscillator; CO2-Reduction Primary Cell for Use on Venus; Cold Atom Source Containing Multiple Magneto- Optical Traps; POD Model Reconstruction for Gray-Box Fault Detection; System for Estimating Horizontal Velocity During Descent; Software Framework for Peer Data-Management Services; Autogen Version 2.0; Tracking-Data-Conversion Tool; NASA Enterprise Visual Analysis; Advanced Reference Counting Pointers for Better Performance; C Namelist Facility; and Efficient Mosaicking of Spitzer Space Telescope Images.

Source record↗

Resonant Tunneling Spin Pump

The resonant tunneling spin pump is a proposed semiconductor device that would generate spin-polarized electron currents. The resonant tunneling spin pump would be a purely electrical device in the sense that it would not contain any magnetic material and would not rely on an applied magnetic field. Also, unlike prior sources of spin-polarized electron currents, the proposed device would not depend on a source of circularly polarized light. The proposed semiconductor electron-spin filters would exploit the Rashba effect, which can induce energy splitting in what would otherwise be degenerate quantum states, caused by a spin-orbit interaction in conjunction with a structural-inversion asymmetry in the presence of interfacial electric fields in a semiconductor heterostructure. The magnitude of the energy split is proportional to the electron wave number. Theoretical studies have suggested the possibility of devices in which electron energy states would be split by the Rashba effect and spin-polarized currents would be extracted by resonant quantum-mechanical tunneling.

Ting, David Z.↗

Electron-Spin Filters Based on the Rashba Effect

Semiconductor electron-spin filters of a proposed type would be based on the Rashba effect, which is described briefly below. Electron-spin filters more precisely, sources of spin-polarized electron currents have been sought for research on, and development of, the emerging technological discipline of spintronics (spin-based electronics). There have been a number of successful demonstrations of injection of spin-polarized electrons from diluted magnetic semiconductors and from ferromagnetic metals into nonmagnetic semiconductors. In contrast, a device according to the proposal would be made from nonmagnetic semiconductor materials and would function without an applied magnetic field. The Rashba effect, named after one of its discoverers, is an energy splitting, of what would otherwise be degenerate quantum states, caused by a spin-orbit interaction in conjunction with a structural-inversion asymmetry in the presence of interfacial electric fields in a semiconductor heterostructure. The magnitude of the energy split is proportional to the electron wave number. The present proposal evolved from recent theoretical studies that suggested the possibility of devices in which electron energy states would be split by the Rashba effect and spin-polarized currents would be extracted by resonant quantum-mechanical tunneling. Accordingly, a device according to the proposal would be denoted an asymmetric resonant interband tunneling diode [a-RITD]. An a-RITD could be implemented in a variety of forms, the form favored in the proposal being a double-barrier heterostructure containing an asymmetric quantum well. It is envisioned that a-RITDs would be designed and fabricated in the InAs/GaSb/AlSb material system for several reasons: Heterostructures in this material system are strong candidates for pronounced Rashba spin splitting because InAs and GaSb exhibit large spin-orbit interactions and because both InAs and GaSb would be available for the construction of highly asymmetric quantum wells. This mate-rial system affords a variety of energy-band alignments that can be exploited to obtain resonant tunneling and other desired effects. The no-common-atom InAs/GaSb and InAs/AlSb interfaces would present opportunities for engineering interface potentials for optimizing Rashba spin splitting.

Ting, David Z.-Y.↗

Electrically controlled spin device concepts

We discuss spin device concepts that exploit spin-orbit coupling in nonmagnetic semiconductor heterostructures, including the resonant interband tunneling spin filter, the bi-directional spin pump,, the bulk inversion asymmetry enhanced spin filter, and resonant spin lifetime devices.

Chang, Y.-C.↗

InAs/GaSb/AlSb resonant tunneling spin device concepts

We discuss device concepts for creating spin polarized current sources without external magnetic fields, using nonmagnetic 6.1 A semiconductor resonant tunneling structures.

spin filter spin pump resonant tunneling bulk inve↗

High‐Asymmetry Metasurface: A New Solution for Terahertz Resonance via Active Learning‐Augmented Diffusion Model

Terahertz (THz) metamaterials with high‐figure‐of‐merit (high‐FoM) performance resonance are essential for advancing sensors, detectors, and imagers. Conventional designs focus on symmetric or low‐asymmetry geometric structures, leaving high‐asymmetry designs largely unexplored due to the inefficiency of trial‐and‐error‐based rational design. Recent deep learning techniques offer automation and acceleration but are constrained by the need for large datasets inherent to their data‐driven nature. Here, a novel prior knowledge‐guided generative model augmented by a physics‐constrained active learning mechanism to design high‐asymmetry metamaterials. An advanced diffusion model learns features from a small set of classical structures with high‐FoM THz resonance and generates new high‐asymmetry structures. To mitigate the limited number of classical structures, the generated high‐asymmetry structures are actively selected and integrated into the initial training dataset based on their physical characteristics. Experimental results demonstrate the superior resonance performance of the generated high‐asymmetry metamaterials over classical designs, exhibiting improvements exceeding 30% in key resonance metrics. Remarkably, this performance is attained using only 68 classical structures as the initial training dataset, significantly reducing the data requirements for deep learning‐based metamaterial design. The proposed scheme for generating high‐asymmetry structures provides a new effective and efficient solution for high‐FoM resonance, expanding applications in high‐sensitivity THz metadevices.

diffusion model↗

The influence of NO and ClO variations at twilight on the interpretation of solar occultation measurements

Measurement of short-lived photochemically-produced species in the stratosphere by solar occultation is difficult because the rapid variation of such species near the terminator introduces ambiguities in interpreting the measured absorption in terms of meaningful atmospheric abundances. These variations produce tangent path concentrations that are asymmetric relative to the tangent point, as opposed to the symmetrical distribution usually assumed in most inversion algorithms. Neglect of this asymmetry may yield an inverted profile that deviates significantly from the true sunset/sunrise profile. In the present paper, the influence of this effect on solar occultation measurements of ClO and NO is examined. The results show that average inhomogeneity factors, which measure the concentration variation along the tangent path and which can be calculated from a photochemical model, can indicate which species require more careful data analysis.

Boughner, R.↗