Final Report - Quench Protection for a Neutron Scattering Magnet
Explore the source record for details and available documents.
Scanlan, Ronald M.↗
SEARCH · Search NASA
Results for “magnetic scattering”
Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.
Quote a phrase for an exact phrase match. Source license links do not imply unrestricted reuse.
Reconciling monolayer and bilayer Jeff = 1/2 square lattices in hybrid oxide superlattice
The number of atomic layers confined in a two-dimensional structure is crucial for the electronic and magnetic properties. Single-layer and bilayer J eff = 1/2 square lattices are well-known examples where the presence of the extra layer turns the XY anisotropy to the c-axis anisotropy. We report on experimental realization of a hybrid SrIrO 3 /SrTiO 3 superlattice that integrates monolayer and bilayer square lattices in one layered structure. By synchrotron x-ray diffraction, resonant x-ray magnetic scattering, magnetization, and resistivity measurements, we found that the hybrid superlattice exhibits properties that are distinct from both the single-layer and bilayer systems and cannot be explained by a simple addition of them. In particular, the entire hybrid superlattice orders simultaneously through a single antiferromagnetic transition at temperatures similar to the bilayer system but with all the J eff = 1/2 moments mainly pointing in the ab plane similar to the single-layer system. The results show that bringing monolayer and bilayer with orthogonal properties in proximity to each other in a hybrid superlattice structure is a powerful way to stabilize a unique state not obtainable in a uniform structure.
2-dimensional systems↗
Three-dimensional structure of hybrid magnetic skyrmions determined by neutron scattering
Magnetic skyrmions are topologically protected chiral spin textures which present opportunities for next-generation magnetic data storage and logic information technologies. The topology of these structures originates in the geometric configuration of the magnetic spins, more generally described as the structure. While the skyrmion structure is most often depicted using a two-dimensional projection of the three-dimensional (3D) structure, recent works have emphasized the role of all three dimensions in determining the topology and their response to external stimuli. Here, grazing-incidence small-angle neutron scattering and polarized neutron reflectometry are used to determine the 3D structure of hybrid skyrmions. The structure of the hybrid skyrmions, which includes a combination of Néel-like and Bloch-like components along their length, is expected to significantly contribute to their notable stability, which includes ambient conditions. To interpret the neutron scattering data, micromagnetic simulations of the hybrid skyrmions were performed, and the corresponding diffraction patterns were determined using a Born approximation transformation. The converged magnetic profile reveals the magnetic structure along with the skyrmion depth profile, including the thickness of the Bloch and Néel segments and the diameter of the core.
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
Simulations of Neutron Scattering and Magnetization Data for the NIPS3 lattice with varying exchanges
This dataset contains simulations generated by Sunny.jl of the magnetic excitations on the NiPS3 lattice. The exchange parameters are varied over the system so these simulations can be used for AI model training.
36 MATERIALS SCIENCE↗
Spinteract: a program to refine magnetic interactions to diffuse scattering data
Magnetic diffuse scattering—the broad magnetic scattering features observed in neutron-diffraction data above a material's magnetic ordering temperature—provides a rich source of information about the material's magnetic Hamiltonian. However, this information has often remained under-utilised due to a lack of available computer software that can fit values of magnetic interaction parameters to such data. Here, an open-source computer program, Spinteract, is presented, which enables straightforward refinement of magnetic interaction parameters to powder and single-crystal magnetic diffuse scattering data. Here, the theory and implementation of this approach are summarised. Examples are presented of refinements to published experimental diffuse-scattering data sets for the canonical antiferromagnet MnO and the highly-frustrated classical spin liquid Gd 3 Ga 5 O 12 . Guidelines for data collection and refinement are outlined, and possible developments of the approach are discussed.
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
Magnetic Diffuse Scattering of YBaCo 4 O 7 and LuBaCo 4 O 7 on Kagome and Triangular Lattices
In this work, the magnetic diffuse scattering of YBaCo 4 O 7 and LuBaCo 4 O 7 with alternating kagome and triangular lattices has been studied through neutron scattering measurements on single-crystal samples. In YBaCo 4 O 7 , the line-shape-magnetic-diffuse scattering is observed around the magnetic transition temperature, which is consistent with the Monte Carlo simulation. In LuBaCo 4 O 7 , the line-shape-magnetic-diffuse scattering has not been detected. At low temperature, the propagation vectors of the observed magnetic reflections are different between YBaCo 4 O 7 and LuBaCo 4 O 7 . The structural distortion in RBaCo 4 O 7 is suggested to play a critical role for the magnetic properties.
72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
Magnetic excitations in Nd 𝑛+1 Ni 𝑛 O 3𝑛+1 Ruddlesden-Popper nickelates observed via resonant inelastic x-ray scattering
Magnetic interactions are thought to play a key role in the properties of many unconventional superconductors, including cuprates, iron pnictides, and square-planar nickelates. Superconductivity was also recently observed in the bilayer and trilayer Ruddlesden-Popper nickelates, the electronic structure of which is expected to differ from that of cuprates and square-planar nickelates. Here we study how electronic structure and magnetic interactions evolve with the number of layers, 𝑛, in thin film Ruddlesden-Popper nickelates Nd 𝑛+1 Ni 𝑛 O 3𝑛+1 with 𝑛 = 1,3, and 5 using resonant inelastic x-ray scattering (RIXS). The RIXS spectra are consistent with a high-spin |3𝑑 8 $\underline{𝐿}$⟩ electronic configuration, resembling that of La 2−𝑥 Sr 𝑥 NiO 4 and the parent perovskite, NdNiO 3 . The magnetic excitations soften to lower energy in the structurally self-doped, higher-𝑛 films. In conclusion, our observations confirm that structural tuning is an effective route for altering electronic properties, such as magnetic superexchange, in this prominent family of materials.
36 MATERIALS SCIENCE↗
Thomson scattering in magnetic fields
The equation of transfer in Thomson scattering atmospheres with magnetic fields is solved using Monte Carlo methods. Two cases, a plane parallel atmosphere with a magnetic field perpendicular to the atmosphere, and a dipole star, are investigated. The wavelength dependence of polarization from plane-parallel atmosphere is qualitatively similar to that observed in the magnetic white dwarf Grw+70 deg 8247, and the field strength determined by the calculation, 320 MG, is quantitatively similar to that determined from the line spectrum. The dipole model does not resemble the data as well as the single plane-parallel atmosphere.
Whitney, Barbara↗
An explicitly solvable energy-conserving algorithm for pitch-angle scattering in magnetized plasmas
In this work, we develop an Explicitly Solvable Energy-Conserving (ESEC) algorithm for the Stochastic Differential Equation (SDE) describing the pitch-angle scattering process in magnetized plasmas. The Cayley transform is used to calculate both the deterministic gyromotion and stochastic scattering, affording the algorithm to be explicitly solvable and exactly energy conserving. An unusual property of the SDE for pitch-angle scattering is that its coefficients diverge at the zero velocity and do not satisfy the global Lipschitz condition. Consequently, when standard numerical methods, such as the Euler-Maruyama (EM), are applied, numerical convergence is difficult to establish. For the proposed ESEC algorithm, its energy-preserving property enables us to overcome this obstacle. We rigorously prove that the ESEC algorithm is order 1/2 strongly convergent. This result is confirmed by detailed numerical studies. For the case of pitch-angle scattering in a magnetized plasma with a constant magnetic field, the numerical solution is benchmarked against the analytical solution, and excellent agreements are found.
70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
Origin of circular dichroism in resonant elastic x-ray scattering from magnetic and polar chiral structures
Circular dichroism in resonant elastic x-ray scattering (CD-REXS) has recently been observed in chiral structures composed of multiferroic materials as well as magnetic moments or electric polarization vectors. In order to comprehensively understand the experimental results of these previous studies, we present here in detail the analytical formulation of CD-REXS for one-dimensional helices composed of magnetic moments and electric polarization vectors, respectively. In particular, by comparing CD-REXS for a proper-screw-shaped Bloch-type helix and cycloid-shaped Néel-type helix, we found that CD-REXS for both magnetic and polar helices can discriminate between both types of helices. We also found that the x-ray polarization factor depending on the scattering geometry is a significant factor in determining the characteristics of CD-REXS for chiral structures. The results obtained from the detailed formulas can be intuitively understood using the concept of mirror reflection. In particular, in this way it can be understood that Bloch- and Néel-type helices correspond to truly chiral and achiral structures, respectively, and why CD-REXS is able to distinguish between these two types of helices.
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
Bremsstrahlung from neutrino scattering via magnetic dipole moments
In this paper, we discuss bremsstrahlung induced by neutrino scattering. This process should exist since neutrinos are expected to couple to photons via magnetic dipole and transition moments. These moments are loop-induced and tiny in the Standard Model with neutrino masses but could be significantly enhanced in extended theories. As concrete example, we study the scattering of the two largest neutrino fluxes on earth, solar neutrinos and Cosmic Neutrino Background (CNB). Finally, it is tempting to consider this as a potential signature for CNB searches but it turns out that the signal is extremely small and unlikely to be observed.
72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
Magnetized stimulated scattering in pulsar winds
The effects of stimulated scattering on a collimated high brightness temperature beam of photons traversing a relativistically streaming magnetized plasma are studied. Under the assumption that the center of the photon beam is parallel to the bulk motion, we calculate the scattering rate as a function of the angular spread of the beam and the Lorentz factor gamma. Magnetization changes the photon recoil, without which stimulated scattering has no effect. It also introduces a strong dependence on frequency and polarization: if the photon frequency matches the electron cyclotron frequency, the scattering rate of photons polarized perpendicular to the magnetic field can be substantially enhanced relative to Thomson, and if the photon frequency is much less than the cyclotron frequency, the scattering is suppressed. Applying these calculations to pulsars, we find that stimulated scattering of the radio beam in the magnetized wind believed to exist outside the light cylinder can substantially alter the spectrum and polarization state of the radio signal. We suggest that the scattering rate is so high in some pulsars that the ability of the radio signal to penetrate the pulsar magnetosphere requires modification of either the conventional model of the magnetosphere or assumptions about the effects of stimulated scattering upon a beam.
Sincell, Mark W.↗
Magnetic structure and resistivity minimum in GdCuAs 2
The electrical resistivity of GdCuAs 2 single crystals exhibits an anomalous Kondo-like resistivity minimum above the antiferromagnetic ordering temperature T N 1 approximate to 10.6 K, which is unusual for a highly localized 4f-moment (Gd 3+ ) system. Using x-ray resonant magnetic scattering, we determined the magnetic structure of GdCuAs 2 , where Gd moments are antiferromagnetically aligned along the crystallographic a axis and in the (+ + --) arrangement in the c direction and ferromagnetically arranged in the b direction. The antiferromagnetic order appears first at q = (δ, 0, 0.5) below 10 K, with an incommensurate modulation along the a axis and locks into a commensurate position at q = (1/3, 0, 0.5) below T N 2 approximate to 6 K. Our high-resolution x-ray diffraction measurements show a two-peak structure at Q = (2, 0, 6) above the resistivity minimum, suggesting a lower-symmetry crystal structure than the reported tetragonal structure, and the Q = (2, 0, 6) peak becomes a sharp one-peak structure below the resistivity minimum, implying a magnetoelastic coupling above T N . In conclusion, our findings suggest a complex interplay between the crystal structure and antiferromagnetic structure through a magnetoelastic coupling, associated with the anomalous resistivity minimum above T N 1 .
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
Unraveling magneto-structural coupling of Ni 2 MnGa alloy under the application of stress and magnetic field using in situ polarized neutron diffraction
The magneto-structural evolution of a Ni 2 MnGa single crystal was investigated by in situ polarized neutron diffraction under both magnetic field and mechanical loading. The ability to separate the nuclear and magnetic scatterings by polarized neutrons enables simultaneous observations of the twin reorientation (through twin boundary motion) and magnetic moment configuration. It is found that under a 1.0 T saturating magnetic field, twin reorientation can be activated by compressive stress and is accompanied by a realignment of the magnetic moment, which follows the easy axis of the twin variant. On the other hand, compressive stress as small as 1.0 MPa can freeze the twin reorientation. The evolution of the magnetic scattering amplitudes suggests that the change in magnetization was mainly achieved through the magnetic domain wall motion, while the twin boundary motion was blocked.
36 MATERIALS SCIENCE↗
Lunar electromagnetic scattering. II - Magnetic fields and transfer functions for parallel propagation
Magnetic field and transfer function amplitudes, resulting from a transverse electromagnetic wave in the interplanetary medium scattering from the moon and its diamagnetic cavity, are presented. Calculations are made using an asymmetric scattering theory for a spherical two-layer model of the lunar electrical conductivity profile and a nonconducting cylindrical model of the downstream lunar plasma void. Both the field and transfer function magnitudes are calculated as functions of position on the surface of the moon for frequencies relevant to the observations of the lunar surface and orbiting magnetometers. The amplitudes of the magnetic field components on the cavity boundary are also computed as functions of frequency and distance downstream from the lunar limb. Comparisons of the results are made with those of (1) spherically symmetric descriptions of lunar electromagnetic scattering, (2) the quasi-static approximation to asymmetric scattering theory, and (3) observations of the scattering phenomenon by lunar surface and orbiting magnetometers.
Schubert, G.↗
Broad-band linear polarization in cool stars. II - Amplitude and wavelength dependence for magnetic and scattering regions
We have developed a model to estimate the amplitude and wavelength dependence of broad-band linear polarization (BLP) from magnetic regions on cool stars. The model includes corrections both for line blends and for the partial cancellation of polarization in the vector sum over the stellar disk. Our results agree with recent calculations of BLP in the red, but show larger amplitudes and a different wavelength dependence in the blue. We find that the detailed wavelength dependence of the polarization is complex and varies with effective temperature and gravity due to changes in line blanketing. The BLP amplitudes depend strongly on field strength, blanketing, and magnetic region filling factor and geometry. We make rough estimates of the maximum BLP for stars of various spectral types and demonstrate a method for deriving a lower limit to the filling factor from the maximum observed BLP. This lower limit is related to the fractional area covered by the spatially asymmetric component of magnetic regions.
Saar, Steven H.↗
Magnetic Compton Scattering Study of Li-Rich Battery Materials
The redox process in a lithium-ion battery occurs when a conduction electron from the lithium anode is transferred to the redox orbital of the cathode. Understanding the nature of orbitals involved in anionic as well as cationic redox reactions is important for improving the capacity and energy density of Li-ion batteries. In this connection, we have obtained magnetic Compton profiles (MCPs) from the Li-rich cation-disordered rock-salt compound LixTi0.4Mn0.4O2 (LTMO). The MCPs, which involved the scattering of circularly polarized hard X-rays, are given by the momentum density of all the unpaired spins in the material. The net magnetic moment in the ground state can be extracted from the area under the MCP, along with a SQUID measurement. Our analysis gives insight into the role of Mn 3d magnetic electrons and O 2p holes in the magnetic redox properties of LTMO.
Suzuki, Kosuke (ORCID:0000000317110604)↗
Electronic scattering off a magnetic hopfion
We study scattering of itinerant electrons off a magnetic hopfion in a three-dimensional metallic magnet described by a magnetization vector S(r). A hopfion is a confined topological soliton of S(r) characterized by an emergent magnetic field Bγ(r)≡ε αβγ S∙(∇ α S×∇ β S)/4≠0 with vanishing average value [B(r)]=0. We evaluate the scattering amplitude in the opposite limits of large and small hopfion radius R using the eikonal and Born approximations, respectively. In both limits, we find that the scattering cross section contains a skew-scattering component giving rise to the Hall effect within a hopfion plane. That conclusion contests the popular notion that the Hall effect in noncollinear magnetic structures necessarily implies [B(r)]≠0. In the limit of small hopfion radius pR<<1, we expand the Born series in powers of momentum p and identify different expansion terms corresponding to the hopfion anisotropy, toroidal moment, and skew scattering.
36 MATERIALS SCIENCE↗