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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 19 records
All sourcesNASA NTRSDOE OSTI
DOE OSTI2021

Spatially co-registered wide-field nonlinear optical imaging of living and complex biosystems in a total internal reflection geometry

Nonlinear optical microscopy that leverages an objective based total internal reflection (TIR) excitation scheme is an attractive means for rapid, wide-field imaging with enhanced surface sensitivity. Through select combinations of distinct modalities, one can, in principle, access complementary chemical and structural information for various chemical species near interfaces. Here, we report a successful implementation of such a wide-field nonlinear optical microscope system, which combines coherent anti-Stokes Raman scattering (CARS), two-photon fluorescence (TPF), second harmonic generation (SHG), and sum frequency generation (SFG) modalities on the same platform. The intense optical fields needed to drive these high order nonlinear optical processes are achieved through the use of femtosecond pulsed light in combination with the intrinsic field confinement induced by TIR over a large field of view. The performance of our multimodal microscope was first assessed through the experimental determination of its chemical fidelity, intensity and polarization dependences, and spatial resolution using a set of well-defined model systems. Subsequently, its unique capabilities were validated through imaging complex biological systems, including Hydrangea quercifolia pollen grains and Pantoea sp. YR343 bacterial cells. Specifically, the spatial distribution of different molecular groups in the former was visualized via vibrational contrast mechanisms of CARS, whereas co-registered TPF imaging allowed the identification of spatially localized intrinsic fluorophores. We further demonstrate the feasibility of our microscope for wide-field CARS imaging on live cells through independent characterization of cell viability using spatially co-registered TPF imaging. Overall, this approach to TIR enabled wide-field imaging is expected to provide new insights into bacterial strains and their interactions with other species in the rhizosphere in a time-resolved and chemically selective manner.

47 OTHER INSTRUMENTATION↗
DOE OSTI2024

Nonexistence of integrable nonlinear magnetic fields with invariants quadratic in momenta

Nonlinear, completely integrable Hamiltonian systems that serve as blueprints for novel particle accelerators at the intensity frontier are promising avenues for research, as Fermilab’s Integrable Optics Test Accelerator (IOTA) example clearly illustrates. Here, we show that only very limited generalizations are possible when no approximations in the underlying Hamiltonian or Maxwell equations are allowed, as was the case for IOTA. Specifically, no such systems exist with invariants quadratic in the momenta, precluding straightforward generalization of the Courant-Snyder theory of linear integrable systems in beam physics. We also conjecture that no such systems exist with invariants of higher degree in the momenta. This leaves solenoidal magnetic fields, including their nonlinear fringe fields, as the only completely integrable static magnetic fields, albeit with invariants that are linear in the momenta. The difficulties come from enforcing Maxwell equations; without constraints, we show that there are many solutions. In particular, we discover a previously unknown large family of integrable Hamiltonians.

97 MATHEMATICS AND COMPUTING↗
DOE OSTI2020

Simple model for the nonlinear radiation field of a free electron laser

It is shown that Jacobi elliptic function solutions of the nonlinear Duffing equation model the radiation field in a high-gain free electron laser through early saturation. After initial start-up, the field can be expressed equivalently with a hyperbolic secant. The model is derived for arbitrary detuning from resonance, which enables study of the spectral properties in the early nonlinear regime.

43 PARTICLE ACCELERATORS↗
DOE OSTI2020

A multi-terawatt two-color beam for high-power field-controlled nonlinear optics

Two-color laser beams are instrumental in light-field control and enhancement of high-order harmonic, spectral supercontinuum, and terahertz radiation generated in gases, plasmas, and solids. Here we demonstrate a multi-terawatt two-color beam produced using a relativistic plasma mirror, with 110 mJ at 800 nm and 30 mJ at 400 nm. Both color components have high spatial quality and can be simultaneously focused, provided that the plasma mirror lies within a Rayleigh range of the driving fundamental beam. Favorable scaling of second-harmonic generation by plasma mirrors at relativistic intensities suggests them as an excellent tool for multi-color waveform synthesis beyond the petawatt level.

42 ENGINEERING↗
DOE OSTI2026

Zonal magnetic fields regulate nonlinear edge-localized-mode dynamics via self-consistent force balance

Edge-localized modes (ELMs) eject intense bursts of heat and particles that threaten plasma-facing components in fusion reactors. Nonlinear full-torus BOUT++ simulations show that turbulence-driven zonal magnetic fields (ZMFs) play an essential role in nonlinear ELM evolution by maintaining self-consistent force balance. Zonal flows mitigate the initial crash through shear but do not prevent continued radial transport. When ZMFs are self-consistently included, turbulence-driven zonal currents modify the parallel current distribution and magnetic tension and are associated with a reduction of the axisymmetric (𝑛 = 0) perturbed radial force imbalance. This coincides with a transition from convective, bursty propagation to more localized, diffusive transport. Similar behavior is observed across the regimes considered, including both resistive-ballooning and peeling-ballooning cases. Finally, associated signatures, including radial electric field shear and parallel current redistribution, provide experimentally accessible diagnostics for present devices and ITER-relevant conditions.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2020

Nonlinear error field response in the presence of plasma rotation and real frequencies due to favorable curvature

This works describes the interaction of an phenomenon known to arise in tokamak fusion experiments with the magnetic perturbations that can arise at the edge of such experiments. We present nonlinear NIMROD resistive MHD simulations of the response of a rotating plasma to an error field when the plasma has weakly damped linear tearing modes (TMs), stabilized by a pressure gradient and favorable curvature. The favorable curvature leads to the Glasser effect: the occurrence of real frequencies and stabilization with positive stability index Δ'.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2024

Quasinormal modes of naked singularities in presence of nonlinear scalar fields

We study linear perturbations against static spherically symmetric background configurations of general relativity with a real scalar field (SF), which is minimally coupled with gravity; it is nonlinear due to the presence of the self-action potential. The background solutions have a naked singularity at the center of the configuration. The focus is on the stability of the background and fundamental frequencies of the quasinormal modes (QNM) of the axial perturbations in the Regge-Wheeler gauge. The problem is reduced to one hyperbolic master equation with an effective potential 𝑊eff, which turns out to be positive for a general non-negative SF potential; this ensures the linear stability with respect to this kind of perturbations. For numerical simulations, the SF potential was chosen in the power-law form 𝑉⁡(𝜙) ∼ 𝜙 2⁢𝑛 with 2 < 𝑛 ≤40. We extracted the fundamental frequencies of QNM for different 𝑛 and various sets of the background configuration parameters. The results show that even for a small background SF, there is a significant difference between the fundamental frequencies and ones in case of the Schwarzschild background. Furthermore, the results are also compared with the case of the Fisher-Janis-Newman-Winicour background dealing with a massless linear scalar field.

General relativity↗
DOE OSTI2023

Near-field terahertz nonlinear optics with blue light

Abstract The coupling of terahertz optical techniques to scattering-type scanning near-field microscopy (s-SNOM) has recently emerged as a valuable new paradigm for probing the properties of semiconductors and other materials on the nanoscale. Researchers have demonstrated a family of related techniques, including terahertz nanoscopy (elastic scattering, based on linear optics), time-resolved methods, and nanoscale terahertz emission spectroscopy. However, as with nearly all examples of s-SNOM since the technique’s inception in the mid-1990s, the wavelength of the optical source coupled to the near-field tip is long, usually at energies of 2.5 eV or less. Challenges in coupling of shorter wavelengths (i.e., blue light) to the nanotip has greatly inhibited the study of nanoscale phenomena in wide bandgap materials such as Si and GaN. Here, we describe the first experimental demonstration of s-SNOM using blue light. With femtosecond pulses at 410 nm, we generate terahertz pulses directly from bulk silicon, spatially resolved with nanoscale resolution, and show that these signals provide spectroscopic information that cannot be obtained using near-infrared excitation. We develop a new theoretical framework to account for this nonlinear interaction, which enables accurate extraction of material parameters. This work establishes a new realm of possibilities for the study of technologically relevant wide-bandgap materials using s-SNOM methods.

47 OTHER INSTRUMENTATION↗
DOE OSTI2024

Three-dimensional continuum point cloud method for large deformation and its verification

This study presents a strong form based meshfree collocation method, which is named Continuum Point Cloud Method, to solve nonlinear field equations derived from classical mechanics for deformed bodies in three-dimensional Euclidean space. The method and its implementation are benchmarked against a nonlinear vector field using manufactured solutions. The analysis of mechanical fields firstly focuses on the study of St. Venant Kirchhoff and compressible neo-Hookean materials. Results for various initial boundary value problems are presented, including benchmark cases involving unidirectional tension and simple shear. Subsequently, the study concludes with an analysis of a displacement-controlled simulation of a compressible neo-Hookean material, specifically a bar that is pulled to 50% of its original length and rotated 90°. The pure tension case yields a 1.5% error in displacement between computed and expected values and a combined tension and torsion loading case provides further insight into material behavior under complex loading conditions. The resulting normal axial and transverse stress-strain curves are also presented. Lastly, the consistency and robustness of the proposed nonlinear numerical schemes are successfully demonstrated through various numerical experiments.

Compressible neo-Hookean materials↗
DOE OSTI2021

On the possibility of footprint compression with one lens in nonlinear accelerator lattice

Electromagnetic interaction of colliding beams along with other nonlinear fields often limits the beams' lifetimes and luminosities. Nonlinearities result in the spread of betatron frequencies (footprint) and, thus, may enhance dynamic diffusion of particles due to high order resonances. One of the possible ways to eliminate nonlinearities and overcome the corresponding difficulties is compensation of nonlinear forces, but, in practice, it is hardly possible to obtain exact linearity of the system. The compensation with a single nonlinear lens cannot cope with distributed nonlinearities, nonlinearities due to parasitic crossings, etc. Here, we present a method to compute parameters of nonlinear element (lens) that eliminates both the footprint and resonance strength without achieving full compensation.

43 PARTICLE ACCELERATORS↗
DOE OSTI2024

Experiments and gyrokinetic simulations of the nonlinear interaction between spinning magnetized plasma pressure filaments

A set of experiments using controlled, skin depth-sized plasma pressure filaments in close proximity have been carried out in a large linear magnetized plasma device. Two- and three-filament configurations have been used to determine the scale of cross field nonlinear interaction. When the filaments are separated by a distance of approximately five times the size of a single filament or less, a significant transfer of charge and energy occurs, leading to the generation of inter-filament electric fields. This has the effect of rotating the filaments and influencing the merging dynamics. Nonlinear gyrokinetic simulations using seeded filaments confirm the presence of unstable drift-Alfvén modes driven by the steep electron temperature gradient. When the filaments are within a few collisionless electron skin depths (separations twice the size of a single filament), the unstable perturbations drive the convective mixing of the density and temperature and rearrange the gradients such that they maximize in the region surrounding the filament bundle.

Sydora, R. D. (ORCID:0000000192543149)↗
DOE OSTI2025

Study of Quadrupole Fringe Fields in the Interaction Region of the Hadron Storage Ring of the Electron Ion Collider

Fringe fields in quadrupole magnets are usually neglected in studies of beam dynamics at accelerators. However, the extreme optical parameters present in the final focus of a collider such as the Electron–Ion Collider (EIC) may give rise to effects that should not be overlooked. The calculation of quadrupole fringe fields presented in this study follows the procedure outlined in Ref. [1], specialized to the case of a straight reference orbit (i.e., with no dipole field component). A right-handed Cartesian coordinate system is employed, with the $z$-axis aligned with the quadrupole axis and $x$ and $y$ denoting the horizontal and vertical transverse coordinates, respectively. The magnetic quadrupole field gradient, $G = \partial B_y / \partial x$, transitions from its peak value inside the quadrupole—where it is nearly independent of the longitudinal coordinate $z$—to zero at some distance beyond the magnet edge. Consequently, $G$ is treated as a function of $z$. The region over which this variation occurs is defined as the quadrupole fringe field region. The study begins with the development of a description of the magnetic field in the fringe region using a power-series expansion in the transverse coordinates $x$and $y$, consistent with the longitudinally varying gradient. A model for the $z$-dependence of the gradient is then proposed and adjusted to reproduce magnetic field data obtained from three-dimensional field calculations. To evaluate the impact of the fringe fields on beam dynamics, the corresponding vector potential is derived and incorporated into a Hamiltonian formulation of particle motion. The significance of the fringe fields is quantified by calculating the amplitude-dependent tune shift from the Hamiltonian. Using linear beam optics parameters of the Hadron Storage Ring (HSR) of the EIC, the tune shift due to the fringe fields of all quadrupole magnets in the IR-6 interaction region is evaluated. Finally, the resulting tune shifts are compared with those arising from other nonlinear field components present in the HSR.

43 PARTICLE ACCELERATORS↗
DOE OSTI2022

Control of second-harmonic generation in all-dielectric intersubband metasurfaces by controlling the polarity of χ (2)

All-dielectric metasurfaces have recently led to a paradigm shift in nonlinear optics as they allow for circumventing the phase matching constraints of bulk crystals and offer high nonlinear conversion efficiencies when normalized by the light-matter interaction volume. Unlike bulk crystals, in all-dielectric metasurfaces nonlinear conversion efficiencies primarily rely on the material nonlinearity, field enhancements, and the modal overlaps, therefore most efforts to date have only focused on utilizing these degrees of freedom. In this work, we demonstrate that for second-harmonic generation in all-dielectric metasurfaces, an additional degree of freedom is the control of the polarity of the nonlinear susceptibility. We demonstrate that semiconductor heterostructures that support resonant nonlinearities based on quantum-engineered intersubband transitions provide this new degree of freedom. We can flip and control the polarity of the nonlinear susceptibility of the dielectric medium along the growth direction and couple it to the Mie-type photonic modes. Here we demonstrate that engineering the χ (2) polarity in the meta-atom enables the control of the second-harmonic radiation pattern and conversion efficiency. Our results therefore open a new direction for engineering and optimizing second-harmonic generation using all-dielectric intersubband nonlinear metasurfaces.

42 ENGINEERING↗
DOE OSTI2023

Exploring the Dynamics of Transverse Inter-planar Coupling in the SC Section of the PIP-II Linac

This study investigates the crucial role that an accurate understanding of inter-planar coupling in the transverse plane plays in regulating charged particle dynamics in a high-intensity linear accelerator and minimizing foil/septum impacts during injection from the linac to a ring. We in-depth analyze the emergence and evolution of transverse inter-planar coupling through multiple active lattice elements, taking into account space charge and field nonlinearities in the superconducting section of the PIP-II linac. The article compares various analytical, numerical, and experimental techniques for measuring transverse coupling using beam and lattice matrices and provides insight into effective strategies for its mitigation prior to ring injection.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2023

Exploring the Dynamics of Transverse Inter-planar Coupling in the Superconducting Section of the PIP-II LINAC

This study investigates the crucial role that an accurate understanding of inter-planar coupling in the transverse plane plays in regulating charged particle dynamics in a high intensity linear accelerator and minimizing foil/septum impacts during injection from the linac to a ring. We performed an in-depth analysis for the emergence and evolution of trans verse inter-planar coupling through multiple active lattice elements, taking into account space charge and field nonlinearities in the superconducting section of the PIP-II linac. The article compares various analytical, numerical, and experimental techniques for measuring transverse coupling using beam and lattice matrices and provides insight into effective strategies for its mitigation prior to ring injection.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2022

Optimization of Superconducting Linac for Proton Improvement Plan-II (PIP-II)

PIP-II is an essential upgrade of the Fermilab complex that will enable the worlds most intense high-energy beam of neutrinos for the international Deep Underground Neutrino Experiment at LBNF and support a broad physics program at Fermilab. Ultimately, the PIP-II superconducting linac will be capable of accelerating the $H-$ CW beam to 800 MeV with an average power of 1.6 MW. To operate the linac with such high power, beam losses and beam emittance growth must be tightly controlled. In this paper, we present the results of global optimization of the Linac options towards a robust and efficient physics design for the superconducting section of the PIP-II linac. We also investigate the impact of the nonlinear field of the dipole correctors on the beam quality and derive the requirement on the field quality using statistical analysis. Finally, we assess the need to correct the quadrupole focusing produced by Half Wave, and Single Spoke accelerating cavities. We assess the feasibility of controlling the beam coupling in the machine by changing the polarity of the field of linac focusing solenoids

43 PARTICLE ACCELERATORS↗