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At least 19 records

Analysis of NCERC Critical Experiments with ENDF/B Nuclear Data Libraries

Nuclear data (ND) libraries are the backbone of the nuclear industry, as they are the collections of tabulated probabilities that define sub-atomic particle interactions with matter. In the areas of criticality safety and experiments, no evaluated nuclear data files (ENDF) are more important than those containing neutron cross section data. It is upon these files, and accompanying radiation transport codes, that practitioners are enabled to safely design both subcritical and critical systems. Likewise, in a symbiotic fashion, it is the same critical assemblies which are used primarily to validate that the cross sections are correct. The ENDF/B library, the United States’ national library maintained by the National Nuclear Data Center (NNDC) at Brookhaven National Laboratory (BNL), is soon releasing a new version, ENDF/B-VIII.1. Prior to the official release, several beta versions of the library were prepared and tested in simulation suites. The work presented here are results comparing the newest ENDF/B beta release (ENDF/B-VIII.1b3) and ENDF/B-VIII.0 with recent experiments done at the National Criticality Experiments Research Center (NCERC) as well as correlated experiments from the Los Alamos Critical Experiments Facility (LACEF). These NCERC and LACEF experiments were performed in part to provide validation for various cross sections that were identified as insufficient in the ENDF/B-VIII.0. In particular, lead, copper, fluorine, and chlorine, as well as the major actinides, were targeted from the last decade of critical experiments.

97 MATHEMATICS AND COMPUTING↗

Scattering Angular Distributions in the ENDF/B Nuclear Data Library

Nuclear reactors function by controlling the chain reaction of fission events in a fissile material. Understanding the gain and loss of neutrons is crucial for controlling this chain reaction. The role of fission in liberating neutrons from nuclei is well known. The fact that neutrons can scatter out of a reactor and therefore be lost is less well appreciated. Scattering can happen within fissile fuel or off of any number of the non-fissile structural components holding a reactor together. The scattering angular distributions for reactor material are the quantity that give the probability for a particle (usually a neutron) to scatter off a nucleus into a given angle. The Evaluated Nuclear Data File/B (ENDF/B) nuclear data library is the most complete and authoritative reference for neutron scattering data, containing reaction cross sections and outgoing particle distributions (including scattering angular distributions). In this project, we will compare the scattering angular distributions given in these ENDF/B data sets with those that can be derived using the Blatt-Biedenharn formalism and the resolved resonance data also in the ENDF/B files. More comparisons between the scattering angular distributions of relevant isotopes will help identify and correct any errors in the ENDF/B files. The results of this study will be an important component of the next major release of the ENDF/B library.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

AMPX: A Modern cross section processing system for generating nuclear data libraries - 14619

Nuclear data libraries are essential for nuclear analysis code systems like SCALE. AMPX has been continuously developed since the early 1970's and is used to generate these data libraries for SCALE. Recently, Oak Ridge National Laboratory (ORNL) initiated a major modernization effort to position AMPX for continued development and deployment on modern computing platforms. An important step toward modernization has been to merge AMPX under the SCALE continuous integration (CI) development framework. As a result, AMPX is now developed under the SCALE software quality assurance plan, providing increased confidence in the quality of data libraries developed and deployed by AMPX. This merge allowed us to develop novel methods to generate self-shielding factors that combine SCALE's resonance self-shielding capabilities with the AMPX library-generation capabilities. AMPX processes Evaluated Nuclear Data Format (ENDF/B) files. The ENDF community is working to develop a more modern format that will replace the existing ENDF/B format. Due to strict space and memory requirements when AMPX was first developed, the original AMPX processing and reading of ENDF data were tightly integrated. On newer computer systems, this is no longer necessary. Now there is a separation between reading and processing which allows for simultaneous support of current and new ENDF formats. As a result, AMPX is positioned to adopt any new ENDF format when available. For end users, the modernization effort has resulted in improved processing capabilities for generating nuclear data libraries. The objective of the paper is to document the latest AMPX cross-section processing capabilities and provide the current status of the AMPX modernization effort. (authors)

42 ENGINEERING↗

TENDL: Complete Nuclear Data Library for Innovative Nuclear Science and Technology

The TENDL library is now established as one of the major nuclear data libraries in the world, striving for completeness and quality of nuclear data files for all isotopes, evaluation methods, processing and applied performance. To reach this status, some basic principles have been applied which sets it apart from other libraries: reproducible dedicated evaluations when differential data are available, through determination of nuclear models implemented in TALYS and their parameters, completeness (with or without experimental data), format and processing standardization, automation of production and reproducibility. In this paper, we will outline how such an approach has become a reality, and recall some of the past successes since the first TENDL release in 2008. Next, we will demonstrate the performance of the latest TENDL releases for different application fields, as well as new approaches for uncertainty quantification based on Bayesian inference methods and possible differential and integral adjustments. Also, current limitations of the library performances due to modelling and needs for new and more precise experimental data will be outlined.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

TENDL-2017: the making of multi-faceted technological nuclear data library - 25340

Multi-purpose methodical nuclear data libraries generated by TALYS/T6 as Evaluated Nuclear Data Library TENDL have been released regularly since 2008. Considerable experience has been acquired during those early production of such unique, truly multi-faceted, multi-particle nuclear data libraries based on the feedback from the developers, evaluators, processing experts and, most importantly, users. The backbone of this achievement is simple and robust: completeness, quality, upgradability and, most of all, reproducibility and methodology. Since TENDL has been seamlessly adopted by many different applications (accelerator, astrophysics, fusion, fission, medical) that require multi-faceted nuclear reaction data forms for shielding, radio-protection, transmutation, materials or earth sciences, it is felt necessary to understand its strengths and remaining weaknesses. The essential knowledge is not the TENDL library itself, but rather the necessary methods, processes, codes, tools and know-how that go into the making of every evaluations of such a library. Current efforts are focused on a proper evaluation of the underlying physics and incorporation of information and metrics into the scientific TALYS/T6 system. (authors)

61 RADIATION PROTECTION AND DOSIMETRY↗

Legacy (NDF & MCF), GNDS and Direct forms of the ENDL2009.5 Evaluated Nuclear Data Library

The ENDL2009.5 Evaluated Nuclear Data Library is now available three different processed forms for users: (1) the Legacy form using NDF and MCF processing of the ENDL files, (2) the GNDS form which uses FUDGE and Merced to process the translations in to GNDS of the ENDL files, and (3) the Direct form which uses FUDGE and Merced to process where available the original ENDF6- format source files used to make the ENDL files. If original files are not available for various protares in the Direct form, then the ENDL forms are used.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

2009.1 Revision of the Evaluated Nuclear Data Library (ENDL2009.1)

LLNL’s Computational Nuclear Data and Theory Group have created a 2009.1 revised release of the Evaluated Nuclear Data Library (ENDL2009.1). This library is designed to support LLNL’s current and future nuclear data needs and will be employed in nuclear reactor, nuclear security and stockpile stewardship simulations with ASC codes. The ENDL2009 database was the most complete nuclear database for Monte Carlo and deterministic transport of neutrons and charged particles. It was assembled with strong support from the ASC PEM and Attribution programs, leveraged with support from Campaign 4 and the DOE/Office of Science’s US Nuclear Data Program. This document lists the revisions and fixes made in a new release called ENDL2009.1, by comparing with the existing data in the original release which is now called ENDL2009.0. These changes are made in conjunction with the revisions for ENDL2011.1, so that both the .1 releases are as free as possible of known defects.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

2009.3 Revision of the Evaluated Nuclear Data Library (ENDL2009.3)

LLNL's Computational Nuclear Data and Theory Group have created a 2009.3 revised release of the Evaluated Nuclear Data Library (ENDL2009.3). This library is designed to support LLNL's current and future nuclear data needs and will be employed in nuclear reactor, nuclear security and stockpile stewardship simulations with ASC codes. The ENDL2009 database was the most complete nuclear database for Monte Carlo and deterministic transport of neutrons and charged particles. It was assembled with strong support from the ASC PEM and Attribution programs, leveraged with support from Campaign 4 and the DOE/Office of Science's US Nuclear Data Program. This document lists the revisions and fixes made in a new release called ENDL2009.3, by com- paring with the existing data in the previous release ENDL2009.2. These changes are made in conjunction with the revisions for ENDL2011.3, so that both the .3 releases are as free as possible of known defects.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Evaluated Nuclear Data Library, with ENDL2009.5-direct (2009.5 Rev.)

LLNL’s Nuclear Data and Theory Group have created a 2009.5 revised release of the Evaluated Nuclear Data Library (ENDL2009.5). This library is designed to support LLNL’s current and future nuclear data needs and will be employed in nuclear reactor, nuclear security and stockpile stewardship simulations with ASC codes. The ENDL2009 database was the most complete nuclear database for Monte Carlo and deterministic transport of neutrons and charged particles. It was assembled with strong support from the ASC PEM and Attribution programs, leveraged with support from Campaign 4 and the DOE/Office of Science’s US Nuclear Data Program. This document lists the revisions and fixes made in a new release called ENDL2009.5, by comparing with the existing data in the previous releases ENDL2009.3 and ENDL2009.4. In addition to the legacy library ENDL2009.5 from ENDL-format files generated by Fete, an ENDL2009.5-direct library is also released, in which ENDF6-formatted sources are used wherever possible to avoid possible translation errors from Fete.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Testing nuclear data libraries with burnup for reactor applications

Recently US and European nuclear data libraries have been released, namely ENDF/B-VIII.0 and JEFF-3.3 libraries, which are the result of years of evaluation and validation work in both communities. Consequently, efforts have been made to validate the evaluations in calculations of integral experiments (critical benchmarks, ..etc). Nevertheless, less stringent testing and validation efforts were performed on burnup applications before releasing the libraries. The presented work focusses on the testing of these recent nuclear data libraries for burnup calculations on two benchmarks at the pin and at the assembly level. Monte-Carlo depletion calculations were performed using the VESTA 2.2 code. The K{sub ∞} results between nuclear data libraries are compared. A strong k{sub ∞} bias is observed with burnup using both JEFF-3.3 and JEFF-4T0 compared to all other libraries, and especially ENDF/B-VIII.0, consisting in a strong k{sub ∞} over-estimation at low burnup and a high under-estimation at high burnup. JEFF-3.3 {sup 235}U and {sup 239}Pu evaluations mainly explain this result, as well as fission yields. New {sup 235}U and {sup 239}Pu evaluations were proposed for JEFF-4T0, but they do not address totally the bias issue, even if JEFF-4T0 {sup 239}Pu allows slightly reducing the k{sub ∞} underestimation at high burnup.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

2011.2 Revision of the Evaluated Nuclear Data Library (ENDL2011.2)

LLNL's Computational Nuclear Physics Group and Nuclear Theory and Modeling Group have col- laborated to create the 2011.2 revised release of the Evaluated Nuclear Data Library (ENDL2011.2). ENDL2011.2 is designed to support LLNL's current and future nuclear data needs and will be em- ployed in nuclear reactor, nuclear security and stockpile stewardship simulations with ASC codes. This database is currently the most complete nuclear database for Monte Carlo and deterministic transport of neutrons and charged particles. This library was assembled with strong support from the ASC PEM and Attribution programs, leveraged with support from Campaign 4 and the DOE/O ce of Science's US Nuclear Data Program. This document lists the revisions made in ENDL2011.2 compared with the data existing in the original ENDL2011.0 release and the ENDL2011.1-rc4 re- lease candidate of April 2015. These changes are made in parallel with some similar revisions for ENDL2009.2.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Reasons for 2011 Release of the Evaluated Nuclear Data Library (ENDL2011.0)

LLNL's Computational Nuclear Physics Group and Nuclear Theory and Modeling Group have collaborated to create the 2011 release of the Evaluated Nuclear Data Library (ENDL2011). ENDL2011 is designed to sup- port LLNL's current and future nuclear data needs. This database is currently the most complete nuclear database for Monte Carlo and deterministic transport of neutrons and charged particles, surpassing ENDL2009.0 [1]. The ENDL2011 release [2] contains 918 transport-ready eval- uations in the neutron sub-library alone. ENDL2011 was assembled with strong support from the ASC program, leveraged with support from NNSA science campaigns and the DOE/Offce of Science US Nuclear Data Pro- gram.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

2011.5 Revision of the Evaluated Nuclear Data Library: ENDL2011.5 (legacy and GNDS), and ENDL2011.5-direct

LLNL’s Nuclear Data and Theory Group has created the 2011.5 revised release of the Evaluated Nuclear Data Library (ENDL2011.5). ENDL2011.5 is designed to support LLNL’s current and future nuclear data needs and will be employed in nuclear reactor, nuclear security and stockpile stewardship simulations with ASC codes. This database is currently the most complete nuclear database for Monte Carlo and deterministic transport of neutrons and charged particles. This library was assembled with strong support from the ASC PEM and Attribution programs, leveraged with support from Campaign 4 and the DOE/Office of Science’s US Nuclear Data Program. This document lists the revisions made in ENDL2011.5 compared with the data existing in the original ENDL2011.2 and ENDL2011.3 releases. These changes are made in parallel with some similar revisions for ENDL2009.5. We also describe ENDL2011.5-direct that directly uses ENDF sources wherever possible.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

AMPX and SCALE Nuclear Data Libraries for Depletion [Slides]

This presentation touches on AMPX and SCALE nuclear data libraries for depletion. AMPX is a nuclear data processing code suite that generates continuous-energy and multigroup neutron and gamma libraries used in SCALE and VERA, covariance data used in S/U calculations, and depletion, activation and decay origin data for Oak Ridge Isotope Generation code (ORIGEN).

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Development and Testing of Nuclear Data Libraries for Improved Energy Deposition Modeling - Paper 144

Accurate calculations of local energy deposition rates require the presence of gamma production data (GPD) in the nuclear data library used by radiation transport codes such as MCNP5, MONACO, or Denovo. The lack of GPD in the underlying nuclear data library can cause significant over-prediction of local heat generation rates with a corresponding under-prediction of heat generation rates away from a region of interest. To address this concern, continuous energy (CE) and multigroup (MG) cross section libraries with additional GPD have been created. Both ACE- and AMPX-formatted CE libraries, as well as ANISN- and AMPX-formatted MG libraries, have been created and are undergoing verification and validation (V and V) testing. A hybrid data set consisting of cross-section evaluations from five different nuclear data repositories has been developed. This hybrid data set, referred to as GPD-Rev0, is intended to support enhanced energy deposition calculations. Code-specific libraries in CE ACE, CE AMPX, MG AMPX, and MG ANISN formats have been created from the GPD-Rev0 data set. V and V testing has demonstrated that these various code-specific libraries are performing well for the intended applications. Localized over- and under-predictions of HFIR heating rates have been addressed without adversely affecting the prediction of other key operating parameters. (authors)

61 RADIATION PROTECTION AND DOSIMETRY↗

2011 Release of the Evaluated Nuclear Data Library (ENDL2011.0)

LLNL’s Computational Nuclear Physics Group and Nuclear Theory and Modeling Group have collaborated to produce the last of three major releases of LLNL’s evaluated nuclear database, ENDL2011. ENDL2011 is designed to support LLNL’s current and future nuclear data needs by providing the best nuclear data available to our programmatic customers. This library contains many new evaluations for radiochemical diagnostics, structural materials, and thermonuclear reactions. We have made an effort to eliminate all holes in reaction networks, allowing in-line isotopic creation and depletion calculations. We have striven to keep ENDL2011 at the leading edge of nuclear data library development by reviewing and incorporating new evaluations as they are made available to the nuclear data community. Finally, this release is our most highly tested release as we have strengthened our already rigorous testing regime by adding tests against IPPE Activation Ratio Measurements, many more new critical assemblies and a more complete set of classified testing (to be detailed separately).

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Expanded Intercomparison of Nuclear Data Libraries Using Jupiter and Jupiter High-240 Experiments

There is a limited availability of plutonium experiments with sensitivity to lead in the ICSBEP (International Handbook of Evaluated Criticality Safety Benchmark Experiments) Handbook. The Jupiter and Jupiter High-240 experiments were performed at the National Criticality Experiments Research Center as a collaborative effort between Los Alamos National Laboratory and the Japan Atomic Energy Agency to assess lead void coefficients in a plutonium-lead system containing weapons- and reactor-grade plutonium, respectively. Concurrent with benchmark development, an intercomparison of calculations using different nuclear data libraries has been performed to assess the usability of the experimental data for nuclear data adjustment in a “softer-that-fast” neutron energy spectrum. Eigenvalue calculations using MCNP with the ENDF/B-VIII.0 and TENDL-2021 nuclear data libraries calculate closest to the benchmark values for Jupiter. Calculations using JENDL-5 and ENDF/B-VIII.1 match best with the Jupiter High-240 values. Lead void worth calculations using the various nuclear data libraries are all within 3σ of their respective measured values. Perturbation studies between ENDF/B-VIII.0 and ENDF/B-VIII.1 demonstrate an approximate increase in calculated eigenvalues for the Jupiter series experiments by ~240 pcm for plutonium (mostly 239 Pu) and ~120 pcm for lead accompanied by a decrease contributed by ~113 pcm for copper and ~13 pcm for stainless steel. Nuclear data sensitivities and uncertainties investigated using Whisper show slightly lower sensitivity to scatter than a lead-reflected plutonium sphere but greater sensitivity to neutron capture. The sensitivities between Jupiter and Jupiter High-240 for lead are very similar for both ENDF/B-VIII.0 and ENDF/B-VIII.1 nuclear data. These benchmarks are more sensitive to neutron capture in lead than other plutonium benchmark experiments and would be useful for both lead and 240 Pu validation. In conclusion, with the high degree of compensating effects between copper, lead, and plutonium cross sections, additional isolated Pb-Pu and Cu-Pu benchmarks would be beneficial in improving these nuclear data.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

The EUCLID Experiment and Nuclear Data Library Comparisons

The EUCLID (Experiments Underpinned by Computational Learning for Improvements in Nuclear Data) project at Los Alamos National Laboratory (LANL) was a Laboratory Directed Research and Development project which aimed to reduce compensating errors in nuclear data. One major component of the project was a series of critical experiments, both measuring k eff and various other observables with the goal of using these experiments to constrain 239 Pu nuclear data uncertainties and identify compensating errors. This paper details some of the experiment design and how various nuclear data libraries simulate the EUCLID system, including sensitivities compared to Jezebel.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗