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The r-, s-, and p-Processes in Nucleosynthesis

Burbidge et al (1957) and Cameron (1957) laid out the framework for our understanding of the formation of the heavy nuclei (those nuclei with mass number A approx. greater than 70). From systematics in the solar system abundance distribution, Burbidge et al determined that the heavy nuclei were formed in three distinct nucleosynthetic processes, which they termed the r-, s-, and p-processes. That we still use these terms today is a credit to the soundness of this work done 37 years ago. We may understand how Burbidge et al and Cameron arrived at their conclusions from Figure 1. One population of nuclei, the s-nuclei, shows an abundance distribution with peaks near mass numbers 87, 138, and 208. These nuclei are made in a slow neutron-capture process, the s-process. A rapid neutron-capture process, the r-process, is responsible for the r-nuclei, whose abundance distribution shows peaks at mass numbers 80, 130, and 195. The p-process is responsible for production of the rarer, more proton-rich heavy isotopes (the p-nuclei) that cannot be made by neutron capture. The first quantitative evaluations of the ideas of Burbidge et al and Cameron came to light in the early 1960s with work on the s-process (Clayton et al 1961, Seeger et al 1965) and the r-process (Seeger et al 1965). These calculations further elucidated the mechanisms for heavy-element formation and showed the plausibility of the framework developed in the 1950s. Subsequent work has focused on determining the astrophysical sites where the r-, s-, and p-processes occurred with the help of improved nuclear details, stellar models, and abundances. A goal of this paper is to review the recent progress astrophysicists, astronomers, and physicists have made in these directions and to point out the problems that remain in our understanding of the formation of the heavy nuclei. Another, perhaps deeper, goal is to to seek some understanding of why there are three major processes available to nature for synthesis of heavy elements. It is impossible for a single paper to cover all relevant aspects of the r-, s-, and p-processes; therefore, where possible, references to other reviews are given. Readers should turn to these reviews for more details. Nevertheless, it is hoped that the present paper gives some flavor for the rich field of heavy-element synthesis.

Meyer, Bradley S.↗

The p-process in explosive nucleosynthesis.

The limiting conditions consistent with p-process synthesis in supernova envelopes are inferred from calculations of the appropriate rates of proton capture and neutron photodisintegration. Temperatures in excess of 2 x 10 to the 9th power K are required, for proton mass densities of the order of 100 g cm to the minus 3rd power, if significant production of p-process nuclei is to take place on a hydrodynamic time scale. It is concluded that these processes must be appropriate to very different stellar or supernova environments.

Truran, J. W.↗

On strontium isotopic anomalies and odd-A p-process abundances

Several aspects of the nucleosynthesis of Sr isotopes are considered in an attempt to shed light on the problem of the Sr isotopic anomalies discovered in an inclusion of the Allende meteorite. Decomposition of the Sr isotopes into average r-, s-, and p-process nucleosynthetic classes is performed. It is suggested that the Allende inclusion most likely has an excess of s-process Sr and that the initial Sr-87/Sr-86 isotopic ratio is probably slightly more primitive than basaltic achondrites. The results also show that Sn-115 is mostly due to the r-process and that odd-A yields are very small. It is concluded that if the Sr anomaly in the inclusion is an average s enhancement, it argues somewhat in favor of a model of gas/dust fractionation of s and r isotopes during accumulation of the inclusion parent in the protosolar cloud.

Clayton, D. D.↗

The r-, s-, and p-Processes in Nucleosynthesis

A goal of this paper is to review the recent progress astrophysicists, astronomers, and physicists have made in the r-, s-, and p-processes in nucleosynthesis and to point out the problems that remain in our understanding of the formation of the heavy nuclei. Another, perhaps deeper, goal is to to seek some understanding of why there are three major processes available to nature for synthesis of heavy elements.

Meyer, Bradley S.↗

Molybdenum Isotopic Composition of Iron Meteorites, Chondrites and Refractory Inclusions

Recent Mo isotopic studies of meteorites reported evidence for differences in isotopic compositions for whole rocks of some primitive and differentiated meteorites relative to terrestrial materials. Enrichments of r- and p-process isotopes of up to 3-4 units (e unit = parts in 10(exp 4) over s-process dominated isotopes are the most prominent features. Certain types of presolar grains show large enrichments in s-process isotopes, however, it was concluded on grounds of mass balance that incomplete digestion of such grains cannot explain the enrichments of r- and p-process isotopes in whole rocks of primitive chondrites. If the reported variability in r- and p-process isotope enrichments reflects the true isotopic characteristics of the whole rocks, the implications are quite profound. It would suggest the presence of large scale Mo isotopic heterogeneity within the solar accretion disk with likely collateral effects for other elements. However, such effects were not found for Ru isotopes, nor for Zr isotopes. Another recent Mo isotopic study by multi collector ICP-MS could not confirm the reported deviations in Allende, Murchison or iron meteorites. Here, we present new results for the Mo isotopic composition of iron meteorites, chondrites and CAIs obtained by negative thermal ionization mass spectrometry (NTIMS). We discuss analytical aspects and the homogeneity of Mo isotopic compositions in solar system materials.

Becker, H.↗

Spectrum of carbonaceous-chondrite fission xenon

Estimations of the fission spectrum in xenon isotopes from the progenitor of the strange carbonaceous-chondrite xenon must take account of p-process nucleosynthesis if the latter is the source of anomalous Xe-124, 126. Sample calculations of the p-process yields illustrate the magnitude of the effect, which can greatly increase the estimated Xe-132 fission yield.

Clayton, D. D.↗

The presence of Sm-146 in the early solar system and implications for its nucleosynthesis

A correlation of Nd-142/Nd-144 with Sm-144/Nd-144 in two meteorites which have a large range in Sm-144/Nd-144 in their constituent mineral phases is presented as evidence for the presence of the p-process nucleus Sm-146 in the early solar system and its alpha-decay into Nd-142. The ratio Sm-146/Sm-144 is estimated to be about 0.015 at the time of solar system formation, 4.56 AE ago. It is suggested that the abundance of Sm-146 is compatible with p-proc ess production rate estimates, but not with the production rate for Sm-146 based on a photodisintegration model for the production of p-process nuclides.

Prinzhoffer, A.↗

More on Ru Endemic Isotope Anomalies in Meteorites

We reported last year on endemic isotope anomalies for Ru in iron meteorites, pallasites, ordinary chondrites, and on a whole-rock sample of Allende. We have extended the Ru measurements to more meteorites, to refractory Ca-Al-rich inclusions (CAI) from Allende, and to a whole rock sample of Murchison (CM2). In a companion abstract we report on new measurements for the Mo isotopes, in some of the same samples. There has been a renewed interest in searching for isotope anomalies in this nuclide region, as Ru and Mo include many isotopes from r-, s-, and p-process nucleosynhesis. Furthermore, the Ru and Mo p-process isotopes show atypically high abundances, which have been hard to explain through the standard nucleosynthetic processes. Effects are possible in Ru-98 and Ru-99 from Tc-98 (with a poorly known t(sub 1/2)=4.2 to 10Ma) and from Tc-99 (t(sub 1/2)=0.21Ma). Natural Tc is now extinct on Earth due to the short half-lives, but may have been present in the early solar system. Both radiogenic and general isotope anomalies are important in understanding the processes for the formation of the early solar system. The current emphasis on Ru and Mo is also the result of the development of Negative-ion Thermal Ionization Mass Spectrometry and of Multiple-Collector, Inductively-Coupled-Mass-Spectrometry. We have also developed specific chemical siparation techniques for Ru, which eliminated mass interference effects.

Papanastassiou, D. A.↗

Samarium-146 in the early solar system - Evidence from neodymiun in the Allende meteorite

A carbon-chromite fraction from the Allende C3V chondrite shows strikingly large isotopic enrichments of neodymium-142 (0.47 percent) and neodymium-143 (36 percent). Both apparently formed by alpha decay of samarium-146 and samarium-147 (half-lives 1.03 x 10 to the 8th and 1.06 x 10 to the 11th years), but the isotopic enrichment was greatly magnified by recoil of residual nuclei into a carbon film surounding the samarium-bearing grains. These data provide an improved estimate of the original abundance of extinct samarium-146 in the early solar system, Sm-146/Sm-144 = (4.5 + or - 0.5) x 10 to the -3rd, higher than predicted by some models of p-process nucleosynthesis. It may be possible to use this isotopic pair as a chronometer of the early solar system.

Lugmair, G. W.↗

Al-26 in the interstellar medium

The amount of dispersed interstellar Al-26 detected by the HEAO 3 gamma-ray spectrometer cannot have been synthesized by supernova explosions if current calculations of the production ratio p(26)/p(27) approximately equal to 0.001 are correct. Simple models of chemical evolution of the Galaxy are presented to explain this point. The observed Al-26 is more likely due to about 100 million dispersed novae, or to a single old (10,000-1,000,000 yr) supernova remnant that today surrounds the solar system. If the Al-26 is dispersed, the high interstellar ratio today Al-26/Al-27 about equal to 0.00002 calls into question the requirement that a supernova trigger for formation of the solar system was the cause of a concentration 3-times larger. Also discussed is p-process production in novae with application to the question of live Sm-146 in the solar system.

Clayton, D. D.↗

Heavy-element abundances from a neutron burst that produces Xe-H

We examine quantitatively the suggestion that the heavy anomalous isotopes of Xe-HL found in meteoritic diamonds were produced by a short intense neutron burst and then implanted into the diamonds. Using a large nuclear reaction network we establish one (out of many) neutron irradiation hostories that successfully reproduces the heavy isotopes of Xe-HL, and then evaluate what that same history would produce in every heavy element. This has become more relevant following recent measurement of anomalous Ba and Sr in those same diamond samples. Therefore we offer these calculations as a guide to the anomalies to be expected in all elements if this scenario is correct. We also discuss several other aspects of the problem, especially the established contradictions for Ba, the observed Kr pattern, the near normalcy of Xe-129 and some related astrophysical ideas. In particular we argue from p-process theory that the observed deficit of Kr-78 in correlation with Xe-(124-126) excess implicates Type II supernovae as the diamond sources.

Howard, W. M.↗

Interstellar grains in primitive meteorites - Diamond, silicon carbide, and graphite

Primitive meteorites contain a few parts per million (ppm) of pristine interstellar grains that provide information on nuclear and chemical processes in stars. Their interstellar origin is proven by highly anomalous isotopic ratios, varying more than 1000-fold for elements such as C and N. Most grains isolated thus far are stable only under highly reducing conditions (C/O greater than 1), and apparently are 'stardust' formed in stellar atmospheres. Microdiamonds, of median size about 10 A, are most abundant (about 400-1800 ppm) but least understood. They contain anomalous noble gases including Xe-HL, which shows the signature of the r- and p-processes. Silicon carbide, of grain size 0.2-10 microns and abundance about 6 ppm, shows the signature of the s-process and apparently comes mainly from red giant carbon (AGB) stars of 1-3 solar masses. Some grains appear to be not less than 10 exp 9 a older than the solar system. Graphite spherules of grain size 0.8-7 microns and abundance less than 2 ppm contain highly anomalous C and noble gases, as well as large amounts of fossil Mg-26 from the decay of extinct Al-26. They seem to come from at least three sources, probably AGB stars, novae, and Wolf-Rayet stars.

Anders, Edward↗