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DOE OSTI2024

Sulfide precipitation characteristics of Mn, Ni, Co, and Zn in the presence of contaminant metal ions

In this study, the effects of Al 3+ and Fe 2+ on the precipitation characteristics of four valuable metals, including Mn 2+ , Ni 2+ , Co 2+ , and Zn 2+ , were investigated by conducting solution chemistry calculations, sulfide precipitation tests, and mineralogy characterizations. It was found that the ability of the valuable metals to form sulfide precipitates followed an order of Zn 2+ > Ni 2+ > Co 2+ > Mn 2+ . The sulfide precipitate of Zn 2+ was the most stable and did not re-dissolve under the acidic condition (pH 4.00 ± 0.05). In addition, the sulfide precipitation characteristics of Zn 2+ was barely affected by the contaminant metal ions. However, in the presence of Al 3+ , the precipitation recoveries of Mn 2+ , Ni 2+ , and Co 2+ were noticeably reduced due to simultaneous hydrolysis and competitive adsorption. The precipitation recoveries of Ni 2+ and Co 2+ in solutions containing individual valuable metals also reduced when Fe 2+ was present, primarily due to competitive precipitation. However, the recovery of Mn 2+ was enhanced due to the formation of ferrous sulfide precipitate, providing abundant active adsorption sites for Mn species. Here, in the solution containing all the valuable metals, Fe 2+ promoted the recovery of the valuable metals due to the higher concentration of Na 2 S and the formation of ferrous sulfide precipitate.

58 GEOSCIENCES↗

NASA NTRS2011

The Precipitation Characteristics of ISCCP Tropical Weather States

We examine the daytime precipitation characteristics of the International Satellite Cloud Climatology Project (ISCCP) weather states in the extended tropics (35 deg S to 35 deg N) for a 10-year period. Our main precipitation data set is the TRMM Multisatellite Precipitation Analysis 3B42 data set, but Global Precipitation Climatology Project daily data are also used for comparison. We find that the most convective weather state (WS1), despite an occurrence frequency below 10%, is the most dominant state with regard to surface precipitation, producing both the largest mean precipitation rates when present and the largest percent contribution to the total precipitation of the tropical zone of our study; yet, even this weather state appears to not precipitate about half the time. WS1 exhibits a modest annual cycle of domain-average precipitation rate, but notable seasonal shifts in its geographic distribution. The precipitation rates of the other weather states tend to be stronger when occurring before or after WS1. The relative contribution of the various weather states to total precipitation is different between ocean and land, with WS1 producing more intense precipitation on average over ocean than land. The results of this study, in addition to advancing our understanding of the current state of tropical precipitation, can serve as a higher order diagnostic test on whether it is distributed realistically among different weather states in atmospheric models.

Lee, Dongmin↗

NASA NTRS2011

Precipitation Characteristics of ISCCP Cloud Regimes for Improving Model Hydrological Budgets

The key in unraveling relationships between precipitation and atmospheric circulations is their common linkage to clouds. Clouds can be described in a variety of ways and several approaches can be adopted to examine their connections to precipitation. We claim that when cloud regimes (aka weather states) from the International Satellite Cloud Climatology Project (ISCCP) are used to conditionally sample/sort and average precipitation data, useful insight and GCM-appropriate diagnostics on the origins and distribution of precipitation can be obtained. The ISCCP cloud regimes are mesoscale (2.5 ) cloud mixtures determined by cluster analysis on joint histograms of cloud optical thickness and cloud top pressure inferred from geostationary and polar orbiter satellite passive retrievals. The ISCCP cloud regime data are combined with GPCP IDD merged surface precipitation data and/or higher temporal and spatial resolution TRMM Multi-Satellite Precipitation Analysis (TMPA) data. The analysis is performed separately for three geographical zones, tropics, and northern/southern midlatitudes (for GPCP; only the tropics can be examined with TMPA data). Our presentation aspires to provide answers to the following questions: (l) What is the mean and variability of surface precipitation produced by each cloud regime at the time of regime occurrence? (2) What is the relative contribution of each cloud regime to the total precipitation within its geographical zone? (3) What is the geographical distribution of precipitation corresponding to particular cloud regime? (4) To what extent are the cloud regimes distinct in terms of their precipitation characteristics and is the regime ordering in terms of convective strength consistent with the observed precipitation intensity?

Lee, D.↗

NASA NTRS1994

A satellite observational and numerical study of precipitation characteristics in western North Atlantic tropical cyclones

Special Sensor Microwave/Imager (SSM/I) observations were used to examine the spatial and temporal changes of the precipitation characteristics of tropical cyclones. SSM/I observations were also combined with the results of a tropical cyclone numerical model to examine the role of inner-core diabatic heating in subsequent intensity changes of tropical cyclones. Included in the SSM/I observations were rainfall characteristics of 18 named western North Atlantic tropical cyclones between 1987 and 1989. The SSM/I rain-rate algorithm that employed the 85-GHz channel provided an analysis of the rain-rate distribution in greater detail. However, the SSM/I algorithm underestimated the rain rates when compared to in situ techniques but appeared to be comparable to the rain rates obtained from other satellite-borne passive microwave radiometers. The analysis of SSM/I observations found that more intense systems had higher rain rates, more latent heat release, and a greater contribution from heavier rain to the total tropical cyclone rainfall. In addition, regions with the heaviest rain rates were found near the center of the most intense tropical cyclones. Observational analysis from SSM/I also revealed that the greatest rain rates in the inner-core regions were found in the right half of fast-moving cyclones, while the heaviest rain rates in slow-moving tropical cyclones were found in the forward half. The combination of SSM/I observations and an interpretation of numerical model simulations revealed that the correlation between changes in the inner core diabetic heating and the subsequent intensity became greater as the tropical cyclones became more intense.

Rodgers, Edward B.↗

NASA NTRS2013

A Canonical Repsonse of Precipitation Characteristics to Global Warming from CMIP5 Models

In this study, we find from analyses of projections of 14 CMIP5 models a robust, canonical global response in rainfall characteristics to a warming climate. Under a scenario of 1% increase per year of CO2 emission, the model ensemble projects globally more heavy precipitation (+7+/-2.4%/K1), less moderate precipitation (-2.5+/-0.6%/K), more light precipitation (+1.8+/-1.3%/K1), and increased length of dry (no-rain) periods (+4.7+/-2.1%/K). Regionally, a majority of the models project a consistent response with more heavy precipitation over climatologically wet regions of the deep tropics, especially the equatorial Pacific Ocean and the Asian monsoon regions, and more dry periods over the land areas of the subtropics and the tropical marginal convective zones. Our results suggest that increased CO2 emissions induce a global adjustment in circulation and moisture availability manifested in basic changes in global precipitation characteristics, including increasing risks of severe floods and droughts in preferred geographic locations worldwide.

CMIP5↗

DOE OSTI2021

Precipitation Characteristics and Future Changes Over the Southern Slope of Tibetan Plateau Simulated by a High-Resolution Global Nonhydrostatic Model

Current climate model resolution cannot accurately describe the complex topography over the Tibetan Plateau, which limits our understanding of past and future precipitation over this region. This study investigates the daily precipitation characteristics and its future changes over the Tibetan Plateau, especially for the southern slope of Tibetan Plateau (SSTP), by 14-km Nonhydrostatic ICosahedral Atmospheric Model (NICAM) with explicitly calculated convection for historical and future 30-years period. By comparing with the satellite Global Precipitation Measurement (GPM), NICAM well reproduces the historical precipitation spatial pattern, seasonal cycle, and the extreme precipitation belt over SSTP, but overestimates precipitation amount by~35%. It is found that heavy precipitation probability decreases as elevation becomes higher while the light precipitation generally shows the opposite. For the precipitation changes during June to September from 1979–2008 to 2075–2104, NICAM predicts that mean precipitation will decrease over low-level SSTP but increase over high-level SSTP. Nonprecipitation and heavy precipitation probability will increase while light precipitation probability will decrease in the future over SSTP. The extreme precipitation probability and intensity will increase ~50%/°C and ~8%/°C over SSTP, and this increase is more obvious as elevation becomes higher. The robust increase of extreme precipitation along the SSTP topography is unique and has not been identified by the climate model simulations before. The strong meridional gradient of specific humidity over SSTP is found to be further enhanced under global warming, and this gradient enhancement is suggested to be responsible for the increase in the extreme precipitation over SSTP.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2020

Can the GPM IMERG Final Product Accurately Represent MCSs’ Precipitation Characteristics over the Central and Eastern United States?

Mesoscale convective systems (MCSs) play an important role in water and energy cycles as they produce heavy rainfall and modify the radiative profile in the tropics and midlatitudes. An accurate representation of MCSs’ rainfall is therefore crucial in understanding their impact on the climate system. The V06B Integrated Multisatellite Retrievals from Global Precipitation Measurement (IMERG) half-hourly precipitation final product is a useful tool to study the precipitation characteristics of MCSs because of its global coverage and fine spatiotemporal resolutions. However, errors and uncertainties in IMERG should be quantified before applying it to hydrology and climate applications. This study evaluates IMERG performance on capturing and detecting MCSs’ precipitation in the central and eastern United States during a 3-yr study period against the radar-based Stage IV product. The tracked MCSs are divided into four seasons and are analyzed separately for both datasets. IMERG shows a wet bias in total precipitation but a dry bias in hourly mean precipitation during all seasons due to the false classification of nonprecipitating pixels as precipitating. These false alarm events are possibly caused by evaporation under the cloud base or the misrepresentation of MCS cold anvil regions as precipitating clouds by the algorithm. IMERG agrees reasonably well with Stage IV in terms of the seasonal spatial distribution and diurnal cycle of MCSs precipitation. A relative humidity (RH)-based correction has been applied to the IMERG precipitation product, which helps reduce the number of false alarm pixels and improves the overall performance of IMERG with respect to Stage IV.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS2017

Changing Circulation Structure and Precipitation Characteristics in Asian Monsoon Regions: Greenhouse Warming vs. Aerosol Effects

Using model outputs from CMIP5 historical integrations, we have investigated the relative roles of anthropogenic emissions of greenhouse gases (GHG) and aerosols in changing the characteristics of the large-scale circulation and rainfall in Asian summer monsoon (ASM) regions. Under GHG warming, a strong positive trend in low-level moist static energy (MSE) is found over ASM regions, associated with increasing large-scale land-sea thermal contrast from 1870's to present. During the same period, a mid tropospheric convective barrier (MCB) due to widespread reduction in relative humidity in the mid- and lower troposphere is strengthening over the ASM regions, in conjunction with expanding areas of anomalous subsidence associated with the Deep Tropical Squeeze (DTS) [Lau and Kim, 2015]. The opposing effects of MSE and MCB lead to enhanced total ASM rainfall, but only a partial strengthening of the southern portion of the monsoon meridional circulation, coupled to anomalous multi-cellar overturning motions over ASM land. Including anthropogenic aerosol emissions strongly masks MSE but enhances MCB via increased stability in the lower troposphere, resulting in an overall weakened ASM circulation with suppressed rainfall. Rainfall characteristics analyses indicate that under GHG, overall precipitation efficiency over the ASM region is reduced, manifesting in less moderate but more extreme heavy rain events. Under combined effects of GHG and aerosols, precipitation efficiency is unchanged, with more moderate, but less extreme rainfall.

Asian monsoon↗

NASA NTRS2017

Precipitation Characteristics in Tropical Africa Using Satellite and In-Situ Observations

Tropical Africa receives nearly all its precipitation as a result of convection. The characteristics of rain-producing systems in this region, despite their crucial role in regional and global circulation, have not been well-understood. This is mainly due to the lack of in situ observations. Here, we have used precipitation records from the Trans-African Hydro-Meteorological Observatory (TAHMO) to improve our knowledge about the rainfall systems in the region, and to validate the recently-released IMERG precipitation product. The high temporal resolution of the gauge data has allowed us to identify three classes of rain events based on their duration and intensity. The contribution of each class to the total rainfall and the favorable surface atmospheric conditions for each class have been examined. As IMERG aims to continue the legacy of its predecessor, TMPA, and provide higher resolution data, continent-wide comparisons are made between these two products. IMERG, due to its improved temporal resolution, shows some advantages over TMPA in capturing the diurnal cycle and propagation of the meso-scale convective systems. However, the performance of the two satellite-based products varies by season, region and the evaluation statistics. The results of this study serve as a basis for our ongoing work on the impacts of biomass burning on precipitation processes in Africa.

TMPA↗

NASA NTRS2017

Precipitation Characteristics in West and East Africa from Satellite and in Situ Observations

Using in situ data, three precipitation classes are identified for rainy seasons of West and East Africa: weak convective rainfall (WCR), strong convective rainfall (SCR), and mesoscale convective systems (MCSs).Nearly 75% of the total seasonal precipitation is produced by the SCR and MCSs, even though they represent only 8% of the rain events. Rain events in East Africa tend to have a longer duration and lower intensity than in West Africa, reflecting different characteristics of the SCR and MCS events in these two regions. Surface heating seems to be the primary convection trigger for the SCR, particularly in East Africa, whereas the WCR requires a dynamical trigger such as low-level convergence. The data are used to evaluate the performance of the recently launched Integrated Multi-satellite Retrievals for Global Precipitation Measurement (IMERG)project. The IMERG-based precipitation shows significant improvement over its predecessor, the Tropical Rainfall Measuring Mission (TRMM) Multi-satellite Precipitation Analysis (TMPA), particularly in capturing the MCSs, due to its improved temporal resolution.

West and East Africa↗

NASA NTRS1993

Comment on 'Mapping the dayside ionosphere to the magnetosphere according to particle precipitation characteristics' by Newell and Meng

Newell and Meng (1992) present maps of the occurrence probability of various classifications of particle precipitation as seen in the dayside topside ionosphere. It is argued that these are maps of the magnetospheric regions, a contention with which their critics disagree. The latter conclude that, because of convection, any one population of particles seen at low altitudes will have originated from a wide variety of locations, and particle characteristics cannot be mapped back to those in the magnetosphere without detailed knowledge of both the convection and magnetic field. Steplike boundaries between the regions will arise from nonsteady-state conditions and cannot be envisaged as steady-state magnetospheric boundaries between two plasma populations. In their reply Newell and Meng contend that convection does not move plasma from the LLBL into the cusp. Most of the LLBL plasma comes from the magnetosheath, so the direction of plasma transfer is in the other direction.

Lockwood, M.↗

DOE OSTI2022

Southern Ocean Precipitation Characteristics Observed From CloudSat and Ground Instrumentation During the Macquarie Island Cloud & Radiation Experiment (MICRE): April 2016 to March 2017

A 1-year blended surface precipitation data set using Parsivel disdrometer, surface W-band radar, and tipping bucket measurements is produced for the Macquarie Island Cloud and Radiation Experiment (MICRE) and compared with retrievals from CloudSat (spaceborne 94 GHz radar). Surface precipitation was observed 44% ± 4% of the time between April 2016 and March 2017. Precipitation composed primarily of small particles (diameter <1 mm) occurred about 36% ± 2% of the time, constituting 10% of total accumulation. Remaining precipitation contained enough large particles such that the disdrometer could be used to identify the precipitation type as rain, ice, snow or wet snow. Seasonal and annual statistics on frequency of occurrence and accumulation for each precipitation type observed during MICRE are presented. Most ice and mixed phase precipitation was shallow, originating at a height of 3 km or lower, and occurred most often when Macquarie Island was to the northwest of the nearest cyclonic low-pressure center. In contrast, rain was more often deep and occurred most frequently when the island was to the southeast of cyclonic lows. A weak diurnal cycle in frequency and mean rate was present with a minimum between 12:00 and 14:00 local time and maximum between 03:00 and 06:00 local time. The CloudSat 2C-Precip-Column product missed the lightest precipitation (because the near-surface reflectivity is <-15 dBZ) and overestimated total liquid precipitation and occurrence of mixed phase precipitation, but captured reasonably well the distribution of rain rates for rates >0.5 mm/hr.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2021

Precipitation Characteristics of Warm Season Weather Types in the Southeastern United States of America

Daily weather types (WTs) over the Southeast United States have been analyzed using 850 hPa winds from reanalysis data from March to October of 1979–2019. Six WTs were obtained. WTs 1–3 represent mid-latitude synoptic systems propagating eastward. WT4 is a summer-type pattern predominantly occurring in June–August, with the center of the North Atlantic Subtropical High (NASH) along the Gulf coast in the southern United States. WT5 is most frequent from August to middle October, with the NASH pushed further north and southerly winds over the northern Great Plains. An anticyclone centered at the Carolina coast characterizes WT6, which occurs in all months but is slightly more frequent in the spring and fall, especially in October, corresponding to fair weather in the region. WTs 1, 2 and 3 can persist for only a few days. WTs 4, 5 and 6 can have long spells of persistence. Besides self-persistence, the most observed progression loop is WT1 to WT2, to WT3, and then back to WT1, corresponding to eastward-propagating waves. WTs 4 and 5 are likely to show persistence, with long periods of consecutive days. WT6 usually persists but can also transfer to WT3, i.e., a change from fair weather in the Southeast U.S. to rainy weather in the Mississippi River Valley. A diurnal cycle of precipitation is apparent for each WT, especially over coastal plains. The nocturnal precipitation in central U.S. is associated with WT3. WTs 1–3 are more frequent in El Niño years, corresponding to stronger westerly wave activities and above normal rainfall in the Southeast U.S. in the spring. The positive rainfall anomaly in the Mississippi and Ohio River valley in El Niño years is also associated with more frequent WT3.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS2019