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At least 19 records

Southeast Regional CO 2 Utilization and Storage Acceleration Partnership (SECARB-USA): Regional Commercialization Plan (Final): Work Products 4.4.b (Regional Commercialization Plan) & 4.3 (Socioeconomic Impacts of CCUS and Workforce Readiness)

Commercialization of carbon capture and storage (CCS) within the SECARB-USA region is scaling up and will continue as governments and private companies expand on current decarbonization efforts. The Inflation Reduction Act (2022) enhanced 45Q tax credits beyond the 2018 Bipartisan Budget Act levels by incentivizing previously uneconomic projects to develop CCS plans and infrastructure. Additionally, the continued interest and support for CCS mitigates the relative risk of commercial-scale projects that are seeking long-term viability to develop capture facilities to accommodate their emissions reduction goals. This multifaceted Commercialization Plan provides an overview of the current status and potential for CCS in the Southeast and the pathways to achieve emissions reduction goals in the region by 2050. Specifically, the study addresses: • The current status of CCS activities in the SECARB region, • Assessment of buildout pathways for CCS projects and carbon transport infrastructure development opportunities, • Estimation of CCS job creation and economic impacts, and • The social justice considerations and public benefits associated with CCS activities in the SECARB-USA region.

42 ENGINEERING↗

The ongoing need for high-resolution regional climate models: Process understanding and stakeholder information

Regional climate modeling addresses our need to understand and simulate climatic processes and phenomena unresolved in global models. High resolution models are generally more skillful in simulating extremes, such as heavy precipitation, strong winds, and severe storms. In addition, research has shown that fine-scale features such as mountains, coastlines, lakes, irrigation, land use, and urban heat islands can substantially influence a region’s climate and its response to changing forcings. Regional climate simulations explicitly simulating convection are now being performed, providing an opportunity to illuminate new physical behavior that previously was represented by parameterizations with large uncertainties. Regional and global models are both advancing toward higher resolution, as computational capacity increases. However, the resolution and ensemble size necessary to produce a sufficient statistical sample of these processes in global models has proven too costly for contemporary supercomputing systems. Regional climate models are thus indispensable tools that complement global models for understanding regional climate variability and change, and are critical for supporting societal responses to changing climate.

Gutowski, William↗

Interannual consistency of migration phenology is season- and breeding region-specific in North American Golden Eagles

Abstract Interannual consistency (an indicator of the strength of adjustments) in migration phenology of Golden Eagles (Aquila chrysaetos) in North America is most strongly associated with the breeding region, the season, and with late-season temperature on breeding and wintering grounds. Consistency was greatest in boreal spring migration and the breeding regions of eastern Canada. Using multi-year GPS tracks of 83 adults breeding in 3 spatially distant regions (Alaska, northeast Canada, and southeast Canada), we quantified the interannual consistency of migration phenology and wintering latitude within and among individuals tracked across multiple years and the repeatability (r) by breeding regions and seasons. By comparing regions and seasons, we found that consistency was highest (r > 0.85) for boreal spring migration in eastern Canada while Alaska had the lowest value (r < 0.15). Because seasonal consistency of migration phenology was only detected in eastern Canada, we conclude that seasonal features are not a primary constraint. While regional differences in consistency were not related to differences in migratory distances, they could be the result of genetic or habitat differences. We also found that temperatures warmer than the decadal average at the region of departure delayed the start of boreal spring migration by ~10 days and advanced boreal autumn migration by ~20 days. These results suggest that warmer temperatures would reduce residence time on breeding grounds, contrary to expectations and trends found in other studies. Wide variations in migratory strategies across a species distribution can add to the list of challenges for conservation but may give migrants the capacity to acclimate to environmental changes.

Zoology↗

Regional Geology Capstone Report for the Midwestern Regional Carbon Sequestration Partnership (Volume V)

The Midwest Regional Carbon Sequestration Partnership (MRCSP) was founded in 2003 as part of the U.S. Department of Energy’s (DOE’s) Regional Carbon Sequestration Partnership initiative. Since its founding, MRCSP has made significant strides toward making CCUS a viable option for states in the region. The public/private consortium, funded through the DOE Regional Carbon Sequestration Initiative, brings together nearly 40 industry partners and 10 states. Battelle, as the project lead, oversees research, development and operations and coordinates activities among the partners. The incremental, phased approach has built a valuable knowledge base for the industry and paved the way for commercial-scale adoption of CCUS technologies. From 2008 to 2020, MRCSP Phase III focused on the development of large-scale injection projects. This report is part of a series of reports prepared under the Midwestern Regional Carbon Sequestration Partnership (MRCSP) Phase III (Development Phase). These reports summarize and detail the findings of the work conducted under the Phase III project. The MRCSP regional geology Capstone report summarizes the regional characterization of geologic storage subtasks performed under MRCSP Phase III. The regional characterization work was completed by the state geological surveys of Delaware, Indiana, Kentucky, Maryland, New York, Ohio, Pennsylvania, and West Virginia along with Western Michigan University and Rutgers University. Building on the Phases I and II, the Phase III research was focused on key research topics identified in previous MRCSP efforts: [1] Regional Geologic Cross Sections for Potential Storage and Containment Zones; [2] Appalachian Basin: Enhanced Recovery Opportunities; [3] Michigan Basin: Assessment of Enhanced Oil Recovery Using Carbon Dioxide in Silurian Pinnacle Reefs; [4] Mid-Atlantic Coastal Plain and Adjacent Offshore Region: Characterization of Carbon Storage Targets; [5] Ordovician-Cambrian Units: Hierarchical Evaluation of Geologic Carbon Storage Resource Estimates; [6] Upper Silurian to Middle Devonian Strata of Ohio: Structural Characterization of Potential CO 2 Reservoirs and Adjacent Strata; [7] Triassic Rift Basins: Preliminary Study of Long-Term CO 2 Storage Potential Together, the regional characterization effort developed useful products to support project developers, policy makers and other stakeholders in the MRCSP region seeking to understand where potential storage exists relative to large stationary sources of CO 2 emissions.

01 COAL, LIGNITE, AND PEAT↗

Multiple Critical Unresolved Region Integral Experiment (MCURIE): A Proposed Integral Critical Experimental Framework for Unresolved Region and Intermediate Energies

The Critical Unresolved Region Integral Experiment (CURIE) critical experiment was performed at the National Criticality Experiments Research Center (NCERC) at the Device Assembly Facility (DAF) at the Nevada Nuclear Security Sites (NNSS) in 2020. The objective of CURIE was to improve the quality of integral nuclear data in the uranium-235 ( 235 U) unresolved resonance region (URR) by performing benchmark integral experiments that were sensitive to the URR energy ranges. The CURIE experiment was evaluated for the International Criticality Safety Benchmark Evaluation Project (ICSBEP) handbook and the benchmark evaluation was accepted in 2022. The URR is a region within the intermediate neutron energy range (the intermediate energy ranges from 0.7 eV to 100 keV). The observed resonance structure in neutron cross sections is due to discrete energy levels in the nucleus and are characterized by resonance parameters. In the URR region, the resonance parameters are only partially resolved as the resolution of the experiment techniques becomes comparable to the average width of the resonances themselves, and the resonances are so close to one another that the structure cannot be determined empirically. The ENDF/B-VIII.0 and JEFF-3.3 nuclear data libraries define the URR as beginning at 2.25 keV and continuing until 25 keV. There are minimal intermediate neutron energy benchmarks available in the ICSBEP benchmark handbook, and aside from CURIE there are none that are highly sensitive in the URR energy region. There is a current need for additional experiments sensitive to the URR energy region. There is a new proposed subgroup for the Organization for Economic Co-operation and Development and Nuclear Energy Agency (OECD NEA) Working Party on International Nuclear Data Evaluation Cooperation (WPEC), so any new models or information will need experimental validation and testing. The NEA Working Party on Nuclear Criticality Safety (WPNCS) recent experimental needs and priority list includes intermediate energy 235 U and 238 U experiments, as does the recent Integral Experiments to Address Nuclear Criticality Safety Needs Meeting (May 2023). A variant on the original CURIE experiment called the Multiple Critical Unresolved Region Integral Experiment (MCURIE) is proposed to provide further investigation of the intermediate and URR energy region for uranium. MCURIE will utilize existing fuels at NCERC but use alternative moderators and reflectors to modify the neutron absorption, scattering, and fission spectra of the experiments, allowing for precise targeting of nuclear data sensitivities. The overall goal of MCURIE is to develop a framework for designing and performing integral benchmark experiments with high sensitivities in the intermediate and URR energy regions for nuclear data validation.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Multi-decade high-resolution regional hindcasts for wave energy resource characterization in U.S. coastal waters

Long-term, high-resolution, regional wave hindcast datasets were generated using unstructured-grid Simulating WAves Nearshore (SWAN) models for the U.S. coastal waters to support nearshore wave energy development in the U.S. including those bordering U.S. territorial islands. The model domains resolved the entire U.S. exclusive economic zones, with a spatial resolution of approximately 200 m nearshore. The regional SWAN models were driven by the global WAVEWATCH III® model outputs and run for a 42-year period from 1979 to 2020. Extensive model validations were performed using buoy observations and altimeter data. Regional resource characterization was performed based on hindcast data points at 2 km from shore and along the 100 m isobath. Aggregations of wave resource parameters were produced, and spatial and seasonal variations were analyzed for all the regions. Wave resource metrics recommended by international standards, including a 3-hour time series of six resource parameters, hourly frequency- and directionally resolved wave spectra at selected “virtual buoy” locations, and average-annual values of omni-directional wave power, significant wave height, and energy period are publicly disseminated through an Amazon Web Service and a Marine Energy Atlas web application tool to facilitate wave energy research and a wide range of coastal ocean applications.

16 TIDAL AND WAVE POWER↗

140,142 Ce Neutron Cross Section Resolved Resonance Region Evaluation

A resolved resonance region evaluation of 140,142 Ce was conducted by Oak Ridge National Laboratory. Requested by the US Nuclear Criticality Safety Program, this evaluation is based on recent high-resolution transmission and capture high-resolution measurements of nat Ce and 142 Ce conducted at JRC-Geel at the Geel Linear Accelerator facility. It is also based on recently measured thermal constants available from the EX FOR database. Starting from the resonance parameters from the ENDF/B-VIII.0 library and following a preliminary R-matrix analysis, an updated set of resonance parameters and corresponding covariance in formation was derived by the fit of these experimental datasets using the Reich–Moore approximation of the R-matrix theory, as implemented in the SAMMY code system. The resolved resonance region upper energy limit for 140 Ce was kept at 200 keV, whereas the 142 Ce resonance region was extended from 13 to 26 keV. This new evaluation was found to be in good agreement not only with several integral quantities of interest to the reactor physics community, but also with the stellar Maxwellian-averaged cross section.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Multi‐Scale Seismic Imaging of the Ridgecrest, CA, Region With Waveform Inversion of Regional and Dense Array Data

Abstract We develop an inversion procedure for deriving multi‐scale velocity models with waveform inversions of earthquake and ambient noise data at multi‐frequency bands recorded by regional and dense sensor configurations. The method is applied for the area around the 2019 Ridgecrest earthquake rupture zones, utilizing data recorded by regional stations and dense 2D and 1D arrays with station spacings of ∼5 km and ∼100 m, respectively. Starting with regional Vp, Vs models and locations of Ridgecrest aftershocks, the velocity models and event locations are improved iteratively by inversions of waveforms recorded by regional stations and the 2D array, using a minimum spectral element size of ∼600 m. Waveforms from local events recorded by dense 1D arrays across the M7.1 rupture zone with frequencies of up to 10 Hz are used to resolve small‐scale features of the rupture zone and shallow crust with a local spectral element size of 80 m. The refined models provide self‐consistent descriptions of the rupture zone and the shallow crust embedded in the regional structures. The results reveal pronounced low Vs and high Vp/Vs in the M6.4 and M7.1 rupture zones coinciding with concentrations of seismicity, and also around the Garlock fault and in several local basins. We also observe clear velocity contrasts across the Garlock fault with polarity reversals along strike and with depth. The obtained multi‐scale velocity models can be used to improve derivations of earthquake source properties, simulations of dynamic ruptures and ground motions, and the understanding of fault and tectonic processes in the region.

Geochemistry & Geophysics↗

Examining Tropical Convection Features at Storm-Resolving Scales Over the Maritime Continent Region

Global Storm Resolving Models (GSRMs) provide a way to understand weather and climate events across scales for better-informed climate impacts. In this work, we apply the recently developed and validated CAM (Community Atmosphere Model)—MPAS (Model for Prediction Across Scales) modeling framework, based on the open-source Community Earth System Model (CESM2), to examine the tropical convection features at the storm resolving scale over the Maritime Continent region at 3 km horizontal spacing. We target two global numerical experiments during the winter season of 2018 for comparison with observation in the region. Here we focus on the investigation of the representations of the convective systems, precipitation statistics, and tropical cyclone behaviors. We found that regional-refined experiments show more accurate precipitation distributions, diurnal cycles, and better agreement with observations for tropical cyclone features in terms of intensity and strength statistics. We expect the exploration of this work will further advance the development and use of the storm-resolving model in precipitation predictions across scales.

54 ENVIRONMENTAL SCIENCES↗

Impacts of Climate Change on Energy Systems in Global and Regional Scenarios

A growing number of studies report the impact of climate change on the supply, demand, transport, and cost of energy. However, there is lack of comprehensive overview and understanding of climate change impacts on energy across technologies and scales. Here, we conduct a systematic assessment of results from 186 papers on potential impacts of climate change on energy. Results show that increased cooling demand and decreased heating demand is anticipated globally. Similarly, increases in bio-energy and hydro power and a possible decrease in thermal electricity supply is projected. Overall changes in heating and cooling demand, increased thermal cooling, and reduced hydropower supply in Europe, India and Latin America are projected 35 at the regional scale. Furthermore, our review revealed that studies use a wide range of inconsistent methods and data sources. To move forward, the study proposes a consistent multi-model assessment framework for a comprehensive understanding of climate impacts on energy.

Yalew, Seleshi G.↗

Potassium-Containing α-MnO 2 Nanotubes: The Impact of Hollow Regions on Electrochemistry

α-MnO 2 type materials have been studied as electrode materials in rechargeable batteries and electrocatalysts due to their 2 × 2 tunneled crystal structures capable of accommodating cations and their tunable physiochemical properties. In this study, we deliberately synthesized K + containing α-MnO 2 (K 0.9 Mn 8 O 16 ) hollow nanotubes varying the dimensions of the hollow regions and level of surface defects. The K 0.9 Mn 8 O 16 nanotube material samples have similar crystallinity, thermal stability, and average Mn oxidation state. Oxygen surface defects in the hollow regions were revealed through detailed studies using electron energy loss spectroscopy. The impact of the hollow regions and associated surface defects on the electrochemistry of K x Mn 8 O 16 were investigated using cyclic voltammetry, galvanostatic intermittent titration technique, and galvanostatic cycling. The K 0.9 Mn 8 O 16 nanotubes with a large hollow region (~30 nm) and higher level of surface defects show higher apparent lithium ion diffusion coefficients and lower polarization compared to the nanotubes with a small hollow region (~10 nm). In-situ lithiation demonstrated that the dimensions of the nanotube walls expanded, but the hollow region did not change in size as result of lithiation. Furthermore, this research demonstrates that tuning particle architecture and surface defects can positively impact functional behavior of electrochemical storage materials.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Regional Geologic Cross Sections for Potential Storage and Containment Zones in the MRCSP Region

The Midwest Regional Carbon Sequestration Partnership (MRCSP) has incorporated the work of geologic research teams (Geoteams) in its regional characterization, project planning and carbon dioxide (CO 2 ) injection implementation work since the partnership was established by the U.S. Department of Energy (DOE) in 2003. Over this 16-year period, the cohort of Geoteams has grown from five to ten states and has contributed to the characterization of geologic sequestration opportunities, refinement of reservoir and seal data, and supported injection efforts through both predictive and post-injection assessments. Five geologic cross sections (labeled A through E) were constructed onshore across the parts of the MRCSP Region west of the Valley and Ridge Province, and one section (labeled F) was constructed beginning onshore in New Jersey and running eastward to offshore areas examined for carbon storage. Regional and local stratigraphic units were used in these cross sections to show current nomenclature as well as highlighting specific units/features pertinent to carbon capture, utilization and storage (CCUS) opportunities in the region. Each cross section uses 15 to 25 deep wells and other geologic information to illustrate the relative depth, thickness and location of rock units in the subsurface.

01 COAL, LIGNITE, AND PEAT↗

Effects of groundwater pumping on ground surface temperature: A regional modeling study in the North China Plain

Over-exploitation of groundwater (GW) in the North China Plain (NCP) since the 1960s has many environmental consequences. However, understanding of the dominant mechanisms remains limited, particularly at regional scale. In this study, the coupled ParFlow.CLM model representing subsurface and land-surface processes and their interactions was applied in the NCP at high spatio-temporal resolutions. The model was validated using the water and energy fluxes reported in previous studies and from the JRA-55 reanalysis. Numerical experiments were designed to examine the relative impacts of GW pumping and irrigation on the ground surface temperature (GST). Results show significant effects of GW pumping on GST in the NCP. Generally, the subsurface acts as a buffer to temporal variations in heat fluxes at the land-surface, but long-term pumping can gradually weaken this buffer, resulting in increases in the spatio-temporal variability of GST, as exemplified by hotter summers and colder winters. Considering that changes of water table depth (WTD) can significantly affect land surface heat fluxes when WTD ranges roughly between 0.01–10 m, the 0.5 m/year increase of WTD simulated by the model due to pumping can continue to increase the average WTD and hence, disturb GST, for about 20 years from the pre-pumping WTD in the NCP, before the WTD exceeds 10 m. The variations of GST are expected to be faster initially and gradually slow down due to the nonlinear behaviors of GST with WTD. The findings from this study in the NCP may also have implications for other regions with GW depletion.

Yang, Chen↗

Summer mean and extreme precipitation over the Mid-Atlantic region: climatological characteristics and contributions from different precipitation types

Based on a long-term observational dataset from the tracking of mesoscale convective systems (MCSs), isolated deep convection (IDC), and tropical cyclones (TCs), we examine the climatological characteristics of summer mean and extreme precipitation during 2004 – 2017 and their respective contributions from MCS, IDC, TC, and non-convective (NC) systems and the local vs. remote influence of MCS and IDC over the MAR. On average, MCS, IDC, TC, and NC contribute 22%, 29%, 4%, and 45% to the total summer mean precipitation in the region. While MCS and TC precipitation primarily occurs in the coastal areas east of the Appalachian Mountains, IDC precipitation is more concentrated in the southern MAR and near the mountain windward slopes. Each summer, ~41 MCSs with an average lifetime of 19.6 hours influence the MAR, with 80% initiated outside and traveling on average 10 hours to the region. Around 13 MCSs initiated in the Great Plains and Midwest propagate across the Appalachian Mountains and contribute 20-40% to summer MCS precipitation in the central Mid-Atlantic coastal areas. In contrast, more than 2000 IDCs with an average lifetime of 2.0 hours influence the MAR each summer, and 77% are initiated locally. MCS, IDC, TC, and NC contribute 31% (30%), 26% (31%), 18% (7%), and 26% (32%) to the top 1% (5%) extreme daily precipitation, respectively. Considering extreme hourly precipitation, however, the IDC contributions increase to 41% (top 1%) and 38% (top 5%) due to the shorter duration of IDC events than the other precipitation types.

Li, Jianfeng↗

WRF-ELM v1.0: a regional climate model to study land–atmosphere interactions over heterogeneous land use regions

Abstract. The Energy Exascale Earth System Model (E3SM) Land Model (ELM) is a state-of-the-art land surface model that simulates the intricate interactions between the terrestrial land surface and other components of the Earth system. Originating from the Community Land Model (CLM) version 4.5, ELM has been under active development, with added new features and functionality, including plant hydraulics, radiation–topography interaction, subsurface multiphase flow, and more explicit land use and management practices. This study integrates ELM v2.1 with the Weather Research and Forecasting (WRF; WRF-ELM) model through a modified Lightweight Infrastructure for Land Atmosphere Coupling (LILAC) framework, enabling affordable high-resolution regional modeling by leveraging ELM's innovative features alongside WRF's diverse atmospheric parameterization options. This framework includes a top-level driver for variable communication between WRF and ELM and Earth System Modeling Framework (ESMF) caps for the WRF atmospheric component and ELM workflow control, encompassing initialization, execution, and finalization. Importantly, this LILAC–ESMF framework demonstrates a more modular approach compared to previous coupling efforts between WRF and land surface models. It maintains the integrity of ELM's source code structure and facilitates the transfer of future developments in ELM to WRF-ELM. To test the ability of the coupled model to capture land–atmosphere interactions over regions with a variety of land uses and land covers, we conducted high-resolution (4 km) WRF-ELM ensemble simulations over the Great Lakes region (GLR) in the summer of 2018 and systematically compared the results against observations, reanalysis data, and WRF-CTSM (WRF coupled with the Community Terrestrial Systems Model). In general, the coupled WRF-ELM model has reasonably captured the spatial distribution of surface state variables and fluxes across the GLR, particularly over the natural vegetation areas. The evaluation results provide a baseline reference for further improvements in ELM in the regional application of high-resolution weather and climate predictions. Our work serves as an example to the model development community for expanding an advanced land surface model's capability to represent fully-coupled land–atmosphere interactions at fine spatial scales. The development and release of WRF-ELM marks a significant advancement for the ELM user community, providing opportunities for fine-scale regional representation, parameter calibration in coupled mode, and examination of new schemes with atmospheric feedback.

54 ENVIRONMENTAL SCIENCES↗

Resolved resonance region evaluations of n+ 206,207,208 Pb for fast spectrum applications

Resolved resonance region evaluations of the major isotopes of natural lead, 206 Pb, 207 Pb, 208 Pb, have been per formed to support the development of Generation IV reactors. In this study, validation of nuclear data for lead fast reactors was performed with simulations of shielding benchmarks, integral critical benchmarks, and quasi-differential scattering measurements. Sensitivity analyses of these systems showed that elastic scattering reactions above 100 keV were the dominant reactions driving system performance. The resolved resonance regions (RRRs) of the lead isotopes extend past 100 keV, making the RRR an ideal starting point to evaluate lead cross sections. Since the R-matrix requires knowledge of bound, distant, and observed resonances, it was necessary to evaluate from 10 -5 eV up to the respective limit of the RRR. The 208 Pb RRR evaluation was extended to 1.5 MeV in order to obtain resonance parameters used to calculate new elastic scattering angular distributions up to 1.5 MeV. Resonance parameter uncertainties and covariance were generated using the R-matrix code SAMMY. The new RRR parameters show a direct improvement to the scattering kernel below 1.5 MeV which in turn greatly improves fast critical experiments over ENDF/B-VIII.0.

206Pb↗

Evaluation of Light-Element Reactions in the Resolved Resonance Region

Light-element reactions at low energies in the resolved resonance region are important for a range of applications in basic and applied sciences including nuclear reactors, nonproliferation, cultural heritage, forensics and environmental control, rare event investigations and nuclear astrophysics. In this paper, we report on an effort to evaluate charged-particle cross sections in the resolved resonance region and produce evaluated nuclear data files for further processing and inclusion in evaluated data libraries. We discuss the open issues in R-matrix calculations as we extend to higher energies, such as dealing with the rapidly growing number of open channels and merging with the regime of smooth cross sections described by the statistical model, and present attempts to address these issues in neutron-induced reactions relevant to nuclear reactor applications.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗