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DOE OSTI2023

Aerosol Optical Depth Best Estimate Value-Added Product Report

Four aerosol optical depth (AOD) products are offered by four collocated ground-based instruments deployed at the U.S. Department of Energy Atmospheric Radiation Measurement (ARM) user facility’s Southern Great Plains (SGP) observatory (SGP Central Facility 1 [C1] and Extended Facility 13 [E13]) for more than two decades. Two of these instruments, the multifilter rotating shadowband radiometers (MFRSRs C1 and E13), are sensors with horizontal hemispherical receivers shaded by rotating shadowbands.

47 OTHER INSTRUMENTATION↗

DOE OSTI2024

Evaluation of the hyperspectral radiometer (HSR1) at the Atmospheric Radiation Measurement (ARM) Southern Great Plains (SGP) site

Abstract. The Peak Design Ltd hyperspectral radiometer (HSR1) was tested at the Atmospheric Radiation Measurement (ARM) user facility Southern Great Plains (SGP) site in Lamont, Oklahoma, for 2 months from May to July 2022. The HSR1 is a prototype instrument that measures total (Ftotal) and diffuse (Fdiffuse) spectral irradiance from 360 to 1100 nm with a spectral resolution of 3 nm. The HSR1 spectral irradiance measurements are compared to nearby collocated spectral radiometers, including two multifilter rotating shadowband radiometers (MFRSRs) and the Shortwave Array Spectroradiometer–Hemispheric (SASHe) radiometer. The Ftotal at 500 nm for the HSR1 compared to the MFRSRs has a mean (relative) difference of 0.01 W m−2 nm−1 (1 %–2 %). The HSR1 mean Fdiffuse at 500 nm is smaller than the MFRSRs' by 0.03–0.04 (10 %) W m−2 nm−1. The HSR1 clear-sky aerosol optical depth (AOD) is also retrieved by considering Langley regressions and compared to collocated instruments such as the Cimel sunphotometer (CSPHOT), MFRSRs, and SASHe. The mean HSR1 AOD at 500 nm is larger than the CSPHOT's by 0.010 (8 %) and larger than the MFRSRs' by 0.007–0.017 (6 %–18 %). In general, good agreement between the HSR1 and other instruments is found in terms of the Ftotal, Fdiffuse, and AODs at 500 nm. The HSR1 quantities are also compared at other wavelengths to the collocated instruments. The comparisons are within ∼ 10 % for the Ftotal and Fdiffuse, except for 940 nm, where there is relatively larger disagreement. The AOD comparisons are within ∼ 10 % at 415 and 440 nm; however, a relatively larger disagreement in the AOD comparison is found for higher wavelengths.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS2003

The "RED Versa NIR" Plane to Retrieve Broken-Cloud Optical Depth from Ground-Based Measurements"

A new method for retrieving cloud optical depth from ground-based measurements of zenith radiance in the RED and near infrared (MR) spectral regions is introduced. Because zenith radiance does not have a one-to-one relationship with optical depth, it is absolutely impossible to use a monochromatic retrieval. On the other side, algebraic combinations of spectral radiances such as NDCI while largely removing nouniquiness and the radiative effects of cloud inhomogeneity, can result in poor retrievals due to its insensitivity to cloud fraction. Instead, both RED and NIR radiances as points on the 'RED vs. NIR' plane are proposed to be used for retrieval. The proposed retrieval method is applied to Cimel measurements at the Atmospheric Radiation Measurements (ARM) site in Oklahoma. Cimel, a multi-channel sunphotometer, is a part of AERONET - a ground-based network for monitoring aerosol optical properties. The results of retrieval are compared with the ones from Microwave Radiometer (MWR) and Multi-Filter Rotating Shadowband Radiometers (MFRSR) located next to Cimel at the ARM site. In addition, the performance of the retrieval method is assessed using a fractal model of cloud inhomogeneity and broken cloudiness. The preliminary results look very promising both theoretically and from measurements.

Marshak, A.↗

NASA NTRS2004

How Can AERONET Help with Monitoring Clouds?

When conditions are inappropriate to make AErosol RObotic NETwork (AERONET) measurements for aerosol studies, new measurements related to cloud physics can be made instead. As such, several AERONET CIMEL sunphotometers have been equipped with a new "cloud mode." This mode allows the CIMELs to make measurements of zenith radiance when the Sun in blocked by clouds. When in cloud mode, a CIMEL points straight up every 10-15 minutes and takes 10 measurements over a 9 second time interval at four wavelengths: 440,670,870, and 1020 nm. For cloudy conditions above green vegetation, the spectral contrast in surface albedo dominates over Rayleigh and aerosol effects. We have developed a new method for retrieving cloud optical depth, even for broken clouds, that uses data from the 670 (and/or 440) and 870 nm channels. In addition to cloud optical depth, the method also infers a "radiatively effective" cloud fraction. The results of the retrievals at the ARM Central Facility in Oklahoma are compared with the ones from Microwave Radiometer (MWR) and Multi-Filter Rotating Shadowband Radiometers (MFRSR).

Marshak, A.↗

NASA NTRS2000

Total Optical Depth Analysis for NO2, O3 and Aerosols by a Multi-Filter Shadowband Radiometer

The main focus of this research is the retrieval of tropospheric aerosol information using a Multi-filter Rotating Shadowband Radiometer, Model MFR-7, placed on the roof of the Science Building at Medgar Evers College. This instrument makes precise measurements of atmospheric extinction of the direct solar beam simultaneously at six wavelengths (475, 500, 615, 670, 840 and 940 nm) at one minute intervals throughout the day. We are interested in measuring the changes in the optical depth of ambient aerosols, mass, effective particle size, aerosol size distribution, and chemical composition of ambient particulate matter in the Greater New York City Area. Results will be compared with data obtained by A. Lacis, B. Carlson and B. Cairns at the NASA Goddard Institute for Space Studies.

Williamson, Lorenzo↗

NASA NTRS2018

Comparisons of Spectral Aerosol Single Scattering Albedo in Seoul, South Korea

Quantifying aerosol absorption at ultraviolet (UV) wavelengths is important for monitoring air pollution and aerosol amounts using current (e.g., Aura/OMI (Ozone Monitoring Instrument)) and future (e.g., TROPOMI (TROPOspheric Monitoring Instrument), TEMPO (Tropospheric Emissions: Monitoring of POllution), GEMS (Geostationary Environment Monitoring Spectrometer) and Sentinel-4) satellite measurements. Measurements of column average atmospheric aerosol single scattering albedo (SSA) are performed on the ground by the NASA AERONET (AEROsol robotic NETwork) in the visible (VIS) and near-infrared (NIR) wavelengths and in the UV-VIS-NIR by the SKYNET (SKY radiometer NETwork) networks. Previous comparison studies have focused on VIS and NIR wavelengths due to the lack of co-incident measurements of aerosol and gaseous absorption properties in the UV. This study compares the SKYNET-retrieved SSA in the UV with the SSA derived from a combination of AERONET, MFRSR (MultiFilter Rotating Shadowband Radiometer), and Pandora (AMP) retrievals in Seoul, South Korea, in spring and summer 2016. The results show that the spectrally invariant surface albedo assumed in the SKYNET SSA retrievals leads to underestimated SSA compared to AMP values at near UV wavelengths. Re-processed SKYNET inversions using spectrally varying surface albedo, consistent with the AERONET retrieval improve agreement with AMP SSA. The combined AMP inversions allow for separating aerosol and gaseous (NO2 and O3) absorption and provide aerosol retrievals from the shortest UVB (305 nanometers) through VIS to NIR wavelengths (870 nanometers).

aerosol and gaseous absorption properties↗

NASA NTRS1998

Aerosol analysis techniques and results from micro pulse lidar

The effect of clouds and aerosol on the atmospheric energy balance is a key global change problem. Full knowledge of aerosol distributions is difficult to obtain by passive sensing alone. Aerosol and cloud retrievals in several important areas can be significantly improved with active remote sensing by lidar. Micro Pulse Lidar (MPL) is an aerosol and cloud profilometer that provides a detailed picture of the vertical structure of boundary layer and elevated dust or smoke plume aerosols. MPL is a compact, fully eyesafe, ground-based, zenith pointing instrument capable of full-time, long-term unattended operation at 523 nm. In October of 1993, MPL began taking full-time measurements for the Atmospheric Radiation Measurement (ARM) program at its Southern Great Plains (SGP) site and has since expanded to ARM sites in the Tropical West Pacific (TWP) and the North Slope of Alaska (NSA). Other MPL's are moving out to some of the 60 world-wide Aerosol Robotic Network (AERONET) sites which are already equipped with automatic sun-sky scanning spectral radiometers providing total column optical depth measurements. Twelve additional MPL's have been purchased by NASA to add to the aerosol and cloud database of the EOS ground validation network. The original MPL vertical resolution was 300 meters but the newer versions have a vertical resolution of 30 meters. These expanding data sets offer a significant new resource for atmospheric radiation analysis. Under the direction of Jim Spinhirne, the MPL analysis team at NASA/GSFC has developed instrument correction and backscatter analysis techniques for ARM to detect cloud boundaries and analyze vertical aerosol structures. A summary of MPL applications is found in Hlavka (1997). With the aid of independent total column optical depth instruments such as the Multifilter Rotating Shadowband Radiometer (MFRSR) at the ARM sites or sun photometers at the AERONET sites, the MPL data can be calibrated, and time-resolved vertical profiles of aerosol optical depth as well as aerosol extinction can be calculated. The techniques used to calibrate the lidar, calculate the aerosol extinction-to-backscatter ratio, and produce profiles of aerosol extinction and aerosol optical depths, will be described. Results using these techniques will be presented for case studies at the ARM site in the Tropical West Pacific and later in the Southern Great Plains.

Hlavka, Dennis L.↗

DOE OSTI2024

Shortwave Array Spectroradiometer-Hemispheric (SAS-He): design and evaluation

A novel ground-based radiometer, referred to as the Shortwave Array Spectroradiometer-Hemispheric (SAS-He), is introduced. This radiometer uses the shadow-band technique to report total irradiance and its direct and diffuse components frequently (every 30 s) with continuous spectral coverage (350–1700 nm) and moderate spectral (~2.5 nm ultraviolet–visible and ~6 nm shortwave-infrared) resolution. The SAS-He's performance is evaluated using integrated datasets collected over coastal regions during three field campaigns supported by the US Department of Energy's Atmospheric Radiation Measurement (ARM) program, namely the (1) Two-Column Aerosol Project (TCAP; Cape Cod, Massachusetts), (2) Tracking Aerosol Convection Interactions Experiment (TRACER; in and around Houston, Texas), and (3) Eastern Pacific Cloud Aerosol Precipitation Experiment (EPCAPE; La Jolla, California). We compare (i) aerosol optical depth (AOD) and total optical depth (TOD) derived from the direct irradiance, as well as (ii) the diffuse irradiance and direct-to-diffuse ratio (DDR) calculated from two components of the total irradiance. As part of the evaluation, both AOD and TOD derived from the SAS-He direct irradiance are compared to those provided by a collocated Cimel sunphotometer (CSPHOT) at five (380, 440, 500, 675, 870 nm) and two (1020, 1640 nm) wavelengths, respectively. Additionally, the SAS-He diffuse irradiance and DDR are contrasted with their counterparts offered by a collocated multifilter rotating shadowband radiometer (MFRSR) at six (415, 500, 615, 675, 870, 1625 nm) wavelengths. Overall, reasonable agreement is demonstrated between the compared products despite the challenging observational conditions associated with varying aerosol loadings and diverse types of aerosols and clouds. For example, the AOD- and TOD-related values of root mean square error remain within 0.021 at 380, 440, 500, 675, 870, 1020, and 1640 nm wavelengths during the three field campaigns.

47 OTHER INSTRUMENTATION↗

DOE OSTI2023

Aerosol Optical Depth Value-Added Product Report

This document describes the process applied to retrieve aerosol optical depth (AOD) from multifilter rotating shadowband radiometers (MFRSR) and normal incidence multifilter radiometers (NIMFR) operated at the ARM Climate Research Facility’s ground-based facilities.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2021

Droplet Number Concentration Value-Added Product

The ndrop_mfrsr value-added product (VAP) provides an estimate of the cloud droplet number concentration of overcast water clouds retrieved from cloud optical depth from the multi-filter rotating shadowband radiometer (MFRSR) instrument and liquid water path (LWP) retrieved from the microwave radiometer (MWR). When cloud layer information is available from vertically pointing lidar and radars in the Active Remote Sensing of Clouds (ARSCL) product, the VAP also provides estimates of the adiabatic LWP and an adiabatic parameter (beta) that indicates how divergent the LWP is from the adiabatic case. quality control (QC) flags (qc_drop_number_conc), an uncertainty estimate (drop_number_conc_toterr), and a cloud layer type flag (cloud_base_type) are useful indicators of the quality and accuracy of any given value of the retrieval. Examples of these major input and output variables are given in sample plots in section 6.0.

97 MATHEMATICS AND COMPUTING↗

DOE OSTI2020

ARM Shortwave Spectral Radiometry Strategy Review Report

A meeting of experts in shortwave (SW) spectral measurements was held in February 2019 to discuss the current state of the U.S. Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) user facility instrumentation and the potential scientific impact of these measurements. Instrument mentors and users reported significant progress in hyperspectral measurement quality, with good-quality data sets now possible at several field campaigns and fixed sites. Ongoing filter-based measurement improvements, including addition of the 1.6-micron channel to the multifilter rotating shadowband radiometer (MFRSR) and lunar tracking mode of the Cimel sun photometers, were also lauded as exciting developments to improve retrievals of aerosol radiative properties and size distributions.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2020

ARM Shortwave Spectral Radiometry Strategy Review Report

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS2002

CIMEL Measurements of Zenith Radiances at the ARM Site

Starting from October 1, 2001, Cimel at the ARM Central Facility in Oklahoma has been switched to a new "cloud mode." This mode allows taking measurements of zenith radiance when the Sun in blocked by clouds. In this case, every 13 min. Cimel points straight up and takes 10 measurements with 9 sec. time interval. The new Cimel's mode has four filters at 440, 670, 870 and 1020 nm. For cloudy conditions, the spectral contrast in surface albedo dominates over Rayleigh and aerosol effects; this makes normalized zenith radiances at 440 and 670 as well as for 870 and 1020 almost indistinguishable. We compare Cimel measurements with other ARM cart site instruments: Multi-Filter Rotating Shadowband Radiometer (MFRSR), Narrow Field of View (NFOV) sensor, and MicroWave Radiometer(MWR). Based on Cimel and MFRSR 670 and 870 nm channels, we build a normalized difference cloud index (NDCI) for radiances and fluxes, respectively. Radiance NDCI from Cimel and flux NDCI from MFRSR are compared between themselves as well as with cloud Liquid Water Path (LWP) retrieved from MWR. Based on our theoretical calculations and preliminary data analysis,there is a good correlation between NDCIs and LWP for cloudy sky above green vegetation. Based on this correlation, an algorithm to retrieve cloud optical depth from NDCI is proposed.

Marshak, Alexander↗

NASA NTRS2003

Inferring Cloud Properties from Passive Solar Sensors

The most common approach for retrieving cloud optical depth from ground-based observations uses downwelling fluxes measured by pyranometers and Multi-Filter Rotating Shadowband Radiometers (MFRSR). The key element in both retrieval techniques is the one-to-one mapping of the "observed" fluxes into cloud optical depth through plane-parallel radiative transfer. Both methods are expected to work well only for completely overcast clouds giving an effective optical depth for the whole sky. To infer cloud optical depth locally one can assume to use a narrow-field-of view radiometer that measures radiances instead of fluxes. However, lack of one-to-one relationships between radiance and cloud optical depth, prevents the direct use of radiances either. Here we discuss a new method for retrieving cloud optical depth from ground-based measurements of zenith radiance in the RED and near infrared (NIR) spectral regions. In addition to an algebraic combinations of spectral radiances such as Normalized Difference Cloud Index (NDCI) that largely removes nonuniqueness and the radiative effects of cloud inhomogeneity but can result in poor retrievals due to its insensitivity to cloud fraction, both RED and NIR radiances as points on the "RED vs. NIR" plane are proposed to be used for retrieval. The proposed retrieval method is applied to a multi- channel sunphotometer (as a part of AERONET) measurements at the ARM site in Oklahoma. The results of retrieval are compared with the ones from Microwave Radiometer (MWR) and MFRSR. In addition to cloud optical depth, the new retrieval method also infers a "radiatively effective" cloud fraction.

Marshak, A.↗

NASA NTRS2020

Ground-based retrievals of aerosol column absorption in the UV spectral region and their implications for GEMS measurements

Quantifying the spectral variation of column aerosol absorption in the ultraviolet (UV) and visible (Vis) wavelengths is required for accurate satellite-based aerosol and trace-gas retrievals. Retrievals of the column-averaged imaginary part of refractive index and single scattering albedo (SSA) in the UV–Vis range have been performed at Yonsei University, Seoul, Korea, since 2016 by combining co-located measurements from the NASA Aerosol Robotic Network (AERONET) Cimel sun-sky photometer, the Ultraviolet Multifilter Rotating Shadowband Radiometer (UV-MFRSR), the SKYNET Prede sky radiometer, and the NASA Pandora sun spectrometer. We investigated the spectral variation of column-averaged imaginary part of refractive index for UV–Vis wavelengths to refine models used in our aerosol retrieval algorithm to process measurements from the upcoming Geostationary Environment Monitoring Satellite (GEMS). The retrieved imaginary part of refractive index for highly absorbing fine pollution particles (BC), dust (DS), and non-absorbing (NA) particles in the selected UV–Vis range (380–440 nm) showed 0–20%, 30%, and 0–40% of spectral dependence, respectively. Retrievals of Ozone Monitoring Instrument (OMI) measurement data using the improved aerosol model showed improved correlation with AERONET data compared to the old algorithm that did not properly account for aerosol absorption effects. These results corroborate the advantage of using local climatology derived from ground-based UV–Vis spectral aerosol absorption measurements for satellite GEMS aerosol retrievals over East Asia. Moreover, this study reveals that spectral variations in the UV column aerosol absorption in East Asia differ from those in other regions.

ultraviolet (UV) and visible (Vis) wavelengths↗

DOE OSTI2020

Physically based correction of systematic errors of Rotating Shadowband Irradiometers

Accurate measurements of direct normal, diffuse horizontal and global horizontal irradiance (DNI, DHI and GHI) are needed for meteorological studies and are essential for the solar resource assessment at potential solar power plant sites. Often, these potential sites are remote and hence require robust sensors that require minimal maintenance that are not affected strongly by soiling. Therefore, Rotating Shadowband Irradiometers (RSI) are widely used for resource assessment. To achieve the required accuracy, corrections for the raw values of RSIs depending on systematic temperature, incidence angle and spectral errors must be used, and a thorough calibration of the sensor head must be applied. The existing correction functions are derived from comparisons of RSIs to thermopile radiometers at selected sites and therefore empirical. Their accuracy is considered to be site dependent. In this work a new correction and calibration method is presented that removes the systematic errors using a physical approach. It is based on information of the sensor properties as well as measurements of its directional response, and incorporates the atmospheric conditions at the measurement site. In this case, no empiric relations obtained from a specific site are required. The method requires estimates of the current DHI and GHI spectra during each measurement of the RSI. Based on these spectra, a spectral correction, which includes a spectrum dependent temperature correction, can be made without employing empirical relationships. The new physical calibration and correction method is tested at three sites and reaches similar results compared to the empirical functions. This is already achieved with rudimentary estimations of the GHI and DHI spectra and we expect that these estimations can be improved in the future. The results indicate that the physical approach reduces the problematic location dependence of the current calibration and correction methods. The physical correction and calibration method show promise for a further improvement of the RSI accuracy.

47 OTHER INSTRUMENTATION↗

NASA NTRS2000

MM-Wave Radiometric Measurements of Low Amounts of Precipitable Water Vapor

An experiment was conducted during March, 1999 to study ways in which to improve techniques for measuring low amounts of total-column precipitable water vapor (PWV). The experiment was conducted at the DOE's ARM program's North Slope of Alaska/Adjacent Arctic Ocean Cloud and Radiation Testbed site (DoE ARM NSA/AAO CaRT) located just outside Barrow, Alaska. NASA and NOAA deployed a suite of radiometers covering 25 channels in the frequency range of 20 GHz up to 340 GHz including 8 channels around the 183 GHz water vapor absorption line. In addition to the usual CaRT site instrumentation the NOAA Depolarization and Backscatter Unattended Lidar (DABUL), the SUNY Rotating Shadowband Spectroradiometer (RSS) and other surface based meteorological instrumentation were deployed during the intensive observation period. Vaisala RS80 radiosondes were launched daily as well as nearby National Weather Service VIZ sondes. Atmospheric conditions ranged from clear calm skies to blowing snow and heavy multi-layer cloud coverage. Measurements made by the radiosondes indicate the PWV varied from approx. 1 to approx. 5 mm during the experiment. The near-surface temperature varied between about -40 C to - 15 C. In this presentation, an overview of the experiment with examples of data collected will be presented. Application of the data for assessing the potential and limitations of millimeter-wave radiometry for retrieving very low amounts of PWV will be discussed.

Racette, P.↗

NASA NTRS2001

A Robust Retrieval of Water Vapor Column In Dry Arctic Conditions Using the Rotating Shadowband Spectroradiometer

A method to retrieve water vapor column using the 940-nm water vapor absorption band in dry Arctic conditions is presented. The retrievals with this method are stable with respect to uncertainties in instrument radiometric calibration, air pressure, solar source function, and aerosols. The water vapor column was retrieved with this method using spectra obtained with the rotating shadowband spectroradiometer (RSS) that was deployed during an intensive observation period near Barrow, Alaska, in March 1999. A line-by-line radiative transfer model was used to compute water vapor transmittance. The retrievals with this method are compared with retrievals obtained from three independent measurements with microwave radiometers. All four measurements show the same pattern of temporal variations. The RSS results agree most closely with retrievals obtained with the millimeter-wave imaging radiometer (MIR) at its 183 GHz +/- 7 double-side band channel. Their correlation over a period of 7 days when water vapor column varied between 0.75 mm and 3.6 mm (according to RSS) is 0.968 with MIR readings 0.12 mm higher on average.

Kiedron, P.↗