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At least 19 records

Spectral zone selection methodology for pebble bed reactors

A methodology is developed for determining boundaries of spectral zones for pebble bed reactors. A spectral zone is defined as a region made up of a number of nodes whose characteristics are collectively similar and that are assigned the same few-group diffusion constants. The spectral zones are selected in such a manner that the difference (error) between the reference transport solution and the diffusion code solution takes a minimum value. This is achieved by choosing spectral zones through optimally minimizing this error. The objective function for the optimization algorithm is the total reaction rate error, which is defined as the sum of the leakage, absorption and fission reaction rates errors in each zone. The selection of these spectral zones is such that the core calculation results based on diffusion theory are within an acceptable tolerance as compared to a proper transport reference solution. Through this work, a consistent approach for identifying spectral zones that yield more accurate diffusion results is introduced.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Full-zone spectral envelope function formalism for the optimization of line and point tunnel field-effect transistors

Efficient quantum mechanical simulation of tunnel field-effect transistors (TFETs) is indispensable to allow for an optimal configuration identification. We therefore present a full-zone 15-band quantum mechanical solver based on the envelope function formalism and employing a spectral method to reduce computational complexity and handle spurious solutions. We demonstrate the versatility of the solver by simulating a 40 nm wide In{sub 0.53}Ga{sub 0.47}As lineTFET and comparing it to p-n-i-n configurations with various pocket and body thicknesses. We find that the lineTFET performance is not degraded compared to semi-classical simulations. Furthermore, we show that a suitably optimized p-n-i-n TFET can obtain similar performance to the lineTFET.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Hitomi X-ray observation of the pulsar wind nebula G21.5–0.9

Here, we present results from the Hitomi X-ray observation of a young composite-type supernova remnant (SNR) G21.5–0.9, whose emission is dominated by the pulsar wind nebula (PWN) contribution. The X-ray spectra in the 0.8–80 keV range obtained with the Soft X-ray Spectrometer (SXS), Soft X-ray Imager, and Hard X-ray Imager (HXI) show a significant break in the continuum as previously found with the NuSTAR observation. After taking into account all known emissions from the SNR other than the PWN itself, we find that the Hitomi spectra can be fitted with a broken power law with photon indices of Γ 1 = 1.74 ± 0.02 and Γ 2 = 2.14 ± 0.01 below and above the break at 7.1 ± 0.3 keV, which is significantly lower than the NuSTAR result (~9.0 keV). The spectral break cannot be reproduced by time-dependent particle injection one-zone spectral energy distribution models, which strongly indicates that a more complex emission model is needed, as suggested by recent theoretical models. We also search for narrow emission or absorption lines with the SXS, and perform a timing analysis of PSR J1833–1034 with the HXI and the Soft Gamma-ray Detector. No significant pulsation is found from the pulsar. However, unexpectedly, narrow absorption line features are detected in the SXS data at 4.2345 keV and 9.296 keV with a significance of 3.65 σ. While the origin of these features is not understood, their mere detection opens up a new field of research and was only possible with the high resolution, sensitivity, and ability to measure extended sources provided by an X-ray microcalorimeter.

(stars:) pulsars: individual↗

ML-Based Pebble Power Reconstruction for Pebble Bed Reactor Analysis

Pebble power reconstruction has been explored to complement the conventional homogenized modeling approach in pebble bed reactor (PBR) analysis, as detailed heterogeneous geometry calculations are computationally expensive. The random distribution of pebble fuels within the core challenges the application of conventional pin power reconstruction methods. To address this, we introduce a machine learning approach based on the transformer model, composed of encoder and decoder layers, to estimate the flux and power form functions for reconstructing individual pebble neutron fluxes and powers. The homogeneous neutron flux distribution within each spectral zone (SZ) is obtained from finite element solutions of global diffusion or transport calculations. Verification tests demonstrate that the trained transformer model accurately predicts power form functions over a range of conditions, including variations in pebble enrichment, location, type, SZ size, and burnup. In particular, verification using a three-dimensional PBR benchmark with burned pebbles shows good agreement in heterogeneous pebble power distributions between Griffin and Serpent. These results highlight the potential of applying conventional pin power reconstruction approaches to PBR cores with randomly distributed pebbles.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

SPITZER EVIDENCE FOR A LATE-HEAVY BOMBARDMENT AND THE FORMATION OF UREILITES IN {eta} CORVI At {approx}1 Gyr

We have analyzed Spitzer and NASA/IRTF 2-35 {mu}m spectra of the warm, {approx}350 K circumstellar dust around the nearby MS star {eta} Corvi (F2V, 1.4 {+-} 0.3 Gyr). The spectra show clear evidence for warm, water- and carbon-rich dust at {approx}3 AU from the central star, in the system's terrestrial habitability zone. Spectral features due to ultra-primitive cometary material were found, in addition to features due to impact produced silica and high-temperature carbonaceous phases. At least 9 Multiplication-Sign 10{sup 18} kg of 0.1-100 {mu}m warm dust is present in a collisional equilibrium distribution with dn/da {approx} a{sup -3.5}, the equivalent of a 130 km radius Kuiper Belt object (KBO) of 1.0 g cm{sup 3} density and similar to recent estimates of the mass delivered to the Earth at 0.6-0.8 Gyr during the late-heavy bombardment. We conclude that the parent body was a Kuiper Belt body or bodies which captured a large amount of early primitive material in the first megayears of the system's lifetime and preserved it in deep freeze at {approx}150 AU. At {approx}1.4 Gyr they were prompted by dynamical stirring of their parent Kuiper Belt into spiraling into the inner system, eventually colliding at 5-10 km s{sup -1} with a rocky planetary body of mass {<=}M{sub Earth} at {approx}3 AU, delivering large amounts of water (>0.1% of M{sub Earth'sOceans}) and carbon-rich material. The Spitzer spectrum also closely matches spectra reported for the Ureilite meteorites of the Sudan Almahata Sitta fall in 2008, suggesting that one of the Ureilite parent bodies was a KBO.

79 ASTRONOMY AND ASTROPHYSICS↗

On the Radio-emitting Particles of the Crab Nebula: Stochastic Acceleration Model

The broadband emission of pulsar wind nebulae (PWNe) is well described by non-thermal emissions from accelerated electrons and positrons. However, the standard shock acceleration model of PWNe does not account for the hard spectrum in radio wavelengths. The origin of the radio-emitting particles is also important to determine the pair production efficiency in the pulsar magnetosphere. Here, we propose a possible resolution for the particle energy distribution in PWNe; the radio-emitting particles are not accelerated at the pulsar wind termination shock but are stochastically accelerated by turbulence inside PWNe. We upgrade our past one-zone spectral evolution model to include the energy diffusion, i.e., the stochastic acceleration, and apply the model to the Crab Nebula. A fairly simple form of the energy diffusion coefficient is assumed for this demonstrative study. For a particle injection to the stochastic acceleration process, we consider the continuous injection from the supernova ejecta or the impulsive injection associated with supernova explosion. The observed broadband spectrum and the decay of the radio flux are reproduced by tuning the amount of the particle injected to the stochastic acceleration process. The acceleration timescale and the duration of the acceleration are required to be a few decades and a few hundred years, respectively. Our results imply that some unveiled mechanisms, such as back reaction to the turbulence, are required to make the energies of stochastically and shock-accelerated particles comparable.

79 ASTRONOMY AND ASTROPHYSICS↗

A Versatile Coupled Test Reactor Concept

A Versatile Coupled Test Reactor (VCTR) is a highly reconfigurable, sodium-cooled, coupled fast and thermal spectrum test reactor, which provides (1) a fast flux irradiation environment prototypical of potential fast reactor designs, (2) thermal and epithermal flux irradiation environments complementary to those of ATR and HFIR, and (3) other possibilities, including beam tubes for scientific experiments, irradiation vehicles for isotope production, etc. The ongoing design of a new versatile coupled thermal-fast test reactor at INL that can accommodate both fast and thermal irradiation, technology and safety features tests is described in this paper. A coupled reactor is defined as a reactor with two distinct spectral zones (Fast and Thermal), which are neutronically coupled to each other: some neutrons born in zone F cause fission in zone T and vice-versa. Only fast neutrons are allowed to go from one zone to the other, which is assured by a thermal neutron filter. A distinction of coupling can be made depending on the main purpose of using fuel assemblies with some level of neutron moderation (thermal zone) together with fuel assemblies with as little moderation as possible (fast zone). It can be used mainly to minimize the core power and fissile inventory, or it can be used mainly to provide additional control of the irradiation conditions in the thermal zone. The steady-state neutronics calculations were performed using the three-dimensional continuous-energy Monte Carlo reactor physics burnup calculation code Serpent2. Although, a few changes were necessary to support the Serpent code in calculating the coupling coefficients. Steady state and transient thermal analyses were performed with RELAP5-3D. RELAP5-3D is the latest in the RELAP5 code series developed at INL. One of the core configurations using only low enriched uranium fuel could provide both a high fast neutron flux and a high thermal neutron flux—respectively 3.5E15 n/s.cm2 and 1E15 n/s.cm2—in large volumes while maintaining core power below 300 MW. The use of plutonium in the fast zone provides more flexibility in fuel assembly design than when low enriched uranium is used, the designer has more degrees of freedom to work with; in particular it could provide additional control of the irradiation conditions in the thermal zone. The results showed that the current design fulfills most R&D needs requirements providing high thermal and fast fluxes and wide possibilities for diversified future reactor features test in appropriate loops, both in steady state and during transients.

coupled spectrum↗

Derivation of the Point-Kinetics Parameters for the Coupled Reactors

The design of coupled reactors, which provide two distinct spectral zones (fast and thermal), has recently drawn attention because it can provide configurations that could not be met in current thermal neutron test reactors and thus allows versatile irradiation tasks. A coupled reactor core is characterized by the neutron multiplicity of each zone as well as by the coupling between the two zones. It is desired to evaluate the integral point kinetics parameters that characterize the neutron physics of the coupled system. This summary provides a derivation of the equations for evaluating these point kinetics parameters. Following the strong and the weak form of the multigroup diffusion equation, the weak forms for the partial forward and adjoint solutions, each for a particular active region of the reactor core, are derived. These partial solutions are then used to collapse the weak form into the coupled-reactor point kinetics equations with the approximation of equilibrium. It is noted that these parameters are not meant for transient analysis because of the equilibrium approximation. They are rather used for characterizing the coupled system. The derived reactivity equations are then compared with those in Ref. 1. The equations are implemented in Rattlesnake, the INL MOOSE-based radiation transport application for multi-physics simulations. Numerical results are presented for a simple two-group problem. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Observation of the spectrally invariant properties of clouds in cloudy-to-clear transition zones during the MAGIC field campaign

We use the spectrally invariant method to study the variability of cloud optical thickness τ and droplet effective radius reff in transition zones (between the cloudy and clear sky columns) observed from Solar Spectral Flux Radiometer (SSFR) and Shortwave Array Spectroradiometer-Zenith (SASZe) during the Marine ARM GPCI Investigation of Clouds (MAGIC) field campaign. The measurements from the SSFR and the SASZe are different, however inter-instrument differences of self-normalized measurements (divided by their own spectra at a fixed time) are small. The spectrally invariant method approximates the spectra in the cloud transition zone as a linear combination of definitely clear and cloudy spectra, where the coefficients, slope and intercept, character-ize the spectrally invariant properties of the transition zone. Simulation results from the SBDART (Santa Barbara DISORT Atmospheric Radiative Transfer) model demonstrate that (1) the slope of the visible band is positively correlated with the cloud optical thickness τ while the intercept of the near-infrared band has high negative cor-relation with the cloud drop effective radius reff even without the exact knowledge of τ; (2) the above relations hold for all Solar Zenith Angle (SZA) and for cloud-contaminated skies. In observations using redundant measure-ments from SSFR and SASZe, we find that during cloudy-to-clear transitions, (a) the slopes of the visible band de-crease, and (b) the intercepts of the near-infrared band remain almost constant near cloud edges. The findings in simulations and observations suggest that, while the optical thickness decreases during the cloudy-to-clear transition, the cloud drop effective radius does not change when cloud edges are approached. These results sup-port the hypothesis that inhomogeneous mixing dominates near cloud edges in the studied cases.

54 ENVIRONMENTAL SCIENCES↗

Stochastic microhertz gravitational radiation from stellar convection

High Reynolds-number turbulence driven by stellar convection in main-sequence stars generates stochastic gravitational radiation. We calculate the wave-strain power spectral density as a function of the zero-age main-sequence mass for an individual star and for an isotropic, universal stellar population described by the Salpeter initial mass function and redshift-dependent Hopkins-Beacom star formation rate. The spectrum is a broken power law, which peaks near the turnover frequency of the largest turbulent eddies. The signal from the Sun dominates the universal background. For the Sun, the far-zone power spectral density peaks at S(f {sub peak}) = 5.2 × 10{sup –52} Hz{sup –1} at frequency f {sub peak} = 2.3 × 10{sup –7} Hz. However, at low observing frequencies f < 3 × 10{sup –4} Hz, the Earth lies inside the Sun's near zone and the signal is amplified to S {sub near}(f {sub peak}) = 4.1 × 10{sup –27} Hz{sup –1} because the wave strain scales more steeply with distance (∝d {sup –5}) in the near zone than in the far zone (∝d {sup –1}). Hence the Solar signal may prove relevant for pulsar timing arrays. Other individual sources and the universal background fall well below the projected sensitivities of the Laser Interferometer Space Antenna and next-generation pulsar timing arrays. Stellar convection sets a fundamental noise floor for more sensitive stochastic gravitational-wave experiments in the more distant future.

79 ASTRONOMY AND ASTROPHYSICS↗

A Chandra grating observation of the dusty Wolf-Rayet star WR 48a

We present results of a Chandra High-Energy Transmission Grating (HETG) observation of the carbon-rich Wolf-Rayet (WR) star WR 48a. These are the first high-resolution spectra of this object in X-ray. Blueshifted centroids of the spectral lines of ∼ – 360 km s{sup –1} and line widths of 1000-1500 km s{sup –1} (FWHM) were deduced from the analysis of the line profiles of strong emission lines. The forbidden line of Si XIII is strong and not suppressed, indicating that the rarified 10-30 MK plasma forms far from strong sources of far-ultraviolet emission, most likely in a wind collision zone. Global spectral modeling showed that the X-ray spectrum of WR 48a suffered higher absorption in the 2012 October Chandra observation compared with a previous 2008 January XMM-Newton observation. The emission measure of the hot plasma in WR 48a decreased by a factor ∼3 over the same period of time. The most likely physical picture that emerges from the analysis of the available X-ray data is that of colliding stellar winds in a wide binary system with an elliptical orbit. We propose that the unseen secondary star in the system is another WR star or perhaps a luminous blue variable.

79 ASTRONOMY AND ASTROPHYSICS↗

Modeling Sequences of Earthquakes and Aseismic Slip (SEAS) in Elasto-Plastic Fault Zones With a Hybrid Finite Element Spectral Boundary Integral Scheme

We present a coupled finite element spectral boundary integral framework for modeling sequences of earthquakes and aseismic slip on a 2-D planar rate-and-state fault with off-fault visco-plastic response in the plane strain approximation. The model resolves both slow aseismic deformation and inertia effects during rapid slip. As an application, we perform two sets of simulations with different choices of cohesion to explore the co-evolution of fault slip, bulk plasticity and local stress fields. The first set implements a relatively large value of the cohesion parameter, which results in limiting inelastic strain accumulation to dynamic rupture phases. The second set implements a smaller cohesion, allowing for plastic strain to accumulate in both seismic and aseismic phases. For the first model, our results indicate that the extent and distribution of plastic strain depend on the angle of maximum compressive principal stress. At larger angles, inelastic strain accumulates on the extensional side of a dynamically propagating rupture. At smaller angles, the extent of plasticity is limited to the compressional side of the domain. At smaller cohesion values, off-fault plasticity may occur during aseismic slip, which alters the nucleation characteristics and earthquake sequence pattern. Furthermore, our results at lower cohesion values indicate that plastic strain accumulation may occur in both the extensional and compressional sides of the off-fault bulk even at higher angles of maximum compression. In conclusion, this produces damage patterns that deviate from the traditional off-fault fan-like distribution observed in dynamic rupture simulations and emphasizes the significance of long-term deformation in interpreting observations.

58 GEOSCIENCES↗

Evaluation of the Effects of Microbes on Autunite Dissolution and the Spectral Induced Polarization Response in Hanford Vadose Zone Sediment - 18440

As a result of the U.S. nuclear weapons program during the second World War and throughout the Cold War, there now exists a significant amount of uranium contamination at the U.S. Department of Energy Hanford site located in Washington State. Much of this contamination is in the form of mobile uranyl carbonates species within the vadose zone, which at Hanford varies up to 100 m thick in the Central Plateau. In-situ immobilization of mobile uranium via injections of a soluble sodium tripolyphosphate amendment may prove effective in the formation of low-solubility uranyl phosphate solid phases, autunite. However, the injected polyphosphate undergoes hydrolysis in aqueous solutions to form orthophosphate, which serves as a readily available nutrient for the various microorganisms in the sediment. Sediment-filled column experiments conducted under saturated oxygen restricted conditions using a geophysical technique known as spectral induced polarization (SIP) have shown the impact of microbes on the dissolution of synthetic autunite. Two sets of experiments were conducted using test columns. Each experiment had a pair of columns inoculated with microbes (with a glucose solution acting as a nutrient source) which were monitored using SIP in conjunction with regular sampling of pore-water. Columns were built with two silver/silver chloride (Ag/AgCl) coiled current electrodes at either end and four Ag potential electrodes along the side, which allowed the measurement of three distinct points along the length of the column. SIP measures phase which is the time delay between an injected current and measured voltage, in this case measured in radians. Three sampling ports were added to correspond with the geophysical measurements. Pore-water samples taken over the course of the experiment were analyzed for dissolved elements including uranium, iron, phosphorous, calcium, and magnesium. SIP results were plotted over time in order to determine correlations between changes in electrical phase and changes in pore-water chemistry. It was determined that changes in the phase and bulk resistivity detected with SIP corresponded to changes in the pore-water chemistry due to the growth of microbes. The first experiment ran for five months and had measurements done once a week, the second only ran one month but had measurements taken five times a week in order to understand initial changes in column chemistry in greater detail. SIP may be an effective way to remotely track changes indicative of bacterial activities on the surrounding environment. This method has the potential for field application at a larger scale for the purpose of tracking microbe growth in response to tripolyphosphate amendment. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Spectral induced polarization (SIP) measurements across a PFAS-contaminated source zone

There is a pressing need for the development of field-scale, in situ screening technologies for assessing variations in aqueous film forming foam (AFFF) concentrations in soils at former fire training and storage sites. Field-scale Spectral Induced Polarization (SIP) geophysical measurements were acquired on a transect crossing an AFFF source zone. Soil samples were acquired from ten locations and used to determine variations in poly- and per-fluoroalkyl substances (PFAS) concentrations in soils and soil texture. These samples were also used to create triplicate soil columns for laboratory-grade SIP measurements. Field and laboratory observations provide evidence that SIP measurements are sensitive to the concentration of AFFF constituents associated with the pore surface in soils. The phase of the SIP measurements on the laboratory samples was linearly correlated with total soil-sorbed PFAS concentration. The phase from the field SIP measurements was highest over the location of maximum PFAS concentration measured on the laboratory samples, although a significant correlation between field-measured phase and laboratory-measured total PFAS concentration was not established. The sensitivity of the SIP response to the removal of soil PFAS using a methanol wash procedure (total PFAS concentration drop of 366 ppb) adds evidence for the case for SIP characterization of AFFF source zones. The results of these studies suggest that SIP might be developed into a field-scale technology for rapid, indirect assessment of AFFF source zones. Such a technology could improve the effectiveness of AFFF source zone characterization at reduced costs.

58 GEOSCIENCES↗

Enhanced photodetection in graphene-integrated photonic crystal cavity

We demonstrate the controlled enhancement of photoresponsivity in a graphene photodetector by coupling to slow light modes in a long photonic crystal linear defect cavity. Near the Brillouin zone (BZ) boundary, spectral coupling of multiple cavity modes results in broad-band photocurrent enhancement from 1530 nm to 1540 nm. Away from the BZ boundary, individual cavity resonances enhance the photocurrent eight-fold in narrow resonant peaks. Optimization of the photocurrent via critical coupling of the incident field with the graphene-cavity system is discussed. The enhanced photocurrent demonstrates the feasibility of a wavelength-scale graphene photodetector for efficient photodetection with high spectral selectivity and broadband response.

36 MATERIALS SCIENCE↗

Ultrafast broadband spectroscopy of crystalline bismuth

Femtosecond spectroscopy in the wavelength range 0.4 - 2.3 {mu}m has been used to probe ultrafast electronic and lattice processes in bismuth. The photoresponse of a bismuth crystal is shown to comprise components with relaxation times of 1 ps, 7 ps, and {approx}1 ns. The electron-hole and electron-phonon interaction strengths in bismuth are found to depend significantly on the wave vector in the {Gamma}-T direction of the Brillouin zone. Comparison of the spectral dependences of the amplitudes of coherent E{sub g} and A{sub 1g} phonons and the corresponding dependences of the Raman scattering cross sections indicates that these phonon modes differ in generation mechanism. The generation of coherent A{sub 1g} phonons is mainly due to displacement of the equilibrium position of atoms in the crystal lattice in a nonequilibrium state. This process differs fundamentally from resonance Raman scattering responsible for the coherent excitation of low-symmetry phonon modes. (extreme light fields and their applications)

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

MULTI-FREQUENCY, MULTI-EPOCH STUDY OF Mrk 501: HINTS FOR A TWO-COMPONENT NATURE OF THE EMISSION

Since the detection of very high energy (VHE) γ-rays from Mrk 501, its broadband emission of radiation was mostly and quite effectively modeled using the one zone emission scenario. However, broadband spectral and flux variability studies enabled by the multi-wavelength campaigns carried out during the recent years have revealed the rather complex behavior of Mrk 501. The observed emission from Mrk 501 could be due to a complex superposition of multiple emission zones. Moreover, new evidence of detection of very hard intrinsic γ-ray spectra obtained from Fermi-LAT observations has challenged the theories about the origin of VHE γ-rays. Our studies based on Fermi-LAT data indicate the existence of two separate components in the spectrum, one for low-energy γ-rays and the other for high-energy γ-rays. Using multi-waveband data from several ground- and space-based instruments, in addition to HAGAR data, the spectral energy distribution of Mrk 501 is obtained for various flux states observed during 2011. In the present work, this observed broadband spectral energy distribution is reproduced with a leptonic, multi-zone synchrotron self-Compton (SSC) model.

79 ASTRONOMY AND ASTROPHYSICS↗

Long-duration superluminous supernovae at late times

Nebular-phase observations and spectral models of Type Ic superluminous supernovae (SLSNe) are presented. LSQ14an and SN 2015bn both display late-time spectra similar to galaxy-subtracted spectra of SN 2007bi, and the class shows strong similarity with broad-lined SNe Ic such as SN 1998bw. Near-infrared observations of SN 2015bn show a strong Ca ii triplet, O i 9263, O i 1.13 μm, and Mg i 1.50 μm, but no distinct He, Si, or S emission. The high Ca ii NIR/[Ca ii] 7291, 7323 ratio of ∼2 indicates a high electron density of n{sub e}≳10{sup 8} cm{sup −3}. Spectral models of oxygen-zone emission are investigated to put constraints on the emitting region. Models require M(O-zone)≳10 M{sub ⊙} to produce enough [O i] 6300, 6364 luminosity, irrespective of the powering situation and the density. The high oxygen-zone mass, supported by high estimated magnesium masses, points to explosions of massive CO cores, requiring M{sub ZAMS}≳40 M{sub ⊙}. Collisions of pair-instability pulsations do not provide enough mass to account for the emission. [O ii] and [O iii] lines emerge naturally in many models, which strengthens the identification of broad [O ii] 7320, 7330, [O iii] 4363, and [O iii] 4959, 5007 in some spectra. A small filling factor f≲0.01 for the O/Mg zone is needed to produce enough luminosity in Mg i] 4571, Mg i 1.504 μm, and O i recombination lines, which shows that the ejecta is clumped. We review the constraints from the nebular spectral modeling in the context of the various scenarios proposed for SLSNe.

79 ASTRONOMY AND ASTROPHYSICS↗