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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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IR pumped third-harmonic generation and sum-frequency generation in diatomic molecules

The potential efficiency of using nonlinear up-conversion techniques for the high efficiency type lasers (CO,CO2, and chemical) is assessed. Results indicate that: the small pump photon energy necessitates the use of molecular media for conversion if resonance enhancement is to be used and that molecular systems present several problems. These difficulties include: their levels are complex; their transition probabilities are often unknown; and the oscillator strengths among vibrational levels in the ground electronic state of a molecule are much smaller than those among electronic states of an atom, thus limiting the magnitude of nonlinear interactions. It is shown that this problem can be eliminated by making use of vibronic transitions which, being primarily electronic transitions have much larger matrix elements and efficient conversion can be achieved with molecular systems.

She, C. Y.↗

Infrared-pumped third-harmonic and sum-frequency generation in diatomic molecules

Using molecular hydrogen as a model system, we present a calculation which demonstrates the feasibility of efficient third-harmonic and sum-frequency generation of IR laser radiation by diatomic molecular gases. A conversion efficiency of 10% without phase matching is achievable with a modest laser intensity of about 20 MW/sq cm. In addition to a two-photon resonance, the efficient conversion depends on a mechanism which makes use of virtual vibronic transitions exclusively. Possible methods for phase matching are also suggested.

She, C. Y.↗

Sum-frequency generation from photon number squeezed light

We investigate the quantum fluctuations of the fields produced in sum-frequency (SF) generation from light initially in the photon number squeezed state. It is found that, to the fourth power term, the output SF light is sub-Poissonian whereas the quantum fluctuations of the input beams increase. Quantum anticorrelation also exists in SF generation.

Wu, Ling-An↗

Diode-pumped laser altimeter

TEM(sub 00)-mode output energies up to 22.5 mJ with 23 percent slope efficiencies were generated at 1.064 microns in a diode-laser pumped Nd:YAG laser using a transverse-pumping geometry. 1.32-micron performance was equally impressive at 10.2 mJ output energy with 15 percent slope efficiency. The same pumping geometry was successfully carried forward to several complex Q-switched laser resonator designs with no noticeable degradation of beam quality. Output beam profiles were consistently shown to have greater than 90 percent correlation with the ideal TEM(sub 00)-order Gaussian profile. A comparison study on pulse-reflection-mode (PRM), pulse-transmission-mode (PTM), and passive Q-switching techniques was undertaken. The PRM Q-switched laser generated 8.3 mJ pulses with durations as short as 10 ns. The PTM Q-switch laser generated 5 mJ pulses with durations as short as 5 ns. The passively Q-switched laser generated 5 mJ pulses with durations as short as 2.4 ns. Frequency doubling of both 1.064 microns and 1.32 microns with conversion efficiencies of 56 percent in lithium triborate and 10 percent in rubidium titanyl arsenate, respectively, was shown. Sum-frequency generation of the 1.064 microns and 1.32 microns radiations was demonstrated in KTP to generate 1.1 mJ of 0.589 micron output with 11.5 percent conversion efficiency.

Welford, D.↗

Program Predicts Performance of Optical Parametric Oscillators

A computer program predicts the performances of solid-state lasers that operate at wavelengths from ultraviolet through mid-infrared and that comprise various combinations of stable and unstable resonators, optical parametric oscillators (OPOs), and sum-frequency generators (SFGs), including second-harmonic generators (SHGs). The input to the program describes the signal, idler, and pump beams; the SFG and OPO crystals; and the laser geometry. The program calculates the electric fields of the idler, pump, and output beams at three locations (inside the laser resonator, just outside the input mirror, and just outside the output mirror) as functions of time for the duration of the pump beam. For each beam, the electric field is used to calculate the fluence at the output mirror, plus summary parameters that include the centroid location, the radius of curvature of the wavefront leaving through the output mirror, the location and size of the beam waist, and a quantity known, variously, as a propagation constant or beam-quality factor. The program provides a typical Windows interface for entering data and selecting files. The program can include as many as six plot windows, each containing four graphs.

Cross, Patricia L.↗

Development of Mesospheric Sodium Laser Beacon for Atmospheric Adaptive Optics

A solid-state source of long pulse length, sodium-resonance radiation was developed for the purpose of generating an artificial star in the earth's mesospheric sodium layer. This radiation is generated by sum-frequency mixing the output of a 1.064 micron Nd:YAG laser with the output of a 1.319-micron Nd:YAG laser. By operating these lasers at wavelengths very close to the peak of their tuning curves, it is possible to match the wavelength of the sum-frequency radiation to that of the sodium D2 adsorption wavelength. Two pulsed laser systems were constructed, one producing as much as 0.6 J of sodium resonance radiation at a 10-Hz repetition rate and another producing as much as 24 mJ at a 840-Hz repetition rate. In both laser systems, the 1.06-micron and 1.32-micron Nd:YAG lasers are configured as mode-locked master oscillators followed by power amplifiers. Other aspects of this project are presented.

Jeys, T. H.↗

Characterization of Artificial Guidestars Generated in the Mesospheric Sodium Layer

Using a 10 W average power sum-frequency laser, we have generated resonant fluorescence beacons in the mesospheric sodium layer and are currently evaluating them for use as an artificial guidestar for atmospheric compensation using adaptive optics. Two flashlamp pumped Nd:YAG lasers operating at 1.064 and 1.319 microns are mixed in a lithium triborate crystal to produce 589 nm light at 840 Hz. The laser emits 47.5 microsec mode-locked pulse trains at 11-14 mJ per pulse and is tuned to the sodium resonance transition with intracavity etalons.

Jelonek, M. P.↗

Digital single-sideband mixer.

Description of a simple single-sideband (SSB) mixer design that yields either a sum-frequency output with the difference-frequency output suppressed or vice-versa, and uses only 'digital' logic devices and no reactive or frequency-selective 'analog' (linear) circuit elements. A pair of outputs is generated in phase quadrature. It is shown that SSB frequency conversion can be accomplished for many applications much more efficiently with simple digital circuitry than in the usual way with complicated linear frequency selective filter and phasing circuits.

Counselman, C. C., III↗