Two-photon processes in the solar X-ray spectrum.
Two photon decay of metastable levels of hydrogenic and He-like ions in solar corona, depopulating via proton collisional excitation to 2p level
Smith, T. S.↗
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Computational study of alkali-metal-noble gas collisions in the presence of nonresonant lasers - Na + Xe + h/2/pi/omega sub 1 + h/2/pi/omega sub 2 system
The collision of Na with Xe in the presence of both the rhodamine-110 dye laser and the Nd-glass laser is investigated within a quantum-mechanical close-coupled formalism, utilizing ab initio potential curves and transition dipole matrix elements. Both one- and two-photon processes are investigated; the Na + Xe system is not asymptotically resonant with the radiation fields, so that these processes can only occur in the molecular collision region. The one-photon processes are found to have measurable cross sections at relatively low intensities; even the two-photon process has a significant section for field intensities as low as 10 MW/sq cm.
Devries, P. L.↗
Optical communication with two-photon coherent stages. I - Quantum-state propagation and quantum-noise reduction
To determine the ultimate performance limitations imposed by quantum effects, it is also essential to consider optimum quantum-state generation. Certain 'generalized' coherent states of the radiation field possess novel quantum noise characteristics that offer the potential for greatly improved optical communications. These states have been called two-photon coherent states because they can be generated, in principle, by stimulated two-photon processes. The use of two-photon coherent state (TCS) radiation in free-space optical communications is considered. A simple theory of quantum state propagation is developed. The theory provides the basis for representing the free-space channel in a quantum-mechanical form convenient for communication analysis. The new theory is applied to TCS radiation.
Yuen, H. P.↗
Theory of a two-photon laser
Equations for describing nonstationary processes in two-photon laser
LASER OUTPUT↗
Two-photon excitation of nitric oxide fluorescence as a temperature indicator in unsteady gasdynamic processes
A laser-induced fluorescence technique based on the pulsed two-photon excitation of NO is presented which is especially suited for the measurement of fluctuating temperatures in cold turbulent flows. The technique uses the fluorescence from the UV gamma bands of NO produced by two-photon excitation of NO (A 2 Sigma +, nu-prime = 0 - X 2 Pi, nu-double prime = 0) to obtain a rotational temperature. An analysis is presented of relevant aspects of the two-photon absorption process including microphysical processes, spectral intensities as a function of transition and laser spectral widths, line-shape integrals, the nonequilibrium response of the medium to a laser pulse, fluorescence energies, signal to noise ratio, and focusing effects. An analysis of absolute two-photon absorptivity measured in a nonflowing cell is then presented and used to predict signal to noise ratios greater than 50 for supersonic flows at temperatures below 300 K.
Mckenzie, R. L.↗
Infrared up-conversion with resonantly two-photon pumped metal vapors
Observation of efficient up-conversion of low-level IR radiation near 10 microns to the near ultraviolet. Radiation at 9.26 micron is converted to 3305 A with a photon conversion efficiency of 58% and a corresponding power gain of 16.2. The process employs resonant two-photon pumping of the nonallowed 3s-3d transition in Na.
Bloom, D. M.↗
Optical stark effect in the 2-photon spectrum of NO
A large optical Stark effect has been observed in the two-photon spectrum X(2)Pi yields A(2)Sigma(+)_ in NO. It is explained as a near-resonant process in which the upper state of the two-photon transition is perturbed by interactions with higher-lying electronic states coupled by the laser field. A theoretical analysis is presented along with coupling parameters determined from ab initio wave functions. The synthetic spectrum reproduces the major experimental features.
Huo, W. M.↗
Two-photon excitation of nitric oxide fluorescence as a temperature indicator in unsteady gas-dynamic processes
A laser induced fluorescence technique, suitable for measuring fluctuating temperatures in cold turbulent flows containing very low concentrations of nitric oxide is described. Temperatures below 300 K may be resolved with signal to noise ratios greater than 50 to 1 using high peak power, tunable dye lasers. The method relies on the two photon excitation of selected ro-vibronic transitions. The analysis includes the effects of fluorescence quenching and shows the technique to be effective at all densities below ambient. Signal to noise ratio estimates are based on a preliminary measurement of the two photon absorptivity for a selected rotational transition in the NO gamma (0,0) band.
Mckenzie, R. L.↗
A status of progress for the Laser Isotope Separation (LIS) process
An overview of the Laser Isotope Separation (LIS) methodology is given together with illustrations showing a simplified version of the LIS technique, an example of the two-photon photoionization category, and a diagram depicting how the energy levels of various isotope influence the LIS process. Applications were proposed for the LIS system which, in addition to enriching uranium, could in themselves develop into programs of tremendous scope and breadth. These include the treatment of radioactive wastes from light-water nuclear reactors, enriching the deuterium isotope to make heavy-water, and enriching the light isotopes of such elements as titanium for aerospace weight-reducing programs. Economic comparisons of the LIS methodology with the current method of gaseous diffusion indicate an overwhelming advantage; the laser process promises to be 1000 times more efficient. The technique could also be utilized in chemical reactions with the tuned laser serving as a universal catalyst to determine the speed and direction of a chemical reaction.
Delionback, L. M.↗
Atomic processes in astrophysics.
Studies of particle excitation processes in the solar corona are reviewed, covering electron affinities, negative ion experiments using two-photon laser and drift tube techniques, geometrical hindrance in molecular ion formation, negative ion-molecule reactions, and negative ions in the ionosphere and astrophysics. Aspects of forbidden atomic transitions are also discussed, including the calculation of transition probabilities, the Fe II problem, and magnetic quadrupole radiation in a relativistic approximation.
Garstang, R. H.↗
Formation of integrated optics components by multiphoton photorefractive processes
Phase holograms have been formed in pure outdiffused LiNbO3 waveguides using the photorefractive effect initiated by two-photon absorption. Efficient holograms were recorded with two guided waves, of less than 100 W peak power, and less than 10 microJ optical energy. This technique automatically compensates for wave front perturbations in the guide and allows the formation of various integrated components such as wavelength multiplexers and optical switches.
Verber, C. M.↗
Pair Production and Annihilation in Strong Magnetic Fields
Electromagnetic phenomena occurring in the presence of strong magnetic fields are currently of great interest in high-energy astrophysics. In particular, the process of pair production by single photons in the presence of fields of order 10 to the 12th power Gauss is of importance in cascade models of pulsar gamma ray emission, and may also become significant in theories of other radiation phenomena whose sources may be neutron stars (e.g., gamma ray bursts). In addition to pair production, the inverse process of pair annihilation is greatly affected by the presence of superstrong magnetic fields. The most significant departures from annihilation processes in free space are a reduction in the total rate for annihilation into two photons, a broadening of the familiar 511-keV line for annihilation at rest, and the possibility for annihilation into a single photon (which dominates the two-photon annihilation for B ( 10 the 13th power Gauss). The physics of these pair conversion processes, which is reviewed briefly, can become quite complex in the teragauss regime, and can involve calculations which are technically difficult to incorporate into models of emission mechanisms in neutron star magnetospheres. However, theoretical work, especially the case of pair annihilation, also suggests potential techniques for more direct measurements of field strengths near the stellar surface.
Daugherty, J. K.↗
Pair production and annihilation in strong magnetic fields
Electromagnetic phenomena occurring in the presence of strong magnetic fields are currently of great interest in high-energy astrophysics. In particular, the process of pair production by single photons in the presence of fields of order 10 to the 12th power Gauss is of importance in cascade models of pulsar gamma ray emission, and may also become significant in theories of other radiation phenomena whose sources may be neutron stars (e.g., gamma ray bursts). In addition to pair production, the inverse process of pair annihilation is greatly affected by the presence of superstrong magnetic fields. The most significant departures from annihilation processes in free space are a reduction in the total rate for annihilation into two photons, a broadening of the familiar 511-keV line for annihilation at rest, and the possibility for annihilation into a single photon which dominates the two-photon annihilation for B (10 to 13th power Gauss) The physics of these pair conversion processes, which is reviewed briefly, can become quite complex in the teragauss regime, and can involve calculations which are technically difficult to incorporate into models of emission mechanisms in neutron star magnetospheres. However, theoretical work, especially the case of pair annihilation, also suggests potential techniques for more direct measurements of field strengths near the stellar surface.
Daugherty, J. K.↗
Optical communication with two-photon coherent states. II - Photoemissive detection and structured receiver performance
In a previous paper (1978), the authors developed a method of analyzing the performance of two-photon coherent state (TCS) systems for free-space optical communications. General theorems permitting application of classical point process results to detection and estimation of signals in arbitrary quantum states were derived. The present paper examines the general problem of photoemissive detection statistics. On the basis of the photocounting theory of Kelley and Kleiner (1964) it is shown that for arbitrary pure state illumination, the resulting photocurrent is in general a self-exciting point process. The photocount statistics for first-order coherent fields reduce to those of a special class of Markov birth processes, which the authors term single-mode birth processes. These general results are applied to the structure of TCS radiation, and it is shown that the use of TCS radiation with direct or heterodyne detection results in minimal performance increments over comparable coherent-state systems. However, significant performance advantages are offered by use of TCS radiation with homodyne detection. The abstract quantum descriptions of homodyne and heterodyne detection are derived and a synthesis procedure for obtaining quantum measurements described by arbitrary TCS is given.
Shapiro, J. H.↗
Radiative cooling of a low-density plasma
The paper extends and improves the radiative cooling coefficient calculations of Cox and Tucker (1969) and Cox and Daltabuit (1971) for a low-density optically thin plasma with no molecules or dust, of cosmic abundances in the range from 10,000 to 100,000,000 K. Earlier rates applied to a plasma containing H, He, C, N, O, Ne, Mg, Si, and S; the present study added Ca, Fe, and Ni. For the elements included, many individual lines are calculated which previously has been averaged together. The cooling processes considered are permitted, forbidden, and semiforbidden line transitions, including contributions from dielectronic recombination and bremsstrahlung, radiative recombination, and two-photon continua. The ionization balance is calculated in collisional equilibrium using an approximate auto-ionization following inner-shell excitation and the low-density limit for the dielectronic recombination rate. Cooling in various observational bands in the soft X-ray region is determined.
Raymond, J. C.↗
Pair annihilation in superstrong magnetic fields
The kinematical and dynamical aspects of the annihilation processes in superstrong magnetic fields are studied. The feasibility and potential significance of detecting from magnetic neutron stars are discussed. The discussion proceeds from the derivation of the fully relativistic differential cross sections and annihilation rates for both one- and two-photon emission from a ground-state gas of electrons and positrons in a static, uniform magnetic field.
Daugherty, J. K.↗
Equilibria in Strongly Magnetized Pair Plasmas
Positron-electron pair densities for a thermal plasma in the steady-state equilibrium where pair production balances pair annihilation are found as a function of temperature kT / mc(2) approx. 1, source size R and magnetic field strength B. When the plasma is strongly magnetized, B 10(12) G, the important processes are synchrotron radiation, one-photon (magnetic) pair production and two-photon pair annihilation. An analytic solution for the equilibrium pair density, found under certain simplifying assumptions, shows that optically thin equilibria exist only for sufficiently small source sizes.
Harding, A. K.↗
Pair production rates in mildly relativistic, magnetized plasmas
Electron-positron pairs may be produced by either one or two photons in the presence of a strong magnetic field. In magnetized plasmas with temperatures kT approximately sq mc, both of these processes may be important and could be competitive. The rates of one-photon and two-photon pair production by photons with Maxwellian, thermal bremsstrahlung, thermal synchrotron and power law spectra are calculated as a function of temperature or power law index and field strength. This allows a comparison of the two rates and a determination of the conditions under which each process may be a significant source of pairs in astrophysical plasmas. It is found that for photon densities n(gamma) or = 10 to the 25th power/cu cm and magnetic field strengths B or = 10 to the 12th power G, one-photon pair production dominates at kT approximately sq mc for a Maxwellian, at kT approximately 2 sq mc for a thermal bremsstrahlung spectrum, at all temperatures for a thermal synchrotron spectrum, and for power law spectra with indices s approximately 4.
Burns, M. L.↗