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Thompson, N.

Publications and source records attributed to Thompson, N..

Measurements of K-edge and L-edge extended x-ray absorption fine structure at the national ignition facility (invited)

High-energy-density laser facilities and advances in dynamic compression techniques have expanded access to material states in the Terapascal regime relevant to inertial confinement fusion, planetary science, and geophysics. However, experimentally determining the material temperature in these extreme conditions has remained a difficult challenge. Extended X-ray Absorption Fine Structure (EXAFS), referring to the modulations in x-ray absorption above an absorption edge from photoelectrons’ interactions with neighboring atoms, has proven to be a versatile and robust technique for probing material temperature and density for mid-to-high Z elements under dynamic compression. The current platform at the National Ignition Facility has developed six configurations for EXAFS measurements between 7 and 18 keV for different absorption edges (Fe K, Co K, Cu K, Ta L3, Pb L3, and Zr K) using a curved-crystal spectrometer and a bright, continuum foil x-ray source. Here, in this work, we describe the platform geometry, x-ray source performance, spectrometer resolution and throughput, design considerations, and data in ambient and dynamic-compression conditions.

36 MATERIALS SCIENCE↗

How to Safely Build 100-plus Kilograms of Weapons-Grade Plutonium

The goal of the EUCLID (Experiments Underpinned by Computational Learning for Improvements in Nuclear Data) project was to reduce compensating errors by utilizing machine learning to both help determine which reactions contain compensating errors as well as optimizing an experiment which can be used to maximally reduce these errors. Compensating errors can adversely impact the predictive power of application simulations, and therefore it’s useful to further constrain nuclear data and reduce these errors. The EUCLID project included building two configurations at the National Criticality Experiments Research Center (NCERC). These two configurations had very different geometries (one was cube-like and one was slab-like). Previous works focus on selection of the target experiment(s), radiation transport capabilities developed in the project, the experiment optimization, and the performance of the experiments. This work will focus only on the safety aspects of performing this experiment, which utilized over 100 kg of weapons-grade plutonium.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Neutron Noise Analysis of the Neptunium Subcritical Observation (NESO) Experiment

The Neptunium Subcritical Observation (NeSO) experiment was a subcritical integral benchmark experiment. This experiment was designed in 2017-2018 and was performed at the National Criticality Experiments Research Center (NCERC) in 2019. Eight different subcritical configurations were measured with varying Nickel reflector thickness. For all configurations, a 3 He detection system was used to record neutron events. The focus of this work is to share neutron noise results of the measured data.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Neutron Noise Analysis of the Neptunium Subcritical Observation (NESO) Experiment

The Neptunium Subcritical Observation (NeSO) experiment was a subcritical integral benchmark experiment. This experiment was designed in 2017-2018 and was performed at the National Criticality Experiments Research Center (NCERC) in 2019. Eight different subcritical configurations were measured with varying Nickel reflector thickness. For all configurations, a 3 He detection system was used to record neutron events. The focus of this work is to share neutron noise results of the measured data.

3-Helium↗

Empirical Bounding Analysis and User Recommendations for a Neutron Multiplicity Detector

Neutron multiplicity detectors are useful for a variety of applications including nuclear emergency response, nuclear nonproliferation, safeguards, and criticality safety. When measuring black-box problems (i.e., when the system being measured is completely unknown) with systems that have relatively low detection efficiency, expert analysis is frequently required to determine appropriate bounds for system parameters such as neutron multiplication and neutron leakage. This is because the detection efficiency can vary wildly, which also means that the resulting system parameters can have large variations. This work applies an empirical approach to provide bounds on system parameters (such as system multiplication, neutron leakage, and detector efficiency). The results of this bounding analysis are then used as inputs to provide recommendations to users regarding criticality safety. In addition to describing the method used, this work provides sample results from a measurement campaign performed at the National Criticality Experiments Research Center (NCERC).

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Zirconium Scattering Sensitivity in Neutron Transport Calculations of Multiplying Systems [Slides]

This presentation touches on motivation and applications of Zirconium. Performance of evaluated libraries on double and quasi differential experiments is considered. Additionally, the performance of evaluated libraries in select ICSBEP benchmarks is considered. Provided is a detailed look in the performance of evaluated libraries in preliminary benchmark configurations for IER-516: Zirconium Test Assembly (ZTA). Conclusions and recommended experiments to satisfy Zirconium scattering nuclear data needs are presented.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Criticality Experiments to Reduce Compensating Errors in Plutonium Nuclear Data

Compensating errors between nuclear data observables in a library can adversely impact application simulations. The primary goal of the EUCLID project (Experiments Underpinned by Computational Learning for Improvements in Nuclear Data) is to reduce compensating errors in nuclear data. A new criticality experiment, described in this work, was designed with the specific target nuclear data of 239 Pu fission, inelastic scattering, elastic scattering, capture, nu-bar, and prompt fission neutron spectrum (PFNS). This work will focus on the design and execution of the EUCLID experiment, performed on the Planet vertical lift critical assembly machine at the National Criticality Experiments Research Center (NCERC). The criticality experiment includes two different configurations with very different geometries: one is cube-like to minimize neutron leakage while the other is slab-like to maximize leakage. Having these two widely varying configurations allows the scattering sensitivities of 239 Pu to the neutron multiplication factor to be greatly changed while minimally impacting the other cross section sensitivities. Both configurations utilize the Pu ZPPR (Zero Power Physics Reactor) plates as fuel. The experiments were designed using a D-Optimality criteria, which is an optimization method minimizing the log-determinant of the adjusted nuclear data covariance for the target reactions. These experiments include not only inference of k eff , as done in all critical benchmark experiments, but several other responses as well, such as neutron multiplication measurements and reaction rate ratios. After analysis of the measured data is complete, adjustment of nuclear data will be performed to assess whether the new experimental data successfully reduced compensating errors.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Reactivity Coefficient Measurements to Aid in Reducing Compensating Errors in Plutonium Nuclear Data

Compensating errors between several nuclear data observables in a nuclear data library can adversely impact application simulations. The primary goal of the EUCLID project (Experiments Underpinned by Computational Learning for Improvements in Nuclear Data) is to reduce compensating errors between fast (0.1–5 MeV) 239Pu nuclear data for prompt fission neutron spectra (PFNS), average prompt fission neutron multiplicities, and neutron induced fission, capture, elastic, and inelastic cross sections. This work will focus on the design and execution of void reactivity coefficient measurements in the EUCLID experiment, performed on the Planet vertical lift critical assembly machine at the National Criticality Experiments Research Center (NCERC). Two different base configurations were designed and measured, one with high neutron leakage, and one with low neutron leakage. Both were primarily made up of plutonium metal (Zero Power Physics Reactor plates) without interstitial moderators and reflected by half-inch aluminum. Design optimization showed that void reactivity coefficient measurements in three locations per configuration was most impactful to reduce nuclear data uncertainties due to the varying impacts from elastic and inelastic scattering, as well as fission and capture. The locations for measurements were chosen based on preliminary studies which balanced measurement uncertainty and measurement practicality. The measurements were also selected to have sensitivities maximally complementary to previous arrangements. Comparisons across nuclear data libraries highlight the potential impact.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗