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DOE OSTI2025

Tuning of electronic properties in highly lattice-mismatched epitaxial SmN

Here, we establish the relationship between native N vacancies, introduced through varying growth parameters, and the structural and transport properties in SmN thin films grown via molecular beam epitaxy grown on MgO(001). The varying levels of N vacancies introduced by varying the ratio of Sm to N atoms during deposition creates excess carriers that radically transform the electrical behavior of the film, over a range of five orders of magnitude, from highly resistive to highly conductive, and unlocking a phase transition evidenced by the presence of a ferromagnetic feature in resistivity. X-ray photoelectron spectroscopy results show that this effect is much less pronounced when varying the available nitrogen species. These samples retain a highly crystal quality despite being grown on a substrate with a lattice mismatch of 20%, alleviating the strain by forming a highly strained SmO oxide layer. The integration between SmN and several transition metal nitride compounds has the potential to unlock new architectures for Josephson junction devices.

36 - MATERIALS SCIENCE↗

DOE OSTI2026

Coupling of Klein-Andreev resonant states in B⁢i 2 ⁢S⁢r 2 ⁢CaC⁢u 2 ⁢O 8+𝑥 -graphene-B⁢i 2⁢ S⁢r 2 ⁢CaC⁢u 2 ⁢O 8+𝑥 devices

Quantum devices require coherent coupling over macroscopic distances. Recently, resonances due to Klein tunneling and Andreev reflection states (KARS) have been observed in a naturally occurring p-n junction at the interface between B⁢i 2 ⁢S⁢r 2 ⁢CaC⁢u 2 ⁢O 8+𝑥 (BSCCO), a high−⁢𝑇 c superconductor (HTS), and graphene. The resonances appear as conductance oscillations with gating. Here, in this study, we show coupling between the KARS in BSCCO-graphene-BSCCO devices of varying separation (L). The coupling is evidenced by a power-law decay of resonance period as L increases from tens of nanometers to microns. These results demonstrate the long-distance coupling of KARS cavities in graphene-HTS junctions. The length dependence seen in experiments is supported by single-particle spectral functions which show KARS are coupled by transport modes in graphene. The strong coupling between KARS in BSCCO-graphene-BSCCO devices showcases the possibility of HTS-graphene junctions for quantum circuits and unconventional Josephson junctions.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

DOE OSTI2024

Performance analysis of superconductor-constriction-superconductor transmon qubits

Here, this work presents a computational analysis of a superconducting transmon qubit design, in which the superconductor-insulator-superconductor (SIS) Josephson junction is replaced by a coplanar, superconductor-constriction-superconductor (ScS) nanobridge junction. Within the scope of Ginzburg-Landau theory, we find that the nanobridge ScS transmon has an improved charge dispersion compared to the SIS transmon, with a tradeoff of smaller anharmonicity. These calculations provide a framework for estimating the superconductor material properties and junction dimensions compatible with gigahertz frequency ScS transmon operation.

36 MATERIALS SCIENCE↗

DOE OSTI2024

Nonlinear inductive response of pinned superconducting vortices in artificial pinning sites

Using the time dependent Ginzburg-Landau equations, we simulate the inductive responses of a variety of thin-film systems containing patterned antidots with different sizes and shapes. The results for all shapes show that the kinetic inductance diverges as the applied current approaches a critical current that is below the BCS depairing current. In conclusion, exploiting the similarity of the observed current-voltage behavior to that of Josephson junctions, we obtain an empirical equation that well fits the inductivity curve as a function of the applied current.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

DOE OSTI2025

Improved receiver noise calibration for ADMX axion search: 4.54 to 5.41 μeV

Axions are a well-motivated candidate for dark matter. The preeminent method to search for axion dark matter is known as the axion haloscope, which makes use of the conversion of axions to photons in a large magnetic field. Because of the weak coupling of axions to photons, however, the expected signal strength is exceptionally small. To increase signal strength, many haloscopes make use of resonant enhancement and high gain amplifiers, while also taking measures to keep receiver noise as low as possible such as the use of dilution refrigerators and ultra-low-noise electronics. In this paper, we derive the theoretical noise model based on the sources of noise found within a typical axion haloscope receiver chain, using the Axion Dark Matter eXperiment (ADMX) as a case study. We present examples of different noise calibration measurements at 1280 MHz taken during ADMX’s most recent data-taking run. These new results shed light on a previously unidentified interaction between the cavity and Josephson Parametric Amplifier as well as provide a better understanding of the systematic uncertainty on the system noise temperature used in the axion search analysis for this data-taking run. Finally, the consistency between the measurements and the detailed model provide suggestions for future improvements within ADMX and other axion haloscopes to reach a lower noise temperature.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2025

ADMX Axion Dark Matter Bounds around 3.3 μ eV with Dine-Fischler-Srednicki-Zhitnitsky Discovery Ability

We report the results of a QCD axion dark matter search with discovery ability for Dine-Fischler-Srednicki-Zhitnitsky (DFSZ) axions using an axion haloscope. Sub-Kelvin noise temperatures are reached with an ultralow noise Josephson parametric amplifier cooled by a dilution refrigerator. This work excludes (with a 90% confidence level) DFSZ axions with masses between 3.27 to 3.34 μ eV , assuming a standard halo model with a local energy density of 0.45 G e V / cm 3 made up 100% of axions. Published by the American Physical Society 2025

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2024

Dephasing in Fluxonium Qubits from Coherent Quantum Phase Slips

Phase slips occur across all Josephson junctions (JJs) at a rate that increases with the impedance of the junction. In superconducting qubits composed of JJ-array superinductors—such as fluxonium—phase slips in the array can lead to decoherence. In particular, phase-slip processes at the individual array junctions can coherently interfere, each with an Aharonov-Casher phase that depends on the offset charges of the array islands. These coherent quantum phase slips (CQPS) perturbatively modify the qubit frequency, and therefore charge noise on the array islands will lead to dephasing. By varying the impedance of the array junctions, we design a set of fluxonium qubits in which the expected phase-slip rate within the JJ array changes by several orders of magnitude. We characterize the coherence times of these qubits and demonstrate that the scaling of CQPS-induced dephasing rates agrees with our theoretical model. Furthermore, we perform noise spectroscopy of two qubits in regimes dominated by either CQPS or flux noise. We find that the noise power spectrum associated with CQPS dephasing appears to be featureless at low frequencies and not 1 / f . Numerical simulations indicate that this behavior is consistent with charge noise generated by charge-parity fluctuations within the array. Our findings broadly inform JJ-array-design trade-offs, relevant for the numerous superconducting-qubit designs employing JJ-array superinductors. Published by the American Physical Society 2024

Physics↗

DOE OSTI2026

Advancements in NbTiN based circuits for Superconducting Digital Logic

Superconducting (SC) electronics have emerged as a promising platform for high-speed, energy-efficient computing and quantum information processing. This work, centered on NbTiN, presents recent advances in material science and fabrication methods leading to significant improvements in performance, scalability and vertical integration. We specifically report on fabrication and characterization of key components, including Josephson junctions (JJs), flux trapping structures and SC interconnects. Together, these efforts represent critical steps towards realizing practical, complex, dense and large-scale SC integrated circuits.

Pokhrel, A. [Imec,Heverlee,Belgium]↗

DOE OSTI2025

Anomalous superconductivity in twisted MoTe 2 nanojunctions

Introducing superconductivity in topological materials can lead to innovative electronic phases and device functionalities. Here, we present a unique strategy for quantum engineering of superconducting junctions in moiré materials through direct, on-chip, and fully encapsulated 2D crystal growth. We achieve robust and designable superconductivity in Pd-metalized twisted bilayer molybdenum ditelluride (MoTe 2 ) and observe anomalous superconducting effects in high-quality junctions across ~20 moiré cells. Unexpectedly, the junction develops enhanced, instead of weakened, superconducting behaviors, exhibiting fluctuations to a higher critical magnetic field compared to its adjacent Pd 7 MoTe 2 superconductor. In addition, the critical current further exhibits a notable V-shaped minimum at zero magnetic field. These features are unexpected in conventional Josephson junctions and absent in junctions of natural bilayer MoTe 2 created using the same approach. We discuss implications of these observations, including the possible formation of mixed even- and odd-parity superconductivity at the moiré junctions. Our results also demonstrate a pathway to engineer and investigate superconductivity in fractional Chern insulators.

Science & Technology - Other Topics↗

DOE OSTI2025

Zero-bias conductance peaks at zero applied magnetic field due to stray fields from integrated micromagnets in hybrid nanowire quantum dots

Many recipes for realizing topological superconductivity rely on broken time-reversal symmetry, which is often attained by applying a substantial external magnetic field. Alternatively, using magnetic materials can offer advantages through low-field operation and design flexibility on the nanoscale. Mechanisms for lifting spin degeneracy include exchange coupling, spin-dependent scattering, spin injection – all requiring direct contact between the bulk or induced superconductor and a magnetic material. Here, we implement locally broken time-reversal symmetry through dipolar coupling from nearby micromagnets to superconductor-semiconductor hybrid nanowire devices. Josephson supercurrent is hysteretic due to micromagnets switching. At or around zero external magnetic field, we observe an extended presence of Andreev bound states near zero voltage bias. We also show a zero-bias peak plateau of a non-quantized value. Our findings largely reproduce earlier results where similar effects were presented in the context of topological superconductivity in a homogeneous wire, and attributed to more exotic time-reversal breaking mechanisms [Nat. Phys. 17, 43 (2020)]. In contrast, our stray field profiles are not designed to create Majorana modes, and our data are compatible with a straightforward interpretation in terms of trivial states in quantum dots. At the same time, the use of micromagnets in hybrid superconductor-semiconductor devices shows promise for future experiments on topological superconductivity.

Jiang, Luyao [Univ. of Pittsburgh, PA (United Stat↗

DOE OSTI2024

Design, Control and Application of Next Generation Qubits

Design, Control and Application of Next Generation Qubits Arun Bansil, Northeastern University (Principal Investigator) Claudio Chamon, Boston University (Co-Investigator) Adrian Feiguin, Northeastern University (Co-Investigator) Liang Fu, MIT (Co-Investigator) Eduardo Mucciolo, Univ. of Central Florida (Co-Investigator) Qimin Yan, Temple University (Co-Investigator) The quest for developing technologies for manipulating and storing information quantum mechanically is currently led by approaches that include Josephson-junctions, ion-traps, and qubits generated by defect spins in solids. Topological qubits, however, are inherently more robust to decoherence by environmental effects, and should be able to sprint ahead once practical barriers have been overcome. At the present stage of the development of the field, it is important to explore a variety of architectures and materials beyond the conventional paradigms in order to seed breakthroughs toward building a scalable quantum computer. Our comprehensive theoretical research program involved four interconnected thrusts as follows. • A materials discovery effort in two-dimensional compounds in search of materials to support Majorana zero modes and defect structures suitable as qubits. • Exploration of architectures for topological quantum computation by investigating both superconducting Majorana qubits, and robust platforms for braiding with new “meta-materials” built of arrays of Majorana qubits. • Investigation of properties of hybrid metal-organic qubits based on transition-metal centers in graphene, and molecular crystals of polyaromatic complexes with embedded transition-metal atoms. • Development of tensor-network and semiclassical approaches to study decoherence in the presence of random and dispersive spin baths, and NV centers in diamond. The full spectrum of theoretical and numerical approaches was used to address the goals of this project including first-principles, density-matrix-renormalization group, tensor networks, and data-driven high-throughput approaches using materials database and machine-learning.

36 MATERIALS SCIENCE↗

DOE OSTI2024

Investigation of cosmic ray impact on transmon qubits with different materials through fast decay detection at Fermilab’s SQMS laboratory

Noise sources affecting superconducting qubits, such as cosmic rays and ambient gamma radiation, have garnered attention for their potential impact. These radiations deposit energy in the qubit's substrate, generating high-energy phonons that break Cooper pairs, leading to the formation of quasi-particles. When these quasi-particles tunnel across Josephson junctions, they induce qubit de-excitation, causing relaxation errors. In this study, we employ a fast feedback mechanism for performing qubit reset to detect decay events with high time resolution. This capability along with frequency multiplexed readout allows us to explore error correlations across time and space. Transmon qubits, manufactured within the Superconducting Quantum Materials and Systems (SQMS) center [1], are investigated at the above-ground lab. We study the impact of cosmic rays on qubits with different encapsulations, geometries, and locations on the same or different chips. We present preliminary findings and discuss the implications for the performance of contemporary quantum hardware.

Roy, Tanay↗

DOE OSTI2024

SQMS science advances impact on Rigetti commercial processors

The collaboration between the Superconducting Quantum Materials and Systems Center (SQMS) and Rigetti Computing produced several advancements in our understanding of the role of materials characteristics in quantum processor performance. This partnership leverages SQMS's extensive characterization infrastructure and cutting-edge research in materials, and Rigetti's expertise in quantum hardware and robust nanofabrication to improve precision and performance of Rigetti's test QPUs. Qubit frequency is determined in large part by the properties of Josephson junctions (JJs) made of amorphous oxide tunnel barriers; the Alternating-Bias Assisted Annealing (ABAA) process allows us to tune JJs to their desired frequency [1]. Work by SQMS researchers in characterizing high-precision JJs post-processed (using ABAA) have yielded crucial information on the nature of the structure and chemical bonding uniformity of the ABAA processed amorphous oxides. Performance has also been improved through a comprehensive series of experiments that tested encapsulation and surface treatment. Encapsulation of the niobium metal layer with tantalum resulted in an T1 improvement of 80%, experimentally confirming the role of Nb surface losses in qubit performance [2]. Pre-treatment of the underlying silicon surface prior to JJ fabrication by replacing a buffered oxide etch (BOE) with hydrofluoric acid (HF) followed by aqueous ammonium fluoride (NH4F) has shown a statistically significant improvement of T1 by 22%, and reduction in the number of strongly-coupled TLS [3]. These examples, as well as many other published and ongoing investigations, demonstrate the mutual benefits that come from Rigetti's involvement in the SQMS collaboration. [1] - Pappas, D.P., et al. (2024). https://doi.org/10.1038/s43246-024-00596-z [2] - Bal, M., et al. (2024). https://doi.org/10.1038/s41534-024-00840-x [3] Kopas, C. J. et al. Preprint at https://doi.org/10.48550/arXiv.2408.02863 (2024).

Lachman, Ella↗

DOE OSTI2024

Quantum sensing for fundamental physics efforts at SQMS

One of the areas of research of the Superconducting Quantum Systems and Materials (SQMS) center is the application of quantum sensing to fundamental physics searches, demonstrating that quantum sensors can greatly improve the sensitivity of experiments searching for Beyond the Standard Model (BSM) physics, or performing high-precision measurements. Theorists have developed many ideas for BSM physics that would result in interactions that can in principle be detected, but with signals small enough that they haven t been observed yet. In this field, the capability to lower the detector s thermal noise to few or dozens of mK, and to use QIS technologies such as Josephson Parametric Amplifiers and photon counters (in-situ or itinerant) enable us to reach unprecedented sensitivities and faster scan rates. Here is presented an overview of the quantum sensing efforts at SQMS [1], focusing on theoretical advancements and experimental searches for Dark Sector particles (as dark matter candidates and not), gravitational waves, and precision measurements. The experiments conducted, or under preparation, include axion dark matter (DM) [2, 3], dark photon DM searches [4,5], light-shining-through-wall experiments [6], cavity-based searches for high frequency gravitational waves [7], and measurements of the electron magnetic moment [8]. [1] Berlin, A., et al. "Searches for new particles, dark matter, and gravitational waves with SRF cavities." arXiv preprint arXiv:2203.12714 (2022). [2] Giaccone, B., et al. "Design of axion and axion dark matter searches based on ultra high Q SRF cavities." arXiv preprint arXiv:2207.11346 (2022). [3] Braggio, C., et al. "Quantum-enhanced sensing of axion dark matter with a transmon-based single microwave photon counter." arXiv preprint arXiv:2403.02321 (2024). [4] Fan, X., et al. "One-electron quantum cyclotron as a milli-eV dark-photon detector." Physical review letters 129.26 (2022): 261801. [5] Cervantes, R., et al. "Deepest sensitivity to wavelike dark photon dark matter with superconducting radio frequency cavities." Physical Review D 110.4 (2024): 043022. [6] Romanenko, A., et al. "Search for dark photons with superconducting radio frequency cavities." Physical review letters 130.26 (2023): 261801. [7] Berlin, A., et al. "Electromagnetic cavities as mechanical bars for gravitational waves." Physical Review D 108.8 (2023): 084058. [8] Fan, X., et al. "Measurement of the electron magnetic moment." Physical review letters 130.7 (2023): 071801.

Giaccone, Bianca↗

DOE OSTI2024

Material and Interface Engineering Strategies to Mitigate Decoherence in Superconducting Qubits

While significant strides have been made to increase the coherence time of superconducting qubits, further advancements are essential for realizing scalable quantum computing. Decoherence is often a result of loss and noise stemming from two-level systems and excess quasiparticles, arising due to material defects, fabrication processes, and ambient exposure, particularly at surfaces and interfaces. Our recent efforts to mitigate these decoherence mechanisms have employed a variety of strategies, including low-loss surface encapsulation materials, advanced substrate preparation techniques, modifications to metal film growth, and the development of novel fabrication processes. The structural and chemical properties of materials, surfaces, and interfaces are studied using scanning probe microscopy, electron microscopy, photoelectron spectroscopy, mass spectrometry, and X-ray diffraction, which is correlated to device performance metrics, including superconducting resonator internal quality factor and qubit T1 time. This information is used to identify and understand material sources of loss and their origins in the device fabrication process. Through multi-institution efforts within SQMS we have identified the loss mechanism of interstitial hydrogen in niobium-based devices and shown how standard fabrication processes introduce these hydrides, developing strategies to mitigate their formation.1 Furthermore, we have characterized the metal-substrate interface, including the loss of niobium-silicides formed at that interface, and developed silicon surface treatments that reduce atomic scale roughness and oxygen content at the metal-substrate and Josephson junction interfaces.2-4 By developing the connection between materials properties and the overall performance of superconducting quantum circuitry, we can develop fabrication strategies to mitigate material losses, thus supporting the ongoing efforts to enhance coherence time in superconducting quantum devices. 1. Torres-Castanedo, C. G.*, Goronzy, D. P.*, et al., Adv. Funct. Mater., 2401365 (2024) 2. Lu, X., et al., Phys. Rev. Materials 6, 064402 (2022) 3. Berti, G., Appl. Phys. Lett. 122, 192605 (2023) 4. Kopas, C. J., Goronzy, D. P., et al., arXiv:2408.02863 (2024)

Goronzy, Dominic P.↗

DOE OSTI2024

SQMS Nanofabrication Taskforce: Towards Fabrication of High Coherence Superconducting Qubits

SQMS Nanofabrication Taskforce, which brings together experts in nanofabrication and materials science at the SQMS Center, has been launched to implement novel materials, substrates, and fabrication techniques for high coherence superconducting quantum devices. In a first coordinated effort, the Nanofabrication Taskforce developed fabrication processes to eliminate the lossy materials at surfaces and interfaces of superconducting qubits to enhance qubit coherence. The initial results of this study demonstrated T1 enhancement by almost an order of magnitude with best T1 s reaching ~ 600 $\mu$s. [1] We attribute this improvement to the replacement of lossy native Nb oxide layer with native Ta oxide, which is thinner and less disordered. we are now currently working on strategies with an aim towards moving qubit coherence times to millisecond timescales and beyond. The results of a systematic study will be presented to address substrate preparation, alternative materials as low loss platforms (Nb, Ta, and Re), novel non-oxide forming low loss capping layers such as proximitized Au, optimized qubit designs, and optimized Josephson junction materials, processing, and design.

Bal, Mustafa↗

DOE OSTI2024

Qubit-Based Detector For Dark Matter Search And Radiation Studies

One of the challenges in exploring promising novel materials for dark matter searches is the detection of sub-eV energy excitations from light-dark matter interaction with a target material. Dark matter interaction can excite sub-eV optical phonon modes in polar materials like sapphire. We plan to utilize superconducting qubits on a sapphire substrate to study their response to energy deposition into the superconducting film and the substrate by irradiating them with photons and particles and also generating phonons in the chip. A fraction of the incident energy is expected to break Cooper pairs in the superconductor, releasing quasiparticles. As the quasiparticles tunnel across the Josephson junction, the charge parity of the qubit changes. The parity switching rate is proportional to the quasiparticle density in the qubit superconductor film and can be measured using standard qubit readout protocol. This presentation describes our ongoing attempt to build such a prototype detector.

Khatiwada, Rakshya↗

DOE OSTI2025

Comparative Study of Quasi-Particle Burst Events in Transmon Qubits made with Different Materials and Geometries

Superconducting qubits are susceptible to various noise sources, including cosmic rays. ambient gamma and infrared radiation, which can significantly impact their performance. High-energy radiations deposit energy into the qubit substrate, generating high-energy phonons that disrupt Cooper pairs and create quasi-particles (QPs). Infrared photons, on the other hand can directly create QPs. The tunneling of these quasi-particles across Josephson junctions leads to qubit de-excitation and causes relaxation errors. In this study, we utilize a fast feedback mechanism for qubit reset to detect QP burst events with high time resolution [1]. We investigate transmon qubits fabricated with different encapsulations [2], geometries, and substrates at the above-ground laboratory of the Superconducting Quantum Materials and Systems (SQMS) center at Fermilab. Our preliminary results are presented, with discussions on their implications for the performance of modern quantum hardware. [1] Dominicis and Roy et al.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗