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At least 181 records · Page 10

Method for calculating radon activity and radon rejection using a beta-gamma detector

Radon interferes with concentration measurements used by atmospheric radioxenon systems. We demonstrate a method to quantify the amount of radon that is present in the detectors, the impact of radon activity on the minimum-detectable-concentrations, and how to determine the needed radon rejection levels. An example calculation shows a radon rejection level of 10 5 is sufficient to limit impact on the detector sensitivity. We anticipate this method will give analysist a better understanding of radon present in their measurements and allow system designers to tailor their systems’ radon rejection better for its location.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗

An all-digital associated particle imaging system for the 3D determination of isotopic distributions

Associated particle imaging (API) is a non-destructive nuclear technique for the 3D determination of isotopic distributions. By detecting the alpha particle associated with the emitted neutron in the deuterium–tritium fusion reaction with a position- and time-resolving detector, the direction of the 14.1 MeV neutron and its time of emission can be determined. Employing this method, isotope characteristic gamma rays emitted in inelastic neutron scattering events can be correlated with the neutron interaction location. Here, an API system consisting of a sealed-type neutron generator, gamma detectors, and a position-sensitive alpha detector was designed, constructed, and characterized. The system was tested with common soil elements and shown to be sensitive to 12 C, 16 O, 28 Si, 27 Al, and 56 Fe. New aspects of our approach are the use of a yttrium–aluminum–perovskite scintillator, using a sapphire window instead of a fiber-optic faceplate for light transport to the photomultiplier, and the all-digital data acquisition system. We present a description of the system with simulations and experimental results that show a position resolution on the alpha detector of 1 mm, a depth resolution using a LaBr 3 detector of 6.2 cm, and an angular resolution of 4.5°. Additionally, we present single-element gamma response measurements for the elements mentioned above together with a comparison to Monte Carlo simulations (MCNP6).

47 OTHER INSTRUMENTATION↗

A telescope for high energy gamma-ray measurements in the Space Station era

This paper describes the concept of a large gamma-ray imaging telescope system (GRITS) which will provide sufficient sensitivity for the identification of faint objects to be catalogued by the Gamma-Ray Observatory. The technique used in this telescope for the detection of gamma rays is based on the conversion of the incident gamma ray into an electron-positron pair which subsequently produces Cherenkov radiation. The gamma ray is identified by a unique signature based on a sequence of time-delayed coincidence events. The GRITS telescope will use the extended Shuttle external tank, ET, as the pressure vessel necessary for the gas-Cherenkov process. Astronauts from the Shuttle or the Space Station performing EVA will convert ET to an autonomous spacecraft and install the telescope inside the ET.

Koch, David G.↗

Neutron capture-induced nuclear recoils as background for CE$v$⁢NS measurements at reactors

Nuclear reactors represent a promising neutrino source for CE⁢v⁢NS (coherent-elastic neutrino-nucleus scattering) searches. However, reactor sites also come with high ambient neutron flux. Neutron capture-induced nuclear recoils can create a spectrum that strongly overlaps the CEv⁢NS signal for recoils ≲100 eV for nuclear reactor measurements in silicon or germanium detectors. This background can be particularly critical for low-power research reactors providing a moderate neutrino flux. Here, in this work we quantify the impact of this background and show that, for a measurement 10 m from a 1 MW reactor, the effective thermal neutron flux should be kept below ~7 × 10 –4 ⁢n/cm 2 s so that the CE⁢v⁢NS events can be measured at least at a 5⁢σ level with germanium detectors in 100 kg yr exposure time. This flux corresponds to 60% of the sea-level flux but needs to be achieved in a nominally high-flux (reactor) environment. Improved detector resolution can help the measurements, but the thermal flux is the key parameter for the sensitivity of the experiment. For silicon detectors, the constraint is even stronger and thermal neutron fluxes must be near an order of magnitude lower. This constraint highlights the need of an effective thermal neutron mitigation strategy for future low threshold CEv⁢NS searches. In particular, the neutron capture-induced background can be efficiently reduced by active veto systems tagging the deexcitation gamma following the capture.

79 ASTRONOMY AND ASTROPHYSICS↗

Modernization of the Radiation Measurements Laboratory at the Advanced Test Reactor Complex

The Advanced Test Reactor (ATR) at the Idaho National Laboratory (INL) is a unique, water-cooled, high-flux test reactor capable of performing tests prototypical of PWR operating conditions. The Radiation Measurements Laboratory (RML) was founded in the 1960s to support reactor operations and to conduct independent scientific research. For nearly six decades RML has performed four primary functions: monitoring of radioactivity by gamma-ray spectroscopy of routine reactor samples, fluence rate determinations for irradiation cycles, fission-rate measurements for the ATR-Critical (ATR-C) Facility, and independent research and development of radiation detection systems and applications. Through the decades, RML has seen technological advancements that have been integrated into each of the critical functions of the laboratory. However, many of the measurement and analysis systems employed to this day can be improved by modernization. Recent progress at RML is improving reliability and accuracy of the radiation measurements performed in support of nuclear energy research for the U.S.A. Department of Energy. The control and data collection systems supporting ATR-C have been upgraded. New High-Purity Germanium (HPGe) spectrometers have been procured with liquid nitrogen recycling capabilities to improve up-time and reduce measurement uncertainties. Fluence-rate measurement techniques are also being improved to ensure accuracy, avoid systemic errors, and identify biases. In a parallel effort, new scientific research avenues are being explored which will provide an opportunity to further enhance the utilization of ATR and ensure the sustainability of the RML as nuclear research continues to evolve. The RML is improving the effectiveness of irradiation services provided by ATR while ensuring a sustainable future for nuclear energy research.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Development and validation of a software for simulating γ-γ coincidence emission and detection probabilities

Gamma-gamma coincidence spectrometers have the potential to significantly enhance detection sensitivity for ultra-trace radionuclide measurements. The implementation of these spectrometers, however, is limited by the complexity of acquisition hardware, data processing and quantification. This work reports development of a novel radionuclide quantification software for γ-γ coincidence measurements. For any radionuclide, the software parses the Evaluated Nuclear Structure Data File (ENSDF) database, recursively simulating all possible γ-γ coincidence signatures and their respective emission and detection probabilities. Implemented using Python programming language, the software employs several strategies to boost overall computational performance. Since coincidence-based spectrometers are of notable interest in monitoring compliance for the Comprehensive Nuclear-Test-Ban Treaty (CTBT), the software’s execution was tested for 84 CTBT-relevant radionuclides. To date, the software has been experimentally validated for 15 radionuclides using the Advanced Radionuclide Gamma spectrOmeter (ARGO) at Pacific Northwest National Laboratory, USA (PNNL). Notably, the software can be operated in convergence mode, whereby coincidence detection efficiency’s convergence behavior can help avoid unreliable radionuclide activity estimates. With growing number of coincidence spectrometers worldwide, this paper aims to assist the radiation metrology community in developing similar software for their system.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Evaluation of Compton suppression for enhancing trace element identification in neutron activation analysis of reference materials

Neutron activation analysis (NAA) is a powerful technique for identifying and quantifying trace elements in materials. However, challenges such as high dead times, spectral interferences, and high Compton continuum often arise. This study employs a Compton suppression system (CSS) to enhance NAA sensitivity by reducing the Compton continuum, thereby improving the peak-to-Compton ratio. National Institute of Standards and Technology certified reference materials 1632d, 1633c, and Canadian National Research Council TORT-1 were irradiated in a thermal and epithermal neutron flux under various irradiation, decay and counting times and analyzed using high-resolution gamma-ray spectroscopy with and without Compton suppression. The reduction factor was calculated to evaluate the effectiveness of the CSS, demonstrating significant background reduction and improved detection limits for trace elements. Additional experiments with a 137Cs point source demonstrated the impact of detector-source geometry on system performance, showing a decrease in the reduction factor as the source was moved further from the NaI detector. An optimum distance between the source and HPGe detector was observed, yielding the highest peak-to-Compton ratio. The results highlight the CSS's ability to minimize spectral interference and enhance elemental identification.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

The Orbital Variation of Non-Thermal X-Ray Emission from eta Carinae

The collision of strong stellar winds in massive binary systems creates powerful shocks,which accelerates a small amount of particles to relativistic energies at the shock interface.This process is important in fundamental astrophysics in two ways;i) some particles may contribute to cosmic-rays observed around the Earth, whose origin is not well known, andii) it provides a good laboratory for particle acceleration physics as the shock occurs steadily in a predictable environment.Some relativistic particles collide with stellar photons or ambient material near the binary systemand emit non-thermal X-rays and gamma-rays, which are good probes of particle acceleration.This emission had been searched for decades but not found convincingly without sensitive high-energy telescopes.The NuSTAR telescope observed the enigmatic supermassive binary system eta Carinae multiple times after 2014 and found conclusive evidence of non-thermal emission from the star in the extremely hard X-ray band.This emission is prominent between 20-50 keV, below which thermal emission from shock colliding plasma dominates.It is relatively stable throughout the binary orbit, but it disappears near periastron when the wind colliding activity shuts off.This variation indicates that the non-thermal X-ray emission originates from the head-on wind-wind collision.The flat spectrum is consistent with inverse-Compton of stellar UV photons by accelerated electrons.The spectrum smoothly connects to a gamma-ray spectrum of a Fermi source detected around eta Carinae,suggesting that acceleration occurs up to the GeV energy.This result provide the strongest evidence so far that particle acceleration occurs at the wind colliding shock of a massive colliding wind binary system.

Hamaguchi, Kenji↗

X-ray and γ-ray beam interstellar communication and implications for SETI

The possibility of detecting artificial signals transmitted by alien civilizations via collimated X-ray or gamma-ray beams is investigated. The prospect of using such beams for human communication within the solar system and beyond is also discussed. Detector responses were simulated for input signals and analyzed using relative entropy. For simplicity, all signals were assumed to use on-off keying (OOK) modulation. “Real” signals were generated by taking digital files and sequentially feeding their raw binary data to the detector simulator, the resulting normalized information content of the detector signals was plotted and compared to random noise signals. Since jpeg files contain compressed information, these served as a proxy for artificial alien signals. This showed that there is a clear difference in measured information content between natural and artificial signals, even with relatively poor time resolution in the detector causing the signals to be smeared (dead-time/rise-time intervals many times longer than the duration between signal pulses). It was found that so long as the signal lasts for at least several rise-time/dead-time intervals, the distinction between random and artificial signals is obvious. A space-telescope with high time resolution for searching for such signals is briefly described and its basic requirements are outlined.

43 PARTICLE ACCELERATORS↗

Embedded acoustic sensing and monitoring techniques for small modular reactors

The goal of this project was to study the applicability of specific innovative instrumentation techniques for assessing parameters needed for safe small modular reactor operation and safeguarding of nuclear material. Small modular reactor core designs are currently being developed to provide energy more effectively and efficiently than in the past because they can be built as modules at fabrication sites and then transported to a power-producing facility. However, these modules and/or the final core will often be sealed and not accessible again until disposal. Instead of instruments that access the core directly, during and after operation, to monitor flux/dose and structural integrity, as current power plants use, new sensors need to be designed that can be built into the reactor initially to determine operating history, structural integrity through operation of the system, and nuclear material accountancy after shutdown and before disposition of the core. Embedded sensors already exist that can provide neutron flux, gamma dose, and temperatures, but techniques to expand upon these for assessing structural health and material inventory in the system over time need to be developed. Structural health assessments include the detection and imaging of cracks in the components that could eventually cause radioactive fission products to be released.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Quantum dot lightning detection and warning system and method

A quantum dot (QD) lightning detection and warning (LDW) system and method. This LDW system and method find broader applicability to spark and other transient optical event detection as well. The QDs are operable for receiving ultraviolet (UV), infrared (IR), visible, x-ray, and/or gamma ray radiation emanating from lightning or the like and generating visible radiation that may be detected and utilized to generate topological event information, such that property, human life, and the like may be safeguarded.

Bahritdinov, Farhod↗

Observing Gamma-ray Bursts with GLAST

The Gamma-ray Large Area Telescope (GLAST) is a satellite-based observatory to study the high-energy gamma-ray sky. The Large Area Telescope, the main instrument, is a pair-conversion telescope which will survey the sky in the energy range 20 MeV to greater than 300 GeV. The LAT's wide field of view (greater than 2 sr), large effective area and low deadtime combine to provide excellent high-energy gamma-ray observations of GRB. To tie these frontier high-energy observations to the better-known properties at lower energies, a second instrument, the GLAST Burst Monitor (GBM) will provide important spectra and timing in the 8 keV to 30 MeV range. Upon detection of a GRB by the LAT or the GBM, the spacecraft can autonomously repoint to keep the GRB location within the LAT field of view, allowing high-energy afterglow observations. We describe how the instruments, spacecraft, and ground system work together to provide observations of gamma-ray bursts from 8 keV to over 300 GeV and provide rapid notification of these observations to the wider gamma-ray burst community. Analysis and simulation tools dedicated to the GRB science have been developed. In this contribution we show the expected LAT sensitivity obtained with such simulations, and illustrate the results we expect from GLAST observations with spectral and temporal analysis of simulated GRB.

McEnery, Julie↗

Detecting Low-level Radiation Sources Using Border Monitoring Gamma Sensors

We consider a problem of detecting a low-level radiation source using a network of Gamma spectral sensors placed on the periphery of a monitored region. We propose a computationally light-weight, correlation-based method which is primarily intended for systems with limited computing capacity. Sensor measurements are combined at the fusion by first generating decisions at each time step and then taking their majority vote within a time widow. At each time step, decisions are generated using two strategies: (i) SUM method based on a threshold decision on a correlation statistic derived from measurements from all sensors, and (ii) OR method based on logical-OR of threshold decisions based on correlations statistics of individual sensor measurements. We derive analytical performance bounds for false alarm rates of SUM and OR methods, and show that their performance is enhanced by the temporal smoothing of majority vote within a time window. Using measurements from a test campaign, we generate a border monitoring scenario with twelve 2"x2" NaI Gamma sensors deployed on the periphery of 42m x 42m outdoor region. A Cs-137 source is moved in a straight-line across this region, starting several meters outside and finally moving away from it. We illustrate the performance of both correlation-based detection methods, and compare their performances with each other and with a particle filter method. Overall, under small false-alarm conditions, the OR fusion is found to produce better detection performance.

Sen, Satyabrata↗

Report on Field Test at INL Cask Farm of Single Detector Fast Neutron Spent Fuel Cask Verification System

Detecting diversion of spent fuel elements in dry storage casks is challenging due to the thick shielding used in cask construction. Measurements on top of the cask to map the underlying arrangement of the fuel elements and looking for anomalous changes over time has proven difficult to achieve using gamma rays due to the high scattering and attenuation from the thick steel structure, weakening information on the present or absence of fuel bundles. Simulations and laboratory experiments suggest that the high-energy neutron flux (>200 keV) measured directly above each fuel bundle is sufficient to produce a position map that enables detection of the present or absence of fuel bundles, and therefore diversion of a spent fuel bundle. A single-detector spent-fuel monitoring technique based on this principle was development at the Lawrence Livermore National Laboratory (LLNL). The INL Cask Farm in the INTEC technical area at Idaho National Laboratory (INL) offers the capability to test this technique on an MC-10 storage cask which has a distribution of full and empty fuel positions. An experimental test plan for the single-detector verification system was developed in consultation with INL personnel to be completed in FY2021. Due to travel advisories related to COVID-19, the experimental test plan was adapted to enable INL personnel to carry out the measurements in consultation with LLNL personnel following shipment of the LLNL system to INL. Field test measurements of the single detector verification system were successfully carried out at the INL cask farm on September 7-9, 2021. This document summarizes results of the field test.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

The consequences of gamma-ray burst jet opening angle evolution on the inferred star formation rate

ABSTRACT Gamma-ray burst (GRB) data suggest that the jets from GRBs in the high redshift universe are more narrowly collimated than those at lower redshifts. This implies that we detect relatively fewer long GRB progenitor systems (i.e. massive stars) at high redshifts, because a greater fraction of GRBs have their jets pointed away from us. As a result, estimates of the star formation rate (SFR; from the GRB rate) at high redshifts may be diminished if this effect is not taken into account. In this paper, we estimate the SFR using the observed GRB rate, accounting for an evolving jet opening angle. We find that the SFR in the early universe (z > 3) can be up to an order of magnitude higher than the canonical estimates, depending on the severity of beaming angle evolution and the fraction of stars that make long GRBs. Additionally, we find an excess in the SFR at low redshifts, although this lessens when accounting for evolution of the beaming angle. Finally, under the assumption that GRBs do, in fact, trace canonical forms of the cosmic SFR, we constrain the resulting fraction of stars that must produce GRBs, again accounting for jet beaming-angle evolution. We find this assumption suggests a high fraction of stars in the early universe producing GRBs – a result that may, in fact, support our initial assertion that GRBs do not trace canonical estimates of the SFR.

79 ASTRONOMY AND ASTROPHYSICS↗

Persistent X-ray emission from a gamma-ray burst source

A quiescent X-ray source detected with the Einstein X-ray Observatory in a location consistent with that of an intense gamma ray burst is shown to be also consistent with the location of the 1928 optical transient, the likely optical counterpart of the gamma ray burst source GBS0117-29. The system appears to be underluminous in X-rays by a factor of 10; possible reasons for this are discussed. The observed X-ray flux would require an accretion rate of about 10 to the -14th (d/1 kpc/)-squared solar masses per year, which is probably too low to be consistent with published nuclear flash models for gamma bursts, unless the distance is substantially greater than about 1 kpc or the burst recurrence time is greater than about 50 yrs, or the accretion rate is highly variable. Such a long recurrence time appears to be inconsistent with the detection of the optical burst.

Grindlay, J. E.↗

IAEA Photonuclear Data Library 2019

Here, photo-induced reaction cross section data are of importance for a variety of current or emerging applications, such as radiation shielding design and radiation transport analyses, calculations of absorbed dose in the human body during radiotherapy, physics and technology of fission reactors (influence of photo-reactions on neutron balance) and fusion reactors (plasma diagnostics and shielding), activation analyses, safeguards and inspection technologies, nuclear waste transmutation, medical isotope production and astrophysical applications. To address these data needs the IAEA Photonuclear Data library was produced in 1999, containing evaluated photo-induced cross sections and neutron spectra for 164 nuclides which were deemed relevant for the applications. Since the release of the IAEA Photonuclear Data Library however, new experimental data as well as new methods to assess the reliability of experimental cross sections have become available. Theoretical models and input parameters used to evaluate photo-induced reactions have improved significantly over the years. In addition, new measurements of partial photoneutron cross sections using mono-energetic photon beams and advanced neutron detection systems have been performed allowing for the validation of the evaluations and assessments of the experimental data. Furthermore, technological advances have led to the construction of new and more powerful gamma-beam facilities, therefore new data needs are emerging. We report our coordinated efforts to address these data needs and present the results of the new up-to-date evaluations included in the new updated IAEA Photonuclear Data Library consisting of 219 nuclides. The new library includes 188 new evaluations produced by the CRP evaluators, and one evaluation taken from the JENDL/PD-2016 library, while 20 evaluations were retained from the previous 1999 IAEA Photonuclear Data Library. In most of the cases, the photon energy goes up to 200 MeV. A total of 55 nuclides are new in this library reflecting the progress in measurements but also the developing data needs. In this paper we discuss the new assessment method and make recommendations to the user community in cases where the experimental data are discrepant and the assessments disagree. In addition, in the absence of experimental data, we present model predictions for photo-induced reaction cross section on nuclides of potential interest to medical radioisotope production.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Prospects for Nuclear-gamma-ray Astronomy

An analysis was made of prospects for gamma rays coming from two sources outside the solar system: (1) radioactive decay of fresh nuclear products to explosive nucleosynthesis, and (2) scattering of low energy cosmic rays. The former should be detectable and will provide a factual base for many suppositions about the site and history of nucleosynthesis. The latter may be detectable and, if so, will probably provide factual information about high-flux regions of cosmic radiation.

Clayton, D. D.↗