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At least 217 records · Page 12

Quantitative molecular characterization of bovine vitreous and lens with non-invasive dynamic light scattering

The non-invasive technique of dynamic light scattering (DLS) was used to quantitatively characterize vitreous and lens structure on a molecular level by measuring the sizes of the predominant particles and mapping the three-dimensional topographic distribution of these structural macromolecules in three spatial dimensions. The results of DLS measurements in five fresh adult bovine eyes were compared to DLS measurements in model solutions of hyaluronan (HA) and collagen (Coll). In the bovine eyes DLS measurements were obtained from excised samples of gel and liquid vitreous and compared to the model solutions. Measurements in whole vitreous were obtained at multiple points posterior to the lens to generate a three-dimensional 'map' of molecular structure. The macromolecule distribution in bovine lens was similarly characterized.In each bovine vitreous (Bo Vit) specimen, DLS predominantly detected two distinct particles, which differed in diffusion properties and hence size. Comparisons with model vitreous solutions demonstrated that these most likely corresponded to the Coll and HA components of vitreous. Three-dimensional mapping of Bo Vit found heterogeneity throughout the vitreous body, with different particle size distributions for Coll and HA at different loci. In contrast, the three-dimensional distribution of lens macromolecules was more homogeneous. Thus, the non-invasive DLS technique can quantitate the average sizes of vitreous and lens macromolecules and map their three-dimensional distribution. This method to assess quantitatively the macromolecular structure of vitreous and lens should be useful for clinical as well as experimental applications in health and disease. Copyright 2001 Academic Press.

Models, Molecular↗

Photon Sieve Design and Fabrication for Imaging Characteristics Using UAV Flight

The Photon Sieve (PS) team at NASA Langley Research Center (LaRC) began receiving support for the development and characterization of PS devices through the NASA Internal Research & Development Program (IRAD) in 2015. The project involves ascertaining the imaging characteristics of various PS devices. These devices hold the potential to significantly reduce mission costs and improve imaging quality by replacing traditional reflector telescopes. The photon sieve essentially acts as a lens to diffract light to a concentrated point on the focal plane like a Fresnel Zone Plate (FZP). PS’s have the potential to focus light to a very small spot which is not limited by the width of the outermost zone as for the FZP and offers a promising solution for high resolution imaging. In the fields of astronomy, remote sensing, and other applications that require imaging of distant objects both on the ground and in the sky, it is often necessary to perform post-process filtering in order to separate noise signals that arise from multiple scattering events near the collection optic. The PS exhibits a novel filtering technique that rejects the unwanted noise without the need for time consuming post processing of the images. This project leverages key Langley resources to design, manufacture, and characterize a series of photon sieve specimens. After a prototype was developed and characterized in the Langley ISO5 optical cleanroom and laboratory, outside testing was conducted via the capture of images of the moon by using a telescopic setup. This next goal of the project is to design and develop a telescope and image capture system as a drone-based instrument payload. The vehicle utilized for the initial demonstration was a NASA hive model 1200 XE-8 research Unmanned Aerial Vehicle (UAV), capable of handling a 20-pound maximum payload with a 25-minute flight time. This NASA Technical Memorandum (NASA-TM) introduces preliminary results obtained using a PS-based imaging system on the UAV. The next version of the telescope structure will be designed around diffractive optical components and commercially available camera electronics to create a lightweight payload.

Kim, Hyun Jung↗

Laboratory simulation of diffuse reflectivity from a cloudy planetary atmosphere.

For the first time measurements in the multiple scattering regime of the diffuse reflectivity as a function of single scattering albedo have been made in a geometry that may be simulated by a plane parallel atmosphere of large optical depth. A comparison between the measurements and a theoretical computation of the diffuse reflectivity is presented. The measurements are within 1% agreement with the theoretical calculations for two different sizes of scattering particles which are larger than and smaller than the wavelength of the incident light, corresponding to the Mie and Rayleigh regimes, respectively.

Margolis, J. S.↗

Velocity visualization in gaseous flows

Techniques yielding simultaneous, multiple-point measurements of velocity in reacting or nonreacting flow fields have the potential to significantly impact basic and applied studies of fluid mechanics. This research program is aimed at investigating several candidate schemes which could provide such measurement capability. The concepts under study have in common the use of a laser source (to illuminate a column, a grid, a plane or a volume in the flow) and the collection of light at right angles (from Mie scattering, fluorescence, phosphorescence or chemiluminescence) using a multi-element solid-state camera (100 x 100 array of photodiodes). The work will include an overview and a status report of work in progress with particular emphasis on the method of Doppler-modulated absorption.

Hanson, R. K.↗

Synchrotron Self-Compton Emission from the Crab and Other Pulsars

Results of a simulation of synchrotron-self Compton (SSC) emission from a rotation-powered pulsar are presented. The radiating particles are assumed to be both accelerated primary electrons and a spectrum of electron-positron pairs produced in cascades near the polar cap. They follow trajectories in a slot gap using 3D force-free magnetic field geometry, gaining pitch angles through resonant cyclotron absorption of radio photons, radiating and scattering synchrotron emission at high altitudes out to and beyond the light cylinder. Full angular dependence of the synchrotron photon density is simulated in the scattering and all processes are treated in the inertial observer frame. Spectra for the Crab and Vela pulsars as well as two energetic millisecond pulsars, B1821-24 and B1937+21 are simulated using this model. The simulation of the Crab pulsar radiation can reproduce both the flux level and the shape of the observed optical to hard X-ray emission assuming a pair multiplicity of M+ = 3x10(exp 5), as well as the very-high- energy emission above 50 GeV detected by MAGIC and VERITAS, with both the synchrotron and SSC components reflecting the shape of the pair spectrum. Simulations of Vela, B1821-24 and B1937+21, for M+ up to 10(exp 5), do not produce pair SSC emission that is detectable by current telescopes, indicating that only Crab-like pulsars produce significant SSC components. The pair synchrotron emission matches the observed X-ray spectrum of the millisecond pulsars and the predicted peak of this emission at 1-10 MeV would be detectable with planned Compton telescopes.

Self-Compton↗

Retrievals of Cloud Droplet Size from the Research Scanning Polarimeter Data: Validation Using In Situ Measurements

We present comparisons of cloud droplet size distributions (DSDs) retrieved from the research scanning polarimeter (RSP) data with correlative in situ measurements made during the North Atlantic Aerosols and Marine Ecosystems Study (NAAMES). The airborne portion of this field experiment was based out of St. John's airport, Newfoundland, Canada with the focus of this paper being on the deployment in May - June 2016. RSP was onboard the NASA C-130 aircraft together with an array of in situ and other remote sensing instrumentation. The RSP is an along-track scanner measuring the polarized and total reflectance in 9 spectral channels. Its uniquely high angular resolution allows for characterization of liquid water droplet sizes using the rainbow structure observed in the polarized reflectance over the scattering angle range from 135 to 165.degrees The rainbow is dominated by single scattering of light by cloud droplets, so its structure is characteristic specifically of the droplet sizes at cloud top (within unit optical depth into the cloud, equivalent to approximately 50m). A parametric fitting algorithm applied to the polarized reflectance provides retrievals of the droplet effective radius and variance assuming a prescribed size distribution shape (gamma distribution). In addition to this, we use a non-parametric method, the Rainbow Fourier Transform (RFT), which allows us to retrieve the droplet size distribution itself. The latter is important in the case of clouds with complex microphysical structure, or multiple layers of cloud, which result in multi-modal DSDs. During NAAMES the aircraft performed a number of flight patterns specifically designed for comparisons between remote sensing retrievals and in situ measurements. These patterns consisted of two flight segments above the same straight ground track. One of these segments was flown above clouds allowing for remote sensing measurements, while the other was near the cloud top where cloud droplets were sampled. We compare the DSDs retrieved from the RSP data with in situ measurements made by the Cloud Droplet Probe (CDP). The comparisons generally show good agreement (better than 1 micron for effective radius and in most cases better than 0.02 for effective variance) with deviations explainable by the position of the aircraft within the cloud, or by the presence of additional cloud layers between the cloud being sampled by the in situ instrumentation and the altitude of the remote sensing segment. In the latter case, the multi-modal DSDs retrieved from the RSP data were consistent with the multi-layer cloud structures observed in the correlative High Spectral Resolution Lidar (HSRL) profiles. The results of these comparisons provide a rare validation of polarimetric droplet size retrieval techniques, demonstrating their accuracy and robustness and the potential of satellite data of this kind on a global scale.

Remote Sensing↗

Diurnal variation of thermal plasma in the plasmasphere

All of the OGO-5 light ion density measurements were used to determine the average global topology of the equatorial plasmasphere density distribution. The variation of the light ion equatorial density at L less than or equal to 3.2 with local time was deduced by determining the average density observed within one hour of a specific local time and within 0.1 of a given L coordinate. The average H(+) density showed a semidiurnal variation with peaks near noon and midnight. The He(+) observations also revealed multiple peaks throughout the day but with smaller amplitudes than those of H(+). At L above 3.2 plasma trough conditions increase the scatter of densities. The average variation of the H(+) density with L within the plasmasphere is found to be steepest near midnight and can be least-squares fitted equally well to either an exponential variation or to a power law.

Chen, A. J.↗

Interferometer Control of Optical Tweezers

This paper discusses progress in using spatial light modulators and interferometry to control the beam profile of an optical tweezers. The approach being developed is to use a spatial light modulator (SLM) to control the phase profile of the tweezers beam and to use a combination of the SLM and interferometry to control the intensity profile. The objective is to perform fine and calculable control of the moments and forces on a tip or tool to be used to manipulate and interrogate nanostructures. The performance of the SLM in generating multiple and independently controllable tweezers beams is also reported. Concurrent supporting research projects are mentioned and include tweezers beam scattering and neural-net processing of the interference patterns for control of the tweezers beams.

Decker, Arthur J.↗

A new technique for the measurement of surface shear stress vectors using liquid crystal coatings

Research has recently shown that liquid crystal coating (LCC) color-change response to shear depends on both shear stress magnitude and direction. Additional research was thus conducted to extend the LCC method from a flow-visualization tool to a surface shear stress vector measurement technique. A shear-sensitive LCC was applied to a planar test surface and illuminated by white light from the normal direction. A fiber optic probe was used to capture light scattered by the LCC from a point on the centerline of a turbulent, tangential-jet flow. Both the relative shear stress magnitude and the relative in-plane view angle between the sensor and the centerline shear vector were systematically varied. A spectrophotometer was used to obtain scattered-light spectra which were used to quantify the LCC color (dominant wavelength) as a function of shear stress magnitude and direction. At any fixed shear stress magnitude, the minimum dominant wavelength was measured when the shear vector was aligned with and directed away from the observer; changes in the relative in-plane view angle to either side of this vector/observer aligned position resulted in symmetric Gaussian increases in measured dominant wavelength. Based on these results, a vector measurement methodology, involving multiple oblique-view observations of the test surface, was formulated. Under present test conditions, the measurement resolution of this technique was found to be +/- 1 deg for vector orientations and +/- 5% for vector magnitudes. An approach t o extend the present methodology to full-surface applications is proposed.

Reda, Daniel C.↗

Measurements of the Vertical Structure of Aerosols and Clouds Over the Ocean Using Micro-Pulse LIDAR Systems

The determination of the vertical distribution of aerosols and clouds over the ocean is needed for accurate retrievals of ocean color from satellites observations. The presence of absorbing aerosol layers, especially at altitudes above the boundary layer, has been shown to influence the calculation of ocean color. Also, satellite data must be correctly screened for the presence of clouds, particularly cirrus, in order to measure ocean color. One instrument capable of providing this information is a lidar, which uses pulses of laser light to profile the vertical distribution of aerosol and cloud layers in the atmosphere. However, lidar systems prior to the 1990s were large, expensive, and not eye-safe which made them unsuitable for cruise deployments. During the 1990s the first small, autonomous, and eye-safe lidar system became available: the micro-pulse lidar, or MPL. The MPL is a compact and eye-safe lidar system capable of determining the range of aerosols and clouds by firing a short pulse of laser light (523 nm) and measuring the time-of-flight from pulse transmission to reception of a returned signal. The returned signal is a function of time, converted into range using the speed of light, and is proportional to the amount of light backscattered by atmospheric molecules (Rayleigh scattering), aerosols, and clouds. The MPL achieves ANSI eye-safe standards by sending laser pulses at low energy (micro-J) and expanding the beam to 20.32 cm in diameter. A fast pulse-repetition-frequency (2500 Hz) is used to achieve a good signal-to-noise, despite the low output energy. The MPL has a small field-of-view (< 100 micro-rad) and signals received with the instrument do not contain multiple scattering effects. The MPL has been used successfully at a number of long-term sites and also in several field experiments around the world.

Welton, Ellsworth J.↗

X-Raying the Ultraluminous Infrared Starburst Galaxy and Broad Absorption Line QSO Markarian 231 with Chandra

With 40 ks of Clzandra ACIS-S3 exposure, new information on both the starburst and QSO components of the X-ray emission of Markarian 231, an ultraluminous infrared galaxy and broad absorption line QSO, has been obtained. The bulk of the X-ray luminosity is emitted from an unresolved nuclear point source, and the spectrum is remarkably hard, with the majority of the flux emitted above 2 keV. Most notably, significant nuclear variability (a decrease of -45% in approximately 6 hr) at energies above 2 keV indicates that Chuizdra has probed within light-hours of the central black hole. Although we concur with Maloney & Reynolds that the direct continuum is not observed, this variability coupled with the 188 eV upper limit on the equivalent width of the Fe K o emission line argues against the reflection-dominated model put forth by these authors based on their ASCA data. Instead, we favor a model in which a small, Compton-thick absorber blocks the direct X-rays, and only indirect, scattered X-rays from multiple lines of sight can reach the observer. Extended soft, thermal emission encompasses the optical extent of the galaxy and exhibits resolved structure. An off-nuclear X-ray source with a 0.35-8.0 keV luminosity of Lx = 7 x 10 sup39 ergs s sup -1 , consistent with the ultraluminous X-ray sources in other nearby starbursts, is detected. We also present an unpublished Faint Object Spectrograph spectrum from the Hirhhle Spuce Telescope archive showing the broad C IV absorption.

Gallagher, S. C.↗

Lectures on the scattering of light

The exact (Mie) theory for the scattering of a plane wave by a dielectric sphere is presented. Since this infinite series solution is computationally impractical for large spheres, another formulation is given in terms of an integral equation valid for a bounded, but otherwise general array of scatterers. This equation is applied to the scattering by a single sphere, and several methods are suggested for approximating the scattering cross section in closed form. A tensor scattering matrix is introduced, in terms of which some general scattering theorems are derived. The application of the formalism to multiple scattering is briefly considered.

Saxon, D. S.↗

Light-flavor particle production in high-multiplicity pp collisions at $\sqrt{\textrm{s}}$ = 13 TeV as a function of transverse spherocity

Results on the transverse spherocity dependence of light-flavor particle production (π, K, p, ϕ, K *0 , K$^{0}_{S}$, Λ, Ξ) at midrapidity in high-multiplicity pp collisions at $\sqrt{\textrm{s}}$ = 13 TeV were obtained with the ALICE apparatus. The transverse spherocity estimator ($S$$^{p_T=1}_{O}$) categorizes events by their azimuthal topology. Utilizing narrow selections on $S$$^{p_T=1}_{O}$, it is possible to contrast particle production in collisions dominated by many soft initial interactions with that observed in collisions dominated by one or more hard scatterings. Results are reported for two multiplicity estimators covering different pseudorapidity regions. The $S$$^{p_T=1}_{O}$ estimator is found to effectively constrain the hardness of the events when the midrapidity (|η| < 0.8) estimator is used.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Nighttime observations of thunderstorm electrical activity from a high altitude airplane

Photographs from a NASA U-2 airplane flying over nocturnal thunderstorms show frequent lightning activity in the upper part of the cloud. In some cases, unobscured segments of lightning channels 1 km or longer are visible in clear air around and above the cloud. Multiple images of lightning channels indicate multiple discharges in the same channel. Photographs taken through a diffraction grating show that the lightning has a spectrum similar to that observed in the lower troposphere. Lightning spectra obtained with a slitless line-scan spectrometer show strong singly ionized nitrogen emissions at 463.0 and 500.5 nm. Field changes measured with an electric field-change meter correlate with pulses measured with a photocell optical system. Optical signals corresponding to dart leader, return stroke, and continuing current events are readily distinguished in the scattered light emerging from the cloud surface. The variation of light intensity with time in lightning events is consistent with predicted modification of optical lightning signals by clouds. It appears that satellite based optical sensor measurements cannot provide reliable information on current rise times in return strokes. On the other hand, discrimination between cloud-to-ground and intracloud flashes and the counting of ground strokes is possible using the optical pulse pairs which have been identified with leader, return-stroke events in the cloud-to-ground flashes studied.

Brook, M.↗

Studies of optical and chemical properties of aged and fresh biomass burning absorbing aerosols for climate models

Particulate emissions from burning fuels from sub-Saharan Africa is currently poorly characterized. With increasing population and industrialization, emissions are expected to grow. Optical methods for measuring light absorption in the ultraviolet (UV) and visible (vis) regions of the spectrum are crucial for understanding the optical properties of BB aerosols (Bond and Bergstrom, 2006; Lack and Cappa, 2010; Moschos et al., 2021). One such instrument is the dual-spot AE33 model aethalometer is a common filter-based instrument that can be used to measure aerosol absorption properties (Hansen et al., 1984). This instrument has many figures of merit; however, the method's limitations include potential biases from scattering within the filter material, multiple scattering effects of the particles, filter loading (i.e. particle shadowing), and the need for wavelength-specific correction factors (Cλ), which depend on accurate intercomparison with other in situ techniques (Bond et al., 1999; Collaud Coen et al., 2010). This work aims to: 1. Optically characterize BB aerosol generated from African fuel 2. Correct the aethalometer at multiple wavelengths 3. Parametrize these correction factors. 4. Combusting the same fuels with two difference tube furnace systems assess the general applicability of this flexible means of producing BB aerosol. This was accomplished by conducting laboratory studies at Los Alamos National Laboratory (LANL) and North Carolina A&T State University (NCA&T), where aethalometer measurements were compared to in situ optical measurements. Mass cross sections of BB aerosol from these under-studied fuels will be determined along with their wavelength dependence.

09 BIOMASS FUELS↗

Monitoring Delamination of Plasma-Sprayed Thermal Barrier Coatings by Reflectance-Enhanced Luminescence

Highly scattering plasma-sprayed thermal barrier coatings (TBCs) present a challenge for optical diagnostic methods to monitor TBC delamination because scattering attenuates light transmitted through the TBC and usually degrades contrast between attached and delaminated regions of the TBC. This paper presents a new approach where reflectance-enhanced luminescence from a luminescent sublayer incorporated along the bottom of the TBC is used to identify regions of TBC delamination. Because of the higher survival rate of luminescence reflecting off the back surface of a delaminated TBC, the strong scattering exhibited by plasma-sprayed TBCs actually accentuates contrast between attached and delaminated regions by making it more likely that multiple reflections of luminescence off the back surface occur before exiting the top surface of the TBC. A freestanding coating containing sections designed to model an attached or delaminated TBC was prepared by depositing a luminescent Eu-doped or Er-doped yttria-stabilized zirconia (YSZ) luminescent layer below a plasma-sprayed undoped YSZ layer and utilizing a NiCr backing layer to represent an attached substrate. For specimens with a Eu-doped YSZ luminescent sublayer, luminescence intensity maps showed excellent contrast between unbacked and NiCr-backed sections even at a plasma-sprayed overlayer thickness of 300 m. Discernable contrast between unbacked and NiCr-backed sections was not observed for specimens with a Er-doped YSZ luminescent sublayer because luminescence from Er impurities in the undoped YSZ layer overwhelmed luminescence originating form the Er-doped YSZ sublayer.

Eldridge, Jeffrey I.↗

Long-term stabilization of intensity-difference squeezing from four-wave mixing in rubidium vapor

Generation of quantum states of light through off-resonance four-wave mixing in rubidium vapor is a straightforward and well-established technique. However, achieving a sufficiently high and consistent level of intensity difference squeezing (IDS) and intrinsic quantum correlations between photon pairs over an extended timescale, necessary for quantum-light-based nonlinear optical spectroscopy and microscopy, remains challenging and largely unexplored. Here, we report a simple stabilization method combining an active periodic laser frequency retuning with an automatic control algorithm based on quantitatively assessing the factors affecting the IDS level and squeezed light intensity. Validation of our method was performed by acquiring data over a 5-hour period, and the results demonstrate a remarkably stable squeezing level of -7.8 dB in combination with a > 4× reduction of the standard deviation of IDS level from 0.46 dB to 0.10 dB. The achieved stabilization further enables us to quantitatively assess the IDS reduction due to the scattering in a polystyrene bead suspension as a function of sample transmission. Our approach should enable a variety of applications requiring an extended squeezing stability over multiple hours, especially for those following biological processes and chemical reactions in real time.

Allen, Christian Harry [Oak Ridge National Laborat↗

100-kHz Interferometric Rayleigh Scattering Flow Diagnostics at 266 nm

Interferometric Rayleigh scattering (IRS) is a laser-based technique capable of spatially and temporally resolved measurement of gas velocity and temperature in unseeded gaseous flows. In the present embodiment of the technique, IRS is performed at 266 nm for the first time. IRS at 266 nm is potentially much less susceptible to interferences from particles and other stray light sources. A pulse-burst laser and high-speed camera provided image rates of 100 kHz, allowing simultaneous space- and time-resolved measurement in high speed flow at multiple points along a line. The use of 266 nm excitation and detection is compared with prior work that used 532 nm. New experimental interferogram modelling and fitting techniques for single and multi-velocity-component IRS were demonstrated in a study of the spatial and temporal variation of the flow along a line through a supersonic jet. Single component velocity and temperature measurements using 266 nm were successfully made and compared with prior 532 nm results. Two-component velocity measurements at 266 nm, using the reflected image method, were compared to single-component measurements.

Andrew D Cutler↗