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At least 253 records · Page 14

Delivery of LiH Shell for DANCE

Material for a new LiH shell for neutron shielding has been obtained for the Detector for Advanced Neutron Capture Experiments. This is a critical component for optimizing sensitivity of neutron capture experiments performed in support of Office of Experimental Sciences mission, particularly in the case of small, rare samples.

42 ENGINEERING↗

MHD-240 Neutron Detection Efficiency and Sensitivity Calibration

The neutron detection efficiency of the MHD-240 scintillation detector was measured at Ohio University Edwards Accelerator Laboratory. Pulsed broad-spectrum sources from the 27 Al(d,n) and 9 Be(d,n) reactions were used to produce the neutrons. The neutron time-of-flight technique was used to make an energy-differential efficiency measurement. The measurements were made in a low rate pulse mode. The pulse height distribution was also recorded, and the data were used to derive a neutron sensitivity that would be applicable in a high rate environment such as a critical assembly where the detector would be expected to operate in a current mode.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Gamma Rays from Kilonova: A Potential Probe of r-process Nucleosynthesis

The mergers of compact binaries with at least one neutron star component are the potential leading sites of the production and ejection of r-process elements. Discoveries of galactic binary pulsars, short gamma-ray bursts, and gravitational-wave detections have all been constraining the rate of these events, while the gravitational wave plus broadband electromagnetic coverage of binary neutron star merger (GW170817) has also placed constraints on the properties (mass and composition) of the merger ejecta. But uncertainties and ambiguities in modeling the optical and infrared emission make it difficult to definitively measure the distribution of heavy isotopes in these mergers. In contrast, gamma rays emitted in the decay of these neutron-rich ejecta may provide a more direct measurement of the yields. We calculate the gamma production in remnants of neutron star mergers, considering two epochs: a kilonova epoch, lasting about two weeks, and a much later epoch of tens and hundreds of thousands of years after the merger. For the kilonova epoch, when the expanding ejecta is still only partially transparent to gamma radiation, we use 3D radiative transport simulations to produce the spectra. Futhermore, we show that the gamma-ray spectra associated with beta- and alpha-decay provide a fingerprint of the ejecta properties and, for a sufficiently nearby remnant, may be detectable, even for old remnants. We compare our gamma spectra with the potential detection limits of next generation detectors, including the Lunar Occultation Explorer (LOX), the All-sky Medium Energy Gamma-ray Observatory (AMEGO), and the Compton Spectrometer and Imager (COSI). We show that fission models can be discriminated via the presence of short-lived fission fragments in the remnant spectra.

79 ASTRONOMY AND ASTROPHYSICS↗

Performance of the CMS Zero Degree Calorimeters in pPb collisions at the LHC

The two Zero Degree Calorimeters (ZDCs) of the CMS experiment are located at ± 140 m from the collision point and detect neutral particles in the |η| > 8.3 pseudorapidity region. This paper presents a study on the performance of the ZDC in the 2016 pPb run. The response of the detectors to ultrarelativistic neutrons is studied using in-depth Monte Carlo simulations. A method of signal extraction based on template fits is presented, along with a dedicated calibration procedure. A deconvolution technique for the correction of overlapping collision events is discussed.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Characterizing Shielded Special Nuclear Material by Neutron Capture Gamma-Ray Multiplicity Counting

We present a new neutron multiplicity counting analysis and measurement method for neutron-shielded fissile material using neutron-capture gamma rays. Neutrons absorbed in shielding produce characteristic gamma rays that preserve the otherwise lost neutron multiplicity signature. Neutron multiplicity counting provides estimates of fission parameters, such as neutron leakage multiplication, spontaneous fissioner (e.g. Pu-240) mass, and (α,n) ratio. Standard neutron multiplicity counting can incorporate the new neutron-capture gamma-ray multiplicity counting technique to characterize previously degenerate or intractable source configurations by maximizing the multiplicity signature. The new method decouples neutron source-detector interferences, such as reflection and thermalization time in the detector, that could improve measurements of the mean neutron lifetime. We also develop a detector prototype for the multiplicity counting of neutron-capture gamma rays and present detector design considerations, such as detection material and shielding, to optimize the detection of the 2.2 MeV hydrogen capture gamma ray. We simulate the prototype neutron- capture gamma-ray multiplicity counter against the BeRP ball in polyethylene shells to inform future measurements.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Numerical relativity simulations of the neutron star merger GW190425: microphysics and mass ratio effects

ABSTRACT GW190425 was the second gravitational wave (GW) signal compatible with a binary neutron star (BNS) merger detected by the Advanced LIGO and Advanced Virgo detectors. Since no electromagnetic counterpart was identified, whether the associated kilonova was too dim or the localization area too broad is still an open question. We simulate 28 BNS mergers with the chirp mass of GW190425 and mass ratio 1 ≤ q ≤ 1.67, using numerical-relativity simulations with finite-temperature, composition dependent equations of state (EOS) and neutrino radiation. The energy emitted in GWs is $\lesssim 0.083\mathrm{\, M_\odot }c^2$ with peak luminosity of 1.1–$2.4\times ~10^{58}/(1+q)^2\, {\rm {erg \, s^{-1}}}$. Dynamical ejecta and disc mass range between 5 × 10−6–10−3 and 10−5–$0.1 \mathrm{\, M_\odot }$, respectively. Asymmetric mergers, especially with stiff EOSs, unbind more matter and form heavier discs compared to equal mass binaries. The angular momentum of the disc is 8–$10\mathrm{\, M_\odot }~GM_{\rm {disc}}/c$ over three orders of magnitude in Mdisc. While the nucleosynthesis shows no peculiarity, the simulated kilonovae are relatively dim compared with GW170817. For distances compatible with GW190425, AB magnitudes are always dimmer than ∼20 mag for the B, r, and K bands, with brighter kilonovae associated to more asymmetric binaries and stiffer EOSs. We suggest that, even assuming a good coverage of GW190425’s sky location, the kilonova could hardly have been detected by present wide-field surveys and no firm constraints on the binary parameters or EOS can be argued from the lack of the detection.

79 ASTRONOMY AND ASTROPHYSICS↗

Many-body Nuclear Dynamics

The principal goal of this work was to better understand the fusion of neutron-rich nuclei a topic relevant to the fields of both nuclear physics and nuclear astrophysics. The work provides insight into the structure and reactions of neutron-rich nuclei namely the extent of their neutron density distribution and its polarizability. By comparing the fusion excitation functions for a chain of isotopes with a common target nucleus changes in the attractive nuclear potential are assessed. This change in the attractive potential is related to changes in the neutron density distribution with increasing number of neutrons or changes in fusion dynamics with increasing neutron number. The impact of the pairing of valence neutrons and protons on the fusion cross-section is also examined. Measurement of an isotopic chain is a powerful tool to address this topic. The experimental program made use of several different accelerator facilities. The core of the experimental work involved experiments at the ReA3 accelerator and the Facility for Rare Isotope Beams (FRIB) situated at Michigan State University, at GANIL, the French national nuclear physics laboratory, and the University of Notre Dame. At ReA3 the degree to which α-clusters associated with fusion of 28,30,32 Si + 28 Si result from the collision dynamics or reflect an initial α-cluster structure was explored. Alpha clusters observed in fusion reactions exceed the predictions of the standard statistical model. This experiment provides a measure of how clusterization is impacted by the increasing neutron-richess of the system. In the experiment at GANIL we investigated fusion in 19 O + 12 C and 20 O + 12 C. This experiment utilized the recently developed active-target detector MuSIC@Indiana. Using this proven, highly efficient, active-target detector we measured the fusion excitation function for these neutron-rich systems. Grounded by these experimental measurements, theoretical models were used to examine the role of unpaired valence neutrons on the fusion cross-section at energies just above the fusion barrier.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

MEASUREMENT OF THE NEUTRON FLUENCE-RATES IN THE ADVANCED TEST REACTOR

The axial neutron fluence-rate distribution at the Advanced Test Reactor (ATR) is determined using a combination of pure nickel and cobalt-aluminium alloy dosimeter wires. Most irradiation programs at ATR need to know the fast neutron fluence-rate surrounding their experiment to correlate post-irradiation examination results with neutron dose. The activated dosimeter wires, which extend beyond the full fuelled region of the reactor core, are highly radioactive following the full cycle in ATR and must therefore be measured in the ATR canal. The system that is employed for these measurements is mechanical scanning mechanism is used to scan the activated wires across the face of a columnated shield and a NaI detector. This detector is not sufficiently calibrated to provide absolute activity measurements, therefore, the count-rate is recorded and normalized to the highest activity for that wire. Then, an approximately 3-mm long portion of the wire is removed from the highest activity region in the wire. The wires are then transferred, and an absolute activity measurement is made using a calibrated ionization chamber. These measurements are combined with corrections for decay, neutron energy spectrum, burnup, dosimeter composition, reactor power fluctuations, and reactor outages to determine the average axial neutron fluence-rate at various locations within ATR during the cycle.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

TINMAN Thermal Neutron Detector for Aircraft

TinMan is the first technology to continuously measure thermal neutron intensity during aircraft flight and to define this environment, an important achievement since changes to semiconductors have led electronic parts to become more sensitive to thermal nuetrons that may lead to disturbances in their operation.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

ResNet and CycleGAN for pulse shape discrimination of He-4 detector pulses: Recovering pulses conventional algorithms fail to label unanimously

Pulse shape discrimination (PSD) capable detectors, such as He-4, that respond to neutron and gamma-ray 7 interactions have a threshold deposited energy value below which n/γ discrimination vanishes when using 8 conventional PSD algorithms. Recent attempts in applying supervised learning based artificial neural 9 networks for PSD use the pulses in the separated regions to train the networks so they can be used to classify 10 another set of separated pulses. In doing so, pulses previously indistinguishable are not recovered for 11 classification, which would have increased the number of neutron and gamma-ray pulses that could be used 12 for further analysis. Assuming the reason why conventional PSD algorithms have unseparated regions is 13 because the parameter space of the algorithms fail to capture the intrinsic (but subtle) distinguishing 14 behavior of some of the neutron and gamma-ray pulses, a cycle-consistent generative adversarial network 15 (CycleGAN) was trained to amplify those differences and extract well separated neutron and gamma-ray 16 clusters. Results show that, once the network is trained with pulses from separated and unseparated regions, 17 it was able to transform the pulses in the unseparated region to improve the PSD. Subsequent n/γ 18 classification was performed using deep residual network (ResNet) that takes pulses with 512 data points 19 as an input. Two different ResNets were explored – simple ResNet and modified ResNet which takes 20 segmented pulse inputs in the first layer and the corresponding time axis values in the last hidden layer. 21 The later approach enables the network to extract time correlated pulse features to enhance its ability to 22 capture the pulse behaviors relevant for PSD. Although it achieves slightly lower accuracy, 99.41% versus 23 99.89%, based on simply counting the number of correct n/γ labels assigned, compared to the simple 24 ResNet, the modified ResNets architecture was able to decreases the cross-entropy loss function by half, 25 which implies that the correct n/γ labels assigned are less likely to be accidental. PSD parameter 26 distributions based on n/γ classification by ResNet before and after transforming unseparated pulses using 27 CycleGAN show that by enhancing the separation between neutrons and gamma-rays, the transformation 28 helps improve the performance of classifier networks that are trained using labeled dataset. The 29 enhancement of neutron and gamma-ray separation by the CycleGAN increased the PSD figure of merit 30 (FOM) by up to 70% in some regions. Here, the results show that, if a given detector achieves clear separation 31 between neutron and gamma-ray pulses in any energy region, such neural network approaches can help 32 lower the energy threshold for the separation and increasing the number of neutron and gamma-ray pulses 33 that can be used for further analysis.

4He↗

Optical versus radiographic imaging and tomography: introduction to the ROADS feature issue

Optical imaging is an ancient branch of imaging dating back to thousands of years. Radiographic imaging and tomography (RadIT), including the first use of X-rays by Wilhelm Röntgen, and then, $γ$ -rays, energetic charged particles, neutrons, etc. are about 130 years young. The synergies between optical and radiographic imaging can be cast in the framework of these building blocks: Physics, Sources, Detectors, Methods, and Data Science, as described in Appl. Opt. 61, RDS1 (2022). Optical imaging has expanded to include three-dimensional (3D) tomography (including holography), due in to part the invention of optical (including infrared) lasers. RadIT are intrinsically 3D because of the penetrating power of ionizing radiation. Both optical imaging and tomography (OIT) and RadIT are evolving into even higher dimensional regimes, such as time-resolved tomography (4D) and temporarily and spectroscopically resolved tomography (4D + ). Further advances in OIT and RadIT will continue to be driven by desires for higher information yield, higher resolutions, and higher probability models with reduced uncertainties. Synergies in quantum physics, laser-driven sources, low-cost detectors, data-driven methods, automated processing of data, and artificially intelligent data acquisition protocols will be beneficial to both branches of imaging in many applications. These topics, along with an overview of the Radiography, Applied Optics, and Data Science virtual feature issue, are discussed here.

47 OTHER INSTRUMENTATION↗

Determining the average prompt-fission-neutron multiplicity for Pu 239 ( n , f ) via a Pu 240 ( α , α ' f ) surrogate reaction

The average prompt-fission-neutron multiplicity ν ¯ is of significance in the areas of nuclear theory, nuclear nonproliferation, and nuclear energy. In this work, the surrogate-reaction method has been used for the first time to indirectly determine ν ¯ for Pu 239 ( n , f ) via Pu 240 ( α , α ' f ) reactions. A Pu 240 target was bombarded with a beam of 53.9-MeV α particles. Scattered α particles, fission products, and neutrons were measured with the NeutronSTARS detector array. Values of ν ¯ were obtained for a continuous range of equivalent incident neutron energies between 0.25 and 26.25 MeV, and the results agree well with direct neutron measurements.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Validation of Light Water Reactor Ex-Core Calculations with VERA

The Consortium for Advanced Simulation of Light Water Reactors (CASL) Virtual Environment for Reactor Applications (VERA) is a reactor simulation software. It offers unique capabilities by combining high-fidelity in-core radiation transport with temperature feedback by using MPACT (a deterministic neutron transport code) and COBRA-TF (a thermal-hydraulic code) with follow-on, fixed-source transport calculations using the Shift Monte Carlo code to calculate ex-core quantities of interest. In these coupled calculations, MPACT provides Shift with the fission source for follow-on ex-core calculations. These ex-core simulations can be set up to calculate detector responses, as well as the flux and fluence in ex-core regions of interest, such as the reactor pressure vessel, nozzle, and irradiated capsules. A Watts Bar Nuclear Plant Unit 1 (WBN1) ex-core model was developed, as described in this paper, and this model was used to perform coupon calculations. The results for the coupon flux calculations show close agreement with the reference values for cycle 1 produced by the two-dimensional Discrete Ordinates Transport (DORT) code and presented in a BWXT Services Inc. report. However, differences in the results (10%) seen in cycles 2 and 3 and the reasons for these differences are discussed in this paper. The VERA WBN1 model was also used to perform a vessel fluence calculation for cycle 1. Additionally, a collaboration between CASL and Duke Energy led to the first code-to-code validation of VERA for reactor ex-core applications that used a model for the Shearon Harris reactor. Results from this collaboration show excellent agreement between VERA and the Monte Carlo N-Particle Transport Code for the detector response calculations. The work performed under this collaboration is also detailed in this paper.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Joint LLNL, LANL, SNL, and IRSN High Multiplication Subcritical (Multiplicity) Benchmark Experiments Execution Plan (IER-518 CED-3a)

As part of the experiment design and planning, the critical experiment design team (CEDT), as well as additional stakeholders, convened a series of meetings to discuss the goals and requirements of execution for this experiment. The slides from these meetings are attached in Appendix A. The following sections summarize the outcome of those discussions and present the planned experimental configurations and measurements. The stated goals of this experiment are as follows: 1) Measure time-tagged list-mode data for configurations exceeding neutron multiplication of 100; 2) Provide intercomparison between LLNL, LANL, and IRSN detector systems and methodologies; 3) Generate experiment execution report(s) useful to a fundamental physics benchmark for the ICSBEP; 4) Leverage existing critical experiment and detector system benchmarks to limit required modeling and uncertainty analysis.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Neutron-Resonance Transmission Analysis with a Compact Deuterium-Tritium Neutron Generator

Neutron Resonance Transmission Analysis (NRTA) is a spectroscopic technique which uses the resonant absorption of neutrons in the epithermal range to infer the isotopic composition of an object. This spectroscopic technique has relevance in many traditional fields of science and nuclear security. NRTA in the past made use of large, expensive accelerator facilities to achieve precise neutron beams, significantly limiting its applicability. Here, we describe a series of NRTA experiments where we use a compact, low-cost deuterium-tritium (DT) neutron generator to produce short neutron beams (2.6 m) along with a 6 Li-glass neutron detector. The time-of-flight spectral data from five elements – silver, cadmium, tungsten, indium, and 238 U – clearly show the corresponding absorption lines in the 1-30 eV range. The experiments show the applicability of NRTA in this simplified configuration, and prove the feasibility of this compact and low-cost approach. This could significantly broaden the applicability of NRTA, and make it practical and applicable in many fields, such as material science, nuclear engineering, and arms control.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Sensor response and radiation damage effects for 3D pixels in the ATLAS IBL Detector

Pixel sensors in 3D technology equip the outer ends of the staves of the Insertable B Layer (IBL), the innermost layer of the ATLAS Pixel Detector, which was installed before the start of LHC Run 2 in 2015. 3D pixel sensors are expected to exhibit more tolerance to radiation damage and are the technology of choice for the innermost layer in the ATLAS tracker upgrade for the HL-LHC programme. While the LHC has delivered an integrated luminosity of ≃ 235 fb -1 since the start of Run 2, the 3D sensors have received a non-ionising energy deposition corresponding to a fluence of ≃ 8.5 × 10 14 1 MeV neutron-equivalent cm -2 averaged over the sensor area. This paper presents results of measurements of the 3D pixel sensors' response during Run 2 and the first two years of Run 3, with predictions of its evolution until the end of Run 3 in 2025. Data are compared with radiation damage simulations, based on detailed maps of the electric field in the Si substrate, at various fluence levels and bias voltage values. These results illustrate the potential of 3D technology for pixel applications in high-radiation

47 OTHER INSTRUMENTATION↗

Report on Task USA A 0931 (A.252) Implementation of Fast, Front-End Electronics for Improved Low-Dead Time Neutron Counting

The International Atomic Energy Agency's (IAEA) Department of Safeguards is working on the elaboration and implementation of advanced Non-Destructive Assay (NDA) methods, generally known as neutron noise analysis, for the verification of critical and sub-critical cores containing substantial quantities of direct use nuclear material. These verification methods rely on interpreting time properties of the neutron multiplication process, which are to be extracted from measured neutron pulse trains. The interpretations are highly dependent on the quality of the measured data, which is directly related to the capability of an employed neutron detector to resolve very close detection events originating from neutron bursts produced in a highly multiplying medium. Therefore, the application of detectors with minimum dead-time, pile-up, and other distortion effects is required. This report describes the work under Task USA A 0931 (A.252 Implementation of fast, front-end electronics for improved low-dead time neutron counting).

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Medium Energy Nuclear Physics Research at the University of Richmond

The first part is a technical paper on the fitting techniques used to extract the neutron detec tion efficiency from the CLAS12 detector at the Thomas Jefferson National Accelerator Facility in Newport News, VA. The second is the masters thesis of Mr. Jude Buckley who also studied the neutron detection efficiency. He was a student at the University of Surrey in the UK and supported by the grant.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗