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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 289 records · Page 16

Helium Degassing Filter for Mercury Process Gas Liquid Separator

Testing was conducted to find a suitable filter to help separate helium gas from the Spallation Neutron Source’s mercury process loop. This filter is proposed for installation on the gas-liquid separator (GLS) vent line to prevent a column of liquid mercury from flowing outside of the process loop shielding in the service bay. The filter’s desired properties are to prevent the passage of liquid mercury, provide minimal resistance to helium flow, resist radiation, operate for the lifetime of the target, be replaceable, and have a reliable construction. Testing concluded that the Mott Corporation POU-10-S series of filters provided the best performance available. The filters could stop most liquid mercury passage while allowing helium passage at nominal pressures above the GLS in standard conditions. This result has several implications for the design of the GLS vent system.

Weinmeister, Justin↗

Implementation of Distributed Memory Computing in MOSAIC to Enable Large 3D Simulations of Irradiated Concrete

The concrete biological shield (CBS) of light-water reactors protects workers and the surrounding environment by absorbing neutron and gamma irradiation emitted from the reactor core. The radiation dose increases with the CBS’s operational time and, in the long term, becomes significant enough to raise the question of irradiation effects on concrete—and particularly on the structural integrity of the CBS. Irradiation-induced damage has been identified as one of the main degradation mechanisms in the CBS. Neutron radiation causes the swelling of aggregate-forming minerals at different rates and amplitudes depending on the mineral’s nature. Silicate-bearing minerals such as quartz are particularly sensitive to neutron radiation and experience up to 17.8% volumetric expansion. Aggregates comprise several minerals with different orientations and are, therefore, subject to cracking as a result of mismatch strains. Additionally, the swelling of aggregates creates significant stresses in the surrounding cement paste matrix, which also results in crack formation. In parallel with the collection of characterization and irradiation test data, development of modeling and simulation tools for irradiated concrete is ongoing with the support of the US Department of Energy Office of Nuclear Energy’s Light Water Reactor Sustainability (LWRS) program. This effort resulted in the development and application of the fast-Fourier transform (FFT)–based code Microstructure-Oriented Scientific Analysis of Irradiated Concrete (MOSAIC) at Oak Ridge National Laboratory.

61 RADIATION PROTECTION AND DOSIMETRY↗

Nuclear Interdiction Through Relocatable Detectors

The NNSA Office of Nuclear Smuggling Detection and Deterrence (NSDD) has investigated a set of minimal-infrastructure radiation detection systems as alternatives to fixed Radiation Portal Monitors (RPMs) for nuclear interdiction applications. These versatile and relocatable systems can improve nuclear security in missions or locations that do not warrant or support a standard fixed radiation detection system. Over 2019, a variety of relocatable detectors were characterized at the Interdiction Technologies Integration Laboratory at Pacific Northwest National Laboratory (PNNL). Evaluated detectors were diverse in their size and capabilities, ranging from backpack-sized systems to lane-spanning cargo scanning portals. Both spectroscopic and non-spectroscopic pedestrian and vehicle detection systems were characterized against uranium and plutonium sources. Signatures from the sources were modulated by both shielding and distance to quantify the performance of the relocatable systems as signal strength was decreased. Findings showed that relocatable spectroscopic detectors with isotope identification capabilities could reduce nuisance alarm rates compared to conventional fixed installation, gross-counting, radiation portal monitors. In vehicle scanning applications, detection ability generally trended with detection volume, regardless of spectral capability. In pedestrian scanning applications, several smaller backpack-sized detector systems were found to be more sensitive to detecting material than pedestrian portal monitors. The results of this characterization effort have helped inform the deployment of versatile equipment to improve nuclear security missions.

relocatable detectors, Nuclear Security↗

JWST Observations of Starbursts: Dust Processing in the M82 Superwind

We present JWST MIRI and NIRCam imaging of the inner ∼5 kpc of the M82 superwind at ~ $0''_{.}05 - 0''_{.}375$(∼0.9–6.5 pc) resolution. Targeted filters probe emission from polycyclic aromatic hydrocarbons (PAHs; F335M, F360M, F770W, F1130W) and continuum (F250M, F360M) The images reveal a network of cool wind filaments traced by PAHs. PAH surface brightness declines with the inverse square of distance to the midplane, suggesting that the incident radiation field from the starburst drives the observed PAH intensity out to ±2.5 kpc. The 3.3/11.3 and 3.3/7.7 μm band ratios show uniformity with distance from the starburst, though comparisons with mid-IR dust emission models indicate a modest shift toward larger PAHs. Outside the disk, 11.3/7.7 μm increases moderately, reflecting that PAHs become more neutral with distance from the starburst as they are exposed to a declining radiation field and ionization parameter. Overall, PAHs in the wind are consistent with standard-to-large sizes and standard-to-high ionization states. Including Spitzer and Herschel data, PAH abundance (q PAH ) is set at ∼1% in the starburst and remains unchanging out to ±5 kpc off the disk. This flat q PAH profile suggests that PAHs are shielded from the hot wind, perhaps residing in the surface layers of cool clouds, with possible replenishment from cloud interiors and enrichment of the halo from previous bursts. In this picture, clouds are not dense enough to promote PAH growth, and they likely undergo radiative cooling and mixing with the hot phase to survive the gauntlet for at least ∼20 Myr.

Cronin, Serena A. [University of Maryland, College↗

Small scale electron linear accelerators for industrial applications

Linear accelerators (linacs), producing electron or X-ray radiation in the MeV range, are critical tools for industrial irradiation, medical device sterilization, food pasteurization, non-destructive testing, security, medical, and many other applications. Many of these applications require compact and flexible radiation sources. In this paper, we present new technologies for small-scale electron linear accelerators and examples of their practical implementations. Furthermore, these developments include low energy accelerators with self-shielding options and form factors, ranging from cabinet-size to hand-portable generators; medium-energy accelerators for novel radiotherapy and security applications; and high-energy 10 MeV linacs capable of reaching 20–35 kW beam power for emerging industrial and phytosanitary applications

43 PARTICLE ACCELERATORS↗

Experiments for SINBAD: Evaluation of Oak Ridge Health Physics Research Reactor Operation Data for CAAS Benchmark Creation [Slides]

This report was a real information preservation and dissemination work with a lot of legacy content that was found and used. There was an abundance of uncertainty, discrepancy, and contradictory information. Yet, a detailed, functional SCALE model was built, and the benchmark created is useful for shielding and CAAs validation work. Sulfur fluence C/E ratios are large (2 to 5), so different benchmark metrics were studied. Neutron fluence, element 57 dose, and other dosimetry responses at 3 meters C/E ratios are below 1.5 for bare and steel configurations. Additional promising metrics as dose per unit fluence and steel shield attenuation were computed.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Demonstration of the On-the-Fly Shielding Analysis Method: Spent Fuel and Waste Disposition

This report documents work performed supporting the US Department of Energy (DOE) Office of Nuclear Energy (NE) Spent Fuel and Waste Disposition (SFWD) Integrated Waste Management activities under work breakdown structure element 1.08.02.04.01, “Data and Tools Development, Validation, and Maintenance.” In particular, this report fulfills milestone M3SF-21OR020401016, “Implement on-the-fly dose analysis methodology in UNF-ST&DARDS” within work package SF-21OR02040101, “Commercial SNF Characterization - ORNL.” The Used Nuclear Fuel - Storage, Transportation & Disposal Analysis Resource and Data System (UNFST& DARDS) enables automated dose rate calculations for spent nuclear fuel (SNF) transportation packages and storage casks using a Monte Carlo radiation transport code. The explicit method uses a detailed model of the SNF system and its contents. Therefore, a dose rate calculation is required for each as-loaded transportation package or storage cask because the SNF assemblies within a canister typically have unique irradiation characteristics. An alternate method, referred to as the “on-the-fly” shielding analysis method, has been proposed that requires only a set of Monte Carlo dose rate calculations for each transportation packaging/storage cask design. The results of the Monte Carlo dose rate calculations are independent of the SNF assembly irradiation and decay characteristics. The dose rate values may then be combined with the radiation source strength of the SNF assemblies associated with a particular transportation packaging/storage cask design to determine actual dose rates. This report presents on-the-fly dose rate calculations for a representative SNF storage cask and verification of the on-the-fly dose rate calculation results by comparison with reference dose rate calculations using the explicit Monte Carlo dose rate calculation. The on-the-fly shielding analysis method was implemented in UNF-ST&DARDS. A Python program was developed to process the MAVRIC dose rate results obtained by source particle type, energy group, and fuel geometry region. A Python processor created binary files, which were saved as a special UNF-ST&DARDS library for on-the- fly shielding analyses. UNF-ST&DARDS uses the precalculated on-the-fly binary libraries generated by the Python data processor and directly executes the Python code for on-the-fly dose analysis. This Python code unzips the pre-generated binary files mentioned above, reads the data, and combines them with user-specified sources for dose and uncertainty calculations. The Python programs were verified using Excel calculations and by comparison with the values obtained with the MAVRIC post-processing utilities applied to the 3dmap files. This method can currently be used to determine dose rates for as-loaded HI-STORM FW storage casks. The UNF-ST&DARDS analysis wizard for on-the-fly shielding analysis is described in this report.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Results for Gamma-Ray Spectroscopy Characterization of Residual Radioactivity on Personal Protective Clothing

In early 2019, Health Physics Services (HPS) personnel put together a test plan to use the shielded gamma-ray spectroscopy instruments in the Health Physics Services Technical Laboratory (HPSTL) to perform a series of measurements on laundered personal protective clothing used in radiological areas at the Savannah River Site (SRS). That test plan describes the methodology used to determine the quantities of laundry to be obtained from operational facilities, the methods for quality control checking the instruments throughout the measurement period, and the physical arrangement of samples in the counting shields. The test plan is documented in SRNS-J6700-2019-00037 (Reference 1).

61 RADIATION PROTECTION AND DOSIMETRY↗

Modelling Tritium Production and Release at High-Energy Proton Accelerators

Tritium is a well-known byproduct of particle accelerator operations. To keep levels of tritium below regulatory limits, tritium production is actively monitored and managed at Fermilab. We plan to study tritium production in the targets, beamline components, and shielding elements of the Fermilab facilities such as NuMI, BNB, and MI-65. To facilitate the analysis, we construct a simple model and use three Monte Carlo radiation codes, FLUKA, MARS, and PHITS, to estimate the amount of tritium produced in these facilities. The analysis could also serve as an intercomparison between these code results related to tritium production. To assess the actual amounts of tritium that would be released from various materials, we employ a semi-empirical diffusion model. The results of this analysis are compared to experimental data whenever possible. This approach also helps to optimize proposed target materials with respect to the tritium production and release.

Georgobiani, Dali [Fermilab]↗

Evaluation of Oak Ridge National Laboratory Health Physics Research Reactor Operation Data for Critical Benchmark Creation [Abstract]

The Oak Ridge National Laboratory (ORNL) Health Physics Research Reactor (HPRR) was a research reactor designed and built at ORNL in 1961. The critical assembly was using a highly enriched uranium and molybdenum alloy as the fuel, and it could be operated in steady-state or burst modes. The reactor was used for about 25 years to produce a lot of publications related to dosimetry, radiobiology and radiation detectors testing before its decommissioning in 1987. In recent years, the idea of using legacy operation data from the to create a valuable critical accident alarm system shielding benchmark arose. Such a benchmark has been submitted to the International Criticality Safety Benchmark Experiment Project (ICSBEP) Technical Review Group for a potential inclusion in the 2022 version of the handbook. Another way to use the valuable data from the operation of the HPRR is to evaluate the feasibility of the creation of a subcritical or prompt supercritical benchmark for inclusion in the ICSBEP or the International Reactor Physics Experiments Evaluation Project (IRPhEP) handbooks. To initiate a burst, the HPRR had to be operated in a slightly subcritical state for a few minutes. Then, the insertion of the burst control rod would greatly increase the reactivity of the system and start the burst. No critical configuration of the HPRR critical assembly could be located. The only information available concerns stable subcritical and prompt supercritical states, found in a burst experiments’ logbook. In the recovered logbook pages, information about 8 different bursts is available. The information includes the rods positions before and during a burst, the recorded subcritical reactor period and reactivity, and the burst fission yield derived from the temperature elevation sulfur pellet irradiation analysis. By using the HPRR logbook information and the as-built drawings of the critical assembly, a highly detailed model of the HPRR was created with SCALE 6.2.4/KENO-VI. Eight KENO-VI models were created to replicate the sub-critical assembly configurations described in the eight bursts from the recovered logbook pages. KENO-VI calculates k eff and it can be linked to a reactivity value in cents by using the delayed neutron fraction B eff , also calculated by KENO-VI. KENO-VI can also be used to model the prompt super-critical configurations of the HPRR and to assess the similarity with the burst measurements by comparing the calculated k eff and the measured fission yields between each burst. Unfortunately, high uncertainty exist and the obtained discrepancies between experiments and calculation results are high, compromising the creation of a valuable critical benchmark from HPRR operation data. The reasons of the discrepancies and potential ways to solve them are explored.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Health Physics Research Reactor Criticality Accident Alarm System Benchmark Overview [Slides]

This presentation discusses the Health Physics Research Reactor (HPRR) or Fast Burst Reactor (FBR) and how available data from Health Physics Research Reactor (HPRR) operation to can be used to create a benchmark report for inclusion in the ICSBEP, as a Criticality Accident Alarm System (CAAS) shielding benchmark. The evaluation of experimental data is also presented, specifically four experimental candidates are considered of potential value for the benchmark: 1. Neutron source estimation from a HPRR pulse (energy spectrum, fission yield), 2. Threshold Detector Unit (TDU) measurements at different distances from a HPRR pulse, shielded and unshielded, 3. Sulfur pellet activation at different distances from a HPRR pulse, shielded and unshielded, and 4. Total neutron fluence from a HPRR pulse measured by Bonner Sphere Spectrometry, shielded and unshielded. Additionally, a benchmark model overview is discussed as are sample calculation results.

61 RADIATION PROTECTION AND DOSIMETRY↗

Fuel Assembly Reference Information for SNF Radiation Source Term Calculations

This report consolidates publicly available information related to pressurized water reactor (PWR) and boiling water reactor (BWR) nuclear fuel physical characteristics and operating conditions. The intent of this report is to provide reference information for use in shielding analyses of spent nuclear fuel transportation packages and storage casks.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Shielding Thickness Recommendations for an Activated Target Segment Vertical Stave

This analysis examines the shielding requirements needed to plan maintenance and handling operations of the target segment assembly vertical stave. It provides the analyses and results that fulfill the requirements of Task Order TO-150. The vertical stave is a stainless-steel welded assembly that carries cooling water to and from the target block. In this report, we characterize the dose rates and shielding requirements for the vertical stave only, i.e., separated from the target block. Shielding and dose rates for the target block only have been calculated in response to TO-008.

61 RADIATION PROTECTION AND DOSIMETRY↗

Parametric model-order reduction for radiation transport using multi-resolution proper orthogonal decomposition

For parametric high-fidelity simulations, it is often desirable to utilize a reduced-order model (ROM) to emulate, at a reduced computational cost, parametric solutions of the governing partial differential equations (PDEs) for unseen parameter values. One commonly employed option is to utilize a data-driven, projection-based ROM supplemented with subspace identification via proper orthogonal decomposition (POD). POD discovers the ROM subspace by computing the singular value decomposition (SVD) of a set of training data from the full-order model (FOM). In streaming-dominated radiation transport simulations with localized sources, solutions often greatly vary over the spatial domain by many orders of magnitude. In such cases, machine-precision arithmetic can be insufficient to obtain an accurate SVD, resulting in a poorly performing ROM. We present a method called multiresolution POD (mrPOD) that mitigates these inaccuracies. The mrPOD method works by decomposing the spatial domain into regions and performing proper orthogonal decomposition on the training dataset separately in each region. In conclusion, mrPOD is tested on single energy group and multigroup atmospheric shielding transport problems and is shown to outperform classic POD.

42 ENGINEERING↗

Changing the Rules of the Game: Used Fuel Studies Outside of a Remote Handling Facility

Recent advances in micro-fabrication tools like the FEI Helios NanoLab 660 dual Focused Ion Beam (FIB) and Scanning Electron Microscope (SEM) now make it possible to easily and reliably prepare micron (or smaller) specimens for analyses or further experimentation. Pacific Northwest National Laboratory (PNNL) has leveraged this capability at the Category II Nuclear Facility, the Radiochemical Processing Laboratory, to facilitate nuclear materials analysis and experimentation of used nuclear fuel. Micron-scale specimens of un-irradiated UO2 fuel pellets of various enrichments from depleted to 4.95% enriched, relative to 235U, were prepared at PNNL and shipped to the University of Missouri’s Research Reactor (MURR) for irradiation. Prior to shipping, samples were attached to commercially available Transmission Electron Microscopy half-grids via ion deposition, which were then housed in specially designed aluminum sample holders approved for use at the reactor facility. This minimized handling and preparation requirements prior to materials analysis after irradiation. Samples were irradiated to a burnup equivalent of 8 – 3,700 MWd/MTU. Additionally, by reducing the size of the specimens, and therefore their emitted radiation dose, the required cooling time after irradiation and prior to analysis was greatly diminished, and handling of these samples could proceed outside of a hot cell facility. Results from these experiments provided insight into the initial production of noble metal phase particles in used nuclear fuel at extremely low burnup levels. Some incompatibility with the container was observed at higher burnup. Micro-scale irradiation experiments were performed at roughly 1/7th of the time, effort and expense a similar bulk-scale study requiring a shielded hot cell facility would require. Conducting nuclear materials analysis at the micron-scale holds the promise of enhancing collaboration and material accessibility to the broader research community, improving accessibility to cutting edge research tools by the nuclear materials science community, lowering the risk to the scientist by reducing radiation dose and exposure, reducing facility and research costs associated with the requirement to conduct nuclear materials science within glovebox or remote handling facilities, and minimizing waste.

Schwantes, Jon M.↗

Development of a High-Energy Neutron Sniffer and Subsequent Dose Quantification for High-Energy Particle Accelerator Shielding Surveys

The objective of this research is to design a portable neutron detector that is lightweight and responds to neutrons with energies of 20 MeV and greater. The instrument will be used as a ‘sniffer’ probe for identifying shielding weaknesses at high-energy particle accelerators and be paired with a plastic scintillator to quantify the high-energy neutron dose equivalent. The sniffer probes are two different sizes and comprised of either cesium iodide or sodium iodide, all doped with thallium, making a total of four detectors. The probes were calibrated to respond only to radiations with 8 MeV electron equivalent energy or higher, vastly reducing detector response from background and lower energy radiations. The sniffer probes were tested using californium- 252 and americium-beryllium sources, followed by high-energy (up to 800 MeV) neutron exposures at the Los Alamos Neutron Science Center Weapons Neutron Research (WNR) facility. The sniffer probes were then used to identify areas around the accelerator facility where elevated levels of high-energy radiation was present and the plastic scintillators were placed in these locations to determine the high-energy neutron dose equivalent. The dose equivalent is calculated by measuring the 12 C(n,2n) 11 C reaction, which has a 20.4 MeV neutron threshold. Two locations behind the WNR facility were identified with the probes and the dose equivalent rates from neutron energies above 20 MeV were calculated to be 1.24 mrem/h behind flightpath 30-left and 1.53 behind flightpath 30-right. Of the four sniffer probes, the 2-inch x 2-inch cesium iodide is the recommended probe for performing high-energy shielding surveys. The larger crystal size yields higher sensitivity at lower count rates and the more dense material increases the likelihood of interaction within the crystal.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗