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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 307 records · Page 17
All sourcesNASA NTRSDOE OSTI
NASA NTRS1974

Two views of cosmic ray propagation in the solar system

Diffusion and scatter free cosmic ray propagation theories are discussed in terms of the quality of their alternate viewpoints. A hypothetical model of conditions in interplantary space is described which aids in the comparison. A plot of the intensity of the interplanetary magnetic field over a long period is presented, and the association of these regions with high velocity streams is shown to support the scatter free viewpoint.

Barouch, E.↗
NASA NTRS1979

An 'adding' algorithm for the Markov chain formalism for radiation transfer

An adding algorithm is presented, that extends the Markov chain method and considers a preceding calculation as a single state of a new Markov chain. This method takes advantage of the description of the radiation transport as a stochastic process. Successive application of this procedure makes calculation possible for any optical depth without increasing the size of the linear system used. It is determined that the time required for the algorithm is comparable to that for a doubling calculation for homogeneous atmospheres. For an inhomogeneous atmosphere the new method is considerably faster than the standard adding routine. It is concluded that the algorithm is efficient, accurate, and suitable for smaller computers in calculating the diffuse intensity scattered by an inhomogeneous planetary atmosphere.

Esposito, L. W.↗
NASA NTRS1981

Mechanisms for intense relativistic electron precipitation

An analysis of data gathered over a period of 14 months by the S3-3 satellite has revealed the detection of 313 relativistic electron precipitation events with isotropic flux over the upward-looking hemisphere, of which the majority occur at night in a narrow latitudinal zone which is embedded within a broader region of intense energetic ion precipitation. Three classes of precipitation are found to be associated with strong, diffusion resonant scattering due to known magnetospheric plasma waves. It is also found that intense electron energy deposition is a major source of middle-atmospheric, odd-hydrogen and odd-nitrogen molecules at sub-auroral latitudes, leading to an observable catalytic destruction of mesospheric ozone.

Thorne, R. M.↗
NASA NTRS1984

Morphology of the scattering targets: Fresnel and turbulent mechanisms, part 2.1A

Refractive index fluctuations cause coherent scattering and reflection of VHF radio waves from the clear air in the altitude region between 0 and approximately 90 km. Similar echoes from the stratosphere/troposphere and the mesosphere are observed at UHF and MF/HF frequencies, respectively. The nature of the refractive index fluctuations has been studied for many years without producing a clear consensus on what mechanism causes them. It is believed that the irregularities can originate from two different mechanisms: turbulent mixing of the gradient of refractive index, and stable horizontally stratified laminae of sharp gradients in the refractive index. In order to explain observations of volume dependence and aspect sensitivity of the echo power in the MST region, a diversity of submechanisms has been proposed. They include isotropic and anisotropic turbulent scattering, Fresnel scattering and reflection, and diffuse reflection. Isotropic turbulent scattering is believed to cause a majority of the clear air echoes observed by MST radars. The mechanism requires active turbulence mixing of a preexisting gradient in the refractive index profile.

Royrvik, O.↗
NASA NTRS1991

VUV-induced degradation of FEP Teflon aboard LDEF

Examination of fluorinated ethylene propylene (FEP) copolymer materials recovered from the Long Duration Exposure Facility (LDEF) reveals differing damage characteristics on leading edge (ram-facing) versus trailing edge (wake-facing surfaces). Silver/Teflon (Ag/FEP) thermal control materials on ram facing surfaces of the LDEF exhibited obvious degradation, with an apparent increase in diffuse light scattering, whereas identical materials on the wake facing surfaces showed little apparent damage with cursory inspection. Microscopic examination of both types of surfaces reveals the nature and extent of environment induced degradation of materials. The ram facing surfaces were clearly eroded by atomic oxygen impingement, while the wake facing material developed a thin, highly embrittled surface layer.

Brinza, David E.↗
NASA NTRS1994

Energetic and radiative constraints on highly relativistic jets

We examine constraints on the energetics and radiative efficiencies of highly relativistic, synchrotron-emitting jets. If the observed intraday radio variability of compact radio sources is intrinsic and results from incoherent synchrotron radiation, then the associated jets must have bulk Lorentz factors in the range Gamma varies approximately 30 to 100, several times larger than the largest values inferred from superluminal expansion, and larger even than the values required to avoid the synchrotron self-Compton catastrophe. We show that such highly relativistic jets produce synchrotron radiation with extremely low radiative efficiency. As a result they must carry enormous kinetic energy fluxes, L(sub j) approximately greater than 10(exp 47)(Delta Omega/0.1 sr), where Delta Omega is the solid angle subtended by the jet, in order to produce 'apparent' synchrotron brightness temperatures approximately greater than 10(exp 16) K. Energy losses by such jets should be strongly dominated by Compton scattering of diffuse ambient radiation, and they should produce large X-ray and gamma-ray fluxes.

Begelman, Mitchell C.↗
NASA NTRS2004

Photophysics of Laser Dye-Doped Polymer Membranes for Laser-Induced Fluorescence Photogrammetry

Laser-induced fluorescence target generation in dye-doped polymer films has recently been introduced as a promising alternative to more traditional photogrammetric targeting techniques for surface profiling of highly transparent or reflective membrane structures. We investigate the photophysics of these dye-doped polymers to help determine their long-term durability and suitability for laser-induced fluorescence photogrammetric targeting. These investigations included experimental analysis of the fluorescence emission pattern, spectral content, temporal lifetime, linearity, and half-life. Results are presented that reveal an emission pattern wider than normal Lambertian diffuse surface scatter, a fluorescence time constant of 6.6 ns, a pump saturation level of approximately 20 micro J/mm(exp 2), and a useful lifetime of more than 300,000 measurements. Furthermore, two demonstrations of photogrammetric measurements by laser-induced fluorescence targeting are presented, showing agreement between photogrammetric and physically measured dimensions within the measurement scatter of 100 micron.

Dorrington, Adrian A.↗
NASA NTRS2023

The Calipso Version 4.5 Stratospheric Aerosol Subtyping Algorithm

The accurate classification of aerosol types injected into the stratosphere is important to properly characterize their chemical and radiative impacts within the Earth climate system. The updated stratospheric aerosol subtyping algorithm used in the version 4.5 (V4.5) release of the Cloud Aerosol Lidar with Orthogonal Polarization (CALIOP) level 2 data products now delivers more comprehensive and accurate classifications than its predecessor. The original algorithm identified four aerosol subtypes for layers detected above the tropopause: volcanic ash, smoke, sulfate/other, and polar stratospheric aerosol (PSA). In the revised algorithm, sulfates are separately identified as a distinct, homogeneous subtype, and the diffuse, weakly scattering layers previously assigned to the sulfate/other class are recategorized as a fifth “unclassified” subtype. By making two structural changes to the algorithm and revising two thresholds, the V4.5 algorithm improves the ability to discriminate between volcanic ash and smoke from pyrocumulonimbus injections, improves the fidelity of the sulfate subtype, and more accurately reflects the uncertainties inherent in the classification process. The 532 nm lidar ratio for volcanic ash was also revised to a value more consistent with the current state of knowledge. This paper briefly reviews the previous version of the algorithm (V4.1 and V4.2) then fully details the rationale and impact of the V4.5 changes on subtype classification frequency for specific events where the dominant aerosol type is known based on the literature. Classification accuracy is best for volcanic ash due to its characteristically high depolarization ratio. Smoke layers in the stratosphere are also classified with reasonable accuracy, though during the daytime a substantial fraction are misclassified as ash. It is also possible for mixtures of ash and sulfate to be misclassified as smoke. The V4.5 sulfate subtype accuracy is less than that for ash or smoke, with sulfates being misclassified as smoke about one-third of the time. However, because exceptionally tenuous layers are now assigned to the unclassified subtype and the revised algorithm levies more stringent criteria for identifying an aerosol as sulfate, it is more likely that layers labeled as this subtype are in fact sulfate compared to those assigned the sulfate/other classification in the previous data release.

Jason L Tackett↗
DOE OSTI2023

Incoherent Dynamics of Intense Proton Beams Under Electron Cooling

The minimum emittance of ion beams achieved using electron cooling is limited by the heating processes of Intra Beam Scattering and diffusion driven by resonance crossing of particles due to space-charge. We describe a new experiment to explore the intense space-charge regime with a transverse tune shift approaching -0.5 using 2.5 MeV protons at the Integrable Optics Test Accelerator (IOTA) at Fermilab. We also report on the results from PyORBIT simulations incorporating transverse space-charge and electron cooling with emphasis on the incoherent dynamics of the particles.

43 PARTICLE ACCELERATORS↗
NASA NTRS2007

Effect of EMIC Wave Normal Angle Distribution on Relativistic Electron Scattering in Outer RB

We present the equatorial and bounce average pitch angle diffusion coefficients for scattering of relativistic electrons by the H+ mode of EMIC waves. Both the model (prescribed) and self consistent distributions over the wave normal angle are considered. The main results of our calculation can be summarized as follows: First, in comparison with field aligned waves, the intermediate and highly oblique waves reduce the pitch angle range subject to diffusion, and strongly suppress the scattering rate for low energy electrons (E less than 2 MeV). Second, for electron energies greater than 5 MeV, the |n| = 1 resonances operate only in a narrow region at large pitch-angles, and despite their greatest contribution in case of field aligned waves, cannot cause electron diffusion into the loss cone. For those energies, oblique waves at |n| greater than 1 resonances are more effective, extending the range of pitch angle diffusion down to the loss cone boundary, and increasing diffusion at small pitch angles by orders of magnitude.

Khazanov, G. V.↗
DOE OSTI2026

Integrated Strategies for Overcoming Resolution Limits in Electron Beam Lithography of Chemically Amplified Resists

Electron beam lithography (EBL) of chemically amplified resists (CARs) faces fundamental challenges, including stochastic electron scattering and acid diffusion, that limit resolution and reproducibility. Using SU-8 as a model CAR, this study systematically investigated complementary strategies to address these challenges, combining multipass exposure, proximity effect correction (PEC) with midrange correction factors, base quencher incorporation, and post-exposure bake (PEB) suppression. Monte Carlo simulations and calibrated PEC modeling revealed that extending the point spread function to include a midrange scattering component significantly improved critical dimension (CD) control across varying pattern densities, correcting deviations that conventional two-term PEC failed to capture. Multipass exposure, particularly 4-pass writing with a 25% offset, redistributed the dose to average stochastic beam and scattering fluctuations, reducing line-width roughness by more than 50% and yielding more uniform nanoscale features. Photoacid confinement was investigated by adding urea as a base quencher, which successfully reduced acid diffusion but introduced substantial sensitivity penalties without improving ultimate resolution or Z-factor performance, underscoring the trade-offs of chemical versus physical confinement. Suppressing PEB most directly minimized acid diffusion, resulting in improved Z-factors and reproducible 30 nm half-pitch dense line/space patterns. Overall, these results demonstrated that PEC with midrange correction, multipass strategies, quencher additives, and PEB-free processing addresses different aspects of the EBL process window and that their integration provides a comprehensive framework for managing stochastic scattering, diffusion, and chemical amplification effects. This framework advances dense nanoscale patterning in CARs and establishes guiding principles for optimizing resist design and process strategies in high-resolution EBL and potentially other advanced lithographies, such as extreme ultraviolet (EUV) lithography.

36 MATERIALS SCIENCE↗
DOE OSTI2022

Li-Ion Diffusion Correlations in LiAlGeO 4 : Quasielastic Neutron Scattering and Ab Initio Simulation

Here, we investigated the impact of Li stoichiometry and host flexibility on Li + diffusion processes in LiAlGeO 4 at the microscopic level using quasielastic neutron scattering (QENS) and ab initio molecular dynamics (AIMD) simulations. Using sufficiently long AIMD trajectories, we could simulate the observed QENS signal and identify the localized dynamics of Li in crystalline LiAlGeO 4 . Such information is vital to identify the bottleneck of diffusion processes and design materials for battery application. Our AIMD simulations in LiAlGeO 4 reveal that the Li + conductivity can be significantly improved by manipulating the Li stoichiometry and/or host flexibility via amorphization. We determined that excess Li stoichiometry enhances the Coulomb repulsion of neighboring Li sites and softens the host structure to enable faster Li + diffusion along the hexagonal c-axis. In the amorphous structure, random orientations of AlO 4 and GeO 4 polyhedral units create a wide distribution of intersite distances and significantly soften the host structure, greatly enhancing the Li + diffusion. The simulations are used to understand the nature of diffusion, especially the role of the host structure, the possible hopping pathways, and the diffusion behavior in various structures of LiAlGeO 4 .

localized dynamics↗
DOE OSTI2021

Stoichiometric tuning of lattice flexibility and Na diffusion in NaAlSiO 4 : quasielastic neutron scattering experiment and ab initio molecular dynamics simulations

We have performed quasielastic neutron scattering (QENS) experiments up to 1243 K and ab initio molecular dynamics (AIMD) simulations to investigate the Na diffusion in various phases of NaAlSiO4 (NASO), namely, low-carnegieite (L-NASO; trigonal), high-carnegieite (H-NASO; cubic) and nepheline (N-NASO; hexagonal) phases. The QENS measurements reveal Na ions localized diffusion behavior in L-NASO and N-NASO, but long-range diffusion behavior in H-NASO. Furthermore, the AIMD simulation supplemented the QENS measurements and showed that excess Na ions in H-NASO enhance the host network flexibility and activate the AlO 4 /SiO 4 tetrahedra rotational modes. These framework modes enable the long-range diffusion of Na across a pathway of interstitial sites. The simulations also show Na diffusion in Na-deficient N-NASO through vacant Na sites along the hexagonal c-axis.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
NASA NTRS1993

Comparative accuracy of diffuse radiative properties computed using selected multiple scattering approximations

Computational results have been obtained for the spherical albedo, global transmission, and global absorption of plane-parallel layers composed of cloud droplets. These computations, obtained using the doubling method for the entire range of single scattering albedos and for optical depths between 0.1 and 100, are compared with corresponding results obtained using selected multiple scattering approximations. The spherical albedo and global absorption computed using asymptotic theory are found to be accurate to better than 5 percent for all values of the single scattering albedo, provided the optical thickness exceeds about 2. The diffuse two-stream approximations have relative accuracies that are much worse than 5 percent for the spherical albedo over most of the parameter space, yet are accurate to within 5 percent in the global absorption when the absorption is significant. The integrated delta-Eddington scheme appears to be the most suitable model over the entire range of variables, generally producing relative errors of less than 5 percent in both the spherical albedo and global absorption.

HARSHVARDHAN↗
NASA NTRS1992

Laser scattering in a hanging drop vapor diffusion apparatus for protein crystal growth in a microgravity environment

One type of hardware used to grow protein crystals in the microgravity environment aboard the U.S. Space Shuttle is a hanging drop vapor diffusion apparatus (HDVDA). In order to optimize crystal growth conditions, dynamic control of the HDVDA is desirable. A critical component in the dynamically controlled system is a detector for protein nucleation. We have constructed a laser scattering detector for the HDVDA capable of detecting the nucleation stage. The detector was successfully tested for several scatterers differing in size using dynamic light scattering techniques. In addition, the ability to detect protein nucleation using the HDVDA was demonstrated for lysozyme.

Casay, G. A.↗
NASA NTRS1999

Radiative Smoothing in Clouds at Transparent and Absorbing Wavelengths

For absorbing and transparent wavelengths, we discuss the effect of horizontal solar radiative fluxes in clouds on the accuracy of a conventional plane-parallel radiative transfer calculations for a single pixel, known as the Independent Pixel Approximation (IPA). We address the question of correlations between horizontal fluxes, IPA accuracies and radiative smoothing. By smoothing we understand a radiative transfer process whereby radiation does not follow the small-scale fluctuations of cloud structure, producing much smoother radiation fields. The scale eta that characterizes this process is called "radiative smoothing scale." We relate radiative smoothing to the photon's horizontal displacement that characterizes a "spot" of reflected light associated with a point source. We generalize the "spot-size" estimate derived for conservative scattering using the diffusion theory to the case of non-conservative scattering. For reflected light, theoretical results are confirmed with numerical simulations. The radiative smoothing scale eta is a critical value where IPA effectively breaks down; for scales smaller than TI, real radiation field are much smoother than their IPA counterparts for the same cloud structure. In addition to the estimate of il for absorbing wavelengths, we show that: (1) with more absorption, the scale break determined by eta in a log-log plot of wavenumber spectra moves towards smaller scales and (2) the smaller eta the flatter the small-scale slope which means less radiative smoothing, thus more accuracy in the IPA reflection.

Marshak, A.↗
DOE OSTI2022

A Cartesian-diffusion Langevin method for hybrid kinetic-fluid Coulomb scattering in particle-in-cell plasma simulations

A novel, drag-diffusion Langevin method of hybrid, kinetic-fluid Coulomb scattering in plasmas is presented. Unlike previous methods, the frictional drag is always applied in the simulation frame of reference. The velocity-space diffusion is performed in the stationary-fluid frame of reference when anisotropic, and in the laboratory frame when isotropic. While the general method is mass-ratio independent, we focus on interactions of kinetic-ions and fluid-electrons to show first-order modifications to the electron velocity distribution function that are an important correction for the accurate calculation of electric resistivity. Inclusion of sub-cycling and a limit to the maximum collision frequency is shown to allow for arbitrarily large timesteps without numerical failure. Here the Langevin method is compared with a grid-based binary method and found to require a much less restrictive timestep in cases of ion–electron slowing and temperature equilibration; this finding differs from previous work and is dependent on the mass ratio.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗