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At least 37 records · Page 2

The Need for a New LLNL Pulsed Sphere Neutron Leakage Spectra Series

Here, it is shown that spectra measured as part of the Lawrence Livermore National Laboratory Pulsed Sphere (LPS) program offer decisive information to locate formatting or physics issues in nuclear data of key interest for fusion reactor simulations. However, experiments from this measurement series are not benchmarks. For instance, their uncertainties are incomplete. There are also many open questions—e.g., on the setup, the detector response, and whether LPS are accurately modeled—that cannot be answered anymore given the limited documentation and that many of the experimenters are no longer actively working. This limited knowledge has implications when one tries to adjust nuclear data to LPS spectra. Usually, one adjusts to benchmarks representing an application with the hope to get more precise nuclear data for the application of interest where differential data might be scarce and/or to reduce nuclear data uncertainties in the application simulations. However, it is demonstrated that adjustment with LPS spectra without accounting for missing uncertainties and modeling potential biases in the experimental data leads to adjusted data that are highly unphysical. That means adjusted data differ significantly from evaluated data based on information from differential experiments; also, application quantities predicted with the adjusted data deviate distinctly from experimental ones. While we can approximate our limited knowledge on these experiments with Gaussian processes in the adjustment process, this modeling of bias is arbitrary rather than based on a physics explanation, calling into doubt the validity of resulting adjusted data. Thus, we discuss here the need for a new measurement series, learning from the strengths and weaknesses of the LPS program, to yield decisive and well-benchmarked integral experiments to support fusion reactor research.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Differential and Integral Data Evaluation for Titanium: An Application to Criticality Safety

The intent of this work is to highlight the role of differential and integral data evaluation to address issues in connection with criticality safety applications. Demonstration is made by using, as an example, differential data measurements and evaluation, and the benchmark integral experiments for titanium. Energy differential data are measured analyzed and evaluated to produce nuclear data libraries for criticality safety applications. Alternatively, integral experiments are performed at critical facilities, small experimental reactors, and play an important part in the validation of the differential nuclear data. The demonstration provided here for titanium gives its importance to criticality safety. Titanium is an effective neutron absorber that serves as baseline material for chemical separation in high-activity waste solutions in US. Titanium has not been considered for use in nuclear applications such as reactor design and analysis. Rather, it appears as a structural material that may be present in fuel cycle facilities or canisters for transport and disposition of nuclear waste. Criticality safety evaluations of systems in which titanium is present require an understanding of the nuclear data and its uncertainty.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Chapter 4 - Recent Advances in Identification of Differential Equations from Noisy Data: IDENT Review

Differential equations and numerical methods are extensively used to model various real-world phenomena in science and engineering. With modern developments, we aim to find the underlying differential equation from a single observation of time-dependent data. If we assume that the differential equation is a linear combination of various linear and nonlinear differential terms, then the identification problem can be formulated as solving a linear system. The goal then reduces to finding the optimal coefficient vector that best represents the time derivative of the given data. We review some recent works on the identification of differential equations. We find some common themes for the improved accuracy: (i) The formulation of linear system with proper denoising is important, (ii) how to utilize sparsity and model selection to find the correct coefficient support needs careful attention, and (iii) there are ways to improve the coefficient recovery. We present an overview and analysis of recent developments on the topic.

97 MATHEMATICS AND COMPUTING↗

Investigation of Benchmark $k$ eff Sensitivity and Uncertainty for 239 Pu fission in Specific Energy Ranges

Nuclear data at intermediate energies (from 1 to 100s of keV) are evaluated based on scarce differential data and theory unable to capture physics’ expected structure. There is also a lack of integral data. This is a known deficiency and is challenging to address. Calculated effective multiplication factor, k eff , values for intermediate energy experiments are ~25× further from experiment than for fast energies and are often well outside the experimental uncertainties. The goal of the PARADIGM (PARallel Approach of Differential and InteGral Measurements) project is to significantly re duce the uncertainties of intermediate energy nuclear data for 239 Pu. To this end, PARADIGM simultaneously optimizes experiments at both the Los Alamos Neutron Science Center (LANSCE) and National Criticality Experiments Research Center (NCERC). The combined set of data will inform new intermediate-energy nuclear data. By execution of differential and integral experiments, establishment of new theory, and undertaking nuclear data evaluation in parallel, the timeline to deliver improved nuclear data to users will be reduced significantly that is to three years. For the PARADIGM project, it was decided to optimize an integral experiment for two neutron energy ranges, within the full intermediate energy range. The low energy range goes from 1 to 30 keV, while the higher energy range goes from 30 to 600 keV. This work focuses on nuclear data sensitivities and uncertainties for 239 Pu fission for existing experiments in the International Criticality Safety Benchmark Evaluation Project (ICSBEP). When designing new experiments, it is important to understand what benchmarks currently exist. For a more traditional experiment design (in which a specific application model(s) exists), comparisons would be made between the application model(s) and existing benchmarks. For PARADIGM, there is no specific application model, but instead the specific nuclear data reaction and energy ranges of interest can be explored for existing benchmarks.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Nuclear Data and Benchmarking Program: Nuclear Data Performance Assessment for Advanced Reactors

Over the last several Evaluated Nuclear Data File (ENDF)/B releases, many updates have been introduced to the nuclear data libraries that can significantly change computational results. These changes can be particularly important for advanced reactor concepts, which are not as thoroughly investigated as those used in light water reactor (LWR) systems. Therefore, a performance assessment of the ENDF/B libraries using the SCALE 6.2.3 code package was conducted under the auspices of the U.S., Department of Energy Office of Nuclear Energy (DOE-NE). The following systems relevant to the advanced reactor community were chosen as subject for investigation in this report: sodium cooled fast reactor systems, graphite moderated high temperature gas-cooled reactors, and several molten salt reactor models. At first, the similarity of the integral performance of the ENDF/B-VII.1 and ENDF/B-VIII.0 nuclear data libraries caused by compensating errors in important differential data was demonstrated. In calculations for a shipping container of high-assay low enriched uranium, the data of individual isotopes were systematically swapped between the two ENDF/B libraries. An eigenvalue difference of up to 450 pcm was found due to the use of 235 U and 238 U from one library and 1 H and 16 O from the other library. This clearly demonstrates a cross-correlation between reaction data sets of different isotopes within a library that should be reported in the evaluations. For sodium-cooled fast reactor (SFR) fuel assemblies, significant eigenvalue (k inf ) differences (200– 450 pcm) were found between calculations using the 2011 ENDF/B-VII.1 data and 2018 ENDF/B-VIII.0 data. These differences were mainly caused by updates of 238 U and 239 Pu neutron cross sections. Results from the multigroup (MG) calculations further revealed that the group structure of the applied MG library strongly influences the MG bias due to the importance of an appropriate energy resolution of the resonances in higher energy ranges. The application of previously used MG libraries requires new verification for advanced reactor simulation in comparisons with reference continuous-energy calculations. Nuclear data uncertainty analyses of these SFR systems resulted in eigenvalue uncertainties between 1,400 and 1,800 pcm, which are three to four times higher than corresponding uncertainties in light water reactor (LWR) systems. The main contributor to this uncertainty was found to be inelastic scattering on 238 U, which shows an uncertainty of up to 50% in the fast energy range. Other important contributors are the scattering reactions of 56 Fe and 23 Na which have so far not appeared in LWR analysis. Since the largest contribution to the eigenvalue uncertainty of SFR systems is coming from scattering reactions, it is expected that uncertainties in the angular scattering distributions also have a significant impact. Those uncertainties are, however, not available for the majority of nuclides, and the capabilities to determine sensitivities to this data are currently underdeveloped. For two graphite moderated high temperature gas-cooled reactor (HTGR) benchmarks, only the ENDF/BVII. 1 calculations resulted in consistent eigenvalues (k eff ) with the corresponding experimental measurements. Eigenvalue differences of about 1,000 pcm were found between the 2006 ENDF/B-VII.0 data and the 2011 ENDF/B-VII.1 data, primarily due to an updated carbon capture cross section in the thermal energy range in the later ENDF/B release. The ENDF/B-VIII.0 eigenvalue was larger than the ENDF/B-VII.1 eigenvalue by about 300 pcm mainly due to updates in multiple 235 U neutron cross sections, with offsetting updates in the 238 U cross sections. With ENDF/B-VIII.0, graphite can be modeled as perfect crystal or with two different porosities. The choice of the graphite evaluation can have a significant influence of the eigenvalue. For a HTGR benchmark, maximum eigenvalue differences as high as 650 pcm due to different porosities were observed. More detailed studies of the impact of the porosity are necessary while considering that the graphite porosity can vary between the used materials and changes as a function of neutron fluence. xii The uncertainty of the HTGR eigenvalues due to nuclear data uncertainties was found between 500 and 600 pcm, with the top contributor being the neutron multiplicity of 235 U. A gap in the form of missing uncertainties in graphite thermal scattering data, that might have significant impact on HTGR reactors, was identified. This gap is being investigated by the DOE-NE Nuclear Data and Benchmarking Program, as documented in a separate report The fast spectrum molten salt reactor calculations revealed similar comparisons as for the SFR assemblies. The eigenvalue uncertainties were significantly influenced by inelastic scattering on 238 U, while the impact of angular scattering distributions is unknown. For the graphite and zirconium hydride moderated system, eigenvalue uncertainties of up to 700 pcm were observed, requiring in depth analyses of the cross sections and corresponding uncertainties of the included materials. In general, it was observed that the flux spectra of the various molten salt reactor systems show significant differences, even between a fresh state and a depleted state. The choice of the energy group structure of MG calculations is therefore highly relevant; the applicability of previously used MG libraries needs to be verified. Due the unavailability of pin power measurements of advanced reactor systems, pin power calculations with both ENDF/B-VII.1 and VIII.0 data were performed for a light water reactor and compared to corresponding measurements. Both calculations show good agreement with the measurements. A comparison between the ENDF/B-VII.1 and VIII.0 results revealed small differences, mostly in the range of about 0.2%.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

The importance of phonon spectrum measurements for accurate prediction of thermal scattering laws [Slides]

Although approximate phonon spectra (e.g. Debye model) are sufficient to reproduce integral quantities (e.g. total INS cross section) in reasonable agreement with the measured data, more accurate phonon spectra are needed to achieve agreement with the differential data. SANS component is essential for reproducing the total scattering cross section; this is the case for nanodiamonds and other materials where SANS components are present (such as porous materials like nuclear graphite). A format proposal for SANS data in ENDF or GNDS is needed. Therefore, differential (e.g. phonon spectrum) and integral (e.g. total cross section) measurements are necessary in the process of creating an ENDF evaluation. We have successfully developed a method by which ENDF evaluations can be directly compared to the relevant experimentally measured quantities. INS experiments at SNS, ILL, ISIS, and, in the future, ESS, as well as total cross section measurements at the VESUVIO instrument at ISIS, are accessible through user programs.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Differential spectra and phase space densities of trapped electrons at Jupiter

Using Pioneer 10 data, differential spectra and phase-space densities have been constructed for trapped electrons at Jupiter. These quantities should assist in calculating synchrotron radiation from these particles and in evaluating the diffusion mechanisms that accelerate the particles. Absorption by the moons Io and Europa is evident, and injection by Io is demonstrated by a density peak in phase space, which demands a local source. There is also a rapid decrease in density between the moons, which could call for either a local loss mechanism or nonlocal losses fed by diffusion.

Mcilwain, C. E.↗

Lunar Gravity Field Determination Using SELENE Same-Beam Differential VLBI Tracking Data

A lunar gravity field model up to degree and order 100 in spherical harmonics, named SGM 100i, has been determined from SELENE and historical tracking data, with an emphasis on using same-beam S-band differential VLBI data obtained in the SELENE mission between January 2008 and February 2009. Orbit consistency throughout the entire mission period of SELENE as determined from orbit overlaps for the two sub-satellites of SELENE involved in the VLBI tracking improved consistently from several hundreds of metres to several tens of metres by including differential VLBI data. Through orbits that are better determined, the gravity field model is also improved by including these data. Orbit determination performance for the new model shows improvements over earlier 100th degree and order models, especially for edge-on orbits over the deep far side. Lunar Prospector orbit determination shows an improvement of orbit consistency from I-day predictions for 2-day arcs of 6 m in a total sense, with most improvement in the along and cross-track directions. Data fit for the types and satellites involved is also improved. Formal errors for the lower degrees are smaller, and the new model also shows increased correlations with topography over the far side. The estimated value for the lunar GM for this model equals 4902.80080 +/- 0.0009 cu km/sq s (10 sigma). The lunar degree 2 potential Love number k2 was also estimated, and has a value of 0.0255 +/- 0.0016 (10 sigma as well).

Goossens, S.↗

The PARADIGM Project: Case Study in Balancing Experiment Uncertainty with Design simplicity

Accurate nuclear data are required for simulations of many applications including nuclear criticality safety. Actinide nuclear data at intermediate energies (from 1 to 100s of keV) are imprecise and inaccurate, because of scarce differential data, and an insufficient theory approach to capture the structures expected in the data to yield evaluated nuclear data, and lack of integral data for proper validation. This is a known deficiency but has proved challenging to address. More specifically, only 5% of integral experiments in the International Criticality Safety Benchmark Evaluation Project (ICSBEP) benchmark suite address intermediate energies (Fig. 1). Associated calculated effective multiplication factor, k eff , values for these experiments are far outside the experimental uncertainties and are 25× further from experiment than for fast energies. These differences could either stem from systematic biases in nuclear data, experiments or both. The goal of the PARADIGM (PARallel Approach of Differential and InteGral Measurements) project is to significantly reduce (by more than tens of percent) the uncertainties of intermediate energy actinide nuclear data. The PARADIGM project designed and intends to execute LANSCE (Los Alamos Neutron Science CEnter) and NCERC (National Criticality Experiments Research Center) intermediate experiments in parallel. They will specifically address a high priority nuclear data need—reducing bias and uncertainty in intermediate plutonium nuclear data. The two experiment will achieve that by informing each other and nuclear theory. By doing all these steps in parallel, the timeline to deliver improved nuclear data to users will significantly be reduced. This work will focus on the integral experiment final design and the balance of design and modeling simplicity while minimizing experiment uncertainty.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Specialized Color Function for Display of Signed Data

This Mathematica script defines a color function to be used with Mathematica's plotting modules for differentiating data attaining both positive and negative values. Positive values are shown as shades of blue, and negative values are shown in red. The intensity of the color reflects the absolute value of the data value.

Kalb, Virginia↗

Uncovering Where Compensating Errors Could Hide in ENDF/B-VIII.0

Unconstrained physics spaces between two or more nuclear data observables in a library occur when their values can be simultaneously adjusted without violating the uncertainties in either differential information or simulations of relevant integral experiments. Differential data are often too imprecise to fully bound all nuclear data observables of interest for application simulations. Integral data are simulated with combinations of nuclear data so that an error in one observable may be hidden by a counterbalancing error in another. In this manner compensating errors may lurk within nuclear data libraries and these errors have the potential to undermine the predictive power of neutron transport simulations, particularly in situations where there is no conclusive validation experiment that resembles the application of interest. The EUCLID project (Experiments Underpinned by Computational Learning for Improvements in Nuclear Data) developed a preliminary workflow to identify these unconstrained physics spaces by bringing together results from a large collection of integral experiments with their simulated counter-parts as well as differential information that have a one-to-one correspondence to nuclear data. This wealth of information is processed by machine learning tools for subsequent refinement by human experts. Here, we show how the EUCLID work-flow is executed by applying it first to 239 Pu and then to 9 Be nuclear data in ENDF/B-VIII.0.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Uncovering Where Compensating Errors Could Hide in ENDF/B-VIII.0

Unconstrained physics spaces between two or more nuclear data observables in a library occur when their values can be simultaneously adjusted without violating the uncertainties in either differential information or simulations of relevant integral experiments. Differential data are often too imprecise to fully bound all nuclear data observables of interest for application simulations. Integral data are simulated with combinations of nuclear data so that an error in one observable may be hidden by a counterbalancing error in another. In this manner compensating errors may lurk within nuclear data libraries and these errors have the potential to undermine the predictive power of neutron transport simulations, particularly in situations where there is no conclusive validation experiment that resembles the application of interest. The EUCLID project (Experiments Underpinned by Computational Learning for Improvements in Nuclear Data) developed a preliminary workflow to identify these unconstrained physics spaces by bringing together results from a large collection of integral experiments with their simulated counter-parts as well as differential information that have a one-to-one correspondence to nuclear data. This wealth of information is processed by machine learning tools for subsequent refinement by human experts. Here, we show how the EUCLID work-flow is executed by applying it first to 239 Pu and then to 9 Be nuclear data in ENDF/B-VIII.0.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

MIC-DP: A Scalable Correlation-Aware Differential Privacy Framework for High-Dimensional Data

Conventional differential privacy (DP) assumes record independence, limiting effectiveness on real-world datasets with temporal, spatial, or structural correlations. These dependencies undermine privacy guarantees and degrade utility in domains like healthcare, IoT, and smart city analytics. We propose Maximum Information Correlated Differential Privacy (MIC-DP), a novel framework that dynamically calibrates noise based on statistical dependencies. MIC-DP uses the Maximum Information Coefficient (MIC) to capture both linear and nonlinear correlations without explicit modeling, enabling adaptive sensitivity adjustment and improved privacy–utility trade-offs. Evaluations on healthcare (MIMIC), demographic (ACI), and synthetic datasets show that MIC-DP reduces mean absolute error (MAE) by up to 5.2% under strict privacy budgets (ϵ≤1), with aggregate utility improvements reaching 18% across datasets and evaluation metrics. MIC-DP provides formal (ϵ,δ)-privacy guarantees, scales efficiently with feature count, and supports deployment in moderate-scale, privacy-sensitive applications. Its tunable performance and runtime efficiency make MIC-DP suitable for privacy-sensitive applications where low-latency analytics and strong privacy guarantees must coexist. These results demonstrate MIC-DP’s effectiveness as a correlation-aware solution for practical DP.

Yang, Wenjun [Univ. of Washington, Tacoma, WA (Uni↗

ORNL FY2024 Nuclear Data Evaluation Contributions: Cu, La, N, and Ta [Slides]

63,65 Cu angular distributions resolved for ENDF/B-VIII.1, consistent with both differential data and integral benchmark performance. 139 La RRR and URR evaluations will be merged with the LANL high energy evaluation, and to be submitted to the future ENDF-B release (post-VIII.1). 14 N RRR evaluation is planned to produce n+ 14 N, p+ 14 C, and a+ 11 B contributions to be submitted to the future ENDF-B release (post-VIII.1). 181 Ta covariances repaired and reported as intended in an errata to ENDF/B-VIII.1.

139-La↗

Flight test evaluation of precision-code differential GPS for terminal approach and landing

A flight test evaluation conducted at the NASA Ames Research Center of precision-code differential GPS for terminal approach and landing is described. Differential corrections to satellite range and range-rate measurements are computed in a stationary ground reference system, uplinked to the test aircraft, and employed to correct corresponding airborne satellite data. Differentially corrected range and range-rate data, combined with inertial data, are then utilized with satellite position and velocity to compute aircraft position and velocity employing an eight-state extended Kalman filter.

Mcnally, B. D.↗

Double Shell Inertial Confinement Fusion X-Ray Spectral Analysis

At the National Ignition Facility (NIF), lasers are used to compress a double shell capsule with deuterium and tritium in order to create nuclear fusion processes. The lasers aim at the inside of a gold hohlraum which excite electrons which further release photons in the range of 0~20keV. The photons randomly disperse, ultimately either going towards the fuel capsule or back out the laser entrance holes. The photons that go towards the fuel capsule work towards the compression of the multi-shell capsule whereas the photons that leave the hohlraum have a chance at being picked up by the Lawrence Livermore National Lab’s ‘Dante’ photon detector. ‘Dante’ analyzes photon data by having 18 planar vacuum x-ray diodes (XRD) behind unique filters to differentiate data amongst various photon energies. The goal of the project was to analyze the characteristics of low and high energy photons released by the gold shell.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

ENDF/B-VIII.0 Augmented Covariance Data The first iteration [Slides]

Nuclear data are necessary for reliable modeling and simulation of the next generation of nuclear reactors. However, the variation in the ratio of the computed to experimental values (C/E) for certain types of nuclear systems is much less than predicted by evaluated nuclear data file (ENDF)/B covariances. Figure 1 provides an example of a set of metal-plutonium-fueled, fast-spectrum (PU-MET-FAST) integral experiments from the International Criticality Safety Benchmark Evaluation Project (ICSBEP) in the Oak Ridge National Laboratory (ORNL) VALID database. The variation in the C/E values, shown with one standard deviation error bars, is 100% covered by both the SCALE and ENDB/VIII.0 covariance data. This is due to the comparisons to integral data that are essential during the evaluation process. However, the ENDF evaluations represent uncertainties and correlations in differential data only; they do not reflect the impact of the comparison to integral data in the covariance evaluations.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

ENDF/B-VIII.0 Augmented Covariance Data The first iteration [Slides]

Nuclear data are necessary for reliable modeling and simulation of the next generation of nuclear reactors. However, the variation in the ratio of the computed to experimental values (C/E) for certain types of nuclear systems is much less than predicted by evaluated nuclear data file (ENDF)/B covariances. Figure 1 provides an example of a set of metal-plutonium-fueled, fast-spectrum (PU-MET-FAST) integral experiments from the International Criticality Safety Benchmark Evaluation Project (ICSBEP) in the Oak Ridge National Laboratory (ORNL) VALID database. The variation in the C/E values, shown with one standard deviation error bars, is 100% covered by both the SCALE and ENDB/VIII.0 covariance data. This is due to the comparisons to integral data that are essential during the evaluation process. However, the ENDF evaluations represent uncertainties and correlations in differential data only; they do not reflect the impact of the comparison to integral data in the covariance evaluations.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗