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Advancing Artificial Intelligence with Liquid Argon Neutrino Experiments (Technical Report)

The grant allowed two main contributions: 1) The development of a first successful demonstration of the employment of Optimal Transport in liquid argon time projection chamber neutrino detectors. Optimal Transport, used in other contexts and specifically with LHC calorimetric data, was adapted to address a key particle identification challenge in LArTPCs: the separation of pi0 backgrounds from single-electrons produced in charged-current electron neutrino interactions. The work, leveraging ML methods such as k-nearest-neighbor (kNN) and support-vector-machine (SVM), showed an increase in background rejection of a factor of two or more. Work is now ongoing to incorporate this development in physics analyses for LArTPC experiments and more broadly expand the use of OT in LArTPC detectors including DUNE. This work was done in collaboration with the phenomenology group led by Nathaniel Craig at UCSB. 2) The deployment of NuGraph2, a graph neural network developed for LArTPC reconstruction, in the MicroBooNE experiment. NuGraph2 uses novel graph-neural-network methods on the rather simple LArTPC inputs of reconstructed hits, greatly simplifying the workflow compared to the use of waveform or signal-deconvolved wire ROIs. The network performed particle classification and was shown to address many challenging problems in LArTPC imaging including track-shower separation and the identification of protons and charged pions from primary muons. Our group collaborated with Giuseppe Cerati (FNAL scientist) who is one of the core developers of NuGraph2 to integrate this tool in MicroBooNE’s analysis framework. This consisted in tow key contributions: a) Studying performance on real data, which came with several months of iterations because the MC-trained version of the network was found to show significant bias that our group investigated and addressed. b) Integrating the output hit labeling of NuGraph2 into the existing particle tracking and shower reconstruction code. As a result of this work led by our team NuGraph2 is now enabling a suite of new analyses which benefit from enhanced capabilities and thus broader physics reach. The grant supported primarily the salary of UCSB graduate student Chuyue “Michaelia” Fang as well as partial summer salary support for PI Caratelli. Some funds were used for travel by Michaelia to ML related schools and conferences.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS

Precision Measurement of the Neutron Magnetic Form Factor via the Ratio Method at Jefferson Lab Hall A

Protons and neutrons, collectively known as nucleons, are composed of quarks and gluons. The Sachs electromagnetic form factors encode information about the spatial distributions of charge and magnetization in the nucleon, particularly at low momentum transfer. In particular, the neutron magnetic form factor (GMn) provides crucial information about the distribution of magnetization inside the neutron and helps constrain theoretical models of nucleon structure. Quasi-elastic electron scattering from deuterium was measured up to Q^2=13.5 GeV^2 using the Super BigBite Spectrometer in Hall A at Jefferson Lab. In this work, the neutron magnetic form factor GMn was extracted at Q^2 = 3.0 GeV^2 and Q^2=4.5 GeV^2 using the Ratio Method. These results represent a subset of the full dataset collected in this experiment, which extended to significantly higher Q^2. The extracted GMn values agree with the existing global fit within approximately two standard deviations at Q^2=3.0 and show excellent agreement at Q^2=4.5. The measurements achieved systematic uncertainties of about 2% and statistical uncertainties below 0.5%, among the most precise determinations of GMn at these kinematics. These results demonstrate the robustness of the experimental technique and provide an important validation point for future extractions at higher Q^2, where data remain scarce. In addition, the GRINCH heavy gas Cherenkov detector—a key component of the experimental apparatus—was commissioned and achieved an electron detection efficiency of approximately 97%, supporting reliable particle identification. Together, the analysis presented here advances both our understanding of nucleon structure and the validation of the experimental methods and instrumentation used to access it.

Satnik, Maria [College of William and Mary, Willia

Discrete fracture network model benchmarks developed and applied in a DECOVALEX-2023 repository performance assessment study

This study presents newly developed benchmarks for modeling flow and transport within discrete fracture networks (DFNs) and useful methods for analyzing the results. The new benchmarks are designed to test modeling approaches for use in probabilistic performance assessment models of deep geologic repositories in fractured rock. The benchmarks simulate flow and transport through a 1 km 3 block of fractured rock. The first simulates migration of a short pulse of tracer through a simple network of four intersecting fractures. The second adds 1089 stochastically generated fractures. The third changes the pulse to a continuous point source. Evaluation of model performance relies on moment analysis and comparison of the results of different models. The expected nondimensional first moment of the conservative tracer for each benchmark is 1. The benchmarks were simulated by teams from Canada, Czechia, Germany, Korea, Sweden, Taiwan, and the United States as part of a DECOVALEX-2023 study (decovalex.org). The teams used various approaches, including explicit DFN modeling, DFN upscaling to an equivalent continuous porous medium (ECPM), and a combination of both methods. Transport mechanisms are modeled using either the advection-dispersion equation or particle tracking. Results demonstrate strong agreement among the models in breakthrough behavior up to the 75th percentile. Significant deviations in first moments and well-clustered outputs led to the identification of inaccuracies in several models. Such findings exemplify the benefit of exercising these benchmarks and using the presented methods to test DFN flow and transport models.

Benchmark

Monte Carlo N-Particle Transport Performance of Predicting Digital Radiographic IQI Inspection

The identification of porosity, geometric noncompliance, and other defect types are critical to the qualification of materials and components. X-ray radiographic nondestructive testing is a common industrial inspection method for process quality control and component qualification and certification. Digital radiography provides a quick and efficient alternative when compared to traditional film-based inspection. The quality of radiographic inspection is dependent on equipment specifications, such as the source spot size and detector pixel size, and the specific parameters selected for use for the radiographic technique. To evaluate if an x-ray system and technique is sufficient for a given requirement, a radiographic image quality indicator (IQI) can be used. Radiographic IQIs in hard to machine materials or hard to manufacture defects can be time consuming and expensive to manufacture. This study was conducted to evaluate current Savannah River National Laboratory (SRNL) x-ray imaging systems with a custom tantalum IQI and using Monte Carlo simulations to predict the performance of future systems. The tantalum IQI was tested using a Siefert Isovolt 420 keV x-ray tube with a Perkin Elmer XRD 1611 flat panel with 100-micron pixels. Using the Monte Carlo N-Particle transport software, the radiographic tally was used to simulate the photon flux through an identical tantalum IQI. These simulations provided a benchmark as to the best theoretical identification on a given system using our tantalum IQI. The simulations were refined to match SRNL’s current systems’ noise levels, leading to confidence in their ability to predict the performance of other systems that may be purchased and deployed in the future at the Savannah River Site. Future studies will be conducted to prove this research can be extended to artificially evaluate the ability for systems to identify critical defect sizes through x-ray radiographic inspection, drastically reducing the cost and time burdens of producing high-fidelity radiographic test articles.

digital X-ray radiography

Summer 2025 SULI: Nucleus ID, TinyTPC, and Scientific Communication

This paper summarizes my work during the Summer 2025 SULI internship, which focused on two main projects and broader scientific development. The first project involved improving the particle identification (PID) of protons, deuterons, and tritons using PIDA distributions and template fitting, with the goal of modeling nuclear final-state interactions (FSI) and testing the robustness of the method against systematic uncertainties. These techniques pave the way for future application to LArTPC data from the ICARUS detector. The second project centered on the optimization and data-taking of the TinyTPC detector, a compact LArTPC used for high-resolution low-energy measurements. I adjusted gain and threshold parameters, performed hardware validation tests, and developed analysis strategies to extract meaningful physics from collected data. Throughout the summer, I also enhanced my scientific communication and mentorship skills through presentations, collaborative analysis, and peer guidance.

McCright, Hannah [Maryland U.]

Identification of $^{3}$He–$^{3}$H clusters in the $^{6}$Li+$^{89}$Y experiment using particle-$\gamma$ coincidence measurement

The 6 Li+ 89 Y experiment was performed to explore the reaction mechanism induced by a weakly bound nucleus 6 Li and its cluster configuration. Here, the particle-$\gamma$ coincidence method was used to identify the different reaction channels. The $\gamma$-rays coincident with 3 He/ 3 H indicate that the 3 H/ 3 He stripping reaction plays a significant role in the formation of Zr/Nb isotopes. The obtained results support the existence of a 3 He- 3 H cluster in 6 Li. Direct and sequential transfer reactions are adequately discussed, and the FRESCO code is used to perform precise finite-range cyclic redundancy check calculations. In the microscopic calculation, direct cluster transfer is more predominant than sequential transfer in 3 H transfer. However, the direct cluster transfer is of comparable magnitude to the sequential transfer in the 3 He transfer.

CRC calculations

Dual particle imaging using time-of-flight neutron classification

Fast-neutron imaging technology is well-suited for passive nuclear material monitoring, secondary inspection of flagged cargo, and wide-area search for lost neutron sources. However, imaging systems that use pulse shape discrimination for event classification require complex pulse waveform analysis. In this work, we evaluate time-of-flight (TOF) based particle classification as an alternative solution for fast-neutron imaging by classifying all events with a TOF above a maximum threshold as neutrons. We measured a Cf-252 source next to Cs-137 using a 12-bar organic-glass scintillator array. By varying the TOF thresholds for neutron identification, we demonstrate a clear trade-off between event yield and backprojection image fidelity, with stricter thresholds improving precision at the cost of statistics, TOF thresholded data generated an image that predicted the neutron source direction with 20% reduced mean central angle prediction error compared to a traditional pulse shape discrimination (PSD) method with comparable event count. Time-of-flight particle classification shows promise as an alternative to pulse shape discrimination systems for fast neutron imaging systems looking to minimize costs and size of electronics with comparable imaging quality. The sources used demonstrate that the method is effective in classifying measured neutrons in a measurement environment with 150 μCi Cs-137 and 1.6 × 10 6 n/s Cf-252 sources positioned at distances of 66 cm and 81 cm from the detector. Additionally, the method classifies low-energy neutron events that pulse shape discrimination removes, so a combination of both methods would result in a higher overall neutron event efficiency.

Heriot, William [Univ. of Michigan, Ann Arbor, MI

Leveraging machine learning to enhance aerosol classification using Single-Particle Mass Spectrometry

Advancing automated classification of atmospheric aerosols from Single-Particle Mass Spectrometry (SPMS) data remains challenging due to overlapping ion signatures, compositional diversity, and limited labeled data. This study evaluates supervised and semi-supervised learning frameworks to enhance aerosol identification by jointly leveraging labeled and unlabeled spectra. Four models were compared: a supervised Support Vector Machine (SVM), a self-training SVM, a stacked autoencoder classifier, and a stacked autoencoder trained using a temporal-ensembling Mean Teacher approach. All models achieved high and stable accuracies (90.0 %–91.1 %), surpassing previous results on the same dataset (87 %) and matching the performance of state-of-the-art deep learning methods. Despite small global metric differences (≤ 1 %), semi-supervised variants yielded up to 5 %–10 % improvements for compositionally rare particle types – such as soot (0.77 % of spectra, F1-score: 0.93–0.97) and hazelnut pollen (0.98 % of spectra, F1-score: 0.97–1.00) – equating to roughly ∼ 187 additional correctly classified spectra. These gains are scientifically significant, as such rare particles exert disproportionate influence on radiative absorption and ice nucleation processes; their improved detection reduces modeled uncertainties in aerosol absorption optical depth and mixed-phase cloud ice nucleation rates. The models' residual misclassifications (≈ 9 %) largely arise from true spectral overlap among chemically adjacent species (e.g., Na- vs. K-feldspar, coated vs. uncoated feldspars), reflecting physical compositional continuity rather than algorithmic error. Collectively, these findings demonstrate that leveraging unlabeled data to learn robust spectral representations and refine classification enhances both fidelity and interpretability, bridging data-driven analysis with aerosol–climate process understanding.

54 ENVIRONMENTAL SCIENCES

Identification of uranium oxidation states using oxygen K-edge scanning transmission X-ray microscopy

The field of nuclear forensics is growing in importance, and the increasing capabilities at synchrotron radiation light sources enable non-destructive characterization of oxide particles with better spatial, compositional, and oxidation state speciation resolution than ever before. Here, uranium oxide particles derived from multiple wet chemical processing methods were examined using a scanning transmission X-ray microscope (STXM), and a weakly-supervised method was developed to automatically analyze the collected data. Multiple uranium oxidation states were observed and quantified within and between samples, yielding information about differences between particles produced via the various processing routes.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH

Online Electron Reconstruction at CLAS12

Online reconstruction plays a crucial role in monitoring and in real-time analysis of high energy and nuclear physics experiments. A vital aspect of reconstruction algorithms is particle identification, which combines information from various detector components to determine the type of particle. Electron identification is particularly significant in electro-production nuclear physics experiments like the CLAS12 spectrometer at Jefferson Laboratory as it is essential in data recording. A machine learning approach has been developed for CLAS12 experiments to reconstruct and identify electrons by combining raw signals from multiple detector components at the data acquisition level. This method achieves high electron identification purity while maintaining nearly 100% efficiency. Furthermore, the machine learning tools operate at rates exceeding data acquisition speed, enabling the real-time electron reconstruction. This advancement significantly improves online analyses and monitoring capabilities for CLAS12 experiments.

Tyson,, Richard [Thomas Jefferson National Acceler

Variable rate neural compression for sparse detector data

Particle colliders produce data at extraordinary rates, posing major challenges for transmission and storage. High-throughput compression algorithms are therefore essential. In the sPHENIX experiment taking data at the Relativistic Heavy Ion Collider, a time projection chamber records three-dimensional (3D) particle trajectories that are highly sparse, making conventional learning-free lossy compression ineffective. Convolutional neural networks have surpassed traditional methods in compression ratio and accuracy. However, they fail to exploit sparsity for efficiency. To address these gaps, we present BCAE-VS, a bicephalous convolutional autoencoder with variable compression ratio for sparse data, which adapts compression to input complexity through key-point identification and sparse convolution. BCAE-VS achieves higher accuracy and compression ratios than prior neural approaches while being orders of magnitude smaller. Moreover, its throughput increases with sparsity—a property not observed in other methods. Although it was developed for collider experiments, BCAE-VS readily extends to other sparse data domains, such as light detection and ranging (LiDAR) sensing and 3D microscopy.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS

Exploring quantum statistics for massive Dirac and Majorana neutrinos using spinor-helicity techniques

Recently, there has been interest in the applicability of quantum statistics to distinguish Dirac from Majorana neutrinos in multineutrino final states. In particular, debate has arisen over the validity of the Dirac-Majorana confusion theorem in these processes, i.e., that any distinction between the Dirac and Majorana processes goes to zero as the neutrino mass goes to zero. Here we approach this problem equipped with spinor-helicity methods generalized for massive Dirac and Majorana fermions. We explicitly calculate all helicity amplitudes, and their squares, for the decay of a light scalar particle to two neutrinos and two oppositely charged leptons. This allows us to pinpoint the crucial steps which could lead to claims of a violation of the confusion theorem. We show that, if the correct antisymmetrization of Dirac to Majorana amplitudes is used, identification of which is clear in this framework, and all relevant contributions are appropriately summed, a scalar decay into two charged leptons and two neutrinos satisfies the Dirac-Majorana confusion theorem.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC

Reconstruction of atmospheric neutrinos in DUNE’s horizontal-drift far-detector module

This paper reports on the capabilities in reconstructing and identifying atmospheric neutrino interactions in one of the Deep Underground Neutrino Experiment’s (DUNE) far detector modules, a liquid argon time projection chamber (LArTPC) with horizontal drift (FD-HD) of ionization electrons. The reconstruction is based upon the workflow developed for DUNE’s long-baseline oscillation analysis, with some necessary machine-learning models’ retraining and the addition of features relevant only to atmospheric neutrinos such as the neutrino direction reconstruction. Where relevant, the impact of the detection of the charged particles of the hadronic system is emphasized, and comparisons are carried out between the case when lepton-only information is considered in the reconstruction (as is the case for many neutrino oscillation experiments), versus when all particles identified in the LArTPC were included. Three neutrino direction reconstruction methods have been developed and studied for the atmospheric analyses: using lepton-only information, using all reconstructed particles, and using only correlations from reconstructed hits. The results indicate that incorporating more than just lepton information significantly improves the resolution of both neutrino direction and energy reconstruction. The angle reconstruction algorithms developed in this work result in no strong dependence on particle direction for reconstruction efficiencies or neutrino flavor identification. This comprehensive review of the reconstruction of atmospheric neutrinos in DUNE’s FD-HD LArTPC is the first step towards developing a first neutrino oscillation sensitivity analysis, which will ready DUNE for its first measurements.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS

Identification of contamination in the pulse-compression chamber of the OMEGA EP Laser System originating from clean room garments

The contamination of optical components with microscopic particles strongly impacts their ability to handle high-power or high-intensity laser pulses via an array of mechanisms. This work explores the nature and origin of a subset of contamination particles found inside the pulse-compression chamber of the OMEGA EP Laser System. Using Raman microscopy accompanied by other analytical methods, it was shown that sodium nitrate constitutes a significant fraction of the particles that possess diameters on the order of a few micrometers. Further investigation aiming to reveal the origin of these particles suggests that these sodium nitrate particles are deposited via shedding from the reusable clean room garments worn in the Laser Bay and compression chamber. Raman microscopy also revealed various plastic particles such as polystyrene, polyethylene, and poly(diallyl isophthalate).

Raman spectroscopy

Direct reactions with the AT-TPC

Direct reactions are crucial tools for accessing properties of the atomic nucleus. Fundamental and exotic phenomena such as collective modes, pairing, weakbinding effects and evolution of single-particles energies can be investigated in peripheral collisions between a heavy nucleus and a light target. The necessity of using inverse kinematics to reveal how these structural properties change with isospin imbalance renders direct reactions a challenging technique when using the missing mass method. In this scenario, Active Target Time Projection Chambers (AT-TPC) have demonstrated an outstanding performance in enabling these types of reactions even under conditions of very low beam intensities. The AT-TPC of the Facility for Rare Isotope Beams (FRIB) is a next generation multipurpose Active Target. When operated inside a solenoidal magnet, direct reactions benefit from the measurement of the magnetic rigidity that enables particle identification and the determination of the excitation energy with high resolution without the need of auxiliary detectors. Additionally, the AT-TPC can be coupled to a magnetic spectrometer improving even further its spectroscopic investigation capability. In this contribution, we discuss inelastic scattering and transfer reaction data obtained via the AT-TPC and compare them to theory. In particular, we present the results for the 14 C(p,p′) and 12 Be (p,d) 11 Be reactions. For 14 C, we compare the experimental excitation energy of the first 1 – excited state with coupled-cluster calculationsbased on nuclear interactions from chiral effective field theory and with available shell-model predictions. For 12 Be, we determine the theoretical spectroscopic factors of the 12 Be (p,d) 11 Be transfer reaction in the shell modeland compare them to the experimental excitation spectrum from a qualitative standpoint.

active target

Characterization Techniques Investigated for Characterization of Anomalous Materials in Plutonium Oxide – 25666

The DOE has adopted a Dilute and Dispose approach for processing surplus plutonium which consists of blending plutonium oxide with adulterants and packaging it in a form which is acceptable for disposal at the Waste Isolation Pilot Plant. The feed material for the downblend process is intended to be pure plutonium oxide powder, however other objects are occasionally encountered within the oxide, particularly with legacy material. Potential technologies which could assist in the resolution of incidents where such anomalies are encountered have been investigated. Resolution of these incidents requires characterization of the anomalous object so that plutonium oxide processing can resume and so that a disposition pathway can be determined for the anomalous material. Technologies including gamma ray spectroscopy, alpha-gamma coincidence, LiDAR volumetric measurements, and surface conductivity measurements were investigated for this purpose, with a focus on systems which can be easily introduced into the processing environment when an anomaly is encountered, then removed from the environment after resolution to avoid impeding normal processing activities. This places an emphasis on small and portable measurement systems and systems that can operate in a high-background, oxide-processing environment. Gamma ray systems investigated include the GR1™a CZT detector and the MicroGe™a germanium detector, with a focus on detecting characteristic gamma rays from Pu-239 and other actinides. A gamma ray and alpha particle coincidence method was investigated with the goal of identifying actinides in the presence of a gamma ray background produced by adjacent plutonium oxide material. Leica™b BLK360 G1 and Keyence™c LJ-X8300 LiDAR systems were investigated for use in conjunction with mass measurements to gain accurate material density values, and a Foerster Sigmatest™d 2.070 was tested to determine surface conductivity. The combination of these properties would allow improved identification and characterization of a wide variety of potential anomalous material.

Munson, Justin M.

Methods development towards automated, physics-informed, quantitative quality control of TRISO-SiC

Tristructural-isotropic (TRISO) fuel particles have been developed as a high-performance fuel for use in high-temperature gas-cooled reactor (HTGR) systems due to their high efficiency and stability under both normal and off-normal conditions. Broader deployment of this technology in advanced nuclear applications may benefit from quantitative quality assurance and quality control (QA/QC) methods that directly link TRISO properties to downstream performance. A key TRISO property is the SiC layer microstructure, which influences fission product retention during irradiation. However, existing QA/QC for the TRISO-SiC microstructure comprises only a qualitative visual inspection; therefore, there is a clear opportunity for the development of quantitative methods for TRISO QA/QC. Here, to this end, previous work has demonstrated an image processing approach to grain boundary (GB) identification and subsequent extraction of microstructural metrics; however, extensive twinning within the SiC layer complicates such analyses because twin GBs significantly influence microstructural metrics but are not expected to contribute to fission product transport. This study presents the initial development, training, and testing of an ML-based image segmentation algorithm designed to identify and remove twin GBs from standard backscattered electron micrographs, providing an industrially applicable, quantitative, and physically meaningful QA/QC approach for the TRISO-SiC microstructure. Although pixel-wise performance metrics for the twin predictions are low, the change in grain area and the number of GB pixels after twin removal predicted by the ML workflow are within 1% of the true values calculated using crystallographic data. This suggests that the model is well capable of predicting overall twin boundary structures and grain morphology, and continued advancement of this approach could enable automated, scalable, and physics-informed QA/QC for TRISO-SiC microstructures, supporting the reliable qualification of coated particle fuels for next-generation reactor systems.

Computer vision

The ICEBERG Test Stand for DUNE Cold Electronics Development

ICEBERG is a liquid argon time projection chamber at Fermilab for the purpose of testing detector components and software for the Deep Underground Neutrino Experiment (DUNE). The detector features a 1.15m x 1m anode plane following the specifications of the DUNE horizontal drift far detector and a newly installed X-ARAPUCA photodetector. The status of ICEBERG is reported along with analysis of noise, pulser, and cosmic ray data from the ninth run beginning May 2024 with the goal of advising the DUNE collaboration on the optimal wire readout electronics configuration. In addition, development of an absolute energy scale calibration method is currently underway using known sources such as cosmic ray muon Michel electrons at the ~10 MeV scale and $^{39}$Ar decay electrons at the ~100keV scale. Research into AI-based identification of such events at the data acquisition level is introduced.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND