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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 37 records · Page 2
All sourcesNASA NTRSDOE OSTI
DOE OSTI2020

Axial proton probing of magnetic and electric fields inside laser-driven coils

In a laser-driven coil, a laser is used to eject electrons from a plate, which then draws a current through a loop. Diagnosing the field strength, geometry, and conditions within these loops has been one of the primary difficulties in fielding this type of target. In this paper, the diagnostic technique of axial proton probing with a mesh fiducial of a laser-driven coil is demonstrated. Multiple coil types were driven by a 1 ns, 1.25 kJ long pulse beam and probed several times. Here, this technique provides significantly more information than transverse probing on electric- and magnetic-field strength in the region of interest and shows in our experiment complex, non-uniform current path structures and charge distribution.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2021

Laser absorption measurements of electron density in nanosecond-scale atmospheric pressure pulsed plasmas

We report on time-resolved measurements of electron number density by continuous-wave laser absorption in a low-energy nanosecond-scale laser-produced spark in atmospheric pressure air. Laser absorption is a result of free-free and bound-free electron excitation, with the absorption coefficient modeled and evaluated using estimates of the time-variation in electron temperature and probe laser absorption path length. Plasma electron number densities are determined to be as high as n e = 7 x 10 19 cm -3 , and decay to 1/e of their peak values over a period of about 50 ns following plasma formation using a 20 mJ, 10 ns pulse width frequency-doubled Nd:YAG laser. The measured plasma densities at later times are shown to be in reasonable agreement with Stark broadening measurements of the 3s[ 5 S o ]-3p[ 5 P] electronic transition in atomic oxygen at 777 nm. This study provides support for the use of such continuous wave laser absorption for time resolved electron density measurements in low energy spark discharges in air, provided that an estimate of the electron temperature and laser path length can be made by accompanying diagnostics.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2021

Free space Thomson scattering to study high energy density shocks

A free space collective Thomson scattering system has been developed to study pulsed power produced plasmas. While most Thomson scattering diagnostics on pulsed power machines use a bundle of fibers to couple scattered light from the plasma to the spectrometer, this system used free space coupling of the light, which enabled a spatially continuous image of the plasma. Initial experiments with this diagnostic were performed on an inverse wire array generated by a 200 kA, 1100 ns rise time pulse power generator. The capabilities of this diagnostic were demonstrated by using the low frequency ion acoustic wave feature of the Thomson scattering spectra to measure the plasma flow velocity. The diagnostic was demonstrated to measure velocities between 20 and 40 km/s with an error of 4.7 km/s when fitting with a 600 μm spatial resolution or 8.9 km/s when fitting with a 150 μm spatial resolution. In some experiments, the diagnostic observed a bow shock in the plasma flow as the scattering intensity increased and flow velocity decreased.

47 OTHER INSTRUMENTATION↗
DOE OSTI2022

Characterization of thermal transport and evolution of Au plasma in ICF experiments by Thomson scattering

Here, this paper demonstrates the capability of optical Thomson scattering (OTS) to measure thermal transport, and provides support to radiation hydrodynamic and kinetic simulations of electron thermal transport and plasma evolution. OTS theory and plasma simulations are applied to the interpretation of experimental measurements of laser-produced plasma from spherical gold targets on the OMEGA laser facility. The dynamical form factor, S($\vec{k}$, ω), of electron density fluctuations that is used in the fitting of Thomson scattering spectra includes ion–ion collisions and effects of non-Maxwellian distribution functions. OTS measurements and their interpretation are consistent with the nonlocal transport model in radiation hydrodynamic simulations as well as with kinetic simulations in the second half of the probe pulse duration. In particular, the reversal of heat transport during cooling is observed to be consistent with simulations, while some discrepancies are noted during the initial heating of the Au targets.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2021

Study of detached plasma profile in the divertor simulation experimental module of tandem mirror GAMMA 10/PDX

A divertor simulation experimental module (D-module) in the tandem mirror GAMMA 10/PDX was used for the study of plasma detachment. In previous studies, it was difficult to measure far-upstream plasma parameters in the D-module, and only electrostatic probes on the target plate were used to perform electron temperature and density measurements. Furthermore, to study the detached plasma structure, a Thomson scattering (TS) system and a microwave interferometer system have been installed to measure the inside plasma parameters of the D-module, and a movable electrostatic probe has been placed at the inlet of the D-module to measure the inlet plasma density and temperature. The TS system in the central cell observed the electron temperature and density of the core plasma simultaneously. These measurements revealed the entire density and temperature structure from the core plasma to the divertor plate. The line average electron density measured by the microwave interferometer showed a rollover behavior during detachment. The results indicated that the ionization region was located around the center of the D-module, and it appears to move upstream along the axis.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2022

Hall instability driven seeding of helical magneto-Rayleigh–Taylor instabilities in axially premagnetized thin-foil liner Z-pinch implosions

Helical magneto-Rayleigh–Taylor instability (MRTI) structures have been observed in z-pinch-driven liner implosion experiments with a pre-imposed axial magnetic field. We show that the formation of these helical structures can be described by a Hall magnetohydrodynamical (HMHD) model. We used the 3D extended magnetohydrodynamics simulation code PERSEUS (which includes Hall physics) [Seyler and Martin, Phys. Plasmas 18, 012703 (2011)] to study these helical instabilities and show that a Hall interchange instability in low-density coronal plasma immediately surrounding the dense liner is responsible for producing helically oriented effects in the magnetic field and current density within the coronal layer. Here, this seeds the helical pitch angle of the MRTI even when other proposed helical seeding mechanisms are either not present in the experiments or not accounted for in the simulations. For example, this mechanism does not require low-density power-feed plasmas to be swept in from large radius or the development of electrothermal instabilities. The Hall Instability is, thus, a new, independent explanation for the origin of the helical instabilities observed in axially premagnetized liner experiments. Simulation results supporting this mechanism are presented.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2023

Self-consistent integrated modeling of combined hybrid discharge-laser produced plasma devices for extreme ultraviolet metrology

Discharge- and laser-produced plasma (DLPP) devices are being used as light sources for extreme ultraviolet (EUV) generation. A key challenge for both, DPP and LPP, is achieving sufficient brightness to support the throughput requirements of nanometrology tools. To simulate the environment of a hybrid DLPP device and optimize the EUV output, we have developed an integrated HEIGHTS-DLPP computer simulation package. The package integrates simulation of two evolving plasmas (DPP and LPP) and includes modeling of a set of integrated self-consistent processes: external power source and plasma energy balance, plasma resistive magnetohydrodynamics, plasma heat conduction, detailed radiation transport (RT), and laser absorption and refraction. We simulated and optimized DLPP devices using Xe gas as a target material. We synchronized the external circuit parameters, chamber gas parameters, and laser beam temporal and spatial profiles to achieve maximum EUV output. The full 3D Monte Carlo scheme was integrated for detailed RT and EUV output calculations in Xe using more than 3600 spectral groups. The modeling results are in good agreement with Julich Forschungszentrum experimental data. Theoretical models, developed and integrated into the HEIGHTS package, showed wide capabilities and flexibility. In conclusion, the models and package can be used for optimization of the experimental parameters and settings, investigation of DLPP devices with complex design, analyzing the impact of integrated spatial effects and working timeline arrangement on the final EUV output, and EUV source size, shape, and angular distribution.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2023

Laboratory study of the PFRC-2's initial plasma densification stages

Initial plasma densification by odd-parity rotating magnetic fields (RMF o ) applied to the linear magnetized Princeton field-reversed configuration (PFRC-2) device with fill gases at pressures near 1 mTorr proceeds through two phases: a slow one, characterized by a rise time $τ_{slow}$ ~ 100 $μ$s, followed by a fast one, characterized by $τ_{fast}$ ~ 10 $μ$s. The transition from slow to fast occurs at a line-integral-averaged electron density, t n e , near 2$\times$ 10 11 cm –3 , independent of magnetic field. Here, over most of the range of experimental parameters investigated, as the PFRC-2 axial magnetic field strength was increased, RMF o power decreased, gas fill pressure lowered, or lower atomic mass unit (AMU) fill gas used, the duration of the slow phase lengthened from 50 $μ$s to longer than 10 ms after the RMF o power began. The post-fast-phase maximum n e increases with the fill-gas AMU, exceeding 5 × 10 13 cm –3 for Ar. The slow phase is consistent with atomic physics processes and field-parallel sound-speed losses. The fast phase may be explained by improved axial confinement, possibly augmented by radial or axial contraction of the plasma. Another possible explanation, a large increase in electron temperature, is inconsistent with x-ray emission. The n e behavior is discussed in relation to the E to H transition.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2023

Weibel-like instability in magnetohydrodynamics

In magnetohydrodynamics (MHD), a density perturbation perpendicular to an electron temperature gradient generates a magnetic field around itself that acts to increase the perturbation, which can lead to instability. An MHD dispersion relation is obtained for perturbations perpendicular to a fixed electron temperature gradient with an initial in-plane magnetic field, including resistivity, viscosity, and the electrothermal coefficient. Instability occurs for sufficiently small electron temperature-gradient scale lengths determined by the ion collisionless skin depth. Both viscosity and resistivity are required to prevent growth at arbitrarily small spatial scales and to give a physical result for the fastest growing mode. The perpendicular electrothermal coefficient is only significant for a narrow range of low electron Hall parameters, causing a modest reduction in magnetic field growth and modifying the criteria for instability in the presence of viscosity. If the definition of the Weibel instabilityis extended to include all instabilities due to anisotropy in the electron velocity distribution, then this is a Weibel-like instability because an electron temperature gradient implies an anisotropic electron velocity distribution. Here, the implications for the formation of filaments in laser-produced plasmas and for the verification of MHD codes are considered.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2024

Plasma sources for advanced semiconductor applications

Semiconductors are the foundation of modern technology, used in our personal, industrial, and military-grade devices. Further, every aspect of U.S. society is closely tied to semiconductors, and our economy cannot progress at the current pace with existing chip manufacturing methods as chip features approach an atomistic scale.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2025

Comparison of laser-produced plasma spatio-temporal electron density evolution measured using interferometry with simulation results

Due to the difficulties associated with experimental measurements of laser-produced plasma (LPP) properties during the earliest stages of plasma evolution, radiation hydrodynamic codes are often used. However, although these codes have been extensively validated in the higher intensity regimes, validation at low to moderate intensities has been limited. In this study, the spatio-temporal electron density evolution in an LPP generated at moderate laser intensities and at various laser wavelengths was validated against the FLASH code for times up to 20 ns. The LPP was generated by focusing the fundamental and various harmonics radiation (1064, 532, and 266 nm) from a 6 ns full width half maximum Nd:YAG laser, at a laser intensity of 10 GW cm -2 , onto a copper target. The spatio-temporal density evolution of the expanding plasma was analyzed using Nomarski interferometry. Experimental measurements were found to be consistent with FLASH simulations, and the dependence of electron densities on wavelength was found to be in agreement with analytical models, varying as n e ∝ λ -0.7 . However, slight differences were noted in the widths and shape functions of the experimental and simulated electron density profiles.

2D fast imaging↗
DOE OSTI2025

Modeled sensitivity of multi-MA accelerator performance to electrode contaminant inventory

Significant particle-in-cell code development has enabled simulations of power flow in multi-MA accelerators to include the desorption of surface contaminants, their ionization into surface plasmas, and the impact of these plasmas on efficiency. The simulations base desorption on an Arrhenius equation, whose most significant unknown is the surface contaminant inventory. The sensitivity of power-flow simulations to this inventory is studied here using Sandia National Laboratories' Z accelerator with a 7-nH MagLIF load [Phys. Plasmas 17, 056303 (2010)]. Simulations are conducted in 3D cylindrical coordinates for the current-adder, or “convolute,” region of Z and in 2D for the final feed only. Simulated contaminant inventories are varied from 1 to 32 monolayers (MLs) in 2D, and 2 to 4 ML in 3D. The results reveal sensitivities to the local ratio of E/B⁠. The high B-field, low E-field region near the short-circuit load is insensitive to the contaminant inventory, where assumed values of 4–32 ML change the load current by ≤ 2%, and agree with experiment to within 2% at peak current. A 1-ML value is the outlier, increasing the load current by 5%, but still within measurement uncertainty. In contrast, the relatively higher E-field, lower B-field convolute region has slower contaminant desorption and higher-magnitude E-field penetration of the surface plasmas. The current loss in the convolute region does increase with contaminant inventory. The loss assuming 4 ML is 12% larger than for 2 ML, with 4 ML being the better match to experiment.

Arrhenius equation↗
DOE OSTI2023

Physical and technical basis of Materials Plasma Exposure eXperiment from modeling and Proto-MPEX results *

Abstract The Materials Plasma Exposure eXperiment (MPEX) is a steady-state linear plasma device that will address plasma-material interaction (PMI) science and enable testing of fusion reactor-relevant divertor plasma-facing materials. The MPEX source concept consists of a helicon plasma source to generate the plasma, electron cyclotron heating (ECH) for electron heating, and ion cyclotron heating (ICH) for ion heating. The MPEX source plasma is then transported axially to the PMI material target region to test material samples in fusion reactor-relevant divertor conditions. This paper will summarize the physical and technical basis of MPEX. The paper will first define the MPEX parameters and scenarios at the target relevant to PMI science for various fusion reactor-relevant divertor conditions and show plasma transport modeling results to set the MPEX source parameters. Recent experimental and modeling results from Proto-MPEX, a short-pulse experiment to develop the plasma production, heating, and transport physics for MPEX, will be shown. From these results, it will be shown that MPEX can reach its desired scenarios. The MPEX physical and technical basis will also determine important functional requirements for magnetic field, radiofrequency (RF) power, RF frequency, and neutral pressure in the helicon, ECH, ICH, and PMI regions that are required to achieve the desired MPEX scenarios. The necessity for key in-vessel components such as skimmers, limiters, and microwave absorbers will also be highlighted.

Lau, C. (ORCID:0000000285765867)↗
DOE OSTI2021

Oxygenate Production from Plasma-Activated Reaction of CO 2 and Ethane

Upgrading ethane with CO 2 as a soft oxidant represents a desirable means of obtaining oxygenated hydrocarbons. This reaction is not thermodynamically feasible under mild conditions and has not been previously achieved as a one-step process. Non-thermal plasma was implemented as an alternative means of supplying energy to overcome activation barriers, leading to the production of alcohols, aldehydes, and acids as well as C 1 -C 5+ hydrocarbons under ambient pressure, with a maximum total oxygenate selectivity of 12%. A plasma chemical kinetic computational model was developed and found to be in good agreement with the experimental trends. Results from this study illustrate the potential to use plasma for the direct synthesis of value-added alcohols, acids, and aldehydes from ethane and CO 2 under mild conditions.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2025

Influence of plasma screening on high-density inverse bremsstrahlung absorption

A spherical-implosion platform diagnosed with the “beamlets” scattered-light detector provides high sensitivity to the impact of plasma screening on inverse bremsstrahlung absorption. Contrary to the more restrictive screening length suggested previously [D. Turnbull et al., Phys. Rev. Lett. 130, 145103 (2023); D. Turnbull et al., Phys. Plasmas 31, 063304 (2024)], the beamlets data indicate that the electron-only Debye length is the relevant screening length for high-density inverse bremsstrahlung absorption. Furthermore, using the updated absorption model, we simulate the OMEGA direct-drive inertial confinement fusion implosion database and show that bang times are well reproduced without any ad hoc multipliers.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2022

Plasma‐driven biocatalysis: In situ hydrogen peroxide production with an atmospheric pressure plasma jet increases the performance of OleT JE when compared to adding the same molar amount of hydrogen peroxide in bolus

Abstract Enzymes like fatty acid peroxygenase OleT JE are desirable enzymes for the industry. While they require inexpensive hydrogen peroxide for activity, the same hydrogen peroxide also causes overoxidation of their reactive heme center. Here, we generate hydrogen peroxide slowly in situ using the Cooperation in Science and Technology (COST)‐Jet, an atmospheric pressure plasma jet, to avoid overoxidizing OleT JE . The COST‐Jet was operated in helium with a water admixture to provide hydrogen peroxide for OleT JE activity. This helium/water admixture produced the highest enzyme turnover numbers after 2 min of treatment. These turnover numbers were even superior to using an equimolar amount of hydrogen peroxide to treat the enzymes exogenously, showing that this plasma source can provide a reliable amount of reaction mediator to support OleT JE activity.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2023

Availability and reactivity of N 2 ( v ) for NH 3 synthesis by plasma catalysis

Production of vibrationally excited N 2 (N 2 (v)) in atmospheric pressure nonthermal plasma and loss of N 2 (v) by gas-phase reactions and reactions on catalytic surfaces are analyzed to examine the role of N 2 (v) in NH 3 formation by plasma catalysis. Vibrational state-to-state kinetic models complemented with molecular beam mass spectrometry (MBMS) measurements demonstrate that N 2 (v> 0) is produced with densities 100× greater than the density of N radicals by a radiofrequency atmospheric pressure plasma jet. The experimentally measured loss of N 2 (v) corresponds with a state-to-state kinetic model that describes loss of N 2 (v) by surface-mediated vibrational relaxation without consideration of reactions that convert N 2 (v) to NH 3 over the catalyst surface. Rate constants for vibrational relaxation of N 2 (v) on catalyst surfaces exceed upper bounds on proposed rate constants for NH 3 formation reactions from N 2 (v) over Fe when v < 9, Ni when v < 18, and Ag when v < 39, which indicates that only higher vibrational levels can possibly contribute to catalytic NH 3 formation faster than they undergo vibrational relaxation on the surface. Densities of N 2 (v> 8), vibrational levels that can possibly react over Fe to form NH 3 faster than they undergo vibrational relaxation, are less than or similar to N densities at the inlet of the catalyst bed and measured NH 3 formation for the investigated conditions in this work, while densities of N 2 (v> 17) and N 2 (v> 38) are orders of magnitude below the N density at the inlet of the catalyst bed and the measured NH 3 formation. The loss of N 2 (v) by vibrational relaxation on the surface limits the ability of N 2 (v) to contribute to catalytic NH 3 formation and explains why N 2 (v) does not produce NH 3 in quantities that are comparable to NH 3 formation from N even though N 2 (v > 0) is more abundantly produced by the plasma.

state-to-state kinetic modeling↗
DOE OSTI2023

Plasma assisted distributed chemical production

The present development is a process to produce commodity chemicals such as methanol and syngas using an integrated plasma catalysis technology. The method comprises providing a fixed or fluidized bed reactor having a microwave plasma flame and a catalyst bed with a catalyst, wherein the catalyst is an alloyed bimetallic nanowire. In the process, the plasma flame fluidizes the catalyst thereby producing a more effective catalyst than the non-fluidized catalyst. It is anticipated that the reactor can have a throughput capacity of up to 30 Lpm/kW and can be effective for the conversion of CO 2 , CH 4 , air, water, and combinations thereof, through reactions such as pure CO 2 splitting, reverse water gas shift (RWGS) for CO production, methanol synthesis, and plasma reforming of methane, thereby making a system that would be attractive for small GTL units.

Sunkara, Mahendra↗