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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 361 records · Page 20

Radiation Hardened Electronics for Reactor Environments

Radiation-hardened (rad-hard) electronics have been the shortcoming in nuclear sensing and instrumentation. Placing advanced sensors and associated electronics closer to a nuclear reactor core will improve reactor control and operation through increased signal accuracy, precision, and fidelity, resulting in safer, more efficient energy production. However, the extreme temperature and bombarding radiation environment of nuclear applications make research and development into electronics and electronic materials technologies essential to enabling improved safety, monitoring, and control of the existing nuclear reactor fleet and the next generation of reactors, including microreactors. To help the US Department of Energy (DOE) define a course for the Office of Nuclear Energy (NE)-funded rad-hard electronics research, Oak Ridge National Laboratory staff present this summary of the state-of-the-art (SOA) technology for the design and implementation of rad-hard electronics and systems, including research efforts and commercial offerings. A collection of technological gaps associated with reactor applications are compiled herein. Based on the radiation degradation mechanisms discussed in this report, along with the state-of-the-art summary survey and a compiled list of gaps, a high-level research plan of future NE funding direction was developed and is provided. This report outlines these activities and provides a summary of SOA electronics technology for rad-hard instrumentation in reactors, a list of the major technology gaps observed, and a draft plan for addressing the present and future needs of reactor instrumentation.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

A Critical Review of Heat Pipe Experiments in Nuclear Energy Applications

This critical review provides heat pipe (HP) experimental data sets that contain pertinent information regarding nuclear technology that may be beneficial to researchers. Heat pipes have been shown to have a tremendously positive impact on nuclear technologies and will continue to become a more prevalent technology as more nuclear reactor concepts embrace this robust technology. Most previous reviews may focus on only a specific HP design or application, and some are backdated. Herein, this critical review extends previous efforts; integrates and summarizes previously reported HP experimental efforts; and provides updates with recently reported results in the literature for HPs in all nuclear-related applications, including space power (thermal radiators, core cooling, and electricity production), microreactors (emergency core cooling, hybrid control rods, and reactor core cooling), and HP involvement in other nuclear-related technologies (spent fuel pool cooling). The two main objectives of this critical review are (1) to facilitate the development of HP codes by outlining some of the existing experimental data sets to validate their codes and directing developers to these efforts and (2) to provide comprehensive information regarding the vast applicability of HPs used in the nuclear industry, including the theory of operation and limitations to supplement researchers in the development of new ideas for potential applications in nuclear-related technologies. The review clearly shows extensive and diverse experimental data sets for HPs developed under diverse testing conditions depending on the available nuclear application for validation purposes. Thus, this critical review is oriented to providing attention to the existing efforts rather than determining gaps in HP research.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Comparison of different noble gas injections by massive gas injection on plasma disruption mitigation on Experimental Advanced Superconducting Tokamak

Massive gas injection (MGI) is a traditional plasma disruption mitigation method. This method directly injected massive gas into the pre-disruption plasma and had been developed on the Experimental Advanced Superconducting Tokamak (EAST). Different noble gas injection experiments, including He, Ne, and Ar, were performed to compare the mitigation effect of plasma disruption by evaluating the key parameters such as flight time, pre-thermal quench (pre-TQ), and current quench (CQ). The flight time was shorter for low atomic number ( Z ) gas, and the decrease in flight time by increasing the amount of gas was insignificant. However, both pre-TQ and CQ durations decreased considerably with the increase in gas injection amount. The effect of atomic mass on pre-TQ and CQ durations showed the opposite trend. The observed trend could help in controlling CQ duration in a reasonable area. Moreover, the analysis of radiation distribution with different impurity injections indicated that low Z impurity could reduce the asymmetry of radiation, which is valuable in mitigating plasma disruption. These results provided essential data support for plasma disruption mitigation on EAST and future fusion devices.

Physics↗

Journal paper

Laser technology is being widely studied for controlled energy deposition for a range of applications, including flow control, ignition, combustion, and diagnostics. The absorption and scattering of laser radiation by liquid droplets in aerosols affects propagation of the laser beam in the atmosphere, while the ignition and combustion characteristics in combustion chambers are influenced by the evaporation rate of the sprayed fuel. In this work, we present a mathematical model built on OpenFOAM for laser heating and evaporation of a single droplet in the diffusion-dominated regime taking into account absorption of the laser radiation, evaporation process, and vapor flow dynamics. The developed solver is validated against available experimental and numerical data for heating and evaporation of ethanol and water droplets. The two main regimes—continuous and pulsed laser heating—are explored. For continuous laser heating, the peak temperature is higher for larger droplets. For pulsed laser heating, when the peak irradiance is close to transition to the boiling regime, the temporal dynamics of the droplet temperature does not depend on the droplet size. With the empirical normalization of time, the dynamics of the droplet shrinkage and cooling are found to be independent of droplet sizes and peak laser intensities.

42 ENGINEERING↗

Numerical Modeling of Laser Heating and Evaporation of a Single Droplet

Laser technology is being widely studied for controlled energy deposition for a range of applications, including flow control, ignition, combustion, and diagnostics. The absorption and scattering of laser radiation by liquid droplets in aerosols affects propagation of the laser beam in the atmosphere, while the ignition and combustion characteristics in combustion chambers are influenced by the evaporation rate of the sprayed fuel. In this work, we present a mathematical model built on OpenFOAM for laser heating and evaporation of a single droplet in the diffusion-dominated regime taking into account absorption of the laser radiation, evaporation process, and vapor flow dynamics. The developed solver is validated against available experimental and numerical data for heating and evaporation of ethanol and water droplets. The two main regimes—continuous and pulsed laser heating—are explored. For continuous laser heating, the peak temperature is higher for larger droplets. For pulsed laser heating, when the peak irradiance is close to transition to the boiling regime, the temporal dynamics of the droplet temperature does not depend on the droplet size. With the empirical normalization of time, the dynamics of the droplet shrinkage and cooling are found to be independent of droplet sizes and peak laser intensities.

42 ENGINEERING↗

Apparatuses and methods for optical code-delay reflectometry (OcoDR)

Apparatuses and methods for optical code-delay reflectometry (OCoDR) are disclosed. An apparatus includes a modulator, a receiver, and control circuitry. The modulator is configured to receive incident electromagnetic (EM) radiation at a substantially fixed frequency generated by one or more EM radiation sources. The incident EM radiation includes continuous-wave EM radiation. The modulator is configured to impart a sequence onto an amplitude, a phase, or both of the incident EM radiation to generate modulated EM radiation. The modulated EM radiation includes continuous-wave EM radiation. The receiver is configured to receive reference EM radiation. The receiver is also configured to receive reflected EM radiation from an optical system responsive to the modulated EM radiation and generate interfered EM radiation responsive to the reference EM radiation and the reflected EM radiation. The receiver is further configured to generate a continuous interferogram responsive to the interfered EM radiation.

Seeley, Ryan↗

Impact of Nd ions on the chemical kinetic behavior of radiolytic transients in molten LiCl-KCl-NdCl3 salt mixtures

Pyrochemical reprocessing technologies can be used to recover valuable materials from used nuclear fuel (UNF), such as uranium. However, other critical materials, such as fission product neodymium, are challenging to recover from molten chloride eutectic mixtures (LiCl-KCl) due to the presence of multivalent states (Nd2+/Nd3+), disproportionation reactions, and re-dissolution in the molten chloride salt. Understanding, predicting, and controlling these processes is further complicated by the presence of ionizing radiation fields, for which little is known on the interaction of neodymium ions with the radiolytic transients (es– and Cl2.–) in molten LiCl-KCl salt mixtures. Here, chemical kinetics, from integrated electron pulse irradiation and transient absorption spectroscopy, are presented for the reaction of Nd3+ ions with es– and Cl2.– as a function of temperature (400–600 ?).

36 - MATERIALS SCIENCE↗

Strong-field QED limitations on TeV-class plasma wakefield accelerators

We demonstrate that quantum and classical radiation effects can become non-negligible for TeV-class beams propagating through plasma channels typical of staged plasma accelerators. Although the quantum nonlinearity parameter χ e remains small under currently envisioned experimental conditions, the cumulative influence of radiation over long acceleration distances can lead to significant modifications to the beam’s energy spread, emittance, and polarization. Our analytic models, validated by particle-in-cell simulations, highlight that for standard Gaussian beams, the orbit-induced energy spread dominates over quantum stochastic effects but can be mitigated by tailoring the beam profile, for example, through ring-shaped transverse distributions. In regimes where the radiation reaction approaches the accelerating force, the emittance may be cooled, forming distinctive ring-shaped phase-space structures. Finally, we analyze the influence of the radiation effect on spin transport inside the wakefield. These findings underscore the importance of considering both classical and quantum radiation dynamics in the design and optimization of future high-intensity plasma accelerators.

accelerator↗

Direct visualization of radiation-induced transformations at alkali halide–air interfaces

Radiation driven reactions at mineral/air interfaces are important to the chemistry of the atmosphere, but experimental constraints (e.g. simultaneous irradiation, in situ observation, and environmental control) leave process understanding incomplete. Using a custom atomic force microscope equipped with an integrated X-ray source, transformation of potassium bromide surfaces to potassium nitrate by air radiolysis species was followed directly in situ at the nanoscale. Radiolysis initiates dynamic step edge dissolution, surface composition evolution, and ultimately nucleation and heteroepitaxial growth of potassium nitrate crystallites mediated by surface diffusion at rates controlled by adsorbed water. Finally, in contrast to in situ electron microscopy and synchrotron-based imaging techniques where high radiation doses are intrinsic, our approach illustrates the value of decoupling irradiation and the basis of observation.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Acoustic Radiation From a Superconducting Qubit: From Spontaneous Emission to Rabi Oscillations

Hybrid quantum systems that utilize controllable coupling between phonons and superconducting qubits could pave the way for a new generation of compact quantum memories and sensor technologies. However, the same electromechanical interaction mechanisms that enable coherent qubit-phonon coupling can also lead to decoherence due to the spontaneous phonon emission. In this paper we study the dynamics of a qubit coupled to an acoustic resonator by a piezoelectric film. By varying the surface topography of the resonator from rough to flat to shaped, we explore the crossover from fast decay of an excited qubit to quantum-coherent coupling between the qubit and an isolated phonon mode. The developed theoretical model allows us to establish and check quantitative links between the results obtained for the rough and shaped topographies. Discrepancy between the theory and the data for the flat resonator points to the imperfections of the studied device. Our experimental approach may be used for precision measurements of crystalline vibrations, the design of quantum memories, and the study of electromechanical contributions to dielectric loss.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

MARVEL Instrumentation, Control, and Software Considerations

This paper details the various I&C considerations and design decisions made throughout the MARVEL (Micro-reactor Applications Research Validation and Evaluation) project, including sensor and actuator selection, safety-related functionality, digital control hardware and software, and testing methodologies. Key challenges such as managing radiation, temperature, and space constraints are discussed, along with the trade-offs between using standard equipment and custom solutions. The successful integration of off-the-shelf components, the emphasis on minimizing safety-related instrumentation, and the lessons learned from prototyping and testing are highlighted. The authors aim to provide insights that can benefit future micro-reactor designs and emphasize the importance of real-world testing in advancing reactor technology.

46 - INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AN↗

Confirming the absence of nuclear warheads via passive gamma-ray measurements

Arms-control agreements between the United States and Russia negotiated after the end of the Cold War have imposed limits on the number of deployed strategic nuclear weapons. Verification of these agreements has relied on onsite inspections, sometimes supported by radiation detection techniques to confirm the absence of a nuclear warhead when ambiguities arise. So far, these measurements have sought to detect neutron emissions associated with the presence of plutonium, but they would be inadequate for uranium devices. In an effort to offer instruments that could be used to confirm the absence of both plutonium and uranium weapons, here we propose an inspection system that uses only passive gamma radiation detection techniques. Such a system would be particularly valuable for next-generation arms-control agreements that limit total numbers of weapons and would involve containerized items in storage. We conducted extensive Monte Carlo simulations to support the development of a verification protocol and detection algorithm. Here, we demonstrate the viability of the technique using standard laboratory check sources and MCNP simulations for simplified configurations of special nuclear material.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗

Investigating the FLASH Effect in a Rat Brain Organotypic Model With a Novel High-Energy Electron Beam

Ultrahigh dose rate (FLASH) radiation therapy is reported to reduce normal tissue toxicity while maintaining tumor control; however, mechanism(s) remain obscure. To study FLASH mechanisms in brain tissue, we developed a novel experimental platform featuring a specialized high-energy electron linear accelerator, High Intensity Gamma Ray Source (HIGS), paired with an organotypic ex vivo brain metastasis model. We varied interpulse spacing to modulate the mean dose rate (MDR) of our unique 35 MeV electron beam, while maintaining extremely high instantaneous dose rate (IDR). We characterized dosimetry and targeting accuracy of the FLASH beam with film dosimetry. We combined this FLASH beam with an organotypic rat brain slice/breast carcinoma coculture model of brain metastasis to assess effects on normal and neoplastic tissues. Live-cell and bioluminescence imaging demonstrated cancer cell growth effects, whereas normal tissue responses and immune activation were assessed using live-cell imaging, cytokine profiles, and confocal microscopy. Here, we performed comparison experiments with 20 MeV electrons from a Varian clinical linear accelerator (VCLA) using conventional dose rates. The highest IDR of the FLASH beam to date was 20.7 ± 0.6 MGy/s, with maximum MDR of 20.7 MGy/s delivered in 1 pulse of 1 µs duration. Beam targeting was accurate to <1 mm and reproducible. HIGS-FLASH and VCLA dose rates equivalently decreased cancer cell growth. HIGS-FLASH irradiation significantly increased tumor necrosis factor α and fractalkine levels and confocal microscopy revealed distinct changes in microglial morphology slices suggesting microglia activation. Our novel experimental platform produces extremely high dose rates and rapid normal/neoplastic tissue readouts for mechanistic research into the effects of FLASH radiation in the brain. HIGS-FLASH irradiation induces comparable cancer cell growth inhibition but differential effects on cytokines and microglial morphology, suggesting that acute innate immune responses may be involved in FLASH normal tissue effects in the brain.

Kay, Tyler V. [Duke University, Durham, NC (United↗

Savannah River National Laboratory Participation in the International Atomic Energy Agency CPC Interlaboratory Comparison Exercise 2

International Atomic Energy Agency Safeguards Analytical Services (IAEA-SGAS) oversees coordinating the second Controlled Potential Coulometry Quality Control Interlaboratory Comparison (CPC QC ILC) on behalf of the Nuclear Material Laboratory (NML). The purpose of the exercise is to: (1) verify the ability of participating laboratories to measure the Pu concentration in the sample solutions, and (2) estimate the method performance (repeatability and intermediate reproducibility). Sample shipping coordination was performed by IAEA-SGAS. The test sample is a plutonium nitrate solution (estimated molarity of 3-5 M), delivered in two PTFE screw-capped quartz ampoules. Each participating laboratory is to receive two ampoules. Each ampoule holds approximately 8 mL of solution containing approximately 10 mg Pu/g. The gross weights of the ampoules were provided. The test sample is assumed to have an iron content below the level of significance for the CPC. The isotopic composition of the plutonium test sample was provided; however, no analysis date was provided. In addition, IAEA-SGAS provided analytical instructions to participants. On September 20, 2022, SRNL received the samples sent by IAEA-SGAS.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗

Neutronic impact of Autonomous Reactivity Control system inclusion in a breed-and-burn core

This work examines the impacts induced in a large breed-and-burn core through the inclusion of Autonomous Reactivity Control (ARC) systems from the neutronics perspective. A combination of numerical and analytical techniques are used to conservatively quantify the reactivity penalty, amount of additional tritium production, and depletion of the system absorber fluid. The reactivity penalty is found to be negligibly small, with the largest impact resulting from the removal of fuel material to make room for the ARC system tubes. Similarly, the depletion of the absorber fluid is found to be negligible compared to the amount of fluid present. It is found that the production of tritium within the active core is also small in comparison to that which is nominally produced, while tritium production within the lower ARC system reservoir may be of concern if not adequately considered during the assembly design phase. This issue is explored and a mitigation technique is proposed. Ultimately this study concludes that there are no issues from the steady-state neutronics perspective preventing incorporation of ARC systems into typical breed-and-burn cores.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Detecting tropospheric composition and climate responses to US air pollution controls in the context of internally-arising variability

Since the 1970s, air pollutant emissions controls in the United States (US) have lowered concentrations of ozone (O 3 ) and aerosols, which have opposing radiative effects on surface temperature. Using a pair of initial-condition ensembles generated by a fully-coupled chemistry-climate model, we simulate the “world avoided” by US air pollution controls. In this counterfactual world, we find tropospheric column O 3 increases, robust to natural internal variability, extending across the Northern Hemisphere. Robust aerosol increases, dominated by sulfate, remain localized near the US. Wintertime Northwest Atlantic cloud droplet number concentration is particularly sensitive to US aerosol. While an ensemble mean US surface cooling signal (−0.4 °C) implies that aerosol-driven cooling prevails over any O 3 -induced warming, we find that large regional internal variability will confound its detection in any single transient realization. Larger signal-to-noise ratios for composition versus climate variables underscore the greater detectability of emissions-driven changes in tropospheric composition compared to their associated climate impacts.

54 ENVIRONMENTAL SCIENCES↗

Disentangling core and edge mechanisms of the density limit in DIII-D negative triangularity plasmas

The density limit is investigated in the DIII-D negative triangularity plasmas which lack a standard H-mode edge. We find the limit may not be a singular disruptive boundary but a multifaceted density saturation phenomenon governed by distinct core and edge transport mechanisms. Sustained, non-disruptive operation is achieved at densities up to 1.8 times the Greenwald limit ($n_\mathrm{G}$) until the termination of auxiliary heating. Systematic power scans show distinct power scalings for the core ($n_e \propto P_\mathrm{SOL}^{0.27\pm0.03}$) and edge ($n_e \propto P_\mathrm{SOL}^{0.42\pm0.04}$) density limits. The edge density saturation is triggered by the onset of a non-disruptive, high-field side radiation front and the associated cooling, which clamps the edge density below . In contrast, the core density continues to rise until it saturates, a state characterized by enhanced core turbulence. Core transport evolves from a diffusive to an intermittent, avalanche-like state, as indicated by heavy-tailed probability density functions (kurtosis ≈ 6), increased Hurst exponents, and a $1/f$-type power spectrum. These findings suggest that the density limit in the low-confinement regime is determined by a combination of edge radiative cooling and core turbulent transport. This distinction provides separate targets for control strategies aimed at extending the operational space of future fusion devices.

density limit↗