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At least 523 records · Page 29

Insulation Activation and Contamination in Low-Power Experiments

Among the diverse advanced nuclear reactor concepts being developed are designs that expect to operate at much higher temperatures than conventional light-water reactors, and therefore require alternative materials for components capable of withstanding these extreme temperatures. Insulation is one such component where alternative high-temperature industrial composites are being considered. Low-power experiments can provide an opportunity for advancing our understanding of material behavior under irradiation; however, these experiments are not without occupational hazards. The focus of this paper is the potential for activation of insulating composites when exposed to neutron fluence during reactor experiments, and to discuss the subsequent contamination of the testing area. This paper will also discuss practical measures for preventing the creation and inhalation of activated particulate matter (i.e., dust), such as engineering and administrative controls and personal protective equipment. This paper evaluates the suitability of several insulation materials for use in reactor experiments based on their activation from neutron irradiation. The materials considered are Pyrogel XTE by Aspen Aerogel, Cerablanket and Kaowool by Morgan Advanced Materials, Thermo-12 Gold by Johns Manville, and Maxsil CF6-2000 by McAllister Mills. Although these materials are not yet widely used in the nuclear industry, they are common in other industries due to their thermal insulating properties. These materials produce dust while handling that can pose health and safety hazards, which could be further exacerbated by activation. The analysis presented in this paper utilizes a deterministic method developed to predict the activation source term of the provided insulation materials. The method calculates the atomic density of each element within the composites and simulates their exposure to a specified neutron flux density representative of low power experimental conditions. During the irradiation phase and throughout the extensive cooling period, neutron absorptions and nuclear decays are tracked for relevant isotopes. The residual activity within each composite is then assessed to identify the material with the lowest potential radiological hazard to workers. Dust will be created during installation and removal of insulating materials and may also be generated during the experiment. Contamination of surrounding surfaces due to dispersion is highly likely unless preventative measures are taken. The results of this analysis are used to estimate an internal dose from inhalation of activated dust, which is significantly lower than the allowable whole-body dose. However, the risk of internal exposure may increase if the dust becomes a transport vector for nuclear material. The goals of this paper are to enhance the understanding of the potential activation and contamination hazards from the use of these insulating materials in low-power nuclear experiments and to foster safer work environments through informed decision-making and strategic planning. This work ultimately contributes to a broader understanding of how new non-nuclear materials for advanced reactors impact the radiological safety of co-located workers, helping to ensure the responsible management of radioactive materials during installation and decommissioning activities.

12 - MGMT OF RADIOACTIVE AND NON-RADIOACTIVE WASTE↗

Initial Design of SABRE Fueled Molten Salt Experiment Irradiation Vehicle

Molten Salt Reactors (MSRs) are emerging as promising advanced reactor technologies, utilizing molten salts for both fuel and primary cooling. These reactors may offer advantages such as passive safety, enhanced economic viability, and efficient waste reprocessing while operating at high temperatures and low pressures, which leads to increased system efficiency and reduced mechanical stress on containment structures. However, challenges arise from the complex chemistry and high corrosion rates of fueled molten salts, alongside the volatility of certain fission products during irradiation. The accumulation of these fission products can alter the fuel salt chemistry, affecting corrosion potential and radioactive source terms. Therefore, understanding these phenomena under neutron irradiation is essential for future MSR designs. The SABRE (Salt and Actinide Burnup in a Reactor Environment) experiment, currently in conceptual design at Idaho National Laboratory (INL), aims to investigate these challenges by conducting a drop-in capsule experiment in the Advanced Test Reactor (ATR). The primary objectives include achieving a minimum burnup of 2 GWd/MTU and characterizing fission products while studying corrosion behavior in molten salt systems. This innovative experiment will leverage recent advancements in ATR capabilities, allowing for the safe irradiation of molten salts, thereby advancing the understanding and qualification of MSR technology for future nuclear power generation.

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Nuclear Safety [Vol. 36, No. 2, July-December 1995]

Nuclear Safety is a journal that covers significant issues in the field of nuclear safety. Its primary scope is safety in the design, construction, operation, and decommissioning of nuclear power reactors worldwide and the research and analysis activities that promote this goal, but it also encompasses the safety aspects of the entire nuclear fuel cycle, including fuel fabrication, spent-fuel processing and handling, and nuclear waste disposal, the handling of fissionable materials and radioisotopes, and the environmental effects of all these activities. Table of Contents for this issue follows. THE CHORNOBYL ACCIDENT: 195 The Chornobyl Accident Revisited, Part III: Chernobyl Source Term Release Dynamics and Reconstruction of Events During the Active Phase, A. R. Sich; GENERAL SAFETY CONSIDERATIONS: 218 Second ANS Workshop on the Safety of Soviet-Designed Nuclear Power Plants, R. A. Bari; 234 Elements of a Nuclear Criticality Safety Program, C. M. Hopper; 243 Rickover, Excellence, and Criticality Safety Programs, R. E. Wilson; ACCIDENT ANALYSIS: 249 Transient Analysis of the PIUS Advanced Reactor Design with the TRAC-PF1/MOD2 Code, B. E. Boyack, J. L Steiner, S. C. Harmony, H. J. Stumpf, and J. F. Lime; 278 The Hierarchy-By-Interval Approach to Identifying Important Models that Need Improvement in Severe-Accident Simulation Codes, T. J. Heames, M. Khatib-Rahbar, J. E. Kelly, R. P. Jenks-Johnson, and Y.-S. Chen; 290 RELAP5/MOD3 Code Coupling Model, R. P. Martin; 299 Missiles Caused by Severe Pressurized-Water Reactor Accidents, R. Krieg; DESIGN FEATURES: 310 Validation of COMMIX with Westinghouse AP-600 PCCS Test Data, J. G. Sun, T. H. Chien, J. Ding, and W T. Sha; ENVIRONMENTAL EFFECTS: 321 Spent Nuclear Fuel Characterization for a Bounding Reference Assembly for the Receiving Basin for Off-Site Fuel, S. D. Kahook, R. L. Garrett, L. R. Canas, and M J. Beckum; OPERATING EXPERIENCES: 332 Reactor Shutdown Experience, Compiled by J. W. Cletcher; U.S. NUCLEAR REGULATORY COMMISSION INFORMATION AND ANALYSES: 335 Reactor Coolant System Blowdown at Wolf Creek on September 17, 1994, J. V. Kauffman and S. L. Israel; RECENT DEVELOPMENTS: 344 Reports, Standards, and Safety Guides, D. S. Oueener; 349 Proposed Rule Changes as of June 30, 1995; ANNOUNCEMENTS: 320 Symposium on Acceptability of Risk From Radiation—Application to Manned Space Flight; 320 24th DOE/NRC Nuclear Air Cleaning and Treatment Conference; 361 Radiation Biology and Radiation Protection— Modern Developments and Tendencies in Radiation Biology; 362 1997 IEEE Sixth Conference on Human Factors and Power Plants; 354 The Authors; 360 Reviewers of Nuclear Safety, Vol. 36.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

A Second Law Based Unstructured Finite Volume Procedure for Generalized Flow Simulation

An unstructured finite volume procedure has been developed for steady and transient thermo-fluid dynamic analysis of fluid systems and components. The procedure is applicable for a flow network consisting of pipes and various fittings where flow is assumed to be one dimensional. It can also be used to simulate flow in a component by modeling a multi-dimensional flow using the same numerical scheme. The flow domain is discretized into a number of interconnected control volumes located arbitrarily in space. The conservation equations for each control volume account for the transport of mass, momentum and entropy from the neighboring control volumes. In addition, they also include the sources of each conserved variable and time dependent terms. The source term of entropy equation contains entropy generation due to heat transfer and fluid friction. Thermodynamic properties are computed from the equation of state of a real fluid. The system of equations is solved by a hybrid numerical method which is a combination of simultaneous Newton-Raphson and successive substitution schemes. The paper also describes the application and verification of the procedure by comparing its predictions with the analytical and numerical solution of several benchmark problems.

Majumdar, Alok↗

Search for correlated radio and optical events in long-term studies of extragalactic sources

For the first time, long-term records of radio and optical fluxes of a large sample of variable extragalactic sources have been assembled and compared, with linear cross-correlation analysis being used to reinforce the visual comparisons. Only in the case of the BL Lac object OJ 287 is the correlation between radio and optical records strong. In the majority of cases there is no evidence of significant correlation, although nine sources show limited or weak evidence of correlation. The results do not support naive extrapolation of the expanding source model. The general absence of strong correlation between the radio and optical regions has important implications for the energetics of events occurring in such sources.

Pomphrey, R. B.↗

A Systematic Search for Short-term Variability of EGRET Sources

The 3rd EGRET Catalog contains 170 unidentified high-energy (E>100 MeV) gamma-ray sources, and there is great interest in the nature of these sources. One means of determining sources class is the study of flux variability on time scales of days; pulsars are believed to be stable on these scales while blazars are known to be highly variable. In addition, previous work has led to the discovery of 2CG 135+01 and GRO J1838-04, candidates for a new high-energy gamma-ray source class. These sources display transient behavior but cannot be associated with any known blazars. These considerations have led us to conduct a systematic search for short-term variability in EGRET data, covering all viewing periods through cycle 4. Three unidentified sources show some evidence of variability on short time scales; the source displaying the most convincing variability, 3EG J2006-2321, is not easily identified as a blazar.

Wallace, P. M.↗

Long-term cycles in cosmic X-ray sources

Data on long-term cycles in galactic X-ray sources are reviewed, and classes of variations are identified including precessional activity, recurrent outbursts in Population II sources, and Be/neutron star flare cycles. Cycles of 30-300 days have been found in LMC X-4, Her X-1, SS433, and Cyg X-1 which represent cyclic variations in both the inner and outer parts of the accretion disk. Quasi-periodic cycles with periods ranging from 1/2 to 2 years have been noted in several low-mass X-ray binaries. It is suggested that periodic outbursts in the Be/neutron star systems may result from variable mass transfer in a wide eccentric orbit.

Priedhorsky, W. C.↗

A Systematic Search for Short-term Variability of EGRET Sources

The 3rd EGRET Catalog of High-energy Gamma-ray Sources contains 170 unidentified sources, and there is great interest in the nature of these sources. One means of determining source class is the study of flux variability on time scales of days; pulsars are believed to be stable on these time scales while blazers are known to be highly variable. In addition, previous work has demonstrated that 3EG J0241-6103 and 3EG J1837-0606 are candidates for a new gamma-ray source class. These sources near the Galactic plane display transient behavior but cannot be associated with any known blazers. Although, many instances of flaring AGN have been reported, the EGRET database has not been systematically searched for occurrences of short-timescale (approximately 1 day) variability. These considerations have led us to conduct a systematic search for short-term variability in EGRET data, covering all viewing periods through proposal cycle 4. Six 3EG catalog sources are reported here to display variability on short time scales; four of them are unidentified. In addition, three non-catalog variable sources are discussed.

Wallace, P. M.↗

Quantifying Sources of Long-Term Voltage Decay for Rutile Iridium Oxide Anodes in Proton Exchange Membrane Water Electrolysis

To achieve aggressive hydrogen cost targets for proton exchange membrane water electrolysis (PEMWE), it is necessary to develop catalyst systems that reduce precious metal loadings while maintaining performance over extended operation. While amorphous iridium (Ir) -based catalysts exhibit high initial activity, their long-term stability remains a key limitation. In this study, the behavior of a rutile IrO2 catalyst is investigated over 4000 h of durability testing and compared to past efforts evaluating a more amorphous material. This study finds that rutile IrO2 results in a smaller decay rate (4.9 ..mu..V h-1) than an amorphous catalyst (28 ..mu..V h-1); additionally, the rutile IrO2 results in a smaller degree of Ir migration (20% to the membrane and cathode) than an amorphous catalyst (35%). This research emphasizes rutile IrO2 as a promising avenue for the development of durable, low-iridium anodes that can meet lifetime and cost targets for next-generation electrolyzer systems.

08 HYDROGEN↗

Tropical Diabatic Heating and the Role of Convective Processes as Represented in Several Contemporary Climate Models

One of the most fundamental properties of the global heat balance is the net heat input into the tropical atmosphere that helps drive the planetary atmospheric circulation. Although broadly understood in terms of its gross structure and balance of source / sink terms, incorporation of the relevant processes in predictive models is still rather poor. The work reported here examines the tropical radiative and water cycle behavior as produced by four contemporary climate models. Among these are the NSIPP-2 (NASA Seasonal to Interannual Prediction Project) which uses the RAS convective parameterization; the FVCCM, a code using finite volume numerics and the CCM3.6 physics; FVCCM-MCRAS again having the finite volume numerics, but MCRAS convective parameterization and a different radiation treatment; and, finally, the NCEP GSM which uses the RAS. Using multi-decadal integrations with specified SSTs we examine the statistics of radiative / convective processes and associated energy transports, and then estimate model energy flux sensitivities to SST changes. In particular the behavior of the convective parameterizations is investigated. Additional model integrations are performed specifically to assess the importance representing convective inhibition in regulating convective cloud-top structure and moisture detrainment as well as controlling surface energy fluxes. To evaluate the results of these experiments, a number of satellite retrievals are used: TRMM retrievals of vertical reflectivity structure, rainfall rate, and inferred diabatic heating are analyzed to show both seasonal and interannual variations in vertical structure of latent heat release. Top-of-atmosphere radiative fluxes from ERBS and CERES are used to examine shortwave and longwave cloud forcing and to deduce required seasonal energy transports. Retrievals of cloud properties from ISCCP and water vapor variations from SSM/T-2 are also used to understand behavior of the humidity fields. These observations are supplemented with output form the DOE Reanalysis-2.

Robertson, Franklin R.↗

Correcting STIS CCD Point-Source Spectra for CTE Loss

We review the on-orbit spectroscopic observations that are being used to characterize the Charge Transfer Efficiency (CTE) of the STIS CCD in spectroscopic mode. We parameterize the CTE-related loss for spectrophotometry of point sources in terms of dependencies on the brightness of the source, the background level, the signal in the PSF outside the standard extraction box, and the time of observation. Primary constraints on our correction algorithm are provided by measurements of the CTE loss rates for simulated spectra (images of a tungsten lamp taken through slits oriented along the dispersion axis) combined with estimates of CTE losses for actual spectra of spectrophotometric standard stars in the first order CCD modes. For point-source spectra at the standard reference position at the CCD center, CTE losses as large as 30% are corrected to within approx.1% RMS after application of the algorithm presented here, rendering the Poisson noise associated with the source detection itself to be the dominant contributor to the total flux calibration uncertainty.

Goudfrooij, Paul↗

Long-Term Stability of Radio Sources in VLBI Analysis

Positional stability of radio sources is an important requirement for modeling of only one source position for the complete length of VLBI data of presently more than 20 years. The stability of radio sources can be verified by analyzing time series of radio source coordinates. One approach is a statistical test for normal distribution of residuals to the weighted mean for each radio source component of the time series. Systematic phenomena in the time series can thus be detected. Nevertheless, an inspection of rate estimation and weighted root-mean-square (WRMS) variations about the mean is also necessary. On the basis of the time series computed by the BKG group in the frame of the ICRF2 working group, 226 stable radio sources with an axis stability of 10 as could be identified. They include 100 ICRF2 axes-defining sources which are determined independently of the method applied in the ICRF2 working group. 29 stable radio sources with a source structure index of less than 3.0 can also be used to increase the number of 295 ICRF2 defining sources.

Engelhardt, Gerald↗

Common Calibration Source for Monitoring Long-term Ozone Trends

Accurate long-term satellite measurements are crucial for monitoring the recovery of the ozone layer. The slow pace of the recovery and limited lifetimes of satellite monitoring instruments demands that datasets from multiple observation systems be combined to provide the long-term accuracy needed. A fundamental component of accurately monitoring long-term trends is the calibration of these various instruments. NASA s Radiometric Calibration and Development Facility at the Goddard Space Flight Center has provided resources to minimize calibration biases between multiple instruments through the use of a common calibration source and standardized procedures traceable to national standards. The Facility s 50 cm barium sulfate integrating sphere has been used as a common calibration source for both US and international satellite instruments, including the Total Ozone Mapping Spectrometer (TOMS), Solar Backscatter Ultraviolet 2 (SBUV/2) instruments, Shuttle SBUV (SSBUV), Ozone Mapping Instrument (OMI), Global Ozone Monitoring Experiment (GOME) (ESA), Scanning Imaging SpectroMeter for Atmospheric ChartographY (SCIAMACHY) (ESA), and others. We will discuss the advantages of using a common calibration source and its effects on long-term ozone data sets. In addition, sphere calibration results from various instruments will be presented to demonstrate the accuracy of the long-term characterization of the source itself.

Kowalewski, Matthew↗

Precipitation fluxes of energetic electrons at Jupiter - An estimated upper limit

Divine's (1976) model for the observed energetic electron fluxes in the inner Jovian magnetosphere is used to calculate space densities, and the combined source and loss term is evaluated for steady-state radial diffusion conserving the first and second adiabatic invariants. Upper-limit estimates for the ionospheric precipitation fluxes at various values of L and over various electron energy ranges are derived by assuming that contributions to the source term are negligible and that particle precipitation due to pitch-angle diffusion in the loss cone is the main contributor to the loss term. The energy deposition rates corresponding to these precipitated particles are estimated, along with the bremsstrahlung X-ray emissions that should result. It is found that the X-ray emissions should be 5 to 6 orders of magnitude below the reported upper observational limit.

Thomsen, M. F.↗

First experimental confirmation of island SOL geometry effects in a high radiation regime on W7-X

Abstract This work characterizes the detachment behavior and radiation characteristics of the low
iota configuration in the Wendelstein 7-X (W7-X) stellarator. The island scrape-off layer (SOL) of the
low iota has a poloidal mode number of 6 islands surrounding the last closed flux surface (LCFS).
The island geometry of the low iota configuration is significantly different to that of the standard
magnetic field configuration, whose detachment characteristics have already been described in previous
work[2, 3, 4]. Experimental results show that the radiation pattern in the low iota configuration
is starkly different to that of the standard magnetic field configuration, with radiation concentrated
at the island SOL O-points, rather than the X-points. Additionally, this O-point localized radiation
pattern is associated with unstable detachment, with both radiation oscillations in experiments and the
lack of a self-consistent plasma solution at high radiated power fraction in EMC3-Eirene simulations.
EMC3-Eirene simulations are used to understand the radiation distribution. It was found that the O-
point localized radiation arises first from local impurity accumulation near the parallel flow stagnation,
which is located close to the geometrical center of the island (”O-point”). The local cooling in this
region leads to plasma condensation in the islands in closest magnetic connection to the divertor target
plates. The heat source to this region of the island, which is thermally isolated from the upstream heat
source in terms of parallel transport, must arise via perpendicular heat transport. This heat source is
expected to be large for the low iota configuration due to its very small internal island field line pitch.
This work highlights the importance (complementary to previous work, e. g. [5, 6]) of the internal
island field line pitch not only on the radiation pattern, but also the detachment performance of the
island divertor.

Winters, Victoria (ORCID:0000000181087774)↗