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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 55 records · Page 3

Accelerated fission rate irradiation design, pre-irradiation characterization, and adaptation of conventional PIE methods for U-10Mo and U-17Mo

Metallic U alloys have high U density and thermal conductivity and thus have been explored since the beginning of nuclear power research. Alloys of U with modest amounts of Mo, such as U-10 wt % Mo (U-10Mo), are of particular interest because the γ-U crystal structure in this alloying addition shows prolonged stability in reactor service. Historically, radiation data on U-10Mo fuels were collected in Na fast reactors or lower temperature research reactor conditions, but little is known about irradiation behavior, particularly swelling and creep, at irradiation temperatures between 250 and 500°C. This work discusses the methodology and pre-irradiation characterization results from a U-Mo irradiation campaign performed in the High Flux Isotope Reactor at Oak Ridge National Laboratory. U-10Mo and U-17Mo samples irradiations are being completed at temperatures ranging from 250 to 500°C to three targeted fission densities between 2 × 10 20 and 1.5 × 10 21 fissions per cubic centimeter. Swelling measurement of the specimen sizes studied here required development and assessment of new methods for volume determination before and after irradiation. Laser profilometry and X-ray computation tomography (XCT) were used to provide preirradiation characterization of samples to determine the error and applicability of each to determine swelling following irradiation. These outcomes are contextualized through use of BISON simulations performed to assess the predicted expansion of U-Mo fuels subjected to the irradiation conditions of this work. Use of existing BISON fuel performance models predicted a maximum of 7% swelling under the irradiation conditions of this study. Pre-irradiation characterization revealed the as-cast U-Mo fuel samples were uniformly large-grained fully cubic U crystals with small U-C/N bearing precipitates and pores distributed throughout. Samples were found to contain a bulk porosity between .4 and 3% because of the casting process. Local porosity in areas far from large, interconnected pores was found by Slice-and-View to be under .2%. Nanometer-sized precipitates rich in C and N were identified in all samples, likely because of impurities during the fabrication process. Dendritic bands were also observed throughout the samples. These bands were characterized by variable Mo content that deviated from the overall Mo content by 2–3 wt %. No other microstructural features were correlated to these bands. Mechanical properties were found to be slightly strengthened compared to literature reports of bulk U-Mo fuels due to the nano-scale precipitates throughout the sample.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

AGR-5/6/7 PIE Overview 2024

This is a status update and description of major post-irradiation examination activities under the DOE's AGR TRISO fuel program. This presentation will be given at the annual program review hosted by INL the week of July 15.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

LaSalle Leaking Pin PIE Proposal

Determine the most probable root cause of the LaSalle fuel rod failure, distinguish primary failure mechanisms from post-failure degradation, and assess whether the condition is isolated or indicative of a broader issue affecting similar rods or assemblies. Results will support decisions related to core operation, fuel management, and corrective actions.

LaSalle↗

Irradiation and PIE of alloys X-750 and XM-19 (EPRI Phase III)

The Nuclear Science User Facilities (NSUF) based at Idaho National Laboratory (INL), along with the Electric Power Research Institute (EPRI), formed an agreement to test representative alloys used as reactor structural materials as a pilot program to establish guidelines for future NSUF research programs. This report contains results from the portion of this program established as Phase III (of three phases), entailing irradiation and post-irradiation examination of select alloys typical of boiling water reactor (BWR) internal structural materials. Phases I and II are the subject of separate reports and represent baseline material test results and irradiation experiment design, respectively. The intent of this Phase III research program is to determine properties for the materials of interest after being irradiated at the Advanced Test Reactor (ATR) to three different target fast (E>1MeV) fluences: 5.0 x 10¹⁹ n/cm², 2.0 x 10²⁰ n/cm², and 1.0 x 10²¹ n/cm². These correspond to irradiation damage levels (displacements per atom [dpa]) of approximately 0.08, 0.30, and 1.4 dpa, which represent comparable levels to (a) a previous study which looked at X-750 irradiated to ~1 x 10¹⁹ n/cm², comparable to the lowest fluence; (b) approximately a medium level of fluence for BWR components; and (c) extended life (60 – 80 years) for BWR components. The materials chosen for this research are the nickel-based alloy X-750 and austenitic stainless steel XM-19. A spare core shroud upper support bracket of alloy X-750 was purchased by EPRI from Southern Co., and a section of XM-19 plate was purchased by EPRI from GE-Hitachi. These materials were sectioned at GE Global Research Center (GE-GRC), and parts were provided to INL for use in this pilot project.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Irradiation and PIE of alloys X-750 and XM-19 (EPRI Phase III)

The Nuclear Science User Facilities (NSUF) based at Idaho National Laboratory (INL), along with the Electric Power Research Institute (EPRI), formed an agreement to test representative alloys used as reactor structural materials as a pilot program to establish guidelines for future NSUF research programs. This report contains results from the portion of this program established as Phase III (of three phases), entailing irradiation and post-irradiation examination of select alloys typical of boiling water reactor (BWR) internal structural materials. Phases I and II are the subject of separate reports and represent baseline material test results and irradiation experiment design, respectively. The intent of this Phase III research program is to determine properties for the materials of interest after being irradiated at the Advanced Test Reactor (ATR) to three different target fast (E>1MeV) fluences: 5.0 x 10¹⁹ n/cm², 2.0 x 10²⁰ n/cm², and 1.0 x 10²¹ n/cm². These correspond to irradiation damage levels (displacements per atom [dpa]) of approximately 0.08, 0.30, and 1.4 dpa, which represent comparable levels to (a) a previous study which looked at X-750 irradiated to ~1 x 10¹⁹ n/cm², comparable to the lowest fluence; (b) approximately a medium level of fluence for BWR components; and (c) extended life (60 – 80 years) for BWR components. The materials chosen for this research are the nickel-based alloy X-750 and austenitic stainless steel XM-19. A spare core shroud upper support bracket of alloy X-750 was purchased by EPRI from Southern Co., and a section of XM-19 plate was purchased by EPRI from GE-Hitachi. These materials were sectioned at GE Global Research Center (GE-GRC), and parts were provided to INL for use in this pilot project.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Status Report on Characterization of High Burnup Fuel with Advanced Nondestructive Pulsed Neutron PIE

Characterizing irradiated or spent nuclear fuels with pulsed neutron techniques provides microstructural data such as phase fractions as well as crystallographic data, e.g. lattice parameters, from diffraction analysis. Diffraction characterization is complemented by spatially resolved mapping of isotope densities from energy-resolved neutron imaging, in particular neutron absorption resonance imaging, and overall bulk isotope assay with better sensitivity for minority isotopes from neutron absorption resonance spectroscopy without spatial resolution. Furthermore, after characterization at ambient condition, heating of irradiated or spent fuel will allow to characterize differences of e.g. lattice thermal expansion or phase transition temperature and kinetics compared to fresh fuel as well as enable the study of disappearance of irradiation defects. This data enables benchmarking of predictions of properties of irradiated fuels for which otherwise experimental data is sparse. The effort described here strives to characterize a section cut from a high-burnup fuel. Volumes smaller than entire fuel pellets or rodlets as proposed here, e.g. sections cut from a fuel pellet, to pave the way to characterize entire pellets or rodlets in the future.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Destructive PIE and Safety Testing of Six AGR-5/6/7 Capsule 2 Compacts

This study evaluates fission product retention and particle failure mechanisms in AGR-5/6/7 Capsule 2 uranium carbide and uranium oxide (UCO) tristructural isotropic (TRISO) fuel under high-temperature gas reactor accident-relevant conditions using high-temperature safety tests and destructive postirradiation examination. Three Capsule 2 compacts were held isothermally at 1600°C for approximately 300 hours and one compact at 1800°C for approximately 300 hours; two additional compacts were examined in the as-irradiated state. Post-test deconsolidation–leach–burn–leach (DLBL) quantified nuclide inventories in matrix and particles. Individual particles were surveyed for radioisotope inventories, and microanalytical approaches resolved microstructural evolution and fission product distributions within the coating layers. At 1600°C, no krypton was detected above the minimum detectable limit, and cesium releases were far below a single particle equivalent, indicating the absence of full TRISO failure or SiC failures. Silver releases were limited and primarily reflected depleted postirradiation inventories, consistent with prior compact-level exams indicating substantial in-pile 110mAg loss. At 1800°C, cumulative 134Cs release of approximately 2.5 particle equivalents and delayed 85Kr totaling approximately 0.53 particle equivalents were consistent with one full TRISO failure and two SiC failures. Europium and strontium releases were roughly one order of magnitude higher than at 1600°C and comparable to AGR-1/AGR-2 high-temperature tests, with sustained late-hold rates indicating diffusion through intact coatings coupled with matrix depletion. Overall, AGR-5/6/7 Capsule 2 UCO fuel demonstrated fission product retention during safety testing consistent with prior AGR campaigns, while distinctive in-pile 110mAg depletion and measurable 1600°C europium loss motivate targeted follow-on studies.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Destructive PIE and Safety Testing of Six AGR-5/6/7 Capsule 2 Compacts

This study evaluates fission product retention and particle failure mechanisms in AGR-5/6/7 Capsule 2 uranium carbide and uranium oxide (UCO) tristructural isotropic (TRISO) fuel under high-temperature gas reactor accident-relevant conditions using high-temperature safety tests and destructive post-irradiation examination. Three Capsule 2 compacts were held isothermally at 1600°C for approximately 300 hours and one compact at 1800°C for approximately 300 hours; two additional compacts were examined in the as-irradiated state. Post-test deconsolidation–leach–burn–leach (DLBL) quantified nuclide inventories in matrix and particles. Individual particles were surveyed for radioisotope inventories, and microanalytical approaches resolved microstructural evolution and fission product distributions within the coating layers. At 1600°C, no krypton was detected above the minimum detectable limit, and cesium releases were far below a single particle equivalent, indicating the absence of full TRISO failure or SiC failures. Silver releases were limited and primarily reflected depleted post-irradiation inventories, consistent with prior compact-level exams indicating substantial in-pile 110m Ag loss. At 1800°C, cumulative 134 Cs release of approximately 2.5 particle equivalents and delayed 85 Kr totaling approximately 0.53 particle equivalents were consistent with one full TRISO failure and two SiC failures. Europium and strontium releases were roughly one order of magnitude higher than at 1600°C and comparable to AGR-1/AGR-2 high-temperature tests, with sustained late-hold rates indicating diffusion through intact coatings coupled with matrix depletion. Overall, AGR-5/6/7 Capsule 2 UCO fuel demonstrated fission product retention during safety testing consistent with prior AGR campaigns, while distinctive in-pile 110m Ag depletion and measurable 1600°C europium loss motivate targeted follow-on studies.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Telescopes on the Moon or pie in the sky?

The question is examined of whether it makes sense to believe that there will one day be an interferometric array of telescopes on the Moon. The question is really one of national commitment to a lunar base, since it is not likely that a scientific undertaking of this magnitude would occur in the absence of permanent human presence on the Moon. A discussion is also given of the real possibility if the exploration of space should be a multinational effort.

Pilcher, Carl B.↗

PIE: A Dynamic Failure-Based Technique

This paper presents a dynamic technique for statistically estimating three program characteristics that affect a program's computational behavior: (1) the probability that a particular section of a program is executed, (2) the probability that the particular section affects the data state, and (3) the probability that a data state produced by that section has an effect on program output. These three characteristics can be used to predict whether faults are likely to be uncovered by software testing. Index Terms: Software testing, data state, fault, failure, testability. 1 Introduction

Voas, Jeffrey M.↗

Modeling of the AGR 3/4 PIE Experiments

TRISO Fuel Accident Scenarios Transport of Fission Products (FP) through modern nuclear-grade graphites is not well established The AGR 3/4 experimental results need to be modeled to extract FP transport characteristics A finite element model using graphite diffusivities from IAEA TECDOC-978 is compared against measured results

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Enhancing Post-Irradiation Examination (PIE) Efficiency with High-Throughput Experiments

Nuclear materials testing is essential for understanding changes in reactor environments, but traditional methods are costly and time-consuming. High-Throughput Experimentation (HTE) enables rapid screening and optimization of material properties by significantly increasing the number of specimens in the experiment. In this work, HTE methods were employed to irradiate novel materials at the Advanced Test Reactor (ATR) at Idaho National Laboratory. A total of 367 sub-sized tensile specimens were irradiated using the standard capsule design. To facilitate HTE, automated systems such as the Automated Mechanical Testing System were implemented for mechanical testing within hot cell environments, thereby reducing the need for manual interaction with hot cell manipulators and significantly lowering both the cost and duration of experiments. Digital image correlation (DIC) was used to measure displacement during mechanical testing, providing precise, non-contact measurement capabilities. The methodologies developed in this research will support the advancement of HTE techniques for future nuclear materials testing experiments at ATR. This approach allows for more efficient and cost-effective evaluation of new materials, ultimately leading to improved reactor performance, enhanced safety, and extended longevity within the nuclear industry.

22 - GENERAL STUDIES OF NUCLEAR REACTORS↗

Limits on Achievable Dimensional and Photon Efficiencies with Intensity-Modulation and Photon-Counting Due to Non-Ideal Photon-Counter Behavior

An ideal intensity-modulated photon-counting channel can achieve unbounded photon information efficiencies (PIEs). However, a number of limitations of a physical system limit the practically achievable PIE. In this paper, we discuss several of these limitations and illustrate their impact on the channel. We show that, for the Poisson channel, noise does not strictly bound PIE, although there is an effective limit, as the dimensional information efficiency goes as e[overline] e PIE beyond a threshold PIE. Since the Holevo limit is bounded in the presence of noise, this illustrates that the Poisson approximation is invalid at large PIE for any number of noise modes. We show that a finite transmitter extinction ratio bounds the achievable PIE to a maximum that is logarithmic in the extinction ratio. We show how detector jitter limits the ability to mitigate noise in the PPM signaling framework. We illustrate a method to model detector blocking when the number of detectors is large, and illustrate mitigation of blocking with spatial spreading and altering. Finally, we illustrate the design of a high photon efficiency system using state-of-the-art photo-detectors and taking all these effects into account.

quantum limited communications↗