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At least 55 records · Page 3

Four-wave mixing with anti-parity-time symmetry in hot 85 Rb vapor

Here, we report an experimental demonstration of anti-parity-time symmetric optical four-wave mixing in thermal rubidium vapor, where the propagation of probe and stokes fields in a double-Λ scheme is governed by a non-Hermitian Hamiltonian. We are particularly interested in studying quantum intensity correlations between the two fields near the exceptional point, taking into account loss and accompanied Langevin noise. Our experimental measurements of classical four-wave mixing gain and the associated two-mode relative-intensity squeezing are in reasonable agreement with the theoretical predictions.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Lattice Resonances of Nanohole Arrays for Quantum Enhanced Sensing

We report periodic arrays of nanoholes perforated in metallic thin films interact strongly with light and produce large electromagnetic near-field enhancements in their vicinity. As a result, the optical response of these systems is very sensitive to changes in their dielectric environment, thus making them an exceptional platform for the development of compact optical sensors. Given that these systems already operate at the shot-noise limit when used as optical sensors, their sensing capabilities can be enhanced beyond this limit by probing them with quantum light, such as squeezed or entangled states. Motivated by this goal, here, we present a comparative theoretical analysis of the quantum enhanced sensing capabilities of metallic nanohole arrays with one and two holes per unit cell. Through a detailed investigation of their optical response, we find that the two-hole array supports resonances that are narrower and stronger than its one-hole counterpart, and therefore have a higher fundamental sensitivity limit as defined by the quantum Cramer-Rao bound. We validate the optical response of the analyzed arrays with experimental measurements of the reflectance of representative samples. The results of this work advance our understanding of the optical response of these systems and pave the way for developing sensing platforms capable of taking full advantage of the resources offered by quantum states of light.

74 ATOMIC AND MOLECULAR PHYSICS↗

Quantum-enhanced Imaging and Spectroscopy and their Relevance to International Safeguards

As a follow-up to our previous report on quantum sensing for safeguards, here we delve deeper into quantum-enhanced imaging & spectroscopy and address their relevance to international safeguards. Much of the approaches rely on entangled photons, a quantum phenomenon not possible with classical physics, although just correlated photons will work for some applications, such as ghost imaging. We provide a comprehensive survey of quantum approaches, including multiple entangled photon ghost imaging and spectroscopy techniques. Entangled photons for noise reduction are also described, as well as Non-Line-Of-Sight imaging, compressive techniques, and squeezed light. Of particular interest is the generation of entangled photons with large wavelength separation, such as infrared/visible entangled photon pairs. Such entangled pairs would allow interaction with objects in the IR, such as in the molecular “fingerprint” wavelength region, while the recording device captures the visible photons, thus leveraging the high efficiency and lower cost of visible detectors. Unfortunately, entangled x-ray photons are not practical, which would have been useful for safeguards to interrogate shielded materials. Entangled gamma rays are even further beyond reason. We provide our assessment for application of quantum-enhanced imaging & spectroscopy for international safeguards, including suggested improvements to existing IAEA instruments and destructive assay measurements that are done at IAEA lab facilities.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Quantum Metrology of Noisy Spreading Channels

We provide the optimal measurement strategy for a class of noisy channels that reduce to the identity channel for a specific value of a parameter (spreading channels). We provide an example that is physically relevant: the estimation of the absolute value of the displacement in the presence of phase randomizing noise. Surprisingly, this noise does not affect the effectiveness of the optimal measurement. We show that, for small displacement, a squeezed vacuum probe field is optimal among strategies with same average energy. A squeezer followed by photodetection is the optimal detection strategy that attains the quantum Fisher information, whereas the customarily used homodyne detection becomes useless in the limit of small displacements, due to the same effect that gives Rayleigh’s curse in optical superresolution. There is a quantum advantage: a squeezed or a Fock state with N average photons allow to asymptotically estimate the parameter with a N better precision than classical states with same energy.

Górecki, Wojciech↗

Preparation of metrological states in dipolar-interacting spin systems

Abstract Spin systems are an attractive candidate for quantum-enhanced metrology. Here we develop a variational method to generate metrological states in small dipolar-interacting spin ensembles with limited qubit control. For both regular and disordered spatial spin configurations the generated states enable sensing beyond the standard quantum limit (SQL) and, for small spin numbers, approach the Heisenberg limit (HL). Depending on the circuit depth and the level of readout noise, the resulting states resemble Greenberger-Horne-Zeilinger (GHZ) states or Spin Squeezed States (SSS). Sensing beyond the SQL holds in the presence of finite spin polarization and a non-Markovian noise environment. The developed black-box optimization techniques for small spin numbers ( N ≤ 10) are directly applicable to diamond-based nanoscale field sensing, where the sensor size limits N and conventional squeezing approaches fail.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Variational quantum state preparation for quantum-enhanced metrology in noisy systems

Here, we investigate optimized quantum state preparation for quantum metrology applications in noisy environments. Using the QFI-OPT package, we simulate a low-depth variational quantum circuit (VQC) composed of a sequence of global rotations and entangling operations applied to a chain of qubits that are subject to dephasing noise. The parameters controlling the VQC are numerically optimized to maximize the quantum Fisher information, which characterizes the ultimate metrological sensitivity of a quantum state with respect to a global rotation. We find that, regardless of the details of the entangling operation implemented in the VQC, the optimal quantum states can be broadly classified into a trio of qualitative regimes, i.e., catlike, squeezed like, and product states, associated with different dephasing rates. Our findings are relevant for designing optimal state-preparation strategies for next-generation quantum sensors exploiting entanglement, such as time and frequency standards and magnetometers, aimed at achieving state-of-the-art performance in the presence of noise and decoherence.

quantum Fisher information↗

Quantum Sensing using Geometrical Phase in Qubit-Oscillator Systems

We present a quantum sensing protocol for coupled qubit-oscillator systems that surpasses the standard quantum limit (SQL) by exploiting a geometrical phase. The signal is encoded in the geometrical phase that is proportional to the area enclosed in oscillator phase space. This area is amplified through squeezing, enabling sensitivities beyond the SQL. Our method is independent of oscillator's initial state, amenable to sensing with high-temperature or logical error-corrected states. The protocol shows robustness to qubit Markovian noise and preserves its state-independence, underscoring its practicality for next-generation quantum metrology. We demonstrate application to force sensing beyond the SQL in longitudinally coupled systems, and to high-precision measurements of couplings and pulse calibration surpassing SQL in dispersively coupled circuit quantum electrodynamics (cQED) architectures.

Suri, Nishchay [LBNL, Berkeley]↗

Quantum Enhanced Probes of Magnetic Circular Dichroism

Magneto-optical microscopies, including optical measurements of magnetic circular dichroism, are increasingly ubiquitous tools for probing spin-orbit coupling, charge-carrier g-factors, and chiral excitations in matter, but the minimum detectable signal in classical magnetic circular dichroism measurements is fundamentally limited by the shot-noise limit of the optical readout field. Here, a two-mode squeezed light source is used to improve the minimum detectable signal in magnetic circular dichroism measurements by 3 decibels compared with state-of-the-art classical measurements, even with relatively lossy samples like terbium gallium garnet. Furthermore, these results provide a framework for new quantum-enhanced magneto-optical microscopies that are particularly critical for environmentally sensitive materials and for low temperature measurements where increased optical power can introduce unacceptable thermal perturbations.

42 ENGINEERING↗

Phase-sensitive optomechanical amplifier for quantum noise reduction in laser interferometers

The sensitivity of future gravitational wave interferometers is expected to be limited throughout the detection band by quantum vacuum fluctuations, which can be reduced by applying quantum optics techniques such as squeezed vacuum injection. However, decoherence caused by optical losses in the readout chain will severely limit the effectiveness of such schemes. It was proposed that effect of losses in the final stage of detection can be mitigated by a phase-sensitive amplifier placed in between the output port of the interferometer and the photodetector. In this paper we propose to implement such amplification using an optomechanical device, study some of its practical limitations, and finally, discuss its applicability to next-generation gravitational-wave detectors.

79 ASTRONOMY AND ASTROPHYSICS↗

Creating large Fock states and massively squeezed states in optics using systems with nonlinear bound states in the continuum

The quantization of the electromagnetic field leads directly to the existence of quantum mechanical states, called Fock states, with an exact integer number of photons. Despite these fundamental states being long-understood, and despite their many potential applications, generating them is largely an open problem. For example, at optical frequencies, it is challenging to deterministically generate Fock states of order two and beyond. Here, we predict the existence of an effect in nonlinear optics, which enables the deterministic generation of large Fock states at arbitrary frequencies. The effect, which we call an n-photon bound state in the continuum, is one in which a photonic resonance (such as a cavity mode) becomes lossless when a precise number of photons n is inside the resonance. Based on analytical theory and numerical simulations, we show that these bound states enable a remarkable phenomenon in which a coherent state of light, when injected into a system supporting this bound state, can spontaneously evolve into a Fock state of a controllable photon number. This effect is also directly applicable for creating (highly) squeezed states of light, whose photon number fluctuations are (far) below the value expected from classical physics (i.e., shot noise). In conclusion, we suggest several examples of systems to experimentally realize the effects predicted here in nonlinear nanophotonic systems, showing examples of generating both optical Fock states with large n (n > 10), as well as more macroscopic photonic states with very large squeezing, with over 90% less noise (10 dB) than the classical value associated with shot noise.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Producing entangled photon pairs and quantum squeezed states in plasmas

Plasma is capable of mediating the conversion of two pump photons into two different photons through a relativistic four-wave mixing nonlinearity. Spontaneously created photon pairs are emitted at symmetric angles with respect to the colinear pump direction, and the emission rate is largest if they have identical frequency. Thus, two orthogonally polarized pumps can produce polarization-entangled photon pairs through a millimeter-long homogeneous plasma. Here, the noise from Raman scattering can be avoided if the pump detuning differs from twice the plasma frequency. However, pump detuning exactly equal to twice the plasma frequency can significantly enhance the interaction rate, which allows for the production of strong two-mode squeezed states. Remarkably, the amplified noise from Raman scattering are correlated and hence can be suppressed in one of the output quadratures, thereby maintaining the squeezing magnitude.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Harnessing quantum light for microscopic biomechanical imaging of cells and tissues

The biomechanical properties of cells and tissues play an important role in our fundamental understanding of the structures and functions of biological systems at both the cellular and subcellular levels. Recently, Brillouin microscopy, which offers a label-free spectroscopic means of assessing viscoelastic properties in vivo, has emerged as a powerful way to interrogate those properties on a microscopic level in living tissues. However, susceptibility to photodamage and photobleaching, particularly when high-intensity laser beams are used to induce Brillouin scattering, poses a significant challenge. This article introduces a transformative approach designed to mitigate photodamage in biological and biomedical studies, enabling nondestructive, label-free assessments of mechanical properties in live biological samples. By leveraging quantum-light-enhanced stimulated Brillouin scattering (SBS) imaging contrast, the signal-to-noise ratio is significantly elevated, thereby increasing sample viability and extending interrogation times without compromising the integrity of living samples. The tangible impact of this methodology is evidenced by a notable three-fold increase in sample viability observed after subjecting the samples to three hours of continuous squeezed-light illumination, surpassing the traditional coherent light-based approaches. The quantum-enhanced SBS imaging holds promise across diverse fields, such as cancer biology and neuroscience where preserving sample vitality is of paramount significance. By mitigating concerns regarding photodamage and photobleaching associated with high-intensity lasers, this technological breakthrough expands our horizons for exploring the mechanical properties of live biological systems, paving the way for an era of research and clinical applications.

Li, Tian↗

Dissipative Superradiant Spin Amplifier for Enhanced Quantum Sensing

Quantum metrology protocols exploiting ensembles of N two-level systems and Ramsey-style measurements are ubiquitous. However, in many cases excess readout noise severely degrades the measurement sensitivity; in particular in sensors based on ensembles of solid-state defect spins. We present a dissipative “spin-amplification” protocol that allows us to dramatically improve the sensitivity of such schemes, even in the presence of realistic intrinsic dissipation and noise. Our method is based on exploiting collective (i.e., superradiant) spin decay, an effect that is usually seen as a nuisance because it limits spin-squeezing protocols. We show that our approach can allow a system with a highly imperfect spin readout to approach standard-quantum-limit-like scaling in N within a factor of 2, without needing to change the actual readout mechanism. Our ideas are compatible with several state-of-the-art experimental platforms where an ensemble of solid-state spins (NV centers, SiV centers) is coupled to a common microwave or mechanical mode.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Lieb-Mattis States for Robust Entangled Differential Phase Sensing

We explore a two-node, entanglement-enhanced sensor network for differential phase sensing that exploits decoherence-free subspaces to suppress common-mode noise, a primary limitation of many state-of-the-art quantum sensors. We identify a class of entangled states that, while not strictly optimal, achieve the same asymptotic sensitivity scaling as optimal states and can be prepared efficiently from initially unentangled atomic ensembles. Importantly, the preparation time decreases with increasing system size, which makes the states compatible with realistic noise processes in present-day quantum sensors that operate with large particle numbers but lack full error correction. We illustrate these ideas using two cavity-mediated preparation protocols: (i) coherent, unitary entanglement generation analogous to bosonic two-mode squeezing, yielding Heisenberg scaling, and (ii) dissipative preparation through collective emission into a shared cavity mode, providing a square-root improvement beyond the standard quantum limit. Numerical simulations show that both approaches remain effective at experimentally realistic cavity cooperativities, establishing a practical path toward scalable, quantum-enhanced differential phase sensing.

Kaubruegger, Raphael [National Institute of Standa↗

Diverging Quantum Speed Limits: A Herald of Classicality

When is the quantum speed limit (QSL) really quantum? While vanishing QSL times often indicate emergent classical behavior, it is still not entirely understood what precise aspects of classicality are at the origin of this dynamical feature. Here, we show that vanishing QSL times (or, equivalently, diverging quantum speeds) can be traced back to reduced uncertainty in quantum observables and can thus be understood as a consequence of emerging classicality for these particular observables. We illustrate this mechanism by developing a QSL formalism for continuous-variable quantum systems undergoing general Gaussian dynamics. For these systems, we show that three typical scenarios leading to vanishing QSL times, namely large squeezing, small effective Planck’s constant, and large particle number, can be fundamentally connected to each other. In contrast, by studying the dynamics of open quantum systems and mixed states, we show that the classicality that emerges due to incoherent mixing of states from the addition of classical noise typically increases the QSL time.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Fluctuation–dissipation relation for a quantum Brownian oscillator in a parametrically squeezed thermal field

In this paper we study the nonequilibrium evolution of a quantum Brownian oscillator, modeling the internal degree of freedom of a harmonic atom or an Unruh–DeWitt detector, coupled to a nonequilibrium and nonstationary quantum field bath and inquire whether a fluctuation–dissipation relation (FDR) can exist after/if it approaches equilibration. This is a nontrivial issue because a squeezed field bath cannot reach equilibration and yet, as this work shows, the system oscillator indeed can, which is a necessary condition for FDRs. We discuss three different settings: (A) The bath field essentially remains in a squeezed thermal state throughout, whose squeeze parameter is a mode- and time-independent constant. This situation is often encountered in quantum optics and quantum thermodynamics. (B) The bath field is initially in a thermal state, but is subjected to a parametric process leading to mode- and time-dependent squeezing. This scenario is encountered in cosmology and dynamical Casimir effects. The squeezing in the bath in both types of processes will affect the oscillator’s nonequilibrium evolution. We show that at late times it approaches equilibration and this stationarity condition warrants the existence of a FDR. The trait of squeezing is marked by the oscillator’s effective equilibrium temperature, and the proportionality factor in the FDR is only related to the stationary component of the noise kernel of the bath field. Setting (C) is more subtle: A finite system–bath coupling strength can set the oscillator in a squeezed state even though the bath field is stationary and does not engage in any parametric process. The squeezing of the system in this case is in general time-dependent but becomes constant when the internal dynamics is fully relaxed. We begin with comments on the broad range of physical processes involving squeezed thermal baths and end with some remarks on the significance of FDRs in capturing the essence of quantum backreaction in nonequilibrium and stochastic systems.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Enabling robust, stable, and accurate nonlinear optical measurements from squeezed light generated in hot rubidium vapor

The feasibility of nonlinear optical (NLO) imaging and spectroscopy using low intensity quantum states of light including entangled photon and squeezed light sources, such as those driven by two-photon absorption (TPA), has been a topic of ongoing debate. An unambiguous identification of the appreciable quantum advantage in such quantum light applications could enable NLO imaging of biological samples without photodegradation and phototoxicity. Recently, we have constructed a two-mode squeezed light source based on four-wave mixing in 85Rb vapor, which is capable of 7.9 dB of intensity-difference squeezing (IDS), corresponding to 8.7 dB upon electronic noise correction. In this talk, we discuss the stability of our system, including implementation details on achieving and maintaining 8.7 dB of IDS for several hours, and ensuring the two spatially multimode beams are properly overlapped in a sample with minimal optical loss.

Allen, Harry [ORNL] (ORCID:0000000190253914)↗

Quantum Frequency Combs with Path Identity for Quantum Remote Sensing

Quantum sensing promises to revolutionize sensing applications by employing quantum states of light or matter as sensing probes. Photons are the clear choice as quantum probes for remote sensing because they can travel to and interact with a distant target. Existing schemes are mainly based on the quantum illumination framework, which requires quantum memory to store a single photon of an initially entangled pair until its twin reflects off a target and returns for final correlation measurements. Existing demonstrations are limited to tabletop experiments, and expanding the sensing range faces various roadblocks, including long-time quantum storage and photon loss and noise when transmitting quantum signals over long distances. We propose a novel quantum sensing framework that addresses these challenges using quantum frequency combs with path identity for remote sensing of signatures (“qCOMBPASS”). The combination of one key quantum phenomenon and two quantum resources—namely, quantum-induced coherence by path identity, quantum frequency combs, and two-mode squeezed light—allows for quantum remote sensing without requiring quantum memory. The proposed scheme is akin to a quantum radar based on entangled frequency-comb pairs that uses path identity to detect, range, or sense a remote target of interest by measuring pulses of one comb in the pair that never traveled to the target but that contains target information “teleported” by quantum-induced coherence by path identity from the other comb in the pair that traveled to the target but is not detected. We develop the basic qCOMBPASS theory, analyze the properties of the qCOMBPASS transceiver, and introduce the qCOMBPASS equation—a quantum analog of the well-known LIDAR equation in classical remote sensing. We also describe an experimental scheme to demonstrate the concept using two-mode squeezed quantum combs. qCOMBPASS can strongly impact various applications in remote quantum sensing, imaging, metrology, and communications. These applications include detection and ranging of low-reflectivity objects, measurement of small displacements of a remote target with precision beyond the standard quantum limit (SQL), standoff hyperspectral quantum imaging, discreet surveillance from space with low detection probability (detect without being detected), very-long-baseline interferometry, quantum Doppler sensing, quantum clock synchronization, and networks of distributed quantum sensors. Published by the American Physical Society 2024

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗