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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 73 records · Page 4
All sourcesNASA NTRSDOE OSTI
DOE OSTI2022

Nuclear Data Sheets for A=24

Here, evaluated spectroscopic data and level schemes from radioactive decay and nuclear reaction studies are presented for 24 N, 24 O, 24 F, 24 Ne, 24 Na, 24 Mg, 24 Al, and 24 Si. This evaluation for A=24 supersedes the earlier one by R. B. Firestone (2007Fi14). Highlights of this evaluation are the following: In 24 O, the 7.4- and 7.65-MeV groups reported in 1 H( 24 O,p') (2012Ts03) and 9 Be( 26 F,nX) (2011Ho05), respectively, are considered as separate states in this evaluation, since the former one was observed to decay by only one neutron emission to 23 O, while the latter one by two sequential neutrons to 22 O. Based on assigned configurations, the 7.4- and 7.6-MeV groups are tentatively assigned negative and positive parities, respectively. Additional study would be useful to determine if these states are same or different. In 24 Na, 2014Fi01 (n,γ) proposed Jπ=(0,1,2) - for 4048.8 keV level based on weaker population from the capture state (J π =1 + ,2 + ) and mentioned to reexamine the J π =0 + assignment, suggested in earlier evaluations (1990En08, 2007Fi02). This evaluation includes the first observation of E0 transition, strength ρ 2 (E0)=0.380 70, for the 6432 keV transition from 0 + state at 6432 to 0 + g.s. in 24 Mg reported in 2020Do10. Authors proposed the first-excited 0+ state of 24 Mg to be superdeformed. In 24 Al, the excited level energies deduced from ( 3 He,t) measurements reported by different research groups vary significantly and it was not clear if some of those levels were same or different. Additional measurements are needed.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2023

WPEC SG50: Developing an Automatically Readable, Comprehensive and Curated Experimental Nuclear Reaction Database

The Organisation for Economic Co-operation and Development (OECD) Nuclear Energy Agency (NEA) Working Party on International Nuclear Data Evaluation Co-operation (WPEC) subgroup (SG) 50 was formed in 2020 to develop an automatically readable, comprehensive and curated experimental nuclear reaction database. This database is called MEDUSAL (Machine-readable Experimental Data User Application & Library), and will draw from EXFOR. The EXFOR database preserves experimental nuclear reaction data true to its original documentation and information from the authors of the data. MEDUSAL will deviate from EXFOR by storing additional information from users of the data for their fields of work (evaluation, model development, validation, etc.). This includes expert judgment on the data sets, identification of data points as outliers, renormalization of the data to the newest monitor reactions, and estimations of missing uncertainty sources. The format for MEDUSAL is being developed to enable easy automatic parsing of large amounts of data. Here, we will summarize the use cases, high-level requirements and first steps towards developing the database MEDUSAL and the API to access it.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2023

Quantification of the 35 Cl($\textit{n, p}$) reaction channel

The evaluated 35 Cl($\textit{n, p}$) cross sections in the ENDF/B-VIII.0 nuclear data library remain uncertain because of the lack of measured data in the neutron energy range between 100-600 keV. In this energy region, the R-matrix analysis relies heavily on estimated ($\textit{n, p}$) partial widths and level density information. This resulted in significant differences of the evaluated cross sections and predicted reactivity in nuclear reactor applications with respect to previous nuclear data libraries. Here, we present a methodology to quantify the cross sections for the 35 Cl($\textit{n, p}$) reaction channel from the combination of measured total cross sections and model calculations.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗
DOE OSTI2026

Nuclear Data Sheets for A=69

Experimental data on ground- and excited-state properties for all known nuclei with mass number A=69 have been compiled and evaluated. States populated in radioactive decay, as well as in nuclear reactions, have been considered. For these nuclei, level and decay schemes, as well as tables of nuclear properties, are given in detail. In conclusion, this work supersedes the 2013 evaluation by C.D. Nesaraja (2014Ne01).

Nesaraja, Caroline D. [Oak Ridge National Laborato↗
DOE OSTI2025

$\mathcal{R}$ -matrix analysis of η + nat Cl reactions relevant to molten-salt reactor designs [Abstract]

Performed with support from the U.S. Nuclear Criticality Safety Program in an effort to provide improved chlorine cross section and corresponding covariance data, the R-matrix analysis of neutron induced reactions for two stable chlorine isotopes, 35,37 Cl, was performed in the energy range of thermal up to 1.2 MeV. Starting from the repository of the ENDF/B-VIII.0 library and following recent measurement campaigns, this work represents a significant improvement in the evaluation of the ( η , p ) reaction channel. The evaluation methodology uses the $\mathcal{R}$ -matrix code SAMMY to generate a set of Reich-Moore resonance parameters. As predicted by recently measured 35 Cl( η , p ) data, the presented evaluation features a dramatic increase in the magnitude of the ( η , p ) reaction channel over the ENDF/B-VIII.0 and previous nuclear data ENDF/B released libraries. Together with details of the evaluation procedure, the impact of the updates in the outgoing proton emissions on reactivity coefficients for different molten-salt reactor designs is presented and discussed.

charged-particle↗
DOE OSTI2021

2H(p, gamma) 3He cross section measurement using high-energy-density plasmas

An absolute cross section for the radiative capture reaction 2H(p, γ ) 3He has been measured at the OMEGA laser facility using inertially confined plasmas. These high-temperature plasmas are created by imploding a fuel containing capsule using laser ablation, and are advantageous in that they better mimic astrophysical systems. We measure an S factor for this reaction of 0.429 ± 0.026stat ± 0.072sys eV b at Ec.m. = 16.35 ± 0.40 keV, which is higher than the adopted evaluations. This reaction is important as a source of nuclear energy in protostars and brown dwarfs. It is also a critical reaction during big-bang nucleosynthesis, and an accurate cross section can be used as a constraint on cosmology.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2023

Evaluation of Light-Element Reactions in the Resolved Resonance Region

Light-element reactions at low energies in the resolved resonance region are important for a range of applications in basic and applied sciences including nuclear reactors, nonproliferation, cultural heritage, forensics and environmental control, rare event investigations and nuclear astrophysics. In this paper, we report on an effort to evaluate charged-particle cross sections in the resolved resonance region and produce evaluated nuclear data files for further processing and inclusion in evaluated data libraries. We discuss the open issues in R-matrix calculations as we extend to higher energies, such as dealing with the rapidly growing number of open channels and merging with the regime of smooth cross sections described by the statistical model, and present attempts to address these issues in neutron-induced reactions relevant to nuclear reactor applications.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

Validation of neutron-induced reactions on natural carbon using an active target at neutron energies up to 22 MeV at LANSCE

A single crystal chemical vapor deposited (sCVD) diamond detector is used as an active target to measure neutron-induced reactions on natural carbon using the neutrons produced by spallation, with a broad energy spectrum at LANSCE. Additionally, the neutron-induced reactions are detected in the diamond as low as E n = 400 keV and up to approximately 100 MeV. Relative cross sections for C 12 ( n , α 0 ) , C 12 ( n , p 0 ) , C 12 ( n , d 0 + p 1 ) , and C 13 ( n , α 0 ) are reported up to E n = 22 MeV and comparisons on detected pulse-height spectra and detector response of scattering reactions are made with GEANT4 simulations using the ENDF/B-VIII.0 evaluated nuclear data library up to 20 MeV. The results are compared with past experimental data, including other works that incorporate diamond detectors as an active carbon target. In addition, R-matrix calculations for the C 13 + n system are presented.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2022

Status of the WPEC subgroup 46 - Efficient and effective use of integral experiments for nuclear data validation

The present paper summarizes the current status of the activities of the on-going WPEC subgroup 46 which was the last significant initiative of Massimo before he passed away. The goal of WPEC/SG46 is to define, test and document a methodology to provide unambiguous feedback to the nuclear data evaluator community, based on the joint use of integral experiments and data assimilation techniques. Part of this effort resulted in a renewed analysis of the original Target Accuracy Requirement (TAR) exercise of WPEC/SG26, by adding more diverse nuclear systems and parameters, including reaction channels correlations and a coarser energy group structure; and making use of the progress made in the most recent evaluations in terms of both nuclear data and covariance matrices. The preliminary outcomes of the updated TAR exercise, documented by various groups worldwide are clear already: uncertainty reductions are required for many nuclide-reaction pairs in a variety of energy range if the target uncertainty requirements set by the industry are to be met, especially for k{sub eff}. The inclusion of correlations between the various reaction channels had a major impact on the magnitude of the required uncertainty reduction. Those uncertainty reductions are unlikely to be met by differential measurements alone. However, the selection of relevant integral experiment and a subsequent adjustment procedure may help meet these requirements. (authors)

22 GENERAL STUDIES OF NUCLEAR REACTORS↗
DOE OSTI2020

2 H(p,γ) 3 He cross section measurement using high-energy-density plasmas

An absolute cross section for the radiative capture reaction 2 H(p,γ) 3 He has been measured at the OMEGA laser facility using inertially confined plasmas. These high-temperature plasmas are created by imploding a fuel-containing capsule using laser ablation, and are advantageous in that they better mimic astrophysical systems. We measure an S factor for this reaction of 0.429 ± 0.026 stat ± 0.072 sys eV b at E c.m . = 16.35 ± 0.40 keV, which is higher than the adopted evaluations. Furthermore, this reaction is important as a source of nuclear energy in protostars and brown dwarfs. It is also a critical reaction during big-bang nucleosynthesis, and an accurate cross section can be used as a constraint on cosmology.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2023

The current status of inelastic and capture Gamma-ray production evaluations in translated ENDF-VIII.0 GNDS files and recommended remediation actions

This report provides the status of discrete nuclear levels and inelastic gamma-ray production for neutron induced reactions in current ENDF-VIII.0 evaluations for the isotopes in the GRIN project. Different categories of issues are identified after a comparison with information from “adopted” ENSDF files. Improvement strategies are given and recommendations are described. We have included a similar, but more limited, analysis for thermal capture data where EGAF and ENSDF thermal libraries are considered. In addition, we provide a validation plan to employ different transport code simulations.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

Measurement of U 238 ( n , n ' γ ) cross section data and their impact on reaction models

A better knowledge of (n,xn) reaction cross sections is important for both reaction modeling and energy applications. This article focuses on inelastic scattering of neutrons off 238 U for which improvements are needed to better constrain evaluations and solve inconsistencies in nuclear power reactor calculations. A new precise measurement of (n,xnγ) reaction cross sections on 238 U has been performed at the GELINA (Geel Electron LINear Accelerator) neutron facility operated by EC-JRC-Geel (Belgium) with the GRAPhEME (GeRmanium array for Actinides PrEcise MEasurements) setup. The prompt γ-ray spectroscopy method coupled to time-of-flight measurements is used to extract (n,xnγ) cross section values which can be further combined to infer the total neutron inelastic scattering cross section. Cross section data for 18 γ transitions (five never measured before) are presented and compared to the data in the literature. Here, emphasis is especially given to the uncertainty determination to produce partial cross section data as accurate as possible. Due to intrinsic limitations of the experimental method, the use of additional nuclear structure information coupled with theoretical modeling is required to determine the total (n, n') cross section over the whole neutron energy range. We have investigated modeling aspects of the 238 U(n,n'γ) cross sections related to the description of compound nucleus and preequilibirum mechanisms as well as the discrete part of nuclear structure. Through comparison between experimental and calculated (n,n'γ) cross sections, we pinpoint inaccuracies in the description of specific reaction mechanisms and challenge recently implemented models. This helps improving the whole modeling of the (n, n') reaction.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

The AME 2020 atomic mass evaluation (I). Evaluation of input data, and adjustment procedures*

Abstract This is the first of two articles (Part I and Part II) that presents the results of the new atomic mass evaluation, AME2020. It includes complete information on the experimental input data that were used to derive the tables of recommended values which are given in Part II. This article describes the evaluation philosophy and procedures that were implemented in the selection of specific nuclear reaction, decay and mass-spectrometric data which were used in a least-squares fit adjustment in order to determine the recommended mass values and their uncertainties. All input data, including both the accepted and rejected ones, are tabulated and compared with the adjusted values obtained from the least-squares fit analysis. Differences with the previous AME2016 evaluation are discussed and specific examples are presented for several nuclides that may be of interest to AME users.

74 ATOMIC AND MOLECULAR PHYSICS↗
DOE OSTI2022

Neutron elastic and inelastic cross section measurements on silicon from 0.8--8 MeV

Neutron elastic and inelastic scattering differential cross sections were measured at angles between 30° and 155° with incident neutron energies between 0.8 and 8 MeV. The measured differential scattering cross sections are compared to existing measurements and the ENDF/B-VIII.0, the JEFF-3.3, and the JENDL-4.0 data evaluations, as well as theoretical calculations from the TALYS-1.95 nuclear reaction code. Our results are reasonably well described by values from the ENDF/B-VIII.0 and JEFF-3.3 compilations. However, below 4 MeV, our backward-angle elastic scattering results tend to be lower than database/calculated values, suggesting that less recoil damage would occur than expected. Above 6 MeV, larger backward-angle cross sections are observed suggesting the opposite. Deexcitation γ rays produced in the inelastic scattering process were also studied for neutron energies between 1.9 and 4.5 MeV. Inelastic neutron scattering cross sections deduced from 28 Si(n,n1γ) γ-ray projection cross sections confirm our 28 Si(n,n1) results. To the extent that data from GELINA and our experimental results can be compared, we have excellent agreement between the inelastic neutron scattering cross sections.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2025

Solar fusion III: New data and theory for hydrogen-burning stars

In stars that lie on the main sequence in the Hertzsprung-Russell diagram, like our Sun, hydrogen is fused to helium in a number of nuclear reaction chains and series, such as the proton-proton chain and the carbon-nitrogen-oxygen cycles. Precisely determined thermonuclear rates of these reactions lie at the foundation of the standard solar model. This review, the third decadal evaluation of the nuclear physics of hydrogen-burning stars, is motivated by the great advances made in recent years by solar neutrino observatories, putting experimental knowledge of the proton-proton (𝑝⁢𝑝)-chain neutrino fluxes in the few-percent precision range. The basis of the review is a one-week community meeting held in July 2022 in Berkeley, California, and many subsequent digital meetings and exchanges. The relevant reactions of solar and stellar hydrogen burning are reviewed here from both theoretical and experimental perspectives. Recommendations for the state of the art of the astrophysical 𝑆 factor and its uncertainty are formulated for each of them. Furthermore, several other topics of paramount importance for the solar model are reviewed as well: recent and future neutrino experiments, electron screening, radiative opacities, and current and upcoming experimental facilities. In addition to reaction-specific recommendations, general recommendations are also formed.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2025

Design of Quasi-Integral Experiments at the Flexible Neutron Source at the University of Tennessee

Nuclear reaction data libraries make use of experimental data that are differential in reaction and neutron energy for evaluation and data that are integral in reaction and energy for validation. In many cases, integral measurements can provide lower experimental uncertainties than differential measurements, but the impact of individual reactions and energies cannot generally be determined from the single experimental observable. “Quasi-integral” or “quasi-differential” measurements, which are integral in one characteristic (energy or reaction) and differential in the other, can often provide a middle ground of lower experimental uncertainties combined with some ability to unpack the impact of individual reactions or energies. Furthermore, the Flexible Neutron Source (FNS) at the University of Tennessee, Knoxville, is a new experimental facility that can perform integral and quasi-integral measurements by removing components of the integral configuration to determine the impact of specific reactions. Possible flux-averaged cross-section measurements, flux perturbation measurements, and neutron downscattering measurements are simulated here to show the value of the FNS to evaluation and validation of nuclear data.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

Correlated energy uncertainties in reaction rate calculations

Monte Carlo methods can be used to evaluate the uncertainty of a reaction rate that arises from many uncertain nuclear inputs. However, until now no attempt has been made to find the effect of correlated energy uncertainties in input resonance parameters. Our goal is to investigate the impact of correlated resonance energy uncertainties on reaction rates. Using a combination of numerical and Monte Carlo variation of resonance energies, the effect of correlations are investigated. Five reactions are considered: two fictional, illustrative cases and three reactions whose rates are of current interest. The effect of correlations in resonance energies depends on the specific reaction cross section and temperatures considered. When several resonances contribute equally to a reaction rate, and when they are located on either side of the Gamow peak, correlations between their energies dilute their effect on reaction rate uncertainties. If they are both located above or below the maximum of the Gamow peak, however, correlations between their resonance energies can increase the reaction rate uncertainties. This effect can be hard to predict for complex reactions with wide and narrow resonances contributing to the reaction rate.

79 ASTRONOMY AND ASTROPHYSICS↗