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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 1,063 records · Page 59
All sourcesNASA NTRSDOE OSTI
NASA NTRS2005

Investigation of Ruthenium Dissolution in Advanced Membrane Electrode Assemblies for Direct Methanol Based Fuel Cell Stacks

Dissolution of ruthenium was observed in the 80-cell stack. Duration testing was performed in single cell MEAs to determine the pathway of cell degradation. EDAX analysis on each of the single cell MEAs has shown that the Johnson Matthey commercial catalyst is stable in DMFC operation for 250 hours, no ruthenium dissolution was observed. Changes in the hydrophobicity of the cathode backing papers was minimum. Electrode polarization analysis revealed that the MEA performance loss is attributed to changes in the cathode catalyst layer. Ruthenium migration does not seem to occur during cell operation but can occur when methanol is absent from the anode compartment, the cathode compartment has access to air, and the cells in the stack are electrically connected to a load (Shunt Currents). The open-to-air cathode stack design allowed for: a) The MEAs to have continual access to oxygen; and b) The stack to sustain shunt currents. Ruthenium dissolution in a DMFC stack can be prevented by: a) Developing an internally manifolded stacks that seal reactant compartments when not in operation; b) Bringing the cell voltages to zero quickly when not in operation; and c) Limiting the total number of cells to 25 in an effort to limit shunt currents.

alternative power sources↗
DOE OSTI2019

Status Report on Uncertainty Quantification and Sensitivity Analysis Tools in the Geologic Disposal Safety Assessment (GDSA) Framework

The Spent Fuel and Waste Science and Technology (SFWST) Campaign of the U.S. Department of Energy (DOE) Office of Nuclear Energy (NE), Office of Fuel Cycle Technology (FCT) is conducting research and development (R&D) on geologic disposal of spent nuclear fuel (SNF) and high-level nuclear waste (HLW). Two high priorities for SFWST disposal R&D are design concept development and disposal system modeling. These priorities are directly addressed in the SFWST Geologic Disposal Safety Assessment (GDSA) control account, which is charged with developing a geologic repository system modeling and analysis capability, and the associated software, GDSA Framework, for evaluating disposal system performance for nuclear waste in geologic media. GDSA Framework is supported by SFWST Campaign and its predecessor the Used Fuel Disposition (UFD) campaign.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2022

Uncertainty and Sensitivity Analysis Methods and Applications in the GDSA Framework (FY2022)

The Spent Fuel and Waste Science and Technology (SFWST) Campaign of the U.S. Department of Energy (DOE) Office of Nuclear Energy (NE), Office of Fuel Cycle Technology (FCT) is conducting research and development (R&D) on geologic disposal of spent nuclear fuel (SNF) and high-level nuclear waste (HLW). Two high priorities for SFWST disposal R&D are design concept development and disposal system modeling. These priorities are directly addressed in the SFWST Geologic Disposal Safety Assessment (GDSA) control account, which is charged with developing a geologic repository system modeling and analysis capability, and the associated software, GDSA Framework, for evaluating disposal system performance for nuclear waste in geologic media. GDSA Framework is supported by SFWST Campaign and its predecessor the Used Fuel Disposition (UFD) campaign.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗
NASA NTRS2015

Affordable Development and Demonstration of a Small NTR Engine and Stage: A Preliminary NASA, DOE, and Industry Assessment

In FY11, NASA formulated a plan for Nuclear Thermal Propulsion (NTP) development that included Foundational Technology Development followed by system-level Technology Demonstrations. The ongoing NTP project, funded by NASA's Advanced Exploration Systems (AES) program, is focused on Foundational Technology Development and includes 5 key task activities: (1) Fuel element fabrication and non-nuclear validation testing of heritage fuel options; (2) Engine conceptual design; (3) Mission analysis and engine requirements definition; (4) Identification of affordable options for ground testing; and (5) Formulation of an affordable and sustainable NTP development program. Performance parameters for Point of Departure designs for a small criticality-limited and full size 25 klb (sub f) (kip, or 1000 pound-force)-class engine were developed during FYs 13-14 using heritage fuel element designs for both Rover NERVA (Nuclear Engine for Rocket Vehicle Applications) Graphite Composite (GC) and Ceramic Metal (Cermet) fuel forms. To focus the fuel development effort and maximize use of its resources, the AES program decided, in FY14, that a leader-follower down-selection between GC and cermet fuel was required. An Independent Review Panel (IRP) was convened by NASA and tasked with reviewing the available fuel data and making a recommendation to NASA. In February 2015, the IRP recommended and the AES program endorsed GC as the leader fuel In FY14, a preliminary development schedule DDTE (Design Development Test and Evaluation) plan was produced by GRC (Glenn Research Center), DOE (Department of Energy) and industry for the AES program. Assumptions, considerations and key task activities are presented here. At the direction of NASA HQ (32515), NASA and DOE are to work together to formulate a detailed development plan and schedule allowing the affordable development of a small (7.5-16.5 klbf) GC engine for possible flight technology demonstration (FTD) mission within a 10-year timeframe.

Lunar Flyby Mission↗
DOE OSTI2017

Classification and imaging of spent nuclear fuel dry casks using cosmic ray muons - 132

The present work explores alternative approaches for in situ monitoring with near real-time data analysis and imaging of dry casks using muons. Monitoring can provide useful signals about the cask contents in a yes/no decision format faster and with fewer muons than traditional imaging. Imaging can be performed as a second step in this process if specific information about the location of the fuel assemblies is needed. To explore and analyze these two modalities, simulations of muon scattering and displacement were performed for various scenarios, including vertical and horizontal fully loaded dry casks, half-loaded dry casks, dry casks with one row of fuel assemblies missing, dry casks with one fuel assembly missing, and empty dry casks. This work demonstrates monitoring can provide fast and reliable indication about the contents of the cask. For 100,000 muons, a few minutes of measurement time with a 3.6 m{sup 2} detector at a 45 deg. zenith angle, 90% detection probability for missing fuel assemblies can be achieved with a false alarm rate lower than 1%. If a positive signal is detected, then longer measurements can be performed and coupled with muon imaging algorithms to determine the location of missing nuclear material. In these cases, transmission muon radiography can produce images of acceptable resolution for all scenarios. In the horizontal dry cask case, all scenarios can be identified and separated adequately. In the vertical dry cask case, similar conclusions can be drawn, but because of shadowing from other fuel assemblies, the location of a missing fuel assembly cannot be identified in the 2-D transmission map. However, views from different directions may resolve this. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗
NASA NTRS1979

Phase 1 of the near term hybrid passenger vehicles development program. Appendix A: Mission analysis and performance specification studies, volume 1

Applicable data was categorized and processed according to vehicle usage and trip parameters with consideration of payload (cargo, people, size) and driving cycles. A mission that maximizes the fuel potential savings for the total 1985 vehicle fleet was selected. Mission requirements that have a bearing on conventional and hybrid vehicle performance and characteristics were identified and formulated and a reference ICE vehicle was selected that meets or exceeds all requirements while maintaining within applicable constraints. Specifications for vehicle performance were established based on mission requirements, mission related vehicle characteristics, and fuel consumption.

Traversi, M.↗
DOE OSTI2020

Microstructure and diffusion behavior of uranium fuel with minor additives

Fission product lanthanides in metallic fuels are known to cause adverse fuel-cladding chemical interaction (FCCI). Tin (Sn) and palladium (Pd) are being explored as the potential additives to reduce or mitigate lanthanide-induced FCCI by forming stable Sn-Ln and Pd-Ln compounds. The current study is an investigation of the fuel alloys, U–4Sn, U–4Sn-4Ln, U–4Pd, and U–4Pd-4Ln (wt. %), and their diffusion behaviors with Fe. Microstructural analysis was performed using scanning electron microscopy (SEM). Further, the binary phases in the UPd and USn alloys are identified as UPd 3 and suspected U 2 Sn, where U 2 Sn is unknown in the literature. The binary phases in the UPdLn alloy are identified as PdLn and Pd-rich Pd-Ln (Pd 4 Ln 3 and Pd 3 Ln 2 ), and in the USnLn alloy is SnLn. Diffusion of Fe with these binary phases is insignificant compared to the diffusion with U. The Ln-induced FCCI can be mitigated by the additives.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2023

Degradation and recovery of solid oxide fuel cell performance by control of cathode surface acidity: Case study – Impact of Cr followed by Ca infiltration

Solid oxide fuel cells (SOFC) have attracted attention as clean and efficient energy conversion devices with low emissions. However, several degradation mechanisms limit the electrochemical performance of current SOFCs, with cathode degradation due to Cr-poisoning from metal interconnects particularly problematic. The acidity/basicity of binary additives has been found to be a sensitive descriptor of the oxygen exchange kinetics, indicating that acidic Cr-species/basic Ca-species can be expected to deactivate/activate the cathode surface, respectively. Inspired by recent advances, the feasibility of relative acidity as a tool for reviving degraded SOFCs is demonstrated by neutralizing Cr-poisoned SOFCs by subsequent serial infiltration of Ca-species. Furthermore, a model mixed ionic and electronic conducting oxide, Pr 0.1 Ce 0.9 O 2-δ (PCO), is selected as the cathode material. Area-specific resistances (ASR) of symmetric cells obtained by electrochemical impedance spectroscopy show that Cr-infiltration results in a seven-fold increase in ASR, while subsequent infiltration of Ca-species leads to complete recovery. Performance degradation and recovery are attributed to depressed/enhanced redox properties at the PCO surface, as supported by XPS analysis. Experiments using anode-supported fuel cells show a reduction in peak power density by 26% upon Cr-infiltration, reversed following Ca-infiltration, after which no degradation is observed during subsequent operation for 100 h.

(Pr,Ce)O2-δ↗
DOE OSTI2025

Experimental and fuel-surrogates modeling study of the high-pressure pyrolysis of specialty cetane number fuels: implications for fall-off in ethylene unimolecular dissociation

Single pulse shock tube experiments were conducted at 50 atm nominal pressure and 4 ms nominal reaction time over a temperature range of 900–1800 K, to study the pyrolysis speciation of a multi-component jet fuel, F-24, and six cetane number (CN) specialty fuels - CN30, CN35, CN40, CN45, CN50, and CN55. Gas chromatography (GC) was used to qualitatively and quantitatively analyze the post shock gases. The relationship between the formation of key pyrolysis species and the chemically controlled combustion propensity as reflected by the cetane number of each fuel was examined. A surrogate-based mechanism from the CRECK Modelling Group and chemical-functional group based optimized surrogates (CFGO) were used to simulate the pyrolysis speciation results. The model was able to capture the chemistry of most species except two important pyrolysis intermediates – ethylene and acetylene. Chemical kinetic analyses were performed to identify the important reactions which affect the chemistry of these species; however, the rate parameters of critical reactions were found to be unsuitable for simulating the present high-pressure studies. Here, to address this unsuitability, a theory-based fall-off analysis for three reactions representing the decomposition of ethylene and subsequent formation of acetylene was performed, and these are included in an updated version of the CRECK mechanism. This update resolves discrepancies between the experimental results and simulations for ethylene and acetylene. Reaction flux analyses using the updated surrogate model were also performed to identify the important reaction pathways responsible for the formation of crucial species and to provide an analysis of the chemistry of complex multi-component fuel systems. The fundamental reactions responsible for driving pyrolysis chemistry were greatly influenced by the chemical functional groups present in these fuels. In addition to updating the rate parameters of specific reactions to improve modeling, this study also emphasizes the effectiveness of the fuel-surrogate approach, where surrogates representing the chemical functional group composition of the parent fuel serve as a valuable tool for predicting the combustion chemistry of novel fuels.

Chemical Kinetics↗
DOE OSTI2015

Passive Tomography for Spent Fuel Verification: Analysis Framework and Instrument Design Study

The potential for gamma emission tomography (GET) to detect partial defects within a spent nuclear fuel assembly is being assessed through a collaboration of Support Programs to the International Atomic Energy Agency (IAEA). In the first phase of this study, two safeguards verification objectives have been identified. The first is the independent determination of the number of active pins that are present in the assembly, in the absence of a priori information. The second objective is to provide quantitative measures of pin-by-pin properties, e.g. activity of key isotopes or pin attributes such as cooling time and relative burnup, for the detection of anomalies and/or verification of operator-declared data. The efficacy of GET to meet these two verification objectives will be evaluated across a range of fuel types, burnups, and cooling times, and with a target interrogation time of less than 60 minutes. The evaluation of GET viability for safeguards applications is founded on a modelling and analysis framework applied to existing and emerging GET instrument designs. Monte Carlo models of different fuel types are used to produce simulated tomographer responses to large populations of “virtual” fuel assemblies. Instrument response data are processed by a variety of tomographic-reconstruction and image-processing methods, and scoring metrics specific to each of the verification objectives are defined and used to evaluate the performance of the methods. This paper will provide a description of the analysis framework and evaluation metrics, example performance-prediction results, and describe the design of a “universal” GET instrument intended to support the full range of verification scenarios envisioned by the IAEA.

spent nuclear fuel assemblies, partial defect veri↗
NASA NTRSDate not supplied

Sizing and Performance Analysis of a MW-Class Electrified Aircraft Propulsion (Eap) System for A Parallel Hybrid Turboprop Concept

Aircraft electrification has emerged as a pivotal research and development focus in the 21st century, gaining international momentum as a strategic approach to curtail fuel consumption and emissions in the civil aviation sector. Under the Electrified Powertrain Flight Demonstration (EPFD) project, NASA and industry partners are raising the technical readiness, addressing integration challenges and gathering data for future standards and regulations for demonstrate Megawatt (MW) class Electrified Aircraft Propulsion (EAP) systems which can be utilized on regional turboprop or single aisle transports. With the rapid emergence of novel EAP concepts, risk reduction efforts are focused on developing the capabilities to evaluate the impacts of electrification at the conceptual design level where high variability in the EAP system architecture must be accounted for. This paper details an integrated, approach to parametric sizing of multi-MW EAP systems with the primary goal of assessing vehicle-level performance sensitivities to variations in electrical system component-level performance metrics. The focus of this work is to investigate the degree to which EAP component parameters such as specific power, efficiency, and energy density impact range and overall fuel savings.

EAP↗
NASA NTRSDate not supplied

Sizing and Performance Analysis of a MegaWatt-Class Electrified Aircraft Propulsion (EAP) System for a Parallel Hybrid Turboprop Concept

Aircraft electrification has emerged as a pivotal research and development focus in the 21st century, gaining international momentum as a strategic approach to curtail fuel consumption and emissions in the civil aviation sector. Under the Electrified Powertrain Flight Demonstration (EPFD) project, NASA and industry partners are raising the technical readiness, addressing integration challenges and gathering data for future standards and regulations for demonstrate Megawatt (MW) class Electrified Aircraft Propulsion (EAP) systems which can be utilized on regional turboprop or single aisle transports. With the rapid emergence of novel EAP concepts, risk reduction efforts are focused on developing the capabilities to evaluate the impacts of electrification at the conceptual design level where high variability in the EAP system architecture must be accounted for. This paper details an integrated, approach to parametric sizing of multi-MW EAP systems with the primary goal of assessing vehicle-level performance sensitivities to variations in electrical system component-level performance metrics. The focus of this work is to investigate the degree to which EAP component parameters such as specific power, efficiency, and energy density impact range and overall fuel savings.

EAP↗
NASA NTRS1986

Impact of mismodeled idle engine performance on calculation and tracking of optimal 4-D descent trajectories

Advanced flight management systems are being developed which are capable of calculating optimal 3-D and 4-D flight trajectories for arbitrary fuel and time costs. These systems require mathematical models of airplane performance in order to compute the optimal profiles. Mismodeled idle engine characteristics can result in descent trajectories requiring excessive throttle and/or speedbrake activity in order to achieve the desired end conditions. This paper evaluates the cost and fuel penalties, trajectory variations, and flight control requirements associated with typical idle engine modeling errors for a twin-jet transport airplane. Variations in idle power setting, thrust, fuel flow, and surge bleed operation were evaluated for a cruise/descent flight segment. The results of this analysis provide insight into the penalties associated with uncertainties in idle engine performance and suggest methods of modeling which minimize these penalties.

Williams, D. H.↗
DOE OSTI2022

An economic analysis of the role of materials, system engineering, and performance in electrochemical carbon dioxide conversion to formate

The development of technologies that utilize carbon dioxide is important to mitigating climate change. The electrochemical reduction of carbon dioxide is one technology that can utilize greenhouse gasses that would be otherwise be emitted to the atmosphere by producing chemicals and fuels from carbon dioxide and electricity. Significant progress has been made in the experimental performance of carbon dioxide reduction systems with novel catalyst designs, new materials, and systems engineering; however, no work has linked such changes in stack design and materials to capital costs for the stack itself. In this study, we present an analysis that accounts for and analyzes the impacts of alternative materials and system architectures on manufactured costs of carbon dioxide reduction stacks, thus providing a framework to understand exactly how these advances impact the at-scale capital costs of these systems. Specifically, we consider the impact that the addition of a catholyte buffer layer has on an electrolyzer reducing carbon dioxide to formate, finding that the cost of manufacturing this part only increases stack costs by about $30/m 2 at high manufacturing rates, while previous work finds that this part improves system performance. This work shows that the links between system performance, materials, and costs are nonlinear, and that achieving low-cost scalability requires optimization of not just performance parameters but also the use of low-cost and highly scalable materials. These results bridge experimental and techno-economic analysis of processes for carbon dioxide reduction, informing researchers by providing a quantifiable estimate of the impact of advances in electrochemical carbon dioxide reduction technology on manufactured stack capital costs.

29 ENERGY PLANNING, POLICY, AND ECONOMY↗
DOE OSTI2023

Life-cycle analysis of sustainable aviation fuel production through catalytic hydrothermolysis

Catalytic hydrothermolysis (CH) is a sustainable aviation fuel (SAF) pathway that has been recently approved for use in aircraft fuel production. In alignment with broader sustainable aviation goals, SAF production through CH requires a quantitative assessment of carbon intensity (CI) impacts. In this study, a current-day life-cycle analysis (LCA) was performed on SAF produced via CH to determine the CI. Various oily feedstocks were considered, including vegetable oils (soybean, carinata, camelina and canola) and low-burden oils and greases (corn oil, yellow grease and brown grease). Life-cycle inventory data were collected on all processes within the CH LCA boundary: feedstock cultivation and/or collection, preprocessing, hydrothermal cleanup and CH, biocrude refining, fuel transportation and end use through combustion. Baseline results show that the CH-produced SAF can be generated with CI reductions ranging from 48 to 82% compared with conventional jet fuel. Modest improvements to CI can be achieved through incremental changes to the brown grease CH process, such as relaxing the dewatering specification and implementing renewable natural gas and electricity, which could decrease the CI from 22.9 to 7.9 g CO 2 e/MJ. Total CH fuel production potential was also assessed on the basis of current or near-future feedstock availability and CI. The total biofuel production potential of CH (SAF and renewable fuel co-products) in the US sums to approximately 3487 million gallons per year, with 97% of these volumes having a CI below 50% of that for petroleum jet fuel. The study shows that from an LCA perspective, CH offers a viable SAF pathway that is comparable with existing SAF pathways like hydroprocessed esters and fatty acids.

09 BIOMASS FUELS↗
DOE OSTI2014

Techno-Economic Analysis of Bioconversion of Methane into Biofuel and Biochemical (Poster)

In light of the relatively low price of natural gas and increasing demands of liquid transportation fuels and high-value chemicals, attention has begun to turn to novel biocatalyst for conversion of methane (CH4) into biofuels and biochemicals [1]. A techno-economic analysis (TEA) was performed for an integrated biorefinery process using biological conversion of methane, such as carbon yield,process efficiency, productivity (both lipid and acid), natural gas and other raw material prices, etc. This analysis is aimed to identify research challenges as well provide guidance for technology development.

03 NATURAL GAS↗
DOE OSTI2022

Assessment and Improvement of Fission Product Transport Predictions of Particle Fuel in BISON

The U.S. Department of Energy’s Nuclear Energy Advanced Modeling and Simulation (NEAMS) program aims to develop predictive capabilities by applying computational methods to the analysis and design of advanced reactor and fuel cycle systems. This program has been providing engineering-scale support for the development of BISON, a high-fidelity and high-resolution fuel performance tool. This study was motivated by the need to incorporate more physics-based models in BISON in order to foster tri-structural isotropic (TRISO) applications. This document details the integration of new modeling capabilities in BISON, including (1) development of pyrolytic carbon (PyC) and silicon carbide (SiC) layer anisotropic thermal and mass transport capabilities, (2) verification of the mass diffusion solution in TRISO modeling, (3) calibration of fission product diffusivity using Advanced Gas Reactor (AGR) experiments, (4) improved fission product release modeling by developing compact diffusion modeling capabilities, and (5) documentation of accelerated failure analysis on the BISON website. Improvements made to the diffusion models and parameters were documented and validated against AGR-1 and -2 experiment data.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
NASA NTRSDate not supplied

Performance Analysis of Magnetohydrodynamic Drag Modulation for Actively Controlled Aerocapture at Neptune

Missions to the Ice Giants are a top priority for flagship missions this coming decade. However, a fully propulsive orbital insertion into these planets requires an immense amount of fuel, taking a significant portion of the spacecraft mass and restricting the scientific payload. To mitigate this, aerocapture has been heavily investigated. Although simulations have shown that aerodynamically controlled aerocapture can successfully insert into an orbit around both Ice Giants, the deep atmospheric pass required necessitates a complex, mass expensive, and sometimes prohibitive thermal protection system. Magnetohydrodynamic drag modulation serves as a potential alternative control method for aerocapture which could not only save propellant mass compared to fully propulsive orbital insertion, but also save thermal protection system mass compared to conventional aerocapture methods. Both aerodynamically controlled and magnetohydrodynamically controlled aerocapture methodologies were simulated in NASA Langley’s high-fidelity six degree-of-freedom flight dynamics code, the Program to Optimize Simulated Trajectories II. Each method was simulated to identical missions to Neptune using a numerical predictor-corrector algorithm to optimize the control towards the target orbit. The results concluded that magnetohydrodynamic drag modulation can successfully capture and performs on par with aerodynamic drag modulation while significantly reducing the heatflux and aeroshell complexity.

Danny N Nguyen↗