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DOE OSTI2024

Single-Shot Readout and Weak Measurement of a Tin-Vacancy Qubit in Diamond

The negatively charged tin-vacancy center in diamond (SnV − ) is an emerging platform for building the next generation of long-distance quantum networks. This is due to the SnV − ’s favorable optical and spin properties including bright emission, insensitivity to electronic noise, and long spin coherence times at temperatures above 1 K. Here, we demonstrate measurement of a single SnV − electronic spin with a single-shot readout fidelity of 87.4%, which can be further improved to 98.5% by conditioning on multiple readouts. In the process, we develop understanding of the relationship between strain, magnetic field, spin readout, and microwave spin control. We show that high-fidelity readout is compatible with rapid microwave spin control, demonstrating a favorable parameter regime for use of the SnV − center as a high-quality spin-photon interface. Finally, we use weak quantum measurement to study measurement-induced dephasing; this illuminates the fundamental interplay between measurement and decoherence in quantum mechanics, and provides a universal method to characterize the efficiency of color-center spin readout. Taken together, these results overcome an important hurdle in the development of the SnV − -based quantum technologies and, in the process, develop techniques and understanding broadly applicable to the study of solid-state quantum emitters.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

DOE OSTI2024

Constraining cosmology with the CMB × line intensity mapping-nulling convergence

Lensing reconstruction maps from the cosmic microwave background (CMB) provide direct observations of the matter distribution of the universe without the use of a biased tracer. Such maps, however, constitute projected observables along the line of sight that are dominated by their low-redshift contributions. To cleanly access high-redshift information, Maniyar et al., [Phys. Rev. D 105, 083509 (2022)] showed that a linear combination of lensing maps from both CMB and line intensity mapping (LIM) observations can exactly null the low-redshift contribution to CMB lensing convergence. In this paper we explore the scientific returns of this nulling technique. Here, we show that LIM-nulling estimators can place constraints on standard Λ⁢CDM plus neutrino mass parameters that are competitive with traditional CMB lensing. Additionally, we demonstrate that as a clean probe of the high-redshift universe, LIM nulling can be used for model-independent tests of cosmology beyond Λ⁢CDM and as a probe of the high-redshift matter power spectrum.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2024

Material exploration towards high quality factor microwave resonators

Niobium and aluminum have been widely used to realize superconducting resonators and qubits. However, the native oxide at the metal air interface limits the devices results. This layer is highly disordered, and it induces losses limiting the performances of the resonators or qubits. Recently, tantalum led to great improvement in qubit relaxation time. This improvement has been attributed to a thinner and less disordered oxide layer compared to Nb and Al. This study is aimed to limit the formation of the oxide layer, by the introduction of novel superconducting materials such as rhenium or by encapsulating the Nb surface with other superconducting materials such as Ta, Al, Re or other non-superconducting materials such as Au. To better understand the results, we are realizing these studies on coplanar waveguide resonators where the relation between surface losses and quality factor is clear. We are also analyzing different fabrication techniques to completely characterize our devices, linking material properties to the performances. In this work we are also varying the participation ratio of the devices in order to extract with higher fidelity and precision the losses introduced by the involved interfaces.

Crisa, F.↗

DOE OSTI2025

Requirements on the gain calibration for LiteBIRD polarisation data with blind component separation

The detection of primordial B modes of the cosmic microwave background (CMB) could provide information about the early stages of the Universe's evolution. The faintness of this signal requires exquisite calibration accuracy and control of instrumental systematic effects which otherwise could bias the measurements. In this work, we study the impact of an imperfect relative polarisation gain calibration on the recovered value of the tensor-to-scalar ratio r for the LiteBIRD experiment, through the application of the blind Needlet Internal Linear Combination (NILC) foreground-cleaning method. We derive requirements on the relative calibration accuracy of the overall polarisation gain (Δg ν ) for each LiteBIRD frequency channel. Our results show that minimum variance techniques, as NILC, are less sensitive to systematic gain calibration uncertainties compared to a parametric approach, if the latter is not equipped with a proper modelling of these instrumental effects. In this study, the most stringent requirements are found in the channels where the CMB signal is relatively brighter, with the tightest constraints at 166 GHz (Δg ν ≈ 0.16%). This differs from the outcome of an analogous analysis performed with a parametric method, where the tightest requirements are obtained for the foreground-dominated channels. Gain calibration uncertainties, corresponding to the derived requirements, are then simultaneously propagated into all frequency channels. By doing so, we find that the overall impact on estimated r is lower than the total gain systematic budget for LiteBIRD approximately by a factor 5, due to the correlations of the impacts of gain calibration uncertainties in different frequency channels. In order to decouple the systematic effect from the specific choice of the model, we derive the requirements assuming constant spectral parameters for the foreground emission. To assess the robustness of the obtained results against more realistic scenarios, we repeat the analysis assuming sky models of intermediate and high complexity. In these further cases, we adopt an optimised NILC pipeline, called the Multi-Clustering NILC (MC-NILC). We find that the impact of gain calibration uncertainties on r is lower than the LiteBIRD gain systematics budget for the intermediate-complexity sky model. For the high-complexity case, instead, it would be necessary to tighten the requirements by a factor 1.8.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2026

Secure Wireless Communication Using Distributed Coherent Transmission and Spatial Signal Decomposition

We present a new approach to secure wireless communications using coherent distributed transmission of signals that are spatially decomposed between a two-element distributed antenna array. High-accuracy distributed coordination of microwave wireless systems supports the ability to transmit different parts of a signal from separate transmitters such that they combine coherently at a designated destination. In this article, we explore this concept using a two-element coherent distributed phased array where each of the two transmitters sends a separate component of a communication signal, where each symbol is decomposed into a sum of two pseudorandom signal vectors, the coherent summation of which yields the intended symbol. By directing the transmission to an intended receiver using distributed beamforming, the summation of the two vector components is largely confined to a spatial region at the destination receiver. We implement the technique in a $50−λ$ array operating at 3 GHz. We evaluate the symbol error rate (SER) in 2-D space through simulation and measurement, showing that the approach yields a spatially confined secure region where the information is recoverable (i.e., the received signal has low SER), and outside of which the information is unrecoverable (high SER). The proposed system is also compared against a traditional beamforming system where each node sends the same data. We validate experimentally that our approach achieves a low SER of 0.0082 at broadside and an SER above 0.25 at all other locations compared to a traditional beamforming approach that achieves a SER of 0 at all locations measured.

Engineering - Electronic and electrical engineerin↗

DOE OSTI2024

Ultrafast all-optical coherence of molecular electron spins in room-temperature water solution

The tunability and spatial precision of paramagnetic molecules makes them attractive for quantum sensing. However, usual microwave-based detection methods have poor temporal and spatial resolution, and optical methods compatible with room-temperature solutions have remained elusive. In this study, we utilized pump-probe polarization spectroscopy to initialize and track electron spin coherence in a molecule. Designed to efficiently couple spins to light, aqueous potassium hexachloroiridate(IV) enabled detection of few-picosecond free-induction decay at room temperature and micromolar concentrations. Viscosity was found to strongly vary decoherence lifetimes. This approach has improved the experimental time resolution by up to five orders of magnitude, making it possible to observe molecular electron spin coherence in a system that only exhibits coherence below 25 kelvin with traditional techniques.

74 ATOMIC AND MOLECULAR PHYSICS↗

DOE OSTI2025

A High-Speed, High-Resolution Transition Edge Sensor Spectrometer for Soft X-Rays at the Advanced Photon Source

This project explores the design and development of a transition edge sensor (TES) spectrometer for resonant soft X-ray scattering (RSXS) measurements developed in collaboration between Argonne National Laboratory (ANL) and the National Institute of Standards and Technology (NIST). Soft X-ray scattering is a powerful technique for studying the electronic and magnetic properties of materials on a microscopic level. However, the lack of high-performance soft X-ray spectrometers has limited the potential of this technique. TES spectrometers have the potential to overcome these limitations due to their high energy resolution, high efficiency, and broad energy range. This project aims to optimize the design of a TES spectrometer for RSXS measurements and more generally soft X-ray spectroscopy at the Advanced Photon Source (APS) 29-ID, leading to improved understanding of advanced materials. We will present a detailed description of the instrument design and implementation. The spectrometer consists of a large array of approximately 250 high-speed and high-resolution pixels. The pixels have saturation energies of approximately 1 keV, sub-ms pulse duration and energy resolution of approximately 1 eV. The array is read out using microwave multiplexing chips with MHz bandwidth per channel, enabling efficient data throughput. To facilitate measurement of samples in situ under ultra-high vacuum conditions at the beamline, the spectrometer is integrated with an approximately 1 m long snout.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

DOE OSTI2026

Quality and Loss Factor Analysis of YBCO Superconducting Transmission Lines for Axion Dark Matter Detection

Axion haloscope experiments aim to detect the conversion of axions into microwave photons in a magnetic field, which produces extremely small signals requiring low-loss cryogenic transmission lines for readout to reduce noise and attenuation. Yttrium Barium Copper Oxide (YBCO) cables are a promising candidate. Unlike commonly used low-loss superconducting cables such as Niobium (Nb) and Niobium Titanium (NbTi), which have low critical fields, YBCO is a high-temperature superconductor that can remain stable in strong magnetic fields. We evaluate their suitability by characterizing the quality and loss factors of five stripline resonators (three YBCO, and copper and silver references) from the Brookhaven Technology Group at 77 K without an external field, and cooled to 30 mK in a 14 T magnet. For measurements at 77 K we recorded scattering parameter data and employed Lorentzian and circle-fitting analysis techniques. We identified the best-performing resonator and developed a cryogenic probe for future testing in the magnet at millikelvin temperatures.

Marinos, Zoe [UCLA]↗

DOE OSTI2025

Signal-preserving CMB component separation with machine learning

Analysis of microwave sky signals, such as the cosmic microwave background, often requires component separation using multifrequency methods, whereby different signals are isolated according to their different frequency behaviors. Many so-called blind methods, such as the internal linear combination (ILC), make minimal assumptions about the spatial distribution of the signal or contaminants, and only assume knowledge of the frequency dependence of the signal. The ILC produces a minimum-variance linear combination of the measured frequency maps. In the case of Gaussian, statistically isotropic fields, this is the optimal linear combination, as the variance is the only statistic of interest. However, in many cases the signal we wish to isolate, or the foregrounds we wish to remove, are non-Gaussian and/or statistically anisotropic (in particular for the case of Galactic foregrounds). In such cases, it is possible that machine learning (ML) techniques can be used to exploit the non-Gaussian features of the foregrounds and thereby improve component separation. However, many ML techniques require the use of complex, difficult-to-interpret operations on the data. We propose a hybrid method whereby we train an ML model using only combinations of the data that , and combine the resulting ML-predicted foreground estimate with the ILC solution to reduce the error from the ILC. We demonstrate our methods on simulations of extragalactic temperature and Galactic polarization foregrounds and show that our ML model can exploit non-Gaussian features, such as point sources and spatially varying spectral indices, to produce lower-variance maps than ILC—e.g., reducing the variance of the B-mode residual by factors of up to 5—while preserving the signal of interest in an unbiased manner. Moreover, we often find improved performance even when applying our ML technique to foreground models on which it was not trained. Published by the American Physical Society 2025

McCarthy, Fiona (ORCID:0000000253893565)↗

DOE OSTI2024

Improving constraints on inflation with CMB delensing

Abstract The delensing of cosmic microwave background (CMB) maps will be increasingly valuable for extracting as much information as possible from future CMB surveys. Delensing provides many general benefits, including sharpening of the acoustic peaks, more accurate recovery of the damping tail, and reduction of lensing-inducedB-mode power. In this paper we present several applications of delensing focused on testing theories of early-universe inflation with observations of the CMB. We find that delensing the CMB results in improved parameter constraints for reconstructing the spectrum of primordial curvature fluctuations, probing oscillatory features in the primordial curvature spectrum, measuring the spatial curvature of the universe, and constraining several different models of isocurvature perturbations. In some cases we find that delensing can recover almost all of the constraining power contained in unlensed spectra, and it will be a particularly valuable analysis technique to achieve further improvements in constraints for model parameters whose measurements are not expected to improve significantly when utilizing only lensed CMB maps from next-generation CMB surveys. We also quantify the prospects of testing the single-field inflation tensor consistency condition using delensed CMB data; we find it to be out of reach of current and proposed experimental technology and advocate for alternative detection methods.

Astronomy & Astrophysics↗

DOE OSTI2025

All-optical photoluminescence response of nitrogen-vacancy ensembles in diamond at low magnetic fields

All-optical (AO) microwave-free magnetometry using nitrogen-vacancy (N-𝑉) centers in diamond is attractive due to its broad applicability and reduced experimental complexity. In this work, we investigate room-temperature AO photoluminescence (PL) at low magnetic fields ( <2 mT) using diamonds with N-𝑉 ensembles at parts-per-million (ppm) concentrations. The measured AO-PL contrast features as a function of the applied magnetic field magnitude and direction are correlated with near-degenerate N-𝑉 electronic spin and hyperfine transitions from different N-𝑉 orientations within the diamond host. Reasonable agreement is found between low-field AO-PL measurements and model-based simulations of the effects of resonant dipolar interactions between N-𝑉 centers. The maximum observed AO-PL contrast depends on both the N-𝑉 concentration and the laser-illumination intensity at 532 nm. These results imply different optimal conditions for low-field AO N-𝑉 sensing compared to conventional optically detected magnetic resonance (ODMR) techniques, suggesting new research and application opportunities using AO measurements with lower system complexity, size, weight, and power.

Dipolar interaction↗

DOE OSTI2026

Radiation modeling and experimental validation of sub-cyclotron frequency microwave synchrotron radiation as a diagnostic tool for runaway electrons in present and future tokamaks

The microwave synchrotron radiation in the sub-cyclotron frequency region has been systematically validated as a diagnostic method for runaway electrons (>1 MeV) with radiation modeling and experiments on the DIII-D tokamak. Experimental observations reveal that sub-cyclotron frequency microwave radiation emerges only after runaway electrons are excited during plasma disruptions. Electron gyro-magnetic radiation modeling confirms that only runaway electrons with energies exceeding 1 MeV can emit radiation in the observed sub-cyclotron frequency band on DIII-D. The synchrotron Razin and Beaming effects are modeled in both the sub-cyclotron and standard Electron Cyclotron Emission (ECE) frequency region. Due to the pronounced beaming effect, the modeling supports that a standard ECE system is insensitive to synchrotron radiation from beamed runaway electrons (p ∥ >> p ⟂ ), but very sensitive to ECE radiation from isotropic suprathermal electrons (100 keV or less). DIII-D experiments further show that combining ECE and sub-cyclotron receivers reveals new insights into transient runaway dynamics during the plateau phase. Certain transient crash events appear only in the sub-cyclotron band or lead to opposite changes on the sub-cyclotron and standard ECE signals, supporting models where transient MHD events can exert a different effect on electrons of different energy levels. This novel diagnostic technique offers a powerful tool for studying and detecting runaway electron dynamics in both present-day and high-field future tokamaks. The diagnostic approach has been extrapolated to the SPARC tokamak, where sub-cyclotron radiation is predicted to respond sensitively and solely to runaway electrons during SPARC’s L-mode startup phase.

Yu, Guanying [Hefei Comprehensive National Science↗

DOE OSTI2025

Sputtered ferroelectric aluminum scandium boron nitride (Al 1−x−y B x Sc y N)/ n -GaN heterostructures

This work demonstrates ferroelectric switching in magnetron sputtered Al 1−x−y B x Sc y N/ n -GaN heterostructures. Using high power impulse magnetron sputtering, a silicon doped n -GaN bottom electrode with an electron concentration of 6.0 × 10 19 cm −3 is grown on c-plane sapphire. Al 1−x−y B x Sc y N films are prepared on the GaN surface with Al:B:Sc ratios that produce tensile, lattice matched, or compressive epitaxial strains. X-ray diffraction shows that lattice matched and compressively strained Al 1−x−y B x Sc y N compositions are pseudomorphic, while partial relaxation is observed for tensilely strained Al 1−x−y B x Sc y N/ n -GaN heterostructures. Electrically, the Al 1−x−y B x Sc y N/ n -GaN stacks show robust hysteresis; the P–E loops are fully saturated with both lattice matched and compressively strained Al 1−x−y B x Sc y N compositions exhibiting remanent polarization values of 135 μC/cm 2 . For comparison, Al 1−x−y B x Sc y N films are also prepared on metal organic chemical vapor deposition and single crystal GaN substrates to extend strain and morphology trends to more common substrate types. This report validates that sputter deposition is a feasible technique for fabricating strain-tunable ferroelectric III–N heterostructures with high crystalline fidelity and smooth surface morphologies.

42 ENGINEERING↗

DOE OSTI2024

Materials for Ultra‐Coherent, Mobile, Electron‐Spin Qubits

This research project has had the goal of gaining a better understanding of the physics of electrons bound to the surface of superfluid helium from both experimental and theoretical perspectives. It has particularly been aimed at two areas which had not been well studied: the relaxation and decoherence of the spin of the electrons on the helium surface and how the properties of underlying metallic layers affect the behavior of the electrons when the helium covering the metal is thin. This work is motivated in part by interest in using the spin of these electrons as a quantum bit, or qubit. Low levels of decoherence are advantageous for qubits, and moving the electrons, as one might do in a quantum processor, will be easiest if thin helium films can be employed. It had been suggested that spin decoherence should be very weak for electrons bound to superfluid He, but before this work there have been no quantitative studies of spin relaxation and decoherence. It is especially important to know how moving the electrons across the helium surface would affect their spin coherence. Calculations performed as part of this project show that the Rashba effective magnetic field, the mechanism which limits the spin coherence of mobile electrons in silicon-based devices (an actively pursued qubit technology), is exceptionally weak for electrons bound to helium. This project has identified other decoherence mechanisms which are stronger, but still weak compared to analogous silicon-based structures. Calculated spin coherence times for mobile electrons approach one day, as compared to microseconds in silicon. With coherence times of this magnitude, the spin qubit errors on helium will be completely dominated by errors in the quantum gates. In related work, the possibility of using an artificial spin-orbit interaction (a gradient magnetic field) for quantum operations on the electrons spins was considered. The calculations show that a moderate gradient field, small enough to be generated by a narrow superconducting wire, will enable high-fidelity quantum operations on electrons held in lithographically-defined quantum dots by driving them with a microwave electric field. The spin and motional coherence of the electrons is sufficient to allow high-fidelity 2-qubit quantum operations between electrons in neighboring quantum dots. As an outgrowth of experiments aiming to measure electron spin coherence it was discovered that very high densities of electrons can be stably supported on thin helium films coating ultra-smooth amorphous metallic layers. The measured densities are high enough that the electron system has almost certainly transitioned from an ordered array of electrons, known as a Wigner crystal (ordered by the electrons’ mutual repulsion), to a quantum fluid known as a Fermi liquid. This transition has been a subject of intense interest for over 40 years, since the electron Wigner crystal was first observed with electrons bound to superfluid helium, but it has never been unambiguously observed. Experiments are still underway in these new structures to definitively determine whether true quantum melting of the Wigner crystal has been demonstrated. This work has also catalyzed the development of a new approach for measuring the transport of electrons across very thin helium films, as will be needed for some of the quantum computing applications. The high electron density experiments as well as experiments with electrons bound in quantum dots have led to new techniques which may enable spin coherence measurements.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

DOE OSTI2024

Local probe of bulk and edge states in a fractional Chern insulator

The fractional quantum Hall effect is a key example of topological quantum many-body phenomena, arising from the interplay between strong electron correlation, topological order and time-reversal symmetry breaking. Recently, a lattice analogue of the fractional quantum Hall effect at zero magnetic field has been observed, confirming the existence of a zero-field fractional Chern insulator (FCI). Despite this, the bulk–edge correspondence—a hallmark of a FCI featuring an insulating bulk with conductive edges—has not been directly observed. In fact, this correspondence has not been visualized in any system for fractional states owing to experimental challenges. Here we report the imaging of FCI edge states in twisted MoTe 2 (t-MoTe 2 ) using microwave impedance microscopy. By tuning the carrier density, we observe the system evolving between metallic and FCI states, the latter of which exhibits insulating bulk and conductive edges, as expected from the bulk–boundary correspondence. Further analysis suggests the composite nature of the FCI edge states. We also observe the evolution of edge states across the topological phase transition as a function of interlayer electric field and reveal exciting prospects of neighbouring domains with different fractional orders. Furthermore, these findings pave the way for research into topologically protected one-dimensional interfaces between various anyonic states at zero magnetic field, such as gapped one-dimensional symmetry-protected phases with non-zero topological entanglement entropy, Halperin–Laughlin interfaces and the creation of non-abelian anyons.

Imaging techniques↗

DOE OSTI2024

One-dimensional mapping of femtosecond laser filaments using coherent microwave scattering

Here, this paper reports on the use of coherent microwave scattering (CMS) for spatially resolved electron number density measurements of elongated plasma structures induced at mid-IR femtosecond filamentation in air. The presented studies comprise one-dimensional mapping of laser filaments induced via 3.9 µm, 127.3 fs laser pulses at output energies up to 15 mJ. The axial electron number density was measured to be invariant (about 2 × 10 15 c⁢m −3 ) along the entire filament length and for all tested laser pulse energies 5–15 mJ, and the corresponding laser intensity in the middle portion of the filament was estimated to be nearly constant for 5–15 mJ pulse energies (about 30−40 TW/c⁢m 2 ). These findings support that intensity clamping conditions were achieved in the experiments. The proposed approach enables capabilities that are currently unavailable to perform absolute and longitudinally resolved measurements of electron number density in laser filaments and to precisely characterize conditions associated with self-focusing and intensity clamping.

plasma diagnostic techniques↗

DOE OSTI2025

Quantifying bias due to non-Gaussian foregrounds in an optimal reconstruction of CMB lensing and temperature power spectra

We estimate the magnitude of the bias due to non-Gaussian extragalactic foregrounds on the optimal reconstruction of the cosmic microwave background (CMB) lensing potential and temperature power spectra. The reconstruction is performed using a Bayesian inference method known as the marginal unbiased score expansion (MUSE). We apply MUSE to a minimum variance combination of multifrequency maps drawn from the Agora publicly available simulations of the lensed CMB and correlated extragalactic foreground emission. Taking noise levels appropriate to the SPT-3G D1 release, we find non-Gaussian foregrounds may bias the MUSE reconstruction of the lensing potential amplitude at the level of (0.7 ± 0.3)σ when using modes up to ℓ max = 3500. We do not detect a statistically significant bias, finding a value of (-0.4 ± 0.3)σ, when restricted to lower angular multipoles, ℓ max = 3000. This work is a first step toward understanding the impact of extragalactic foregrounds on optimal reconstructions of CMB temperature and lensing potential power spectra.

Statistical sampling techniques↗

DOE OSTI2025

A unified realization of electrical quantities from the quantum International System of Units

In the revised International System of Units (SI), the ohm and the volt are realized from the von Klitzing constant and the Josephson constant, and a practical realization of the ampere is possible by applying Ohm’s law directly to the quantum Hall and Josephson effects. As a result, it is possible to create an instrument capable of realizing all three primary electrical units, but the development of such a system remains challenging. Here, in this study, we report a unified realization of the volt, ohm and ampere by integrating a quantum anomalous Hall resistor (QAHR) and a programmable Josephson voltage standard (PJVS) in a single cryostat. Our system has a quantum voltage output that ranges from 0.24 mV to 6.5 mV with combined relative uncertainties down to 3 μV V −1 . The QAHR provides a realization of the ohm at zero magnetic field with uncertainties near 1 μΩ Ω −1 . We use the QAHR to convert a longitudinal current to a quantized Hall voltage and then directly compare that against the PJVS to realize the ampere. We determine currents in the range of 9.33–252 nA, and our lowest uncertainty is 4.3 μA A −1 at 83.9 nA. For other current values, a systematic error that ranges from −10 μA A −1 to −30 μA A −1 is present due to the imperfect isolation of the PJVS microwave bias.

Quantum metrology↗