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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 1,405 records · Page 78

Imaging Macromolecular Structural Dynamics with Low-Dose, Time-Resolved Transmission Electron Microscopy

All well-established experimental methods for investigating the structure of biological macromolecules have spatial and/or temporal limitations inherent to the technique that limit their applicability to studying macromolecular dynamics. The ability to measure macromolecular dynamics is key to gaining predictive mastery of biological systems. This work demonstrates that sufficient data can be acquired from low-Z soft materials using dynamic transmission electron microscopy (DTEM) to potentially allow measurements of macromolecular motion. While a dynamic measurement of macromolecular motion or structural change requires further effort, it is evident from this work that this is feasible under specific experimental conditions that can be achieved using low-dose, time-resolved transmission electron microscopy.

59 BASIC BIOLOGICAL SCIENCES↗

Investigations of plasma evolution in Laser Ablation Z-Pinch Experiments using Time-Resolved Optical Spectroscopy

In this dissertation, investigations of the temporal evolution of magnetically driven plasmas are presented. These studies were carried at the Nevada Terawatt Facility using the Zebra pulsed-power accelerator to magnetically compress and confine a cylindrical plasma column. Important parameters needed to characterize these laboratory plasmas include magnetic field strength and orientation, as well as electron number density and temperature. To fully understand the characteristics of a plasma, accurate experimental measurement of these parameters is essential. To determine the electron temperature, the Boltzmann plot method was used. Simulated spectra from PrismSPECT were compared to experimental measurements in order to measure electron number density and temperature early in the pinched plasma formation. Simultaneously, Mach-Zehnder laser interferometry was used to provide complementary measurements of the electron number density. A novel method, streaked Zeeman-induced Magnetic Splitting optical spectroscopy, was developed to measure time- and space-resolved magnetic field strengths in these hot, dense plasmas. This technique has also been applied to diagnose the magnetic field strengths in laser ablation Z-pinch experiments, wherein a pulsed power driver pinches a laser ablated plume.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DARHT Axis 1 Time-Resolved Injector Energy Measurement

The Dual-Axis Radiographic Hydrodynamic Test (DARHT) facility provides flash radiography capabilities using electron Linear Induction Accelerators (LIA’s). The strict requirements for flash radiography require a detailed understanding of the LIA’s performance, including precision measurements of the injected electron beam energy. The DARHT Axis 1 injector of produces a 3-4 MeV, 1-2 kA, 80-ns-FWHM electron beam. Injector capacitive monitors (EVACSUM) are summed to give the injector beam energy. Calibration of EVACSUM was last done in 1999 and is needed. In addition, the flatness of the injector drive voltage is controlled by a peaking capacitor in a Blumlien that is charged by the prime power tank. Time resolved measurements are used to optimize the value of this capacitor.

47 OTHER INSTRUMENTATION↗

Evolution of Precipitation Structure During the November DYNAMO MJO Event: Cloud-Resolving Model Inter-comparison and Cross-Validation using Radar Observations

Evolution of precipitation structures are simulated and compared with radar observations for the November Madden-Julian Oscillation (MJO) event during the DYNAmics of the MJO (DYNAMO) field campaign. Three ground-based, ship-borne, and space-borne precipitation radars and three Cloud-Resolving Models (CRMs) driven by observed large-scale forcing are used to study precipitation structures at different locations over the central equatorial Indian Ocean. Convective strength is represented by 0-dBZ echo-top heights, and convective organization by contiguous 17-dBZ areas. The multi-radar and multi-model framework allows for more stringent model validations. The emphasis is on testing models’ ability to simulate subtle differences observed at different radar sites when the MJO event passed through. The results show that CRMs forced by site-specific large-scale forcing can reproduce not only common features in cloud populations, but also subtle variations observed by different radars. The comparisons also revealed common deficiencies in CRM simulations where they underestimate radar echo-top heights for the strongest convection within large, organized precipitation features. Cross-validations with multiple radars and models also enable quantitative comparisons in CRM sensitivity studies using different large-scale forcing, microphysical schemes and parameters, resolutions, and domain sizes. In terms of radar echo-top height temporal variations, many model sensitivity tests have better correlations than radar/model comparisons, indicating robustness in model performance on this aspect. It is further shown that well-validated model simulations could be used to constrain uncertainties in observed echo-top heights when the low-resolution surveillance scanning strategy is used.

54 ENVIRONMENTAL SCIENCES↗

Time-resolved measurement of electron beam neutralization

An intense relativistic electron beam (IREB) incident on a target generates positive ions by stimulated and thermal desorption of adsorbed gas, and subsequent electron impact ionization. These ions are accelerated upstream by the beam space-charge potential, thereby partially neutralizing the beam. If there is enough neutralization, the repulsive space-charge force can be overcome by the magnetic-pinch force due to the beam current. This so-called ion focusing is responsible for time dependent defocusing of the radiographic source spot. Since a single monolayer of adsorbed gas has a surface density of about 10 15 /cm 2 and is formed in about one second in a one micro-Torr vacuum, there is always enough adsorbed gas to make this a concern in our accelerators. Therefore, time-resolved measurements of the degree of neutralization are valuable for better understanding of this process with an eye to mitigation for improvement of our radiography. Moreover, these measurements would aid quantification of uncertainties due to these effects when using invasive beam diagnostics, such as OTR imaging targets.

43 PARTICLE ACCELERATORS↗

Time-Resolved PIV Measurements of Flow Field at the Exit of a Diffuser Mounted on a Rotating Detonation Combustor

Time-resolved particle image velocimetry at 30 kHz is applied to the exhaust flow field of a RDC system configured with a diffuser geometry and a converging-diverging (CD) nozzle. The RDC is operated with methane fuel and oxygen-enriched air, motivated by power generation applications. The measured flow-field is discretized into axial and non-axial velocity components. Results are shown to characterize the flow-field across a cord length at the exit plane. Instantaneous contours of the two velocity components, and 1D histograms of velocity components, and 2D histograms of total velocity and tilt angle are shown at multiple locations in the flow. Repeatability of the data is evaluated by comparing tests conducted at similar flow rates. Results are presented for a baseline test case, and test cases showing the effect of reactant higher flow rate and CD nozzle geometry. Finally, the results are compared to a previous RDC study without the diffuser to compare the effectiveness of the diffuser and CD nozzle designs in mitigating the flow periodicity at the combustor exit.

particle image velocimetry, pressure gain combusti↗

Spatially and Temporally Resolved Velocimetry for Hypersonic Flows

The development of new hypersonic flight vehicles is limited by the physical understanding that may be obtained from ground test facilities. This has motivated the present development of a temporally and spatially resolved velocimetry measurement for Sandia National Laboratories (SNL) Hypersonic Wind Tunnel (HWT) using Femtosecond Laser Electronic Excitation Tagging (FLEET). First, a multi-line FLEET technique has been created for the first time and tested in a supersonic jet, allowing simultaneous measurements of velocities along multiple profiles in a flow. Secondly, two different approaches have been demonstrated for generating dotted FLEET lines. One employs a slit mask pattern focused into points to yield a dotted line, allowing for two- or three-component velocity measurements free of contamination between components. The other dotted-line approach is based upon an optical wedge array and yields a grid of points rather than a dotted line. Two successful FLEET measurement campaigns have been conducted in SNL’s HWT. The first effort established optimal diagnostic configurations in the hypersonic environment based on earlier benchtop reproductions, including validation of the use of a 267 nm beam to boost the measurement signal-to-noise ratio (SNR) with minimal risk of perturbing the flow and greater simplicity than a comparable resonant technique at 202 nm. The same FLEET system subsequently was reconstituted to demonstrate the ability to make velocimetry measurements of hypersonic turbulence in a realistic flow field. Mean velocity profiles and turbulence intensity profiles of the shear layer in the wake of a hypersonic cone model were measured at several different downstream stations, proving the viability of FLEET as a hypersonic diagnostic.

33 ADVANCED PROPULSION SYSTEMS↗

Size and Time-Resolved Automated Aerosol Sampling Field Campaign Report

To improve the understanding of the impacts of the vertical distribution of aerosol chemical composition on radiative forcing of aerosol, we performed a detailed physicochemical characterization of aerosol particles sampled during ARM deployment of the tethered balloon system at two ARM sites. We used multi-modal microscopy/spectroscopy techniques and advanced mass spectrometry platforms for the analysis of particles. We found variations in size-resolved aerosol composition at different altitudes. We also observed changes in aerosol composition during different seasons. Some of our observations at ARM’s Oliktok Point, Alaska site suggest cloud processing of aerosol while sampling in clouds, below clouds, and above clouds.

54 ENVIRONMENTAL SCIENCES↗

Receiving flat bands near the Fermi level in 1T-VSe2 by using angle resolved photoemission spectroscopy

Here, we study the surface electronic structure of 1T-VSe 2 by means of angle resolved photoemission spectroscopy and uncover a dispersion-less emission located in the vicinity of the Fermi level. Its crystal momentum dependency reveals that it occupies large portions of the Brillouin zone (BZ), where no bulk band is expected. Upon electron doping (deposition of Rb-atoms), the system evolves in a surprising way. Besides the expected down-shifting of the bands, a splitting of both bulk and dispersion-less emission is observed. This peculiar behavior strongly suggests the intrinsic nature of the dispersion-less emission. Its characterization may therefore be relevant to a deeper understanding of the physics of transition metal dichalcogenides.

43 PARTICLE ACCELERATORS↗

Resolved Resonance Region Evaluation of n+ 140,142 Ce [Slides]

ORNL has completed new resolved resonance region (RRR) evaluations for 140,142 Ce, which were carried out using Reich-Moore formalism instead of MLBW. Lack of integral measurements makes validation difficult, but difference from Kadonis values suggest more investigation of capture cross section are warranted. The complete file (with updated File2 & File32) was submitted to NNDC repository for inclusion in next release of ENDF. Sponsor report and journal publication are in progress.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Time-Resolved Beam Position Measurements for the Scorpius Multipulse Linear Induction Accelerator

Beam position monitors (BPMs) provide time-resolved measurements of the current and centroid position of high-current electron beams in linear induction accelerators (LIAs). One of the types of detectors used in BPMs is the B-dot loop, which generates a signal from the EMF due to the time varying magnetic flux through the loop. If some of the boundaries of the loop are composed of thick metal walls with finite conductivity, the resulting signal must be corrected for the magnetic field diffusion into the metal. The theoretically predicted flux due to diffusion is in remarkable agreement with experimental measurements. Although accurate BPM measurements of beam current require correction of magnetic field diffusion, accurate measurement of beam position requires no correction. In this note, we present a theoretical derivation and the experimental validation of this result.

43 PARTICLE ACCELERATORS↗

140,142 Cerium Resolved Resonance Region Evaluation [Slides]

The presentation covers an overview of 140,142 Ce Isotopes, including new evaluations of 140,142 Ce that were requested by the Hanford Plutonium Finishing plant to the Nuclear Criticality Safety Program. It also discusses current ENDF/B-VIII.0 evaluation, which has an error in the 1-2 keV range. It was evaluated using multi-level Breit-Wigner and 142Ce has room for extending resolved resonance region current upper limit from 13 keV. The presentation also discusses new transmission and capture measurements of nat Ce and 142 Ce from Klaus Guber. It also states that no known integral experiments prominently feature Cerium.

07 ISOTOPE AND RADIATION SOURCES↗

Updates to the n+ 63,65 Cu Evaluations in the Resolved Resonance Region [Slides]

This presentation discusses the motivation and background of the n+ 63,65 Cu Evaluations in the Resolved Resonance Region which is to study the interaction of neutrons with copper as it is important in nuclear applications since critical assembly configurations include metallic copper as reflector. In support to the U.S. Department of Energy (DOE) Nuclear Criticality Safety Program (NCSP), measurements and related evaluations of 63,65 Cu isotopes were selected to improve the agreement with the benchmarks and to assess the importance of the angular distribution data for reactor calculations. Previous and current evaluation work is supported by an experimental campaign initiated before 2010, the 63,65 Cu R-matrix analysis generated resonance parameters up to 300 keV. However, due to outstanding issues in the benchmark performance, ENDF/B-VIII.0 library released a truncated set of resonance parameters up to 100 keV. The goal of this work is to generate an updated set of resonance parameters in the 100-300 keV range to improve the benchmark performance of 63,65 Cu isotopes. In conclusion, R-matrix analysis to update 63,65 Cu evaluations was performed to simultaneously improve benchmark performance and extend the RRR to 300 keV. The benchmark calculations suggest the increased capture cross sections are beneficial, however, further investigation of the measured capture data is needed to understand the large normalization scaling factor needed to improve the reactivity. Also, the copper-reflected benchmarks indicate the need to further investigate angular distributions and extension of RRR to 300 keV is aided well by level statistics considerations. Work to refine the fit of individual resonances is ongoing.

07 ISOTOPE AND RADIATION SOURCES↗

NucD-24 Nuclear Diagnostics Development: Time resolved 12 C-rhoR on GCD and NIS technology development for polar LOS and data quality [Slides]

The Neutron Imaging team is readying for the NIS2 polar LOS development and future improvements to data quality on all LOS given consistently higher yields at NIF. Next-gen nano guide scintillators for NIS2 and CMOS cameras to replace outdated CCDs will be studied. Digital image plates will be tested for better data quality on passive imaging systems. The transition into the ignition regime is expected to show a significant signature in the ablator areal density. In the marginal ignition regime, a decrease of 12C-rhoR (ablator areal density) is expected but once the burn propagation produces a shock and compresses the ablator the trend reverses. GCD with the PD-PMT can resolve this effect in the ablator areal density by a temporal shift in the carbon signal. To give quantitative results a calibration of the detector for the Hohlraum/TMP signal is needed. Shots using Al, Si, and Au pucks will yield the needed information to move forward with this project.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Highly Resolved Projections of Passenger Electric Vehicle Charging Loads for the Contiguous United States: Results From and Methods Behind Bottom-Up Simulations of County-Specific Household Electric Vehicle Charging Load (Hourly 8760) Profiles Projected Through 2050 for Differentiated Household and Vehicle Types

This report documents enhancements made to the TEMPO (Transportation Energy & Mobility Pathway Options TM ) model to project spatially, demographically, and temporally resolved national-scale EV charging load profiles and describes three scenarios and corresponding datasets created for the NREL demand-side grid (dsgrid) project in support of bulk power systems modeling. In brief, TEMPO was enhanced to disaggregate national and annual energy demand projections into household and county-level projections of passenger electric vehicle (EV) hourly charging load profiles (8760 profiles), accounting for consumer, travel, and temperature variations that impact EV energy demand. In alignment with NREL's forward-looking grid modeling, three scenarios for EV adoption covering 2020-2050 were created-- Annual Energy Outlook (AEO) Reference Case, Electrification Futures Study (EFS) High Electrification, and All EV Sales by 2035 --and associated datasets have been included in the dsgrid platform for public use.

29 ENERGY PLANNING, POLICY, AND ECONOMY↗

R-matrix Resolved Resonance Region Evaluation of 140,142 Ce

Oak Ridge National Laboratory completed the resolved resonance region (RRR) evaluation of the two most abundant cerium isotopes, 140 Ce (88.45%) and 142 Ce (11.11%), as requested by the US Nuclear Criticality Safety Program. These evaluations are based on recent high-resolution transmission and capture measurements performed on nat Ce and highly enriched 142 Ce samples at the JRC-Geel Linear Accelerator facility, as well as measured thermal constants available from the EXFOR database. Starting from the resonance parameters of the ENDF/B-VIII.0 library followed by a preliminary R-matrix analysis, an updated set of resonance parameters and corresponding covariance information were derived by fitting these measured data using the Reich–Moore approximation of the R -matrix theory, as implemented in the SAMMY code system. The 140 Ce RRR upper energy limit was kept at 200 keV, whereas the 142 Ce resonance region was extended from 13 to 26 keV. Updated statistical properties were obtained for the new evaluations and compared to those derived from the ENDF/B-VIII.0 nuclear data library. The new evaluation work improved some of the discrepancies found in previous work, such as the capture resonance integral and stellar Maxwellian-averaged cross sections. These integral quantities were mainly derived from the fit of the latest measured data, especially the neutron capture yield data for 142 Ce isotope.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗