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At least 145 records · Page 8

An Analysis of Methanol and Hydrogen Production via High-Temperature Electrolysis Using the Sodium Cooled Advanced Fast Reactor

Integration of an advanced, sodium-cooled fast spectrum reactor into nuclear hybrid energy system (NHES) architectures is the focus of the present study. A techno-economic evaluation of several conceptual system designs was performed for the integration of a sodium-cooled Advanced Fast Reactor (AFR) with the electric grid in conjunction with wind-generated electricity. Cases in which excess thermal and electrical energy would be reapportioned within an integrated energy system to a chemical plant are presented. The process applications evaluated include hydrogen production via high temperature steam electrolysis and methanol production via steam methane reforming to produce carbon monoxide and hydrogen which feed a methanol synthesis reactor. Three power cycles were considered for integration with the AFR, including subcritical and supercritical Rankine cycles and a modified supercritical carbon dioxide modified Brayton cycle. The thermal efficiencies of all of the modeled power conversions units were greater than 40%. A thermal efficiency of 42% was adopted in economic studies because two of the cycles either performed at that level or could potentially do so (subcritical Rankine and S-CO2 Brayton). Each of the evaluated hybrid architectures would be technically feasible but would demonstrate a different internal rate of return (IRR) as a function of multiple parameters; all evaluated configurations showed a positive IRR. As expected, integration of an AFR with a chemical plant increases the IRR when “must-take” wind-generated electricity is added to the energy system. Additional dynamic system analyses are recommended to draw detailed conclusions on the feasibility and economic benefits associated with AFR-hybrid energy system operation.

09 BIOMASS FUELS↗

Feasibility study of Self Powered Neutron Detectors in Fast Reactors for detecting local change in neutron flux distribution

Neutron flux monitoring system forms an integral part of the design of a Generation IV sodium cooled fast reactor system. Diverse possibilities of detector systems installation have to be investigated with respect to practicality and feasibility according to the detection parameters. In this paper, we demonstrate the feasibility of using self powered neutron detectors as in-core detectors in fast reactors for detecting local change in neutron flux distribution. We show that the gamma contribution from fission products decay in the fuel and activation of structural materials is very small compared to the fission gammas. Thus, it is possible for the in-core SPND signal to follow changes in local neutron flux as they are proportional to each other. This implies that the signal from an in-core SPND can provide dynamic information on the neutron flux perturbations occurring inside the reactor core. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Core and Fuel Cycle Performance of a Molten Salt Fast Reactor

This paper discusses the reactor core design and modeling approaches for a specific molten salt fast reactor (MSFR) design that is started up with high-assay low-enriched uranium (HALEU) within a chloride fuel salt and focuses on the technical assumptions and design choices. These include the fuel salt properties, first core and make-up heavy metal requirements, fuel composition evolution, equilibrium fission product concentration, etc. This MSFR concept was developed as part of a wider study that sought to compare the fuel cycle performance tradeoffs between deploying a fleet of sodium-cooled fast reactors (SFRs) and deploying a fleet of MSFRs. MSFRs that use flowing liquid fuel salt and on-line salt processing are of particular interest because these technology characteristics are significantly different from those of SFRs and can lead to major differences in fuel cycle impacts. The goal of this study was not to draw general conclusions based on a direct comparison of two very specific point designs for an SFR and MSFR, but rather to use this example MSFR design and associated parametric studies to gain insight into the key technology characteristics that impact fuel cycle performance as it relates to resource utilization (i.e., uranium consumption). The MSFR reactor physics, fission product removal, and fuel salt mass flows were modeled using Argonne’s recently-developed molten salt reactor (MSR) analysis tools while the time-dependent fuel cycle performance of this specific reactor was compared to that of a representative SFR design using the fuel cycle system dynamics code DYMOND.

chloride salt↗

Stationary Liquid Fuel Fast Reactor

For effective burning of hazardous transuranic (TRU) elements of used nuclear fuel, a transformational advanced reactor concept named SLFFR (Stationary Liquid Fuel Fast Reactor) was proposed based on stationary molten metallic fuel. The fuel enters the reactor vessel in a solid form, and then it is heated to molten temperature in a small melting heater. The fuel is contained within a closed, thick container with penetrating coolant channels, and thus it is not mixed with coolant nor flow through the primary heat transfer circuit. The makeup fuel is semi- continuously added to the system, and thus a very small excess reactivity is required. Gaseous fission products are also removed continuously, and a fraction of the fuel is periodically drawn off from the fuel container to a processing facility where non-gaseous mixed fission products and other impurities are removed and then the cleaned fuel is recycled into the fuel container. A reference core design and a preliminary plant system design of a 1000 MWt TRU- burning SLFFR concept were developed using TRU-Ce-Co fuel, Ta-10W fuel container, and sodium coolant. Conservative design approaches were adopted to stay within the current material performance database. Detailed neutronics and thermal-fluidic analyses were performed to develop a reference core design. Region-dependent 33-group cross sections were generated based on the ENDF/B-VII.0 data using the MC2-3 code. Core and fuel cycle analyses were performed in theta-r-z geometries using the DIF3D and REBUS-3 codes. Reactivity coefficients and kinetics parameters were calculated using the VARI3D perturbation theory code. Thermo-fluidic analyses were performed using the ANSYS FLUENT computational fluid dynamics (CFD) code. Figure 0.1 shows a schematic radial layout of the reference 1000 MWt SLFFR core, and Table 0.1 summarizes the main design parameters of SLFFR-1000 loop plant. The fuel container is a 2.5 cm thick cylinder with an inner radius of 87.5 cm. The fuel container is penetrated by twelve hexagonal control assembly (CA) guide tubes, each of which has 3.0 mm thickness and 69.4 mm flat-to-flat outer distance. The distance between two neighboring CA guide tube is selected to be 26 cm to provide an adequate space for CA driving systems. The fuel container has 18181 penetrating coolant tubes of 6.0 mm inner diameter and 2.0 mm thickness. The coolant tubes are arranged in a triangular lattice with a lattice pitch of 1.21 cm. The fuel, structure, and coolant volume fractions inside the fuel container are 0.386, 0.383, and 0.231, respectively. Separate steel reflectors and B4C shields are used outside of the fuel container. Six gas expansion modules (GEMs) of 5.0 cm thickness are introduced in the radial reflector region. Between the radial reflector and the fuel container is a 2.5 cm sodium gap. The TRU inventory at the beginning of equilibrium cycle (BOEC) is 5081 kg, whereas the TRU inventory at the beginning of life (BOL) was 3541 kg. This is because the equilibrium cycle fuel contains a significantly smaller fissile fraction than the LWR TRU feed. The fuel inventory at BOEC is composed of 34.0 a/o TRU, 41.4 a/o Ce, 23.6 a/o Co, and 1.03 a/o solid fission products. Since uranium-free fuel is used, a theoretical maximum TRU consumption rate of 1.011 kg/day is achieved. The semi-continuous fuel cycle based on the 300-batch, 1- day cycle approximation yields a burnup reactivity loss of 26 pcm/day, and requires a daily reprocessing of 32.5 kg of SLFFR fuel. This yields a daily TRU charge rate of 17.45 kg, including a makeup TRU feed of 1.011 kg recovered from the LWR used fuel. The charged TRU-Ce-Co fuel is composed of 34.4 a/o TRU, 40.6 a/o Ce, and 25.0 a/o Co.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Investigations of Properties of {sup 89}Y Levels with Reactor Fast Neutrons

By employing a beam of reactor fast neutrons, the spectrum of gamma rays up to an energy of 4.6MeV and their angular distributions with respect to the neutron-beamaxis aremeasured in the reaction {sup 89}Y(n, n'γ). The multipolarities and multipole-mixture parameters for 34 gamma transitions and the spin–parities J{sup π} of states excited in this reaction are determined. The lifetimes of the lowest 32 levels of 89Y were measured by the Doppler shift attenuation method, and the reduced probabilities for the respective gamma transitions were calculated. Levels of the K{sup π} = +5/2{sup +} and K{sup π} = −7/2{sup +} bands associated with, respectively, prolate and oblate deformation shapes are found in {sup 89}Y at low excitation energies.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Graphite Moderation in Fast Reactors

With the renewed interest in designing and building a fast test reactor in the U.S., several new reactor concepts have been emerging. Although the main mission of a fast test reactor would be to enable high fast flux irradiation capability, there could be added value for such a fast test reactor to also offer thermal neutron irradiation capabilities. As such, several of these concepts considered the use of a moderator material in a Sodium-cooled Fast Reactor (SFR), which is claimed to also offer benefits with respect of mass of fuel required. The work discussed in this paper focuses on exploring and assessing the benefits and challenges resulting from making use of thermalized neutrons to reduce the critical fuel mass. The analyses are performed for a graphite moderating material, using a simple core model to easily identify the phenomena observed. It is found that it is necessary to reduce the fuel enrichment near the moderated regions in order to avoid unacceptable power peaking. In the end, use of moderating materials outside a SFR core does not provide significant benefit in term of fuel volume reduction, but allows for a noticeable reduction of the mass of fissile material needed. However, it also implies a number of additional challenges which are highlighted in this paper.

core optimization↗

GIF sodium fast reactor project R and D on safety and operation

The 'Safety and Operation' project is started in 2009 within the framework of Generation-IV International Forum (GIF) Sodium Fast Reactor (SFR) research and development program. In the safety area, the project involves R and D activities on phenomenological model development and experimental programs, conceptual studies in support of the design of safety provisions, preliminary assessment of safety systems, framework and methods for analysis of safety architecture. In the operation area, the project involves R and D activities on fast reactors safety tests and analysis of reactor operations, feedback from decommissioning, in-service inspection technique development, under-sodium viewing and sodium chemistry. This paper presents a summary of such activities and the main achievements. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Mobile heat pipe cooled fast reactor system

A mobile heat pipe cooled fast nuclear reactor may be configured for transportation to remote locations and may be able to provide 0.5 to 2 megawatts of power. The mobile heat pipe cooled fast reactor may contain a plurality of heat pipes that are proximate to a plurality of fuel pins inside the reactor. The plurality of heat pipes may extend out of the reactor. The reactor may be configured to be placed in a standard shipping container, and may further be configured to be contained within a cask and attached to a skid for easier transportation.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Mobile heat pipe cooled fast reactor system

A mobile heat pipe cooled fast nuclear reactor may be configured for transportation to remote locations and may be able to provide 0.5 to 2 megawatts of power. The mobile heat pipe cooled fast reactor may contain a plurality of heat pipes that are proximate to a plurality of fuel pins inside the reactor. The plurality of heat pipes may extend out of the reactor. The reactor may be configured to be placed in a standard shipping container, and may further be configured to be contained within a cask and attached to a skid for easier transportation.

McClure, Patrick Ray↗

Innovative technologies on fuel assemblies cleaning for sodium fast reactors: First considerations on cleaning process

Within the framework of Sodium Fast Reactor development, innovative fuel assembly cleaning operations are investigated to meet the GEN IV goals of safety and of process development. One of the challenges is to mitigate the Sodium Water Reaction currently used in these processes. The potential applications of aqueous solutions of mineral salts (including the possibility of using redox chemical reactions) to mitigate the Sodium Water Reaction are considered in a first part and a new experimental bench, dedicated to this study, is described. Anhydrous alternative options based on Na/CO{sub 2} interaction are also presented. Then, in a second part, a functional study conducted on the cleaning pit is proposed. Based on experimental feedback, some calculations are carried out to estimate the sodium inventory on the fuel elements, and physical methods like hot inert gas sweeping to reduce this inventory are also presented. Finally, the implementation of these innovative solutions in cleaning pits is studied in regard to the expected performances. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

An Efficient 1-D Thermal Stratification Model for Pool-Type Sodium-Cooled Fast Reactors

Investigating thermal stratification in the upper plenum of a sodium fast reactor (SFR) is presently a technology gap in SFR safety analysis. Understanding thermal stratification will promote safe operation of the SFR before its commercial deployment. Stratified layers of liquid sodium with a large vertical temperature gradient could be established in the upper plenum of an SFR during a down-power or a loss-of-flow transient. These stratified layers are unstable and could result in uncertainties for the core safety of an SFR. In order to predict the occurrence of the thermal stratification efficiently, we developed a one-dimensional (1-D) transport model to estimate the temperature profile of the ambient fluid in the upper plenum. This model demands much less computational effort than computational fluid dynamics (CFD) codes and provides calculations with higher fidelity than historical system-level codes. Two flow conditions were considered separately in the current study depending on if in-vessel components are presented in the upper plenum. For the condition where in-vessel components, specifically the upper internal structure, are presented, we assumed that the impinging sodium was evenly dispersed in the ambient fluid within the distance between the bottom of the in-vessel component and the jet inlet surface. For the condition where no in-vessel components are presented, we assumed that the impinging sodium was evenly dispersed in the ambient fluid within the jet length, which was determined through data-driven trainings. The newly developed 1-D model showed similar performance with the CFD model in both cases. However, due to the assumption of flat profiles of the impinging jet axial dispersion rate, nonnegligible discrepancies between the 1-D prediction and the measured data were observed.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Validation of Fast Reactor Depletion Tools Using EBR-II Measured Data

The validation of simulation tools for calculating fuel depletion and evolution in fast reactors is vital for design, licensing, deployment, operations, and material accountancy. The Physics Analysis Database (PADB) and Analytical Laboratory (AL) database contain measured data collected from Experimental Breeder Reactor II (EBR-II) and were used to validate the most recent versions of the Argonne Reactor Computation (ARC) tool suite and ORIGEN-S for calculating isotopic compositions in irradiated fast reactor fuel. The PADB contains important modeling and operational information about the EBR-II core design, fuel cycle, and analytical results from the legacy versions of the ARC tool suite. The AL database contains the measured isotopic compositions of irradiated samples taken from core subassemblies. A new procedure was developed for the ARC tool suite to perform the EBR-II depletion simulation, as well as to perform more detailed isotopic calculations using ORIGEN-S calculations by coupling it with the ARC suite. Both the ARC and ARC-ORIGEN results were compared with the AL measured data for all relevant samples and showed good agreement for the major actinides. Good agreement with measured data was also achieved using the ARC-ORIGEN approach for several fission products.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Multi-principal element alloys for fast reactor cladding applications

Given the extensive list of multi-principal element alloys (MPEAs) within literature and the overwhelming number of alloys that can be made from only a handful of elements, this article proposes a methodology for prioritizing alloys for use as cladding within advanced reactors. This paper applies neutronic, mechanical, and chemical assessments to a collection of MPEAs available within literature for use as advanced reactor cladding. The results are compared to a reference design of HT9, a ferritic/martensitic steel, for employed in sodium-cooled fast reactor. Mechanical assessments determined pressure limits for a thin-walled tube pressure boundary, thus relating the material's mechanical properties to a minimum acceptable wall thickness. Neutronic analyses reveal a maximum allowable wall thickness that a given material must meet to provide a level of neutronic economy that is equivalent to than that of HT9. Lastly, each alloying element is compared to typical fission products found in a fast reactor fuels to mitigate deleterious phenomena such as fuel-cladding chemical interactions (FCCI). These analyses indicate that Mo-Nb-Ti-V-based alloys are likely to be advantageous and that the inclusion of elements with a high neutronic penalty (e.g., Hf) could be considered with minimal consequences.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Shielding Design for Prototype Generation-IV Sodium-Cooled Fast Reactor

A Prototype Generation-IV Sodium-cooled Fast Reactor (PGSFR) with 150 MWe power rating is being developed jointly by the Korea Atomic Energy Research Institute (KAERI) and Argonne National Laboratory (ANL). KAERI is responsible for the overall project with the ANL contributions integrated into the KAERI activities. Shielding concept of PGSFR was developed to ensure that the safety limit on internal structural damage and working personnel received dose is not exceeded. The first part evaluated the Displacement Per Atoms (DPA) and fast neutron fluence on the structures inside the reactor vessel, such as lower grid, Upper Internal Structure (UIS), barrel, Redan, and reactor vessels. The analysis determined the thickness of shields required to satisfy the DPA and fast fluence limit. The second part of the shielding analysis evaluated the radiation dose rate above the reactor head due to the primary sodium activation inside the reactor vessel. The analysis determined the necessary thickness of reactor head and additional shield to ensure that the dose rate received by personnel working on top of the reactor is below the safety limit. The last part of the shielding analysis investigated the dose rate received by personnel working near the secondary loop. The secondary sodium is activated inside the Intermediate heat exchanger (IHX). The activated secondary sodium flows out of the reactor vessel and emits high energy photons along the way. The shielding designs both inside the reactor vessel and around the pipes of the secondary loop were investigated. The shielding concept for the PGSFR was developed to minimize radiation exposure to plant personnel and the irradiation damage of the internal structural components. The damage of the internal structural components are mainly due to the loss of the ductility by the neutron irradiation, and the activated gammas of primary and secondary sodium coolants are the major radiation sources that are required to be shielded. Thicker and denser shielding structures are favorable to reduce the radiation dose and protect personnel who work in the plant; however, which enlarges the in-vessel space to accommodate the shielding structures. Thus, in order to install the shielding structures in a reasonable reactor to satisfy the DPA or dose rate limit size, the PGSFR shielding parameters were determined from the sensitivity study, which includes the compositions of the shielding materials and dimensions. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

About the Impact of the Unresolved Resonance Region in Monte Carlo Simulations of Sodium Fast Reactors

In the last few years, and within the framework of different European projects, KENO-VI code from SCALE system has been employed to perform detailed continuous-energy Mon-te Carlo transport calculations for advanced fast reactors. The core characterization of both the sodium-cooled ASTRID and the lead-cooled ALFRED reactors was performed during the FP7 cross-cutting ESNII+ project; more recently, core calculations for the sodium-cooled Superphénix reactor and the improved European Sodium Fast Reactor design were performed within the HORIZON2020 ESFR-SMART project. In all cases, the effective multiplication factor predicted by KENO-VI was systematically higher (around 400-500 pcm) than the values computed by MCNP and Serpent Monte Carlo codes, using the same nu-clear data library.In order to provide insight into the origin of the observed discrepancies, a simplified 2D MOX-fueled SFR pin-cell benchmark has been launched. The multiplication factor, as well as 1-group and VITAMINJ 175-group cross-sections computed by KENO-VI, Serpent and MCNP codes employing ENDF/B-VII.1 data library, have been compared.Significant differences between KENO-VI and the other codes have been found in the un-resolved resonance regions of 239Pu and 241Pu capture and production cross sections, while negligible differences appeared outside those energy ranges. On the other hand, calculations without using probability tables have shown very good agreement. Quantita-tive comparison is presented and analyzed, along with a discussion of the impact of the probability-table treatment in the three codes for MOX-fueled systems with typical SFR spectrum.

Jimenez carrascosa, A↗

Irradiation performance of nonfertile (Pu-MA-Zr) fast reactor metal fuels

This work was part of a program begun in 2001 to develop advanced nuclear fuels, originally as carriers for plutonium and minor actinides (neptunium, curium, and americium) taken from spent commercial light-water reactors (LWR) so that the plutonium and minor actinides could be ‘burned’ or transmuted in an accelerator or a fast nuclear reactor. A central part of these experiment programs has been the development of advanced fast reactor fuels, because a fast reactor was considered the most efficient vehicle to transmute the actinide waste products, and metallic fuels is a central focus of these tests. An experiment design was developed in which a thermal test reactor, the Advanced Test Reactor (ATR), was used to test small fuel pin prototypes, by creating areas in the core shielded by cadmium filters to produce a largely epithermal and fast neutron spectrum environment in which the pins could be irradiated. The results of non-fertile metallic fuel (no uranium) tests are presented here. Pu-Am-Np-Zr fuels were irradiated to fission densities up to 33 × 10 20 fission/cm 3 and Pu-239 depletions of up to 39%. The depletions were created by roughly 2/3 by fission and 1/3 by transmutation neutron capture. Up to five fuel ‘rodlets’ were irradiated in three sealed capsules stacked axially in the core, and the peak cladding temperatures ranged from 300°C to 500°C, depending on axial location as those near the core centerline are operating hotter and to higher fission densities. Several post-irradiation examinations (precision gamma scanning and fission gas release) were similar to other historical metal fuel experiments in fast reactors. However, optical metallography indicated that two of the rodlets had breached. The exact reasons are unclear. Due to the design of this irradiation experiment a rodlet breach could have increased the temperature in others in the same capsule by contaminating the thermal gap helium with heavier and less conductive fission product gases. Finally, some of those rodlets showed high amounts of fuel/cladding chemical interaction (FCCI).

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Enhanced Performance Fast Reactors with Engineered Passive Safety Systems

This report summarizes the work and results of NEUP Project #15-8251, "Enhanced Performance Fast Reactors with Engineered Passive Safety System," performed from 2015-2018 at UC Berkeley and Argonne National Laboratory. This project concerns the incorporation of a novel engineered passive safety system, called the Autonomous Reactivity Control (ARC) system, into Sodium-cooled Fast Reactors (SFRs) to improve their transient and economic performance. The first part of this project consisted of fleshing out the basic principles and the manufacturing process for an SFR fuel assembly with the ARC system installed, with the details provided in high-quality, step-by-step CAD drawings. Once the detailed design is laid out, high-fidelity simulations were performed to optimize the dimensions of important ARC system components and to quantify the standalone time-response of ARC systems in a typical SFR environment. These high-fidelity simulations were used to create reduced-order models of ARC system response which could be incorporated into the SAS4A/SASSYS-1 whole-core transient models. In order to accurately account for the time-response of ARC systems in whole-core transient simulations, modifications were made to the SAS4A/SASSYS-1 transient code. These new capabilities were tested and incorporated into the production version of the code, and have been used extensively in this analysis. Before performing whole-core transient calculations, the two reference cores selected for this study to cover a wide design space were simulated and characterized. The two reference cores, (1) a medium-sized oxide-fueled Advanced Burner Reactor and (2) a large metal-fueled Breed-and-Burn core, challenge conventional means of achieving passive safety. Because the two cores vary substantially, simulating the ARC system in both allows for conclusions to be drawn about the applicability of ARC systems in different SFRs. Once both cores were fully characterized, transient calculations were performed to understand the complicated interplay between the ARC system and other inherent reactivity feedback mechanisms. By performing parametric studies of the transient behavior, ARC system designs that best improve transient performance in each core were identified. Once transient improvements were established, the transient calculations were extended to improve reactor economics through design modifications. Upon establishing the potential benefits of ARC system inclusion, the study examines the negative neutronic implications of incorporating ARC systems into the reference cores. The study concludes by discussing a number of knowledge gaps that exist which may have important implications for ARC system implementation. Ultimately, the results of this project indicate that ARC systems may provide an effective means to improve transient performance in certain types of systems. The transient simulations in the oxide Advanced Burner Reactor showed that significant margin to coolant boiling and fuel melting could be gained through the use of a properly designed ARC system, thus improving inherent safety. While oscillatory behavior was induced in the transient response for certain combinations of ARC system parameters, the oscillation-free design space that can be effectively used to improve performance was found to be large, and the additional margin was demonstrated to allow economical improvements to the core design. Conversely, difficulties were encountered in the Breed-and-Burn core due to fundamental aspects of the core design. The combination of a particularly strong positive coolant void feedback and the use of metallic fuel allowed for diverging oscillations to manifest in response to certain transient initiators, and in the end it was found that the current ARC system design could not simultaneously enable passive safety in all transients examined. In order for complete passive safety to be achieved, a mechanism for slowing the reverse actuation of ARC systems is necessary. Regardless, the standard ARC system was able to improve the performance of two out of the three examined transients by increasing the margin to boiling in Loss of Heat Sink transients and avoiding boiling in Transient Overpower accidents. Additionally, no significant barriers to implementation were found, although the issue of tritium production should be closely monitored in any core incorporating ARC systems. Still, a number of technology gaps exist, and these are discussed at the conclusion of the report to recommend directions for future work.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗