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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 163 records · Page 9
All sourcesNASA NTRSDOE OSTI
DOE OSTI2023

Spiroligomer‐Based Macrocycles for Atomically Precise Membranes

Abstract Here, we report a new class of peptidomimetic macrocycles with well‐defined three‐dimensional structures and low conformational flexibility. They are assembled from fused‐ring spiro‐ladder oligomers (spiroligomers) by modular solid‐phase synthesis. Two‐dimensional nuclear magnetic resonance confirms their shape persistency. Triangular macrocycles of tunable sizes assemble into membranes with atomically precise pores, which exhibit size and shape‐dependent molecular sieving towards a series of structurally similar compounds. The exceptional structural diversity and stability of spiroligomer‐based macrocycles will be explored for more applications.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
NASA NTRS1988

Influence of the interplanetary magnetic field orientation on polar cap ion trajectories - Energy gain and drift effects

The influence of the interplanetary magnetic field (IMF) orientation on the transport of low-energy ions injected from the ionosphere is investigated using three-dimensional particle codes. It is shown that, unlike the auroral zone outflow, the ions originating from the polar cap region exhibit drastically different drift paths during southward and northward IMF. During southward IMF orientation, a 'two-cell' convection pattern prevails in the ionosphere, and three-dimensional simulations of ion trajectories indicate a preferential trapping of the light ions H(+) in the central plasma sheet, due to the wide azimuthal dispersion of the heavy ions, O(+). In contrast, for northward IMF orientation, the 'four-cell' potential distribution predicted in the ionosphere imposes a temporary ion drift toward higher L shells in the central polar cap. In this case, while the light ions can escape into the magnetotail, the heavy ions can remain trapped, featuring more intense acceleration (from a few electron volts up to the keV range) followed by precipitation at high invariant latitudes, as a consequence of their further travel into the tail.

Delcourt, D. C.↗
NASA NTRSDate not supplied

3-D Mapping of the Magnetic Field in the Active Region by the CLASP2.1 Rocket Experiment

Comprehensive magnetic field measurements of the solar atmosphere are crucial for understanding energy transport from the photosphere to the corona and its dissipation. However, observations of the magnetic field in the chromosphere and the upper atmospheric layers above the chromosphere, where the gas pressure dominance changes from (β>1) to magnetic pressure dominance (β<1), are overwhelmingly lacking. Therefore, we have focused on the polarization of ultraviolet radiation emitted from the upper chromosphere and transition layer and have conducted the Japan-U.S.-EU observation rocket experiment CLASP in order to demonstrate its usefulness. In CLASP2.1 conducted on October 8, 2021, scan observations were made at 16 locations in the active region, and Stokes (intensity $I$, linearly polarized $Q$, $U$, circularly polarized $V$) spectra in the 280~nm wavelength range were obtained. Looking at the observed region with AIA 171~{¥AA} on board the SDO satellite, we see that it consists of a region where a structure corresponding to the foot of a high-temperature loop called moss (moss) is seen, and a region where a low-temperature loop spreading from a sunspot is seen. We focused on the ionized magnesium $h$ & $k$ lines (emitted from the middle and uppermost of the chromosphere) and the manganese lines (emitted from the low part of the chromosphere), which show particularly prominent circular polarization, and derived the line-of-sight magnetic fields in the low, middle and uppermost parts of the chromosphere by applying weak field approximation to them. Furthermore, by combining the results with observations by the Solar Optical Telescope onboard the solar observing satellite HINODE, we obtained three-dimensional information on the magnetic field in the active region from the photosphere to the uppermost part of the chromosphere. In general, the magnetic field in the active region becomes weaker and smoother as one goes up in the sky, as reported by the CLASP2 observation (Ishikawa et al. 2021). However, in some regions, polarity reversal was observed only in the uppermost part of the chromosphere, and comparison with high spatial resolution transition layer and coronal images recorded by SDO/AIA revealed the connection between the magnetic field structure in the chromosphere and coronal loops.

R. Ishikawa↗
DOE OSTI2023

Synthesis and physical properties of a new layered ferromagnet Cr 1.21 Te 2

Single crystals of a new layered compound, Cr 1.21 Te 2 , were synthesized via a vapor transport method. The crystal structure and physical properties were characterized by single crystal and powder x-ray diffraction, temperature- and field-dependent magnetization, zero-field heat capacity, and angle-resolved photoemission spectroscopy. Cr 1.21 Te 2 , containing two Cr sites, crystalizes in a trigonal structure with a space group P-3 (No. 147). The Cr site in the interstitial layer is partially occupied. Physical property characterizations indicate that Cr 1.21 Te 2 is metallic with hole pockets at the Fermi energy and undergoes a ferromagnetic phase transition at ~ 173 K. The magnetic moments align along the c axis in the ferromagnetic state. Based on low-temperature magnetization, the spin stiffness constant, D, and spin excitation gap, Δ , were estimated according to Bloch's law to be D = 94 ± 17 meV Å 2 and Δ = 0.45 ± 0.33 meV, suggesting its possible application as a low dimensional ferromagnet.

36 MATERIALS SCIENCE↗
DOE OSTI2022

Electronic and magnetic properties of quasi-one-dimensional osmium halide OsCl 4

Using ab initio density functional theory, we study the electronic and magnetic properties of the van der Waals chain material OsCl 4 . In the nonmagnetic state, a strongly anisotropic band structure was observed, in agreement with its anticipated one-dimensional crystal geometry. Based on Wannier functions, we found that the four electrons of the 5d Os atom form a low-spin S = 1 state, with a large crystal field between the d xz/yz and d xy orbitals, corresponding to a strong Jahn–Teller distortion (Q 3 < 0). As a consequence, the magnetic properties are mainly contributed by the d xz/yz states. Furthermore, when a Mott gap develops after the introduction of the Hubbard U and Hund coupling J, we found that the staggered spin order is the most likely magnetic state, namely, spins arranged as (↑-↓-↑-↓) with π wavevector along the chain. In addition, the energy differences between various spin states are small, suggesting a weak magnetic exchange coupling along the chain. Overall, our results provide guidance to experimentalists and theorists working on quasi-one-dimensional osmium halides chain materials.

36 MATERIALS SCIENCE↗
NASA NTRS1990

Mid- and low-latitude model of thermospheric emissions. I - O(+) (2P) 7320 A and N2 (2P) 3371 A

This paper presents an interhemispherically coupled model of airglow emissions of the O(+) (2P) metastable state (7320 A) and the 0-0 band of the N2 second positive system (3371 A), covering mid- and low-latitudes. The model produces volume emission rates as a function of altitude, latitude, longitude, and local time for any selected data and solar and magnetic conditions, and, thus, can be used to provide three-dimensional maps of the selected emission for comparison with data obtained from orbiting vehicles. The semiglobal graphical maps of the 7320 A and 3371 A emissions illustrate the seasonal, diurnal, and solar cyclic variations on a scale that covers mid- and low-latitudes, as well as the effects of interhemispheric coupling (conjugate photoelectrons). It is shown that, in both cases, conjugate photoelectrons result in excitation at mid- to high- nighttime-latitudes in the winter hemisphere.

Torr, Marsha R.↗
NASA NTRS1989

Low-frequency electrostatic instabilities excited by injections of an electron beam in space

One-dimensional particle simulations have been carried out to study the low-frequency broadband electrostatic noise that propagates almost perpendicularly from the magnetic field line when a nonrelativistic electron beam is injected into space from a spacecraft. For T(e) = T(i) the electrostatic ion cyclotron waves appear as well as the waves near the lower hybrid frequency. When the magnetic field is reduced so that Omega(e) is much less than omega(pe) in a nonisothermal plasma, T(e) greater than T(i) oblique ion acoustic instabilities appear to propagate almost perpendicular to the magnetic field. In addition, a very low frequency mode at omega much less than Omega(i) is found to be generated by the electrons flowing into the conductor. Both the injected beam electrons as well as the ambient electrons flowing into the spacecraft are responsible for generating those instabilities, which accelerate ions perpendicular to the magnetic field.

Hwang, Y. S.↗
DOE OSTI2024

High-temperature quantum valley Hall effect with quantized resistance and a topological switch

Edge states of a topological insulator can be used to explore fundamental science emerging at the interface of low dimensionality and topology. Achieving a robust conductance quantization, however, has proven challenging for helical edge states. In this work, we show wide resistance plateaus in kink states—a manifestation of the quantum valley Hall effect in Bernal bilayer graphene—quantized to the predicted value at zero magnetic field. The plateau resistance has a very weak temperature dependence up to 50 kelvin and is flat within a dc bias window of tens of millivolts. We demonstrate the electrical operation of a topology-controlled switch with an on/off ratio of 200. These results demonstrate the robustness and tunability of the kink states and its promise in constructing electron quantum optics devices.

Science & Technology - Other Topics↗
DOE OSTI2025

Shubnikov–de Haas oscillations reaching the quantum limit in two-dimensional electron systems at SrTi⁢O 3 (111) interfaces

Transition metal oxides in the (111) orientation have been predicted to harbor topological phases and unconventional quantum states because of their hexagonal crystal symmetry and strong interactions between charge, spin, and orbital degrees of freedom. We report Shubnikov–de Haas oscillations into the quantum limit at magnetic fields up to 35 T in high-mobility (>20 000 c⁢m 2 V −1 s −1 ) two-dimensional electron liquids at (111)-oriented SrTi⁢O 3 interfaces with controllable carrier densities. Spin splitting is observed at low Landau levels, which is attributed to the interplay between the Zeeman splitting and Rashba spin-orbit coupling according to our theoretical modeling, yielding Landé factor 𝑔 = 0.29 and Rashba coefficient 𝛼 = 0.6 meV nm. Furthermore, at high magnetic field after the system reaches the lowest Landau level, the temperature dependence of the resistance shows a metallic to insulating state transition with the magnetoresistance changing significantly from a primarily quadratic to a large linear field dependence.

Magnetoresistance↗
NASA NTRS1986

Three-dimensional magnetostatic models of the large-scale corona

A special class of magnetostatic equilibria is described, which are mathematically simple and yet sufficiently versatile so as to fit any arbitrary normal magnetic flux prescribed at the photosphere. With these solutions, the corona can be modeled with precisely the same mathematically simple procedure as has previously been done with potential fields. The magnetostatic model predicts, in addition to the coronal magnetic field, the three dimensional coronal density which can be compared with coronagraph observations.

Bogdan, T. J.↗
DOE OSTI2023

Bond-dependent anisotropy and magnon decay in cobalt-based Kitaev triangular antiferromagnet

Following tremendous success of the graphene-derived fundamental and applied research, the magnetic van der Waals materials that can be cleaved into monolayer two-dimensional atomic crystals have emerged as a new platform in the studies of low-dimensional physics and in the design of artificial heterostructures with novel properties. Because of that, the family of dihalides and trihalides of the 3d transition group receive a strong renewed interest. Together with our experimental collaborators, we have investigated the novel dynamical properties of one of such promising material CoI 2 , and demonstrated that spin excitations in it are prone to substantial breakdown and complex level repulsion, the important quantum effects whose theoretical understanding has been significantly advanced by our group in the last two decades. Both phenomena are dramatically revealed by experiments and verified by the theory in our joint study, published in Nature Physics. Altogether, our results pave the way toward a new research direction for the magnetic van der Waals materials.

36 MATERIALS SCIENCE↗
NASA NTRS1982

Crustal interpretation of the MAGSAT data in the continental United States

The processing of MAGSAT scalar data to construct a crustal magnetic anomaly map over the continental U.S. involves removal of the reference field model, a path-by-path subtraction of a low order polynomial through a least-squares fit to reduce orbital offset errors, and a two dimensional spectral filtering to mitigate the spectral bias induced by the path-by-path orbital correction scheme. The resultant anomaly map shows reasonably good correlations with an aeromagnetic map derived from the project MAGNET. Prominent satellite magnetic anomalies are identified in terms of geological provinces and age boundaries. An inversion method was applied to MAGSAT data which produces both the Curie depth topography and laterally varying magnetic susceptibility of the crust. A contoured Curie depth map thus derived shows general agreements with a crustal thickness map based on seismic data.

Won, I. J.↗
DOE OSTI2025

Three-Dimensional Helical-Rotating Plasma Structures in Beam-Generated Partially Magnetized Plasmas

Azimuthal structures emerging in beam-generated partially magnetized plasmas are investigated using three-dimensional particle in cell-Monte Carlo collision simulations. Two distinct instability regimes are identified at low pressures. Furthermore, when the gas pressure is sufficiently high, quasineutrality is attained and 2D spiral-arm structures form as a result of the development of a lower-hybrid instability, resulting in enhanced cross-field transport. At lower pressures, quasineutrality is not achieved and a 3D helical-rotating plasma structure forms due to development of the diocotron instability. Analytical formulas are proposed for the critical threshold pressure between these regimes and for the rotation frequency of the helical structures. Preliminary experimental verification is provided.

Penning discharges↗
NASA NTRS1989

Self-consistent model of the low-latitude boundary layer

A simple, two-dimensional, steady state, viscous model of the dawnside and duskside low-latitude boundary layer is presented. The model described boundary layer currents, magnetic fields, and plasma flow in a self-consistent way. Coupling to the ionosphere via field-aligned currents and associated field-aligned potential drops governed by a simple conductance law are included in the model. The model equations are given and the results from the model are compared with observations.

Phan, T. D.↗
DOE OSTI2022

Bicircular Light Floquet Engineering of Magnetic Symmetry and Topology and Its Application to the Dirac Semimetal Cd 3 As 2

Here, we show that bicircular light (BCL) is a versatile way to control magnetic symmetries and topology in materials. The electric field of BCL, which is a superposition of two circularly polarized light waves with frequencies that are integer multiples of each other, traces out a rose pattern in the polarization plane that can be chosen to break selective symmetries, including spatial inversion. Using a realistic low-energy model, we theoretically demonstrate that the three-dimensional Dirac semimetal Cd 3 As 2 is a promising platform for BCL Floquet engineering. Without strain, BCL irradiation induces a transition to a noncentrosymmetric magnetic Weyl semimetal phase with tunable energy separation between the Weyl nodes. In the presence of strain, we predict the emergence of a magnetic topological crystalline insulator with exotic unpinned surface Dirac states that are protected by a combination of twofold rotation and time reversal (2') and can be controlled by light.

36 MATERIALS SCIENCE↗
NASA NTRS1992

The dynamics of low-beta plasma clouds as simulated by a three-dimensional, electromagnetic particle code

A 3D electromagnetic and relativistic particle simulation code is used to investigate the dynamics of low-beta plasma clouds moving perpendicular to an ambient magnetic field in vacuum and in a background plasma. The simulations show the formation of the space charge sheaths at the sides of the cloud with the associated polarization electric field which facilitate the cross-field propagation, as well as the sheaths at the front and rear end of the cloud caused by the larger ion Larmor radius, which allows ions to move ahead and lag behind the electrons as they gyrate. It is found that, in a background plasma, electron and ion sheaths expand along the magnetic field at the same rate, whereas in vacuum the electron sheath expands much faster than the ion sheath. Sheath clouds are accelerated up to relativistic energies, which indicates that artificial plasma clouds released in the ionosphere or magnetosphere may generate optical emissions as energetic sheath electrons scatter in the upper atmosphere.

Neubert, T.↗
DOE OSTI2022

Elucidating proximity magnetism through polarized neutron reflectometry and machine learning

Polarized neutron reflectometry is a powerful technique to interrogate the structures of multilayered magnetic materials with depth sensitivity and nanometer resolution. However, reflectometry profiles often inhabit a complicated objective function landscape using traditional fitting methods, posing a significant challenge for parameter retrieval. In this work, we develop a data-driven framework to recover the sample parameters from polarized neutron reflectometry data with minimal user intervention. We train a variational autoencoder to map reflectometry profiles with moderate experimental noise to an interpretable, low-dimensional space from which sample parameters can be extracted with high resolution. We apply our method to recover the scattering length density profiles of the topological insulator–ferromagnetic insulator heterostructure Bi2Se3/EuS exhibiting proximity magnetism in good agreement with the results of conventional fitting. We further analyze a more challenging reflectometry profile of the topological insulator–antiferromagnet heterostructure (Bi,Sb)2Te3/Cr2O3 and identify possible interfacial proximity magnetism in this material. We anticipate that the framework developed here can be applied to resolve hidden interfacial phenomena in a broad range of layered systems.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2023

Designing the stripe-ordered cuprate phase diagram through uniaxial-stress

The ability to efficiently control charge and spin in the cuprate high-temperature superconductors is crucial for fundamental research and underpins technological development. Here, we explore the tunability of magnetism, superconductivity and crystal structure in the stripe phase of the cuprate La 2-x Ba x CuO 4 , with x = 0.115 and 0.135, by employing temperature-dependent (down to 400 mK) muon-spin rotation and AC susceptibility, as well as X-ray scattering experiments under compressive uniaxial stress in the CuO 2 plane. A sixfold increase of the 3-dimensional (3D) superconducting critical temperature T c and a full recovery of the 3D phase coherence is observed in both samples with the application of extremely low uniaxial stress of 0.1 GPa. This finding demonstrates the removal of the well-known 1/8-anomaly of cuprates by uniaxial stress. On the other hand, the spin-stripe order temperature as well as the magnetic fraction at 400 mK show only a modest decrease under stress. Moreover, the onset temperatures of 3D superconductivity and spin-stripe order are very similar in the large stress regime. However, a substantial decrease of the magnetic volume fraction and a full suppression of the low-temperature tetragonal structure is found at elevated temperatures, which is a necessary condition for the development of the 3D superconducting phase with optimal T c . Our results evidence a remarkable cooperation between the long-range static spin-stripe order and the underlying crystalline order with the three-dimensional fully coherent superconductivity. Overall, these results suggest that the stripe- and the SC order may have a common physical mechanism.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗