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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 163 records · Page 9
All sourcesNASA NTRSDOE OSTI
DOE OSTI2023

Characterizing random-singlet state in two-dimensional frustrated quantum magnets and implications for the double perovskite Sr 2 CuTe 1 – x W x O 6

Motivated by the experimental observation of a nonmagnetic phase in compounds with frustration and disorder, we study the ground state of a spin-1/2 square-lattice Heisenberg model with randomly distributed nearest-neighbor J 1 and next-nearest-neighbor J 2 couplings. By using the density matrix renormalization group (DMRG) calculation on a cylinder system with a circumference of up to ten lattice sites, we identify a disordered phase between the Néel and stripe magnetic phase with growing J 2 /J 1 in the presence of strong bond randomness. The vanished spin-freezing parameter indicates the absence of spin-glass order. The large-scale DMRG results unveil the size-scaling behaviors of the spin-freezing parameter, the power-law decay of the average spin correlation, and the exponential decay of the typical spin correlation, which all agree with the corresponding behavior in the one-dimensional random-singlet (RS) state and characterize the RS nature of this disordered phase. The DMRG simulation also provides insights and opportunities for characterizing a class of nonmagnetic states in two-dimensional frustrated magnets with disorder. Here, we also compare with existing experiments and suggest more measurements for understanding the spin-liquid-like behaviors in the double perovskite Sr 2 CuTe 1–x W x O 6 .

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2020

Intertwined density waves in a metallic nickelate

Nickelates are a rich class of materials, ranging from insulating magnets to superconductors. But for stoichiometric materials, insulating behavior is the norm, as for most late transition metal oxides. Notable exceptions are the 3D perovskite LaNiO 3 , an unconventional paramagnetic metal, and the layered Ruddlesden-Popper phases R 4 Ni 3 O 10 , (R = La, Pr, Nd). The latter are particularly intriguing because they exhibit an unusual metal-to-metal transition. Here, we demonstrate that this transition results from an incommensurate density wave with both charge and magnetic character that lies closer in its behavior to the metallic density wave seen in chromium metal than the insulating stripes typically found in single-layer nickelates like La 2-x Sr x NiO 4 . We identify these intertwined density waves as being Fermi surface-driven, revealing a novel ordering mechanism in this nickelate that reflects a coupling among charge, spin, and lattice degrees of freedom that differs not only from the single-layer materials, but from the 3D perovskites as well.

36 MATERIALS SCIENCE↗
DOE OSTI2025

Phase diagram of a bilayer superconductor under an in-plane magnetic field

We study a double layer superconductor in the presence of a parallel magnetic field Bby obtaining self-consistent solutions of the Bogoliubov-de Gennes equations, and also using the Pakrovsky- Talapov model for the free energy expressed in terms of the relative phase, namely the difference in the phases of the superconducting order parameters in the two layers. We find that with increasing B, a continuous transition occurs from the Bardeen-Cooper-Schrieffer (BCS) state, where the relative phase is constant, into a state which contains stripes of the BCS state separated by localized vortices in the relative phase. This state is predicted to manifest through oscillations in the amplitude of the superconducting gap and an alternating pattern of supercurrents. With increasing B, the BCS stripe state continuously evolves into the Fulde-Ferrell-Larkin-Ovchinnikov state with linearly varying relative phase and a constant gap amplitude. Furthermore, these predictions apply to superconductivity in bilayer transition-metal-dichalcogenide systems with Ising spin-orbit coupling, and ought to be testable in a recently studied experimental system.

2-dimensional systems↗
DOE OSTI2025

Synthesis and Self-Assembly of Monodisperse Graphene Nanoribbons: Access to Submicron Architectures with Long-Range Order and Uniform Orientation

Fabricating organic semiconducting materials into large-scale well-organized architectures is critical for building high performance molecular electronics. While graphene nanoribbons (GNRs) hold enormous promise for various device applications, their assembly into a well-structured monolayer or multilayer architecture poses a substantial challenge. Here we report the preparation of length-defined monodisperse GNRs via the integrated iterative binomial synthesis (IIBS) strategy and their self-assembly into submicron-architectures with long-range order, uniform orientation as well as regular layers. Further, the use of short alkyl side chains benefits forming stable multi-layers through interlocking structures. By changing the length and backbone shapes of these monodisperse GNRs, various three-dimensional assemblies including multilayer stripes, monolayer stripes, and nanowires, can be achieved, leading to different photophysical properties and band gaps. The discovery of these intriguing self-assembly behaviors of length-defined GNRs is expected to open the door for various future applications.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2022

SrV 0.3 Fe 0.7 O 2.8 : A Vacancy-Ordered Fe-Based Perovskite Exhibiting Room-Temperature Magnetoresistance

We report room-temperature (RT) magnetoresistance (MR) in a novel Fe-based perovskite, SrV 0.3 Fe 0.7 O 2.8 . This compound contains ordered oxygen vacancies in every fifth primitive perovskite (111)p plane, leading to a layered structure consisting of triple-octahedral and double-tetrahedral layers. Along with the oxygen vacancies, the transition-metal ions are also ordered: the octahedral sites are occupied by 100% of Fe ions, while the tetrahedral sites are occupied by 25% of Fe ions and 75% of V ions. As a result, SrV 0.3 Fe 0.7 O 2.8 forms a magnetically striped lattice in which the octahedral layers with 100% of magnetic Fe ions are separated by the diluted magnetic layer. Finally, the compound exhibits weak ferromagnetism and shows a large negative MR (-5% at 3 T) at RT, despite the small saturation moment (0.4 μB/Fe atom). Thus, this type of layered compound is promising for further large MR by an increase of magnetization through chemical substitution.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
NASA NTRS2019

GOES-16 ABI Solar Reflective Channel Validation for Earth Science Application

This paper presents the validation results of GOES-16 Satellite's Advanced Baseline Imager (ABI) obtained from a reflectance-based field campaign undertaken at the Salar de Uyuni in Bolivia in June 2017. In situ ground measurements are used to characterize the surface reflectance and the atmosphere in order to constrain the radiative transfer code and predict at-sensor reflectance (also referred to as top-of-atmosphere (TOA) reflectance) to compare with concurrent GOES-16 ABI measurements. The five-day field campaign provided repeated TOA reflectance estimates, allowing assessment not only of the calibration accuracy of the ABI reflective channels 1, 2, 3, 5 and 6, but also of its stability over the duration of the campaign. The results show that the accuracy of the ABI reflective channels calibration is within specification for channels 1, 3, 5, and 6 - average biases within 2%; for channel 2 the bias is 5%. The estimated uncertainty on the derived biases is 2–2.4%. Some calibration stability issues were present in the ABI calibration at the time of the campaign: (i) a jump on the order of 2% in channels 1 and 6, coincident with an ABI solar calibration event, reflects an instability of the ABI gains in these channels, and (ii) short-term variability in channels 1 and 2 is due to striping (ABI detector-todetector calibration differences). Continued validation and subsequent reprocessing of ABI reflectance imagery would allow Earth scientists to fully benefit from the high spatial and spectral fidelity of the GOES-16 ABI diurnal measurements at the continental scale.

Joel McCorkel↗
DOE OSTI2023

BeyondPlanck: V. Minimal ADC Corrections for Planck LFI

We describe the correction procedure for Analog-to-Digital Converter (ADC) differential non-linearities (DNL) adopted in the Bayesian end-to-end BEYONDPLANCK analysis framework. This method is nearly identical to that developed for the official Planck Low Frequency Instrument (LFI) Data Processing Center (DPC) analysis, and relies on the binned rms noise profile of each detector data stream. However, rather than building the correction profile directly from the raw rms profile, we first fit a Gaussian to each significant ADC-induced rms decrement, and then derive the corresponding correction model from this smooth model. The main advantage of this approach is that only samples which are significantly affected by ADC DNLs are corrected, as opposed to the DPC approach in which the correction is applied to all samples, filtering out signals not associated with ADC DNLs. The new corrections are only applied to data for which there is a clear detection of the non-linearities, and for which they perform at least comparably with the DPC corrections. Out of a total of 88 LFI data streams (sky and reference load for each of the 44 detectors) we apply the new minimal ADC corrections in 25 cases, and maintain the DPC corrections in 8 cases. All these corrections are applied to 44 or 70 GHz channels, while, as in previous analyses, none of the 30 GHz ADCs show significant evidence of non-linearity. By comparing the BEYONDPLANCK and DPC ADC correction methods, we estimate that the residual ADC uncertainty is about two orders of magnitude below the total noise of both the 44 and 70 GHz channels, and their impact on current cosmological parameter estimation is small. However, we also show that non-idealities in the ADC corrections can generate sharp stripes in the final frequency maps, and these could be important for future joint analyses with the Planck High Frequency Instrument (HFI), Wilkinson Microwave Anisotropy Probe (WMAP), or other datasets. We therefore conclude that, although the existing corrections are adequate for LFI-based cosmological parameter analysis, further work on LFI ADC corrections is still warranted.

79 ASTRONOMY AND ASTROPHYSICS↗
NASA NTRS2012

The Atacama Cosmology Telescope: Data Characterization and Map Making

We present a description of the data reduction and mapmaking pipeline used for the 2008 observing season of the Atacama Cosmology Telescope (ACT). The data presented here at 148 GHz represent 12% or the 90 TB collected by ACT from 2007 to 2010. In 2008 we observed for 136 days, producing a total of 142h of data (11 TB for the 148 GHz band only), with a daily average of 10.5 h of observation. From these, 108.5 h were devoted to 850 sq deg stripe (11.2 h by 9 deg.1) centered on a declination of -52 deg.7, while 175 h were devoted to a 280 square deg stripe (4.5 h by 4 deg.8) centered at the celestial equator. We discuss sources of statistical and systematic noise, calibration, telescope pointing and data selection. Out of 1260 survey hours and 1024 detectors per array, 816 h and 593 effective detectors remain after data selection for this frequency band, yielding a 38 % survey efficiency. The total sensitivity in 2008, determined from the noise level between 5 Hz and 20 Hz in the time-ordered data stream (TOD), is 32 muK square root of s in CMB units. Atmospheric brightness fluctuations constitute the main contaminant in the data and dominate the detector and noise covariance at low frequencies in the TOD. The maps were made by solving the lease squares problem using the Preconditioned Conjugate Gradient method, incorporating the details of the detector and noise correlations. Cross-correlation with WMAP sky maps as well as analysis from simulations reveal the our maps are unbiased at l > 300. This paper accompanies the public release of the 148 GHz southern stripe maps from 2008. The techniques described here will be applied to future maps and data releases.

Duenner, Rolando↗
NASA NTRS1988

GaAs/GaAlAs distributed Bragg reflector laser with a focused ion beam, low dose dopant implanted grating

The performance of a GaAs/GaAlAs distributed Bragg reflector (DBR) laser using a focused ion beam implanted grating (FIB-DBR) is reported for the first time. Stripes of Si(2+) with a period of 2300 A and a dose about 10 to the 14th/sq cm are directly implanted into the passive large optical cavity layer to provide the distributed feedback. Surface-emitting light from the second-order grating is observed. Threshold current of 110 mA and single DBR mode operation from 20 to 40 C are obtained. The wavelength tuning rate with temperature is 0.8 A/C. The coupling coefficient is estimated to be 15/cm. The results show that FIB technology is practical for distributed feedback and DBR lasers and optoelectronic integrated circuits.

Wu, M. C.↗
NASA NTRS1993

Vertical-Bloch-Line Memory

Vertical-Bloch-line memory is developmental very-large-scale integrated-circuit block-access magnetic memory. Stores data in form of localized pairs of twists (VBL pairs) in magnetic field at edge of ferromagnetic domain in each stripe. Presence or absence of VBL pair at bit position denotes one or zero, respectively. Offers advantages of resistance to ionizing radiation, potential areal storage density approximately less than 1 Gb/cm squared, data rates approximately less than 1 Gb/s, and average access times of order of milliseconds. Furthermore, mass, volume, and demand for power less than other magnetic and electronic memories.

Katti, Romney R.↗
DOE OSTI2026

Photodynamic melting of phase-reversed charge stripes and enhanced condensation

The interplay between charge stripes and pairing has long been a subject of scrutiny in a broad class of unconventional superconductors, as in some cases it is unclear whether this interplay benefits the ensuing superfluidity. Experiments that explore the out-of-equilibrium dynamics of these systems aim to tip the balance toward one phase or the other by selectively coupling to relevant modes. Leveraging the fact that competition between stripes and pairing is not exclusive to fermionic systems, we explore the photoirradiation dynamics of interacting hardcore bosons in which density-wave phase-reversal melting leads to enhanced phase-coherent transport response, as quantified by the dynamic amplification of both the zero-momentum occupancy and the condensate fraction, as well as finite out-of-equilibrium charge stiffness and superfluid weight, for a given system size. Finally, our results, obtained using unbiased methods for an interacting system on a ladder geometry, demonstrate how one can engineer time-dependent perturbations to release suppressed orders, potentially providing insight into the underlying mechanism in related experiments.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2020

Dust Reverberation Mapping in Distant Quasars from Optical and Mid-infrared Imaging Surveys

The size of the dust torus in active galactic nuclei (AGNs) and their high-luminosity counterparts, quasars, can be inferred from the time delay between UV/optical accretion disk continuum variability and the response in the mid-infrared (MIR) torus emission. This dust reverberation mapping (RM) technique has been successfully applied to ~70 z ≲ 0.3 AGNs and quasars. Here we present first results of our dust RM program for distant quasars covered in the Sloan Digital Sky Survey Stripe 82 region combining ~20 yr ground-based optical light curves with 10 yr MIR light curves from the WISE satellite. Here, we measure a high-fidelity lag between W1 band (3.4 μm) and g band for 587 quasars over 0.3 ≲ z ≲ 2 () and two orders of magnitude in quasar luminosity. They tightly follow (intrinsic scatter ~0.17 dex in lag) the IR lag–luminosity relation observed for z < 0.3 AGNs, revealing a remarkable size–luminosity relation for the dust torus over more than four decades in AGN luminosity, with little dependence on additional quasar properties such as Eddington ratio and variability amplitude. This study motivates further investigations in the utility of dust RM for cosmology and strongly endorses a compelling science case for the combined 10 yr Vera C. Rubin Observatory Legacy Survey of Space and Time (optical) and 5 yr Nancy Grace Roman Space Telescope 2 μm light curves in a deep survey for low-redshift AGN dust RM with much lower luminosities and shorter, measurable IR lags. The compiled optical and MIR light curves for 7384 quasars in our parent sample are made public with this work.

79 ASTRONOMY AND ASTROPHYSICS↗
NASA NTRS2014

Calibrating Historical IR Sensors Using GEO, and AVHRR Infrared Tropical Mean Calibration Models

Long-term, remote-sensing-based climate data records (CDRs) are highly dependent on having consistent, wellcalibrated satellite instrument measurements of the Earth's radiant energy. Therefore, by making historical satellite calibrations consistent with those of today's imagers, the Earth-observing community can benefit from a CDR that spans a minimum of 30 years. Most operational meteorological satellites rely on an onboard blackbody and space looks to provide on-orbit IR calibration, but neither target is traceable to absolute standards. The IR channels can also be affected by ice on the detector window, angle dependency of the scan mirror emissivity, stray-light, and detector-to-detector striping. Being able to quantify and correct such degradations would mean IR data from any satellite imager could contribute to a CDR. Recent efforts have focused on utilizing well-calibrated modern hyper-spectral sensors to intercalibrate concurrent operational IR imagers to a single reference. In order to consistently calibrate both historical and current IR imagers to the same reference, however, another strategy is needed. Large, well-characterized tropical-domain Earth targets have the potential of providing an Earth-view reference accuracy of within 0.5 K. To that effort, NASA Langley is developing an IR tropical mean calibration model in order to calibrate historical Advanced Very High Resolution Radiometer (AVHRR) instruments. Using Meteosat-9 (Met-9) as a reference, empirical models are built based on spatially/temporally binned Met-9 and AVHRR tropical IR brightness temperatures. By demonstrating the stability of the Met-9 tropical models, NOAA-18 AVHRR can be calibrated to Met-9 by matching the AVHRR monthly histogram averages with the Met-9 model. This method is validated with ray-matched AVHRR and Met-9 biasdifference time series. Establishing the validity of this empirical model will allow for the calibration of historical AVHRR sensors to within 0.5 K, and thereby establish a climate-quality IR data record.

Scarino, Benjamin↗
DOE OSTI2022

Single-shot measurements of pulse-front tilt in intense ps laser pulses and its effect on accelerated electron and ion beam characteristics (invited)

Here we report recent single-shot spatiotemporal measurements of laser pulses, including pulse-front tilt (PFT) and spatial chirp, taken at the Compact Multipulse Terawatt laser at the Jupiter Laser Facility in Livermore, CA. STRIPED FISH, a device that measures the complete 3D electric field of fs to ps laser pulses on a single shot, was adapted to near infrared for these measurements. We present the design of the instrument used for these experiments, the on-shot measurements of systematic high-order PFT, and shot-to-shot variations in the measurements of spatiotemporal couplings. Finally, we simulate the effect of PFT in target normal sheath acceleration experiments. These simulations showed that pulse front tilt can steer hot electrons, shape the distribution of the accelerating sheath field, and increase the variability of cutoff energy in the resulting proton spectra. While these effects may be detrimental to experimental accuracy if the pulse front tilt is left unmeasured, hot electron steering shows promise for precision manipulation of the particle source for a range of applications, including irradiation of secondary targets for opacity measurements, radiography, or neutron generation.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2023

Competing incommensurate spin fluctuations and magnetic excitations in infinite-layer nickelate superconductors

The recently discovered infinite-layer nickelates show great promise in helping to disentangle the various cooperative mechanisms responsible for high-temperature superconductivity. However, lack of antiferromagnetic order in the pristine nickelates presents a challenge for connecting the physics of the cuprates and nickelates. Here, by using a quantum many-body Green’s function-based approach to treat the electronic and magnetic structures, we unveil the presence of many two- and three-dimensional magnetic stripe instabilities that are shown to persist across the phase diagram of LaNiO 2 . Our analysis indicates that the magnetic properties of the infinite-layer nickelates are closer to those of the doped cuprates, which host a stripe ground state, rather than the undoped cuprates. The computed longitudinal-spin, transverse-spin, and charge spectra of LaNiO 2 are found to contain an admixture of contributions from localized and itinerant carriers. Theoretically obtained dispersion of magnetic excitations (spin-flip) is found to be in good accord with the results of recent resonant inelastic X-ray scattering experiments. Our study gives insight into the origin of strong magnetic competition in the infinite-layer nickelates and their relationship with the cuprates.

36 MATERIALS SCIENCE↗
NASA NTRS1986

Comparison of the 1984 and 1985 AIS data over the Singatse Range (Yerington), Nevada

The Singatse Range is composed of a series of 53 types of volcanic, plutonic, metamorphic, and sedimentary rocks. In addition the Jurassic plutonic rocks are also of economic interest for their copper mineralization which is contained in a porphyry dike swarm. The 1984 and 1985 flight results from the Airborne Imaging Spectrometer (AIS) instrument flown in the NASA/JPL C-130 aircraft are contrasted and compared. The 1984 data are less noisy than the 1985, in which many sets of vertical stripings from bad detectors can be seen. Significantly however, enough of the hydrothermal alteration patterns can be seen in each line at the mutual crossing points that one can say that the specific targets were detected in both year's flights. The spectra of both years are corrupted by the second-order effect from the grating, but 0-H bond absorption at essentially correct wavelengths for sericite and/or kaolinite can be seen.

Lyon, R. J. P.↗
DOE OSTI2020

Itinerant ferromagnetism in van der Waals Fe 5 – x Ge Te 2 crystals above room temperature

Two-dimensional (2D) van der Waals (vdW) magnets have recently attracted increasing attention, as they provide a novel system for exploring 2D magnetism. However, intrinsic ferromagnetism in 2D systems has almost exclusively been observed at low temperatures, limiting their technological relevance. Fe N Ge Te 2 ( N = 3 , 4, and 5) systems are currently becoming the most attractive 2D vdW materials due to their relatively high Curie temperatures and large saturation magnetization. However, the nature of their complex yet intriguing magnetic behaviors is still unclear, in part due to the multiple inequivalent iron sites and iron vacancies. In this study, we show evolution of magnetic ordering transitions in Fe 5 – x Ge Te 2 with high Curie temperature and a strong saturation magnetization using photoemission electron microscopy and transport measurements. At 275 K, the ferromagnet transitions to a ferrimagnet, and below 110 K transitions to a state with glassy clusters. These are evidenced from temperature-dependent magnetic stripe domain evolution and anisotropic magnetoresistance measurements. Our findings show a clear magnetic ground state of Fe 5 – x Ge Te 2 at room temperature which signals that Fe 5 – x Ge Te 2 system is a very promising candidate for spintronic devices and provides a material design pathway to further increase the Curie temperature and saturation moments in vdW ferromagnets.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
NASA NTRS1978

The 1.1 micrometer and visible emission semiconductor diode lasers

In (AlGa)As, the first of three alloy systems studied, Continuous Wave (CW) operation was obtained at room temperature at a wavelength as low as 7260 A. Reliability in this system was studied in the incoherent mode. Zinc doped devices had significant degradation, whereas Ge or Ge plus Zi doped devices had none. The Al2O3 facet coatings were shown to significantly reduce facet deterioration in all types of lasers, longer wavelength units of that type having accumulated (at the time of writing) 22,000 hours with little if any degradation. A CL study of thin (AlGa)As layers revealed micro fluctuation in composition. A macro-scale fluctuation was observed by electroreflectance. An experimental and theoretical study of the effect of stripe width on the threshold current was carried out. Emission below 7000 A was obtained in VPE grown Ga(AsP) (In,Ga)P with CW operation at 10 C. Lasers and LED's were made by LPE in (InGa) (AsP). Laser thresholds of 5 kA/cm2 were obtained, while LED efficiences were on the order of 2%. Incoherent life test over 6000 hours showed no degradation.

Ladany, I.↗