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Results for “Curved scintillator”

Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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9 records
All sourcesNASA NTRSDOE OSTI
DOE OSTI2025

Portable Distortion Free Large Solid Angle Coverage Detector

Neutron single crystal diffractometers require large solid angle coverage for optimum performance. This can be achieved by tiling flat detectors in a cylindrical or spherical geometry, but results in large gaps in detector coverage and parallax distortion. The detector edges exhibit degraded resolution, distortion, and gamma rejection. Since the detector edge regions are a significant fraction of the detector active area, they must be removed from the experimental data set, requiring extra beam time to collect enough analysis data. A spherical detector with a continuous surface would effectively address this issue while eliminating most boundary ‘dead’ areas. Here we report on the development of a novel hemispherical shaped neutron detector using seamlessly tiled readout modules to form the desired shape. The heart of the detector is a specially developed curved neutron scintillator coupled to high resolution silicon photomultiplier (SiPM) Anger cameras via custom made fiber optic tapers (FOTs). The detector has been assembled and initial tests have been conducted at the High Flux Isotope Reactor (HFIR) beamlines at Oak Ridge National Laboratory (ORNL). Here, in this work, we describe details of the scintillator design, fabrication and characterization, evaluation of individual detector modules, the details of the detector design implementation, and evaluation of the assembled detector at ORNL beamlines.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2025

Energy migration and scintillation kinetics in compositionally complex (Gd 1/4 Y 1/4 Tb 1/4 Lu 1/4 ) 3 Al 5 O 12 :Ce single crystal scintillator

It is well-established that compositional tuning through binary admixture can improve scintillation performance in several materials systems, including Ce-activated garnets. Although recent work on ternary or quaternary cation admixture shows promise, the impact of this increased compositional complexity on thermal stability and carrier-defect dynamics has not been addressed. Here, we investigate a compositionally complex garnet, (Gd 1/4 Y 1/4 Tb 1/4 Lu 1/4 ) 3 Al 5 O 12 :Ce (GYTLAG), grown by the Czochralski method using temperature-dependent photoluminescence (PL), PL decay, and thermoluminescence (TL). PL and PL decay measurements support a thermally activated Tb 3+ -Ce 3+ energy transfer, where Tb 3+ emission dominates below 60 K, but Ce 3+ emission increases from 20-300 K. Thermal quenching of Ce 3+ emission occurs around T 50 = 508 K, with an activation energy of 0.6 eV. TL and wavelength-resolved TL spectra from 20–500 K show that GYTLAG contains similar trap groups to LuAG but with a broader distribution of glow peaks below room temperature, possibly caused by quaternary cation mixing. A combination of dose dependence, partial cleaning and initial rise, and glow curve fitting to a first order continuous Gaussian distribution model are used to understand the contribution of electronic point defects to scintillation decay and afterglow at room temperature. Furthermore, these results inform how increased compositional complexity influences recombination dynamics in garnet scintillators.

Compositionally complex↗
DOE OSTI2024

Nonlinear light-output calibration of the oxygenated xylene scintillators used in OMEGA neutron time-of-flight spectrometers

Neutron time-of-flight (nTOF) spectrometers are essential instruments for measuring and evaluating the performance of inertial confinement fusion implosions. The neutron spectrometers utilized for the OMEGA laser include two liquid-based scintillators, each consisting of a large volume filled with xylene that is coupled to four photomultiplier tubes. Analysis of the signal from these detectors requires detailed knowledge of the scintillator’s light output, which is needed to fit the nTOF spectrum, from which the neutron energy spectrum is informed. The light output is nonlinearly proportional to the neutron energy, which, in turn, affects the interpretation of the neutron energy spectrum from a TOF signal. A recent campaign on OMEGA was performed to calibrate the xylene detectors and infer the shape of the light-output curve. The campaign utilized materials with increasing Z placed in the OMEGA target chamber to initiate scattering events with the 14 MeV fusion neutrons. This process leads to the production of backscatter neutrons of varying energies that appear as peaks in the nTOF data. Simulations using a neutron transport code were combined with the measured deuterium–tritium neutron yields to calculate the expected backscattered neutron yields from the well-known scattering cross sections of each material. Furthermore, the neutron-energy dependent light output of the scintillator inferred from the experiment is compared to the light-output curve simulated with a neutron transport code for the following neutron energies: 1.5, 2.5, 6, and 14 MeV.

47 OTHER INSTRUMENTATION↗
DOE OSTI2025

PMT calibration for the JSNS^2-II far detector with an embedded LED system

The JSNS^2-II (the second phase of JSNS^2, J-PARC Sterile Neutrino Search at J-PARC Spallation Neutron Source) is an experiment aimed at searching for sterile neutrinos. Here, this experiment has entered its second phase, employing two liquid scintillator detectors located at near and far positions from the neutrino source. Recently, the far detector of the experiment has been completed and is currently in the calibration phase. The following properties of all functioning Photo-Multiplier-Tubes (PMTs) to detect the neutrino events in the far detector have been calibrated: PMT gain, its dependence of supplied High Voltage (HV), Peak-to-Valley (PV), and signal timing. This paper presents a detailed description of the calibration process utilizing the LED system. The LED system of the far detector uses two Ultra-Violet (UV) LEDs, which are effective in calibrating all of the PMTs at once. The UV light is converted into the visible light wavelengths inside liquid scintillator via the wavelength shifters, providing pseudo-isotropic light. To achieve a good energy resolution for physics events, a relative gain adjustment of up to 10% is required for all functioning PMTs. This will be achieved using the HV curves measured and the results of the LED calibration. The Peak-to-Valley (PV) ratio values, which distinguish the single photo-electron signal from the pedestal, are similar to those from the production company. Additionally, the precision of the PMT signal timing is measured to be 2.1 ns. This meets the event reconstruction requirement of 10 ns.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2026

Visualization of Thermal and Strain Dynamics in X-ray Optics by Time-Resolved Rocking Curve Imaging

The absorption of intense X-ray pulses from free-electron lasers by X-ray crystal optics triggers rapid thermal and mechanical responses, including lattice compression, expan- sion, and strain-wave propagation, which dynamically modify diffraction conditions and wavefront properties. These effects pose significant challenges for next-generation high- repetition-rate X-ray sources, particularly for crystal monochromators used in XFEL beam- lines and self-seeding. Here, we demonstrate time-resolved rocking curve imaging (TrRCI) of X-ray Bragg optics with high spatial resolution (6.4 μm) and sub-1-μrad angular resolu- tion, enabling direct visualization of lattice dynamics from nanoseconds to microseconds. By combining a high-flux beamline at SPring-8, a scintillator-coupled sCMOS detector, and a synchronized femtosecond laser system, we capture lattice dynamics induced by tran- sient laser heating with a strain sensitivity on the order of 10−6 . Our results reveal transient lattice deformation and the propagation of laser-induced strain waves over millimeter-scale distances. This approach provides experimental benchmarks for understanding heat-load effects in high-repetition-rate X-ray optics.

Source record↗
DOE OSTI2026

Deuterated Xylene-Based Neutron Spectrometry

Deuterated scintillators, such as deuterated xylene (C8D10) have been theorized to offer better pulse shape discrimination (PSD) and neutron spectrometry performance than traditional protiated scintillators due to the anisotropy of neutron scattering on deuterium. However, the light output responses of said deuterated scintillators to monoenergetic has not been characterized in its entirety at both high and low energies. Several time-of-flight experiments were conducted at the Idaho national Laboratory to characterize a pair of EJ-301D deuterated xylene detectors. The low energy detector response to quasi-monoenergetic neutrons was measured using a Cf-252 source, and the high energy detector response was measured using a D-T source and angles of 20, 45, and 60 deg, corresponding to theoretical neutron energies of 13.2, 10.4, and 8.2 MeV. During post-processing, the neutron and gamma bands were clearly able to be separated, even at low light outputs, solidifying the superior PSD capability of deuterated xylene. An exponential of fit of LO=0.63E-2.22*(1-exp(-0.25E)), which has good agreement with previously measured data, was found as the light output response from deuteron recoils. Additionally, measurements of AmBe, D-T, and D-D sources were unfolded using the light output response curve, which resulted in favorable agreement with theoretical values. Further testing of the response matrix by unfolding more sources (such as PuBe) needs to be done, but the unfolding accuracy for currently available sources suggests that deuterated xylene can be used to measure and unfold both fission, monoenergetic, and continuous spectra.

scintillator↗
DOE OSTI2025

Detection and quantification of trace technetium in the presence of molybdenum using laser-induced breakdown spectroscopy

Technetium (Tc) is a very important element that is encountered in many aspects, from its presence in radioactive waste and its potential environmental impact to its use as a medical radioisotope. Its detection and quantification in liquid samples is traditionally cumbersome, involving detailed sample preparation and analysis by mass spectrometry or scintillation. This article demonstrates the first comprehensive emission spectral analysis of Tc from a liquid sample by immobilization in a polymer and analysis by laser-induced breakdown spectroscopy (LIBS). A survey of LIBS spectra was completed to identify the strongest analytical lines for quantification of trace Tc in the presence of Mo. The quantification of Tc in a Mo-containing matrix was selected because Tc radioisotopes are the daughter products of Mo isotope decay. The first reported calibration curves by LIBS are provided with limits of detection and quantification down to 0.710 µg mL −1 and 1.39 µg mL −1 , respectively. Ultimately, this study demonstrated the feasibility of trace Tc quantification using LIBS and will serve as a reference for future research related to monitoring this radioactive species.

Andrews, Hunter B. [Oak Ridge National Laboratory ↗
DOE OSTI2024

LLNL measurements of thermally irradiated HEU sample and saltwater-matrixed HEU sample

Two scintillation vials, kindly provided by the PNNL team, were received in the LLNL radiochemistry building on June 10, 2024; one containing approximately 2 mL dissolved thermally-irradiated HEU, and the other containing dried salt from irradiated seawater. A quick, semiquantitative screening count of the salt showed that the activation product activities were very low, with the highest activity being ~1 Bq 24 Na. The dissolved HEU solution was transferred to a Prindle vial (LLNL standard counting geometry) and weighed. Approximately 2 mL 3 M HNO 3 was added so that the solution completely covered the bottom of the vial and Gamanal software would be able to accurately generate an efficiency curve. This sample, called “PNNLFP24” is the irradiated HEU solution received, gravimetrically diluted by a factor of 1.7356 ± 0.0003, and was sent for quick gamma counting prior to further modification. Meanwhile the salt was quantitatively transferred to a 250 mL polyethylene bottle and dissolved in 160 mL 3 M HNO 3 . After counting, 50 µL PNNLFP24 was aliquoted for Resonance Ionization Mass Spectrometry (RIMS) analysis, and then 10.0 mL of the salt solution (6.03% of the total salt, gravimetrically) was added to the remaining PNNLFP24 solution to make “PNNLFPSW24”. After weighing, two 100 µL aliquots were removed for RIMS and DES, and 3 mL was aliquoted for microfluidic chemistry. The remaining “PNNLFPSW24” solution was weighed and proceeded for singles and coincidence counting on the MCBOS system.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2026

Characterization of lateral amorphous selenium photodetectors for low-photon and VUV detection at cryogenic temperatures

The performance of amorphous selenium (a-Se) as a cryogenic photodetector material is evaluated through a series of experiments using laterally structured devices operated in a custom optical test stand. These studies investigate the response of a-Se detectors to low-photon fluxes at high electric fields near avalanche conditions, the linearity of the photoconductive response over a wide dynamic range and the direct detection of narrowband 130 nm vacuum ultraviolet (VUV) illumination. At 87 K, matched-filter analysis shows reliable single-shot detection with efficiencies ≥80% and area under the curve (AUC) ≥ 0.85 using as few as ∼ 6800 incident 401 nm photons, corresponding to ∼ 3400 photons within field-active regions after accounting for geometric constraints. Measurements are performed at cryogenic temperatures using calibrated photon fluxes derived from a silicon photomultiplier reference and a characterized optical filter stack. Additional experiments using a tellurium-doped a-Se (a-SeTe) device explore the material's behavior under identical test conditions and demonstrate that avalanche is achievable in a-SeTe at cryogenic temperatures. The results demonstrate reproducible low-noise operation, VUV sensitivity and field-dependent gain behavior in a lateral a-Se architecture, representing the first reported observation of avalanche multiplication in laterally structured a-Se and a-SeTe devices at cryogenic temperatures. These findings support the potential integration of laterally structured a-Se devices into next-generation pixelated liquid-argon time projection chambers (TPCs) requiring scalable, high-field-compatible photon detection systems.

Amorphous selenium↗