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At least 19 records

Development of Shielding Benchmarks Using the Godiva IV Assembly

The Nuclear Criticality Safety Program (NCSP) is developing a shielding benchmark using the Godiva IV assembly as a source. Its present status is reviewed herein. Even eight decades into the nuclear era, substantial work remains to develop a database of shielding benchmarks to support future nuclear development. A nuclear simulation is only as good as its supporting data, inputs, and validation basis. Uncertainty in these areas is addressed using conservatism, which adds margin and, occasionally, cost. In many shielding situations, high accuracy is not necessary because additional material is not particularly expensive. After all, 1–2 cm of lead often reduces the gamma ray dose substantially. However, in certain areas, conservatism can add unnecessary cost. These areas include mobile shielding applications such as casks, ships, microreactors, and spacecraft, where weight and, thus, margin is expensive. Although these characteristics are side benefits for NCSP shielding benchmark development, the main driver is enabling more reliable placement of criticality accident alarm systems (CAASs) in nuclear material facilities, such as those dedicated to the production of advanced reactor fuels. CAAS placement relies on more than accurate data and code validation. It also relies on sufficiently accurate materials specifications, geometry specifications, and a well-defined, alarm-producing baseline accident. All these things require tacit knowledge and understanding of the problem being evaluated. Benchmarks can help ensure this understanding.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Godiva-IV Critical Assembly [Slides]

Objectives: Familiarization of the Godiva-IV assembly; Understand the criticality safety parameters that effect Godiva IV; Understand the differences between subcritical, delayed-critical, and prompt-critical operations; and, Understand the concept of temperature-dependent reactivity feedback.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Yield and PDV Measurements of the Godiva-IV Critical Assembly

A high dynamic range, scinillator based detector, the MHD-240, was used to measure the gamma and neutron flux of several prompt critical bursts of the Godiva-IV assembly. The measurements provided the alpha and FWHM for several different burst temperatures. Calibrations of the MHD240 gamma and neutron sensitivity along with MCNP based simulation of the Godiva-IV assembly allowed us to also determine the total fission yield of the burst integrated over approximately 5 ms. In addition a Photo Doppler Velocimetry measurement was conducted to determine the surface motion vibrational frequency of Godiva-IV assembly during the bursts. The combined data were collected to be used as input to multi-physics simulation of the Godiva-IV assembly. This is a preliminary report, there is an ongoing effort to update the MCNP simulations used in the analysis and develop a correction for the room return component of the measured signal.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Yield and PDV Measurements of the Godiva-IV Critical Assembly (Preliminary Report)

A high dynamic range, scinillator based detector, the MHD-240, was used to measure the gamma and neutron flux of several prompt critical bursts of the Godiva-IV assembly. The measurements provided the alpha and FWHM for several different burst temperatures. Calibrations of the MHD240 gamma and neutron sensitivity along with MCNP based simulation of the Godiva-IV assembly will allow us to also determine the total fission yield of the burst integrated over approximately 5 ms. Work is ongoing to check the calibrations of the MHD-240, and improve the MCNP simulations. This is a preliminary report, and the fission yields reported here are not final and are likely inaccurate. The measured alpha and FWHM are not impacted by the calibration issues and are considered final.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Godiva-IV Critical Assembly [Slides]

The objectives of this presentation are to: (1) gain awareness of the Godiva-IV assembly, including its design and intent; (2) create familiarization of the differences between subcritical, delayed-critical, and prompt-critical; and (3) observe the effects of temperature-dependent reactivity feedback.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Photo Doppler Velocimetry and Gamma/Neutron Yield Measurements of Godiva-IV Critical Assembly

The purpose of this experiment was to collect data for a dynamic benchmark of the Godiva-IV burst assembly. Data were taken using two different measurement systems. The gamma & neutron flux was measured using a calibrated, high-dynamic-range scintillator detector, the MHD-240. The measurement will be used to determine the total fission yield and alpha throughout the burst and shutdown sequence of Godiva-IV. The Photon Doppler Velocimetry (PDV) measurement detected the surface motion of the burst assembly as a function of time. The combined data will be used in a multi-physics simulation of the Godiva-IV burst assembly.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

A neutron fluence map of the Los Alamos National Laboratory Godiva IV critical assembly

A neutron fluence map and a total ionizing dose map of the Los Alamos National Laboratory Godiva IV fast burst critical assembly was generated using passive reactor dosimetry, comprised of sulfur pellets and thermoluminescent dosimeters. Godiva IV is an unmoderated, fast burst, critical assembly constructed of approximately 65 kg of highly enriched uranium fuel alloyed with 1.5 % molybdenum for strength. The mapping was performed during a single 75.6 ºC temperature rise burst operation, with the top and sides of the cylindrical Godiva-IV Top Hat covered in passive dosimetry. Dosimetry was placed in a symmetric pattern around the Top Hat, with higher concentrations near the control rods and burst rod. A specific portion of the lower quadrant of the burst rod was mapped to confirm a testing region where the neutron fluence varied by no more than ± 5%. The results will be used to assess the neutron, gamma, and total ionizing dose environment in three-dimensional space around the assembly for higher fidelity experiment placement, active dosimetry positioning, and radiation field characterization.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Radiation Characterization Summary: Godiva IV Critical Assembly Environments at the In-Core, Top Hat, 1m, and 2m Irradiation Locations

This document presents the facility-recommended characterization of the neutron, prompt gamma ray, and delayed gamma ray radiation fields at the Godiva IV critical assembly at the National Criticality Experiments Research Center (NCERC). The environments assessed include the In-Core location, a location on the Top Hat, 1m away from the assembly, and 2m away from the assembly. The neutron, prompt gamma ray, and delayed gamma ray energy spectra, uncertainties, and covariance matrices are presented as well as radial and axial neutron and gamma ray fluence profiles on the Top Hat surrounding the critical assembly. Recommended constants are given to facilitate the conversion of various dosimetry readings into radiation metrics desired by experimenters. Representative pulse operations are presented with conversion examples.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

237 Np Fission Spectrum Cumulative Fission Product Yield Measurement Using Godiva IV Critical Assembly

Precise integral measurement of fast neutron-induced fission product yields for various actinides is of high interest for applied nuclear science. The goal of this effort is to improve uncertainties in fission product yield values of 237 Np. Fission was induced in a NpO 2 (NO 3 ) target using the Godiva IV critical assembly in burst mode. The irradiated sample was transferred to a high-resolution γ-ray detection setup within 50 minutes. γ-ray list mode data was collected from 50 minutes to 1 week after the irradiation. γ-ray spectroscopy was performed to analyze the time dependent γ-ray yields using an automated peak search algorithm to identify isotopes by their decay γ-ray energy and half-life. Finally, the initial activity for each isotope identified was used to calculate their fission product yield.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

239 Pu Fission Spectrum Cumulative Fission Product Yield Measurement Using Godiva IV Critical Assembly

Precise integral measurement of fast neutron-induced fission product yields for various actinides is of high interest for applied nuclear science. The goal of this effort is to improve uncertainties in fission product yield values of 239 Pu. Fission was induced in a pure 239 Pu (>99%) target using the Godiva IV critical assembly in burst mode. Further, the irradiated sample was transferred to a high-resolution γ-ray detector within 45 minutes. γ-ray list mode data was collected from 45 minutes to 1 week after the irradiation. γ-ray spectroscopy was performed to analyze the time dependent γ-ray yields using an automated peak search algorithm to identify isotopes by their decay γ-ray energy and half-life. The initial activity for each isotope identified was used to calculate their fission product yield.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

New constraint on the Np 237 ( n , γ ) Np 238 integral cross section using the Godiva-IV critical assembly

Accurate knowledge of the 237 Np(n, γ) 238 Np cross section at fast neutron energies is important for applied nuclear science. The presently available experimental data has large disagreements in the fast neutron region. Perform a model-independent measurement of the 237 Np(n, γ) 238 Np integral cross section using a well characterized fast neutron source and compare the result with previous measurements and current nuclear data evaluations. Provide an integral measurement that can be used as a benchmark for current evaluations. Multiple samples of 237 Np were irradiated in the Godiva-IV critical assembly. Following the irradiation, the samples placed in a γ-ray counting setup and the γ-rays emitted from the decay of 238 Np were measured over a time period of approximately 7 days. Multiple γ-ray decay branches of 238 Np were observed. The observed activity of 238 Np was used to calculate the amount of 238 Np produced during the irradiation via the 237 Np(n, γ) 238 Np reaction and an integral cross section of 342(11) mb was measured for the Godiva-IV neutron spectrum. Further, the 238 Np half-life has been measured with a result of 50.31(5) hours. The 237 Np(n, γ) 238 Np integral cross section measured in this work is in agreement with overlapping 1σ error bands to ENDF/B-VIII.0. However, the measured value is 3σ away from the calculated integral cross section using JENDL-5. This measurement offers a reliable benchmark for future 237 Np(n, γ) 238 Np cross section evaluations.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

R-Value Measurements Performed on Actinide Targets Irradiated using the GODIVA IV Critical Assembly in FY22

The separation and characterization of two irradiated uranium targets, a depleted uranium (DU) and a highly enriched uranium (HEU) target as well as a plutonium (Pu) target, was conducted in April of 2022. The three targets were assembled at Los Alamos National Laboratory (LANL) and irradiated using the GODIVA critical assembly at the National Criticality Experiments Research Center (NCERC). Splits of the dissolved targets were received by Pacific Northwest National Laboratory (PNNL) after which the PNNL and LANL teams chemically separated the solutions using independent separation schemes and analyzed the separated fractions for short lived actinides and fission products. Chemical separations were traced with stable or radioactive tracers to allow for the determination of chemical yields, analyzing using either inductively coupled plasma optical emission spectroscopy (ICP-OES), inductively coupled plasma mass spectrometry (ICP-MS) or gamma emission analysis (GEA) depending on the nature of the tracer. The Pu target solution was traced with stable elements at LANL to follow elemental fractionation during a Pu removal step. Many analytical techniques were used by PNNL including kinetic phosphorescence analysis (KPA), ICP-OES, ICP-MS, GEA, and thermal ionization mass spectrometry (TIMS) depending on the analyte’s need.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

IER 555: Godiva Benchmark Update CED-2 (Final Design Report)

The International Criticality Safety Benchmark Evaluation Project (ICSBEP) evaluation of the Godiva IV critical assembly, HEU-MET-FAST-086: GODIVA-IV DELAYED-CRITICAL EXPERIMENTS (HMF-086), was completed by Russ Mosteller. Five critical experiment configurations performed at the Los Alamos National Laboratory (LANL) Technical Area (TA)-18 were evaluated as acceptable benchmark cases. The five cases consist of four delayed critical configurations which differ in control rod positions and one prompt critical configuration. All cases calculated a lower $k_{eff}$ than measured by experiment. This data is referred to as the TA-18 Godiva IV benchmark in this report. In 2005, Godiva IV was disassembled for relocation to the Nevada Test Site (NTS), now Nevada National Security Site (NNSS), at the National Criticality Experiments Research Center (NCERC). Following the disassembly and subsequent reassembly and startup of Godiva IV at NCERC, additional information about the Godiva IV components was obtained. An errata note was added to the HMF-086 evaluation in the ICSBEP handbook to provide this new information until a revision to the benchmark evaluation could be performed. In addition to those corrections, there are differences between the Godiva IV assembly at TA-18 and the Godiva IV assembly at NCERC. These differences include both assembly-specific differences (differences in the safety block gap, differences in the control rod positions, a new NCERC Top Hat and contamination shield) as well as environmental differences, such as the size and shape of the experimental building where the assembly is located. An additional model with similar cases, referred to as the NCERC Godiva IV benchmark in this report, will be added to the revised HMF-086 to capture these additional differences. This will provide the best benchmark model of Godiva for use by those performing experiments at NCERC. The IER 555 CED-2 report documents the information that will be updated in the HMF-086 revision, both the corrections to the TA-18 Godiva IV benchmark and the subsequent changes to create a NCERC Godiva IV benchmark. It describes the measurements that will be performed for cases similar to those performed at TA-18. It also describes measurements that will be included in the evaluation as additional data.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Hands-On Experimental Training [Slides]

Training provided includes: Nuclear Criticality Safety Fundamentals, Sub-Critical "Hands On" Demonstration, Hand-Stacking and Remote Approach to Critical Using the Planet Assembly, Flattop Free-Run Demonstration, and Godiva-IV Critical Assembly Demonstration.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗