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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 19 records

Optical shock-enhanced self-photon acceleration

Photon accelerators can spectrally broaden laser pulses with high efficiency in moving electron density gradients driven in a rapidly ionizing plasma. When driven by a conventional laser pulse, the group velocity walk-off experienced by the accelerated photons and deterioration of the gradient from diffraction and plasma-refraction limit the extent of spectral broadening. In this work, we show that a laser pulse with a shaped space-time and transverse intensity profile overcomes these limitations by creating a guiding density pro le at a tunable velocity. Self-photon acceleration in this profile leads to dramatic spectral broadening and intensity steepening, forming an optical shock that further enhances the rate of spectral broadening. In this new regime, multi-octave spectra extending from 400nm to 60nm wavelengths, which support near-transform limited < 400 as pulses, are generated over < 100 μm of interaction length.

74 ATOMIC AND MOLECULAR PHYSICS↗

Advanced Photon Acceleration Schemes for Tunable XUV/Soft X-Ray Sources

We report on the advances made under the purview of DOE award number DE-SC0019135 that was active during the period: 09/01/2018–08/31/2021. The grant investigated the application of a “flying focus” to the problem of photon acceleration—in which a dynamic refractive index gradient is used to continuously upshift a probe beam’s frequency. Codes were written to describe the creation of ionization waves of arbitrary velocity (IWAVs) for use as a photon-accelerating medium, as well as the behavior of a witness pulse residing in said medium. Experiments first verified the spatiotemporal control over laser intensity provided by a chromatic flying focus, then used that ability to produce small-diameter IWAVs in the far-field with the expected dynamics, and finally demonstrated even further flexibility by producing large-diameter IWAVs in the laser quasi-far-field that maintained the beneficial dynamics. Multiple innovative diagnostics—spectrally resolved Schlieren and spectrally resolved interferometry—were pioneered in order to diagnose the IWAVs. For IWAV production in the laboratory, however, beam quality was identified as a key limitation in the quasi-far-field. Since the original chromatic flying focus was found to result in relatively long (ps duration) intensity peaks, which could limit some applications including photon acceleration, additional techniques were invented to provide similar spatiotemporal control while also retaining ultrashort intensity peaks. While simulations have identified several interesting regimes for photon acceleration—first predicting the upshift of a counterpropagating witness pulse from the optical to the extreme ultraviolet in less than 1 cm, and later obtaining similar shifts in less than 100 μm in a simpler self-seeded configuration—experimental demonstration is left for future work.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Performance of an optical TPC Geant4 simulation with opticks GPU-accelerated photon propagation

We investigate the performance of Opticks, a NVIDIA OptiX API 7.5 GPU-accelerated photon propagation tool compared with a single-threaded Geant4 simulation. We compare the simulations using an improved model of the NEXT-CRAB-0 gaseous time projection chamber. Performance results suggest that Opticks improves simulation speeds by between 58.47 ± 0.02 and 181.39 ± 0.28 times relative to a CPU-only Geant4 simulation and these results vary between different types of GPU and CPU. A detailed comparison shows that the number of detected photons, along with their times and wavelengths, are in good agreement between Opticks and Geant4.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Photon acceleration of high-intensity vector vortex beams into the extreme ultraviolet

Extreme ultraviolet (XUV) light sources allow for the probing of bound electron dynamics on attosecond scales, interrogation of high-energy-density matter, and access to novel regimes of strong-field quantum electrodynamics. Despite the importance of these applications, coherent XUV sources remain relatively rare, and those that do exist are limited in their peak intensity and spatio-polarization structure. Here, we demonstrate that photon acceleration of an optical vector vortex pulse in the moving density gradient of an electron beam–driven plasma wave can produce a high-intensity, tunable-wavelength XUV pulse with the same vector vortex structure as the original pulse. Quasi-3D, boosted-frame particlein- cell simulations show the transition of optical vector vortex pulses with 800-nm wavelengths and intensities below 10 18 W/cm 2 to XUV vector vortex pulses with 36-nm wavelengths and intensities exceeding 10 20 W/cm 2 over a distance of 1.2 cm. The XUV pulses have sub-femtosecond durations and nearly flat phase fronts. The production of such high-quality, high-intensity XUV vector vortex pulses could expand the utility of XUV light as a diagnostic and driver of novel light–matter interactions.

43 PARTICLE ACCELERATORS↗

Study of photon emission by electron capture during solar nuclei acceleration. 3: Photon production evaluations

Lower limits of photon fluxes were evaluated from electron capture during acceleration in solar flares, because the arbitrary q sub c asterisk assumed in this work evolves very slow with velocity, probably much more slowly than the physical actual situation: in fact, more emission is expected toward the IR region. Nevertheless the authors claim to show that the factibility of sounding acceleration processes, charge evolution processes and physical parameters of the source itself, by the observational analysis of this kind of emissions. For instance, it would be interesting to search observationally, for the predicted flux and energy drift of F sub e ions interacting with the atomic 0 and F sub e of the source matter, or, even more feasible for the X-ray lines at 4.2 keV and 2.624 + 0.003 KeV from Fe and S ions in ionized Fe at T = 10 to the 7th power K respectively, the 418 + or - 2 eV and 20 + or - 4 eV lines of Fe and S in ionized Fe at 5 x 10 to the 6th power K, which are predicted from Fermi acceleration.

Perez-Peraza, J.↗

Nonlinear Shock Acceleration and Photon Emission in Supernova Remnants

We have extended a simple model of nonlinear diffusive shock acceleration (Berezhko & Ellison 1999: Ellison &, Berezhko 1999a) to include the injection and acceleration of electrons and the production of photons from bremsstrahlung, synchrotron, inverse Compton, and pion-decay processes. We argue that, the results of this model, which is simpler to use than more elaborate ones, offer a significant improvement, over test-particle, power-law spectra which are often used in astrophysical applications of diffusive shock acceleration. With an evolutionary supernova remnant (SNR) model to obtain shock parameters as functions of ambient interstellar medium parameters and time, we predict broad-band continuum photon emission from supernova remnants in general, and SN1006 in particular, showing that our results compare well with the more complete time-dependent and spherically symmetric nonlinear model of Berezhko, Ksenofontov, & Petukhov (1999a). We discuss the implications nonlinear shock acceleration has for X-ray line emission, and use our model to describe how ambient conditions determine the TeV/radio flux ratio, an important parameter for gamma-ray observations of radio SNRs.

Ellison, Donald C.↗

Flexible silicon photonic architecture for accelerating distributed deep learning

The increasing size and complexity of deep learning (DL) models have led to the wide adoption of distributed training methods in datacenters (DCs) and high-performance computing (HPC) systems. However, communication among distributed computing units (CUs) has emerged as a major bottleneck in the training process. In this study, we propose Flex-SiPAC, a flexible silicon photonic accelerated compute cluster designed to accelerate multi-tenant distributed DL training workloads. Flex-SiPAC takes a co-design approach that combines a silicon photonic hardware platform with a tailored collective algorithm, optimized to leverage the unique physical properties of the architecture. The hardware platform integrates a novel wavelength-reconfigurable transceiver design and a micro-resonator-based wavelength-reconfigurable switch, enabling the system to achieve flexible bandwidth steering in the wavelength domain. The collective algorithm is designed to support reconfigurable topologies, enabling efficient all-reduce communications that are commonly used in DL training. The feasibility of the Flex-SiPAC architecture is demonstrated through two testbed experiments. First, an optical testbed experiment demonstrates the flexible routing of wavelengths by shuffling an array of input wavelengths using a custom-designed spatial-wavelength selective switch. Second, a four-GPU testbed running two DL workloads shows a 23% improvement in job completion time compared to a similarly sized leaf-spine topology. We further evaluate Flex-SiPAC using large-scale simulations, which show that Flex-SiPAC is able to reduce the communication time by 26% to 29% compared to state-of-the-art compute clusters under representative collective operations.

Wu, Zhenguo (ORCID:0000000322847985)↗

Longitudinal position dependence of dark line defect growth rate in high-power diode lasers at 790 nm

Using a nondestructive, in situ near-infrared defect imaging technique, we obtained time-resolved images of dark line defect (DLD) growth in the cavities of several high-power 790-nm diode lasers and calculated individual DLD growth rates. A clear longitudinal spatial dependence in the DLD growth rate was observed, in which the DLD growth rate was faster near the anti-reflective (AR) facet. Longitudinal spatial hole burning simulation results indicate that the total photon density increases toward the AR facet, while the carrier density decreases toward the AR facet. Here, these results suggest that photon absorption plays a key role in enhancing DLD growth beyond the contribution of the traditional carrier capture mechanism. Asymmetric DLD growth that was preferentially directed toward the high-reflectivity facet was also observed, providing further support for the role of photon absorption in the growth process. To account for these findings, we propose a photon-accelerated mechanism for the enhancement of DLD growth in which the slower carrier capture process in the traditional recombination-enhanced dislocation glide mechanism is replaced by a faster photon absorption process.

Engineering - Electronic and electrical engineerin↗

Ultrafast Wavefront Shaping via Space-Time Refraction

A myriad of metasurfaces have been demonstrated that manipulate light by spatially structuring thin optical layers. Manipulation of the optical properties of such layers in both space and time can unlock new physical phenomena and enable new optical devices. Examples include photon acceleration and frequency conversion, which modifies Snell’s relation to a more general, nonreciprocal form. Here, we combine theory and experiment to realize wavefront shaping and frequency conversion on subpicosecond time-scales by inducing space-time refractive index gradients in epsilon-near-zero (ENZ) films with femtosecond light pulses. Furthermore, we experimentally tune wavefront steering by controlling the incident angle of the beams and the pump–probe delay without the need for nanostructure fabrication. As a demonstration of this approach, we leverage the ultrafast, high-bandwidth optical response of transparent oxides in their ENZ wavelength range to create large refractive index gradients and new types of nonreciprocal, ultrafast two-dimensional (2D) optics, including an ultrathin transient lens.

36 MATERIALS SCIENCE↗

DOE Plasma Science Center - Predictive Control of Plasma Kinetics: Multi-Phase and Bounded Systems (Final Report DE-SC0001939)

Low temperature plasmas (LTPs) are the plasmas of electron-volt (eV) physics and eV technologies. LTPs have characteristic electron temperatures of a few eV and fractional ionizations that are typically small. Since LTPs have electron temperatures commensurate with the threshold energies of excited states in neutral atoms and molecules, power transfer from electrons to these atoms and molecules efficiently produces activated species (e.g., radicals, excited states, photons). Acceleration of ions in the sheaths of LTPs to energies of tens to hundreds of eV enable activation of surface modifying processes – sputtering, etching, deposition. With such properties, LTPs are often and beneficially used in technological devices, ranging from etching and deposition in microelectronics and solar cell fabrication, to hardening of surgical instruments. LTPs harbor fundamental science issues that are intellectually challenging and rewarding. At the same time, there are enormous societal benefits that are enabled by LTPs. The entire present-day and future information technology infrastructure owes its very existence to LTPs. Renewable energy sources, such as solar cell arrays, could not be economically produced in the absence of deposition and etching by LTPs. In acknowledgment of the importance of LTPs, the DOE Office of Fusion Energy Sciences supported the Plasma Science Center for Predictive Control of Plasma Kinetics: Multi-Phase and Bounded Systems from August 2009 to July 2021, consisting of an initial 5-year grant, 3 funded extensions and 2 no-cost extensions. This is the final report of the Center in which the productivity of the Center is discussed in terms of publications, impact and personnel. High-lights of the research performed in the Center are provided.

36 MATERIALS SCIENCE↗

Photon phase-space dynamics in a plasma wakefield accelerator

Frequency up-shifting of laser light in a beam-driven plasma wakefield has the potential to provide high-intensity sources of short wavelength radiation. Simulations have demonstrated that a laser pulse can undergo large frequency shifts, limited only by the drive beam energy, when the plasma density is tailored to match the accelerating phase of the wake to the group velocity of the pulse. Here, we study the dynamical evolution of photons in the 1D1P phase-space vicinity of the plasma wake-phase matching condition. Numerical calculations using a photon kinetic model are validated by direct comparison with 1D and quasi-3D particle-in-cell simulations. These calculations form the basis of a linear theory of the photon dynamics which reveals several important results, including scalings for the properties of the witness pulse and a self-similar solution for the photon phase-space dynamics. One prediction of the analytic theory is that the pulse can be compressed indefinitely, though the amount of compression would ultimately be limited by practical constraints. These results suggest that photon acceleration can provide a novel source of sub-femtosecond, short wavelength radiation.

XUV generation↗

Design of a multichannel photonic crystal dielectric laser accelerator

To be useful for most scientific and medical applications, compact particle accelerators will require much higher average current than enabled by current architectures. For this purpose, we propose a photonic crystal architecture for a dielectric laser accelerator, referred to as a multi-input multi-output silicon accelerator (MIMOSA), that enables simultaneous acceleration of multiple electron beams, increasing the total electron throughput by at least 1 order of magnitude. To achieve this, we show that the photonic crystal must support a mode at the Γ point in reciprocal space, with a normalized frequency equal to the normalized speed of the phase-matched electron. We show that the figure of merit of the MIMOSA can be inferred from the eigenmodes of the corresponding infinitely periodic structure, which provides a powerful approach to design such devices. Additionally, we extend the MIMOSA architecture to electron deflectors and other electron manipulation functionalities. These additional functionalities, combined with the increased electron throughput of these devices, permit all-optical on-chip manipulation of electron beams in a fully integrated architecture compatible with current fabrication technologies, which opens the way to unconventional electron beam shaping, imaging, and radiation generation.

43 PARTICLE ACCELERATORS↗

Particle acceleration and production of energetic photons in SN1987A

A pulsar wind model for the acceleration of particles in SN1987A is discussed. The expected photon flux is investigated in terms of the spectrum of parent protons and electrons, the nature of the region in which they propagate after acceleration, and the magnetic field and radiation environment which determines the subsequent fate of produced photons. The model is found to produce observable signals if the spin period of the pulsar is 10 ms or less.

Gaisser, T. K.↗

The Orbital Variation of Non-Thermal X-Ray Emission from eta Carinae

The collision of strong stellar winds in massive binary systems creates powerful shocks,which accelerates a small amount of particles to relativistic energies at the shock interface.This process is important in fundamental astrophysics in two ways;i) some particles may contribute to cosmic-rays observed around the Earth, whose origin is not well known, andii) it provides a good laboratory for particle acceleration physics as the shock occurs steadily in a predictable environment.Some relativistic particles collide with stellar photons or ambient material near the binary systemand emit non-thermal X-rays and gamma-rays, which are good probes of particle acceleration.This emission had been searched for decades but not found convincingly without sensitive high-energy telescopes.The NuSTAR telescope observed the enigmatic supermassive binary system eta Carinae multiple times after 2014 and found conclusive evidence of non-thermal emission from the star in the extremely hard X-ray band.This emission is prominent between 20-50 keV, below which thermal emission from shock colliding plasma dominates.It is relatively stable throughout the binary orbit, but it disappears near periastron when the wind colliding activity shuts off.This variation indicates that the non-thermal X-ray emission originates from the head-on wind-wind collision.The flat spectrum is consistent with inverse-Compton of stellar UV photons by accelerated electrons.The spectrum smoothly connects to a gamma-ray spectrum of a Fermi source detected around eta Carinae,suggesting that acceleration occurs up to the GeV energy.This result provide the strongest evidence so far that particle acceleration occurs at the wind colliding shock of a massive colliding wind binary system.

Hamaguchi, Kenji↗

Exploration of Defect Dynamics and Color Center Qubit Synthesis with Pulsed Ion Beams

Short-pulse ion beams have been developed in recent years and now enable applications in materials science. A tunable flux of selected ions delivered in pulses of a few nanoseconds can affect the balance of defect formation and dynamic annealing in materials. We report results from color center formation in silicon with pulses of 900 keV protons. G-centers in silicon are near-infrared photon emitters with emerging applications as single-photon sources and for spin-photon qubit integration. G-centers consist of a pair of substitutional carbon atoms and one silicon interstitial atom and are often formed by carbon ion implantation and thermal annealing. Here, we report on G-center formation with proton pulses in silicon samples that already contained carbon, without carbon ion implantation or thermal annealing. The number of G-centers formed per proton increased when we increased the pulse intensity from 6.9 × 10 9 to 7.9 × 10 10 protons/cm 2 /pulse, demonstrating a flux effect on G-center formation efficiency. We observe a G-center ensemble linewidth of 0.1 nm (full width half maximum), narrower than previously reported. Pulsed ion beams can extend the parameter range available for fundamental studies of radiation-induced defects and the formation of color centers for spin-photon qubit applications.

43 PARTICLE ACCELERATORS↗

Strain-graded quantum dots with spectrally pure, stable and polarized emission

Structural deformation modifies the bandgap, exciton fine structure and phonon energy of semiconductors, providing an additional knob to control their optical properties. The impact can be exploited in colloidal semiconductor quantum dots (QDs), wherein structural stresses can be imposed in three dimensions while defect formation is suppressed by controlling surface growth kinetics. Yet, the control over the structural deformation of QDs free from optically active defects has not been reached. Here, we demonstrate strain-graded CdSe-ZnSe core-shell QDs with compositionally abrupt interface by the coherent pseudomorphic heteroepitaxy. Resulting QDs tolerate mutual elastic deformation of varying magnitudes at the interface with high structural fidelity, allowing for spectrally stable and pure emission of photons at accelerated rates with near unity luminescence efficiency. We capitalize on the asymmetric strain effect together with the quantum confinement effect to expand emission envelope of QDs spanning the entire visible region and exemplify their use in photonic applications.

77 NANOSCIENCE AND NANOTECHNOLOGY↗